Magnon-phonon hybrid excitations are studied theoretically in a two-dimensional antiferromagnet with an easy axis normal to the plane. We show that two magnon bands and one phonon band are intertwined by the magnetoelastic coupling through a nontrivial SU(3) topology, which can be intuitively perceived by identifying a skyrmion structure in the momentum space. We develop a continuum theory as the long-wavelength approximation to the tight-binding model, showing our results are insensitive to lattice details and generally applicable to two-dimensional antiferromagnets. The theoretical results can be probed by measuring the thermal Hall conductance as a function of the temperature and the magnetic field. We envision that the magnetoelastic coupling in antiferromagnets can be a promising venue in search of various topological excitations, which cannot be found in magnetic or elastic models alone.
We study magnon hybridization in a ferrimagnetic heterostructure consisting of ultrathin gadolinium iron garnet and yttrium iron garnet layers and show the localized and extended spatial profiles of the magnon modes with different polarizations. These modes are expected to have distinct thermal excitation properties in the presence of a temperature gradient across the heterostructure. From a quantitative analysis of their consequences on longitudinal spin Seebeck effect, we predict an observable shift of the sign-changing temperature with respect to the one previously observed in gadolinium ir…
We study the exchange between electron and magnon spins at the interface of an antiferromagnet and a heavy metal at finite temperatures. The underlying physical mechanism is based on spin torque associated with the creation/annihilation of thermal magnons with right-hand and left-hand polarization. The creation/annihilation process depends strongly on the relative orientation between the polarization of the electron and the magnon spins. For a sufficiently strong spin transfer torque (STT), the conversion process becomes nonlinear, generating a nonzero net spin pumping current in the AFM that …
Strong coupling between magnon and electromagnetic wave can lead to the formation of a coupled spinphoton quasiparticle named as magnon-polariton. The phenomenon is well studied for ferromagnetic systems inside microwave cavities in recent years. However, formation of magnon-polariton is rarely seen for an antiferromagnet (AFM) because the strong coupling condition is not easily fulfilled. Here we present time-domain terahertz measurement on a multiferroic polar antiferromagnet Fe2Mo3O8. We find clearly beating between two modes at frequencies above and below the electric-active magnon frequen…
Van der Waals magnets are uniquely positioned at the intersection between two-dimensional materials, antiferromagnetic spintronics, and magnonics. The interlayer exchange interaction in these materials enables antiferromagnetic resonances to be accessed at GHz frequencies. Consequently, these layered antiferromagnets are intriguing materials out of which quantum hybrid magnonic devices can be fashioned. Here, we use both a modified macrospin model and micromagnetic simulations to demonstrate a comprehensive antiferromagnetic resonance spectra in van der Waals magnets near the ultrathin (monola…
We theoretically study the interaction of magnons, quanta of spin waves, and a domain wall in a one-dimensional easy-axis antiferromagnet in the presence of an external magnetic field applied along the easy axis. To this end, we begin by obtaining the exact solution for spin waves in the background of a domain wall magnetized by an external field. The finite magnetization inside the domain wall is shown to give rise to reflection of magnons scattering off the domain wall, deviating from the well-known result of reflection-free magnons in the absence of a magnetic field. For practical applicati…
We theoretically study magnon-phonon hybrid excitations (magnon-polarons) in two-dimensional antiferromagnets on a honeycomb lattice. With an in-plane Dzyaloshinskii-Moriya interaction (DMI) allowed from mirror symmetry breaking from phonons, we find non-trivial Berry curvature around the anti-crossing rings among magnon and both optical and acoustic phonon bands, which gives rise to finite Chern numbers. We show that the Chern numbers of the magnon-polaron bands can be manipulated by changing the magnetic field direction or strength. We evaluate the thermal Hall conductivity reflecting the no…
D-Wave Phonon Angular Momentum Texture in Altermagnets by Magnon-Phonon Hybridization
Institute of Physics, Martin Luther University Halle-Wittenberg and Halle-Berlin-Regensburg Cluster of Excellence “Center for Chiral Electronics”（马丁·路德哈雷-维滕贝格大学物理研究所）；Institute of Physics, Otto von Guericke University Magdeburg（奥托·冯·格里克马格德堡大学物理研究所）；Institute of Solid State Theory, University of Münster（明斯特大学固体理论研究所）；Institute of Physics, Johannes Gutenberg University Mainz（约翰内斯·古腾堡美因茨大学物理研究所）
