Optical activity, the power of a medium to rotate the polarization of a light beam, has contributed significantly to molecular structure assessments in stereochemistry, biomolecular science and crystallography. Thus far, it is commonly believed that optical activity is manifested only in the chiral media which can give rise to circular birefringence of light. Here, we experimentally demonstrate that free space can also support the implementation of non-reciprocal optical activity with Bessel beams by spin-orbital interaction. Specifically, non-diffractive optically active beams are realized, with their optical rotatory power readily controlled by simple optical elements. We show that such free-space optical activity can be exploited to form non-reciprocal optical components such as polarization rotators, isolators, and circulators. Our results may bring about new possibilities of media-independent optical activity to other transverse waves