We investigate magnonic band structure in thin homogeneous permalloy film decorated with periodic array of elliptically shaped permalloy dots and separated by non-magnetic Pt spacer. We demonstrated experimentally formation of the magnonic band structure for Damon-Eshbach wave propagating in permalloy film with the band gap opened at the Brillouin zone border and band splitting at smaller wavenumbers, due to the Bragg interference and interaction of propagating wave of the continuous film with a standing resonant mode of the nano-ellipses, respectively. The shape anisotropy of the permalloy na…
We present a theoretical study of excitations formed by hybridization between magnons and phonons - magnon-polarons - in antiferromagnets. We first outline a general approach to determining which magnon and phonon modes can and cannot hybridize in a system thereby addressing the qualitative questions concerning magnon-polaron formation. As a specific and experimentally relevant case, we study Nickel Oxide quantitatively and find perfect agreement with the qualitative analysis, thereby highlighting the strength of the former. We find that there are two distinct features of antiferromagnetic mag…
In this paper, we introduce Berry curvature, topological Chern number and topological chiral edge mode, that emerge from a hybridization between magnon and electromagnetic wave in a ferromagnet insulator. By focusing on the energy conservation, we first reformulate the Landau-Lifshitz-Maxwell equation into a Hermitian eigenvalue equation. From the eigenvalue equation, we define the Berry curvature of the magnon-photon coupled waves. We show that the Berry curvature thus introduced shows a prominent peak around a hybridization point between magnon mode and photon mode, and a massive hybrid mode…
We generalize the concept of the spin-momentum locking to magnonic systems and derive the formula to calculate the spin expectation value for one-magnon states of general two-body spin Hamiltonians. We give no-go conditions for magnon spin to be independent of momentum. As examples of the magnon spin-momentum locking, we analyze a one-dimensional antiferromagnet with the Néel order and two-dimensional kagome lattice antiferromagnets with the 120$^\circ$ structure. We find that the magnon spin depends on its momentum even when the Hamiltonian has the $z$-axis spin rotational symmetry, which can…
Topological Magnetic Phases and Magnon-Phonon Hybridization in the Presence of Strong Dzyaloshinskii-Moriya Interaction
School of Physics and Astronomy, Shanghai Jiao Tong University（上海交通大学物理与天文学院）；Wilczek Quantum Center, School of Physics and Astronomy, Shanghai Jiao Tong University（上海交大物理与天文学院李政道量子中心）；Shanghai Research Center for Quantum Sciences（上海量子科学研究中心）；Department of Physics, The Chinese University of Hong Kong（香港中文大学物理系）；Institute for Quantum Science and Technology, Shanghai University（上海大学量子科学与技术研究院）；Department of Physics, Shanghai University（上海大学物理系）
The richness in both the dispersion and energy of antiferromagnetic magnons has spurred the magnetism community to consider antiferromagnets for future spintronic/magnonic applications. However, the excitation and control of antiferromagnetic magnons remains challenging, especially when compared to ferromagnetic counterparts. A middle ground is found with synthetic antiferromagnet metamaterials, where acoustic and optical magnons exist at GHz frequencies. In these materials, the magnon energy spectrum can be tuned by static symmetry-breaking external fields or dipolar interactions hybridizing …
We study a bilayer structure consisting of an antiferromagnetic insulator and a normal metal. An electron current is driven in the normal metal with direction parallel to the interface between the materials. Due to interfacial exchange coupling between the localized spins in the antiferromagnet and the itinerant electrons in the normal metal, a magnon current can then be induced in the antiferromagnet. Using an uncompensated antiferromagnetic interface, creating an asymmetry in the interfacial coupling to the two degenerate magnon modes, we find that it is possible to generate a magnon spin-cu…
We theoretically study the Berry curvature of the magnon induced by the hybridization with the acoustic phonons via the spin-orbit and dipolar interactions. We first discuss the magnon-phonon hybridization via the dipolar interaction, and show that the dispersions have gapless points in momentum space, some of which form a loop. Next, when both spin-orbit and dipolar interactions are considered, we show anisotropic texture of the Berry curvature and its divergence with and without gap-closing. Realistic evaluation of the consequent anomalous velocity is given for yttrium iron garnet.
We predict that a temperature gradient can induce a magnon-mediated spin Hall response in an antiferromagnet with non-trivial magnon Berry curvature. We develop a linear response theory which gives a general condition for a Hall current to be well defined, even when the thermal Hall response is forbidden by symmetry. We apply our theory to a honeycomb lattice antiferromagnet and discuss a role of magnon edge states in a finite geometry.
In this Letter, we study the spin Nernst effect (SNE) of magnons in the nonlinear response regime. We derive the formula for the nonlinear magnon spin Nernst current by solving the Boltzmann equation and find out that it is described by an extended Berry curvature dipole of magnons. The nonlinear magnon SNE is expected to occur in various Néel antiferromagnets without Dzyaloshinskii-Moriya interaction. In particular, the nonlinear spin Nernst current in the honeycomb and diamond lattice antiferromagnets can be controlled by strain/pressure.
In this work, we theoretically study the magnon spin transport in easy-plane antiferromagnetic insulators in the presence of an in-plane magnetic field. By exactly calculating the magnon spectrum, we find the band splitting due to the magnetic anisotropy can be fully compensated by the external field at a particular strength, which makes its dynamics nearly equivalent to an easy-axis antiferromagnet. As a result, the intrinsic magnon spin Hall effect due to the dipole-dipole interaction, previously predicted in easy-axis antiferromagnets is activated in easy-plane antiferromagnets. The compens…
We theoretically investigate the transport of magnon orbitals in a honeycomb antiferromagnet. We find that the magnon orbital Berry curvature is finite even without spin-orbit coupling and thus the resultant magnon orbital Hall effect is an intrinsic property of the honeycomb antiferromagnet rooted only in the exchange interaction and the lattice structure. Due to the intrinsic nature of the magnon orbital Hall effect, the magnon orbital Nernst conductivity is estimated to be orders of magnitude larger than the predicted values of the magnon spin Nernst conductivity that requires finite spin-o…
In this Letter we present a comprehensive study of topological magnon bands and thermal Hall effect in non-collinear antiferromagnetic systems on the honeycomb lattice with an intrinsic Dzyaloshinskii-Moriya interaction. We theoretically show that the system possesses topological magnon bands with Chern number protected edge modes accompanied by a nonzero thermal magnon Hall effect. These features result from non-collinearity of the magnetic moments due to an applied out-of-plane magnetic field. Our results provide an experimental clue towards the realization of topological magnon transports i…
We report broadband microwave absorption spectroscopy of the layered antiferromagnet CrCl3. We observe a rich structure of resonances arising from quasi-two-dimensional antiferromagnetic dynamics. Due to the weak interlayer magnetic coupling in this material, we are able to observe both optical and acoustic branches of antiferromagnetic resonance in the GHz frequency range and a symmetry-protected crossing between them. By breaking rotational symmetry, we further show that strong magnon-magnon coupling with large tunable gaps can be induced between the two resonant modes.
We explore routes to realize electrically driven Bose-Einstein condensation of magnons in insulating antiferromagnets. Even in insulating antiferromagnets, the localized spins can strongly couple to itinerant spins in adjacent metals via spin-transfer torque and spin pumping. We describe the formation of steady-state magnon condensates controlled by a spin accumulation polarized along the staggered field in an adjacent normal metal. Two types of magnons exist in antiferromagnets, which carry opposite magnetic moments. Consequently, and in contrast to ferromagnets, Bose-Einstein condensation ca…
We consider a hybrid structure formed by graphene and an insulating antiferromagnet, separated by a dielectric of thickness up to $d\simeq 500 \,nm$. When uncoupled, both graphene and the antiferromagnetic surface host their own polariton modes coupling the electromagnetic field with plasmons in the case of graphene, and with magnons in the case of the antiferromagnet. We show that the hybrid structure can host two new types of hybrid polariton modes. First, a surface magnon-plasmon polariton whose dispersion is radically changed by the carrier density of the graphene layer, including a change…
We observe a strong thermally-controlled magnon-mediated interlayer coupling of two ferromagnetic layers via an antiferromagnetic spacer in spin-valve type trilayers. The effect manifests itself as a field-induced coherent switching of the two ferromagnets, which can be controlled by varying temperature and the spacer thickness. We explain the observed behavior as due to a strong hybridization of the ferro- and antiferro-magnetic magnon modes in the trilayer at temperatures just below the Néel temperature of the antiferromagnetic spacer.
We investigated the topological property of magnon bands in the collinear magnetic orders of zigzag and stripy phases for the antiferromagnetic honeycomb lattice and identified Berry curvature and symmetry constraints on the magnon band structure. Different symmetries of both zigzag and stripy phases lead to different topological properties, in particular, the magnon bands of the stripy phase being disentangled with a finite Dzyaloshinskii-Moriya (DM) term with non-zero spin Chern number. This is corroborated by calculating the spin Nernst effect. Our study establishes the existence of the non…
Gilbert damping is a key property governing magnetization dynamics in ordered magnets. We present a theoretical study of intrinsic Gilbert damping induced by magnon decay in antiferromagnetic metals through $s$-$d$ exchange interaction. Our theory delineates the qualitative features of damping in metallic antiferromagnets owing to their bipartite nature, in addition to providing analytic expressions for the damping parameters. Magnon-induced intraband electron scattering is found to predominantly cause magnetization damping, whereas the Néel field is found to be damped via disorder. Depending …
A magnon spin-orbit coupling, induced by the dipole-dipole interaction, is derived in monoclinic-stacked bilayer honeycomb spin lattice with perpendicular magnetic anisotropy and antiferromagnetic interlayer coupling. Linear crossings are predicted in the magnon spectrum around the band minimum in G valley, as well as in the high frequency range around the zone boundary. The linear crossings in K and K' valleys, which connect the acoustic and optical bands, can be gapped when the intralayer dipole-dipole or Kitaev interactions exceed the interlayer dipole-dipole interaction, resulting in a pha…
Magnon excitations in antiferromagnetic materials and their physical implications enable novel device concepts not available in ferromagnets, emerging as a new area of active research. A unique characteristic of antiferromagnetic magnons is the coexistence of opposite spin polarization, which mimics the electron spin in a variety of transport phenomena. Among them, the most prominent spin-contrasting phenomenon is the magnon spin Nernst effect (SNE), which refers to the generation of transverse pure magnon spin current through a longitudinal temperature gradient. We introduce selected recent p…
Antiferromagnetic materials host pairs of spin-up and spin-down magnons which can be described in terms of a magnonic pseudospin. The close analogy between this magnonic pseudospin systems and that of electronic charge carriers led to the prediction of fascinating phenomena in antiferromagnets. Recently, the associated dynamics of antiferromagnetic pseudospin has been experimentally demonstrated and, in particular, the first observation of the magnon Hanle effect has been reported. We here expand the magnonic spin transport description by explicitly taking into account contributions of finite-…
In the absence of an external magnetic field and a spin-polarized charge current, an antiferromagnetic system supports two degenerate magnon modes. An applied thermal bias activates the magnetic dynamics, leading to a magnon flow from the hot to the cold edge (magnonic spin Seebeck current). Both degenerate bands contribute to the magnon current but the orientations of the magnetic moments underlying the magnons are opposite in different bands. Therefore, while the magnon current is nonzero, the net spin current is zero.
Ultrastrong magnon-photon coupling in superconductor/antiferromagnet/superconductor heterostructures at terahertz frequencies
Moscow Institute of Physics and Technology（莫斯科物理技术学院）；School of Physics, Huazhong University of Science and Technology（华中科技大学物理学院）；National Research University Higher School of Economics（国立研究型高等经济大学）
We propose a general theory of microwave absorption spectroscopy for symmetry-breaking synthetic antiferromagnets (SAFs). Generally, inhomogeneity or different thickness of the two ferromagnetic sublayers of a SAF results in the intrinsic symmetry breaking, while out-of-plane components of dc magnetic fields lead to the extrinsic one. The broken symmetry of SAFs excludes the original symmetry-protected crossing between pure in-phase and out-of-phase resonance modes with opposite parity. Alternatively, new frequency branches become hybridization of original bare modes in terms of symmetry-break…
In this work, we study magnon-magnon coupling in synthetic antiferromagnets (SyAFs) using microwave spectroscopy at room temperature. Two distinct spin-wave modes are clearly observed and are hybridised at degeneracy points. We provide a phenomenological model that captures the coupling phenomena and experimentally demonstrate that the coupling strength is controlled by the out-of-plane tilt angle as well as the interlayer exchange field. We numerically show that a spin-current mediated damping in SyAFs plays a role in influencing the coupling strength.
The Stern-Gerlach (SG) effect is well known as the spin-dependent splitting of a beam of atoms carrying magnetic moments by a magnetic-field gradient, leading to the concept of electron spin. Antiferromagnets can accommodate two magnon modes with opposite spin polarizations, which is equivalent to the spin property of electrons. Here, we propose the existence of an all-magnonic SG effect in antiferromagnetic magnonic system, where a linearly polarized spin-wave beam is deflected by a straight Dzyaloshinskii-Moriya interaction (DMI) interface into two opposite polarized spin-wave beams propagat…
We investigate the intrinsic magnon spin current in a noncollinear antiferromagnetic insulator. We introduce a definition of the magnon spin current in a noncollinear antiferromagnet and find that it is in general non-conserved, but for certain symmetries and spin polarizations the averaged effect of non-conserving terms can vanish. We formulate a general linear response theory for magnons in noncollinear antiferromagnets subject to a temperature gradient and analyze the effect of symmetries on the response tensor. We apply this theory to single-layer potassium iron jarosite KFe$_3$(OH)$_6$(SO…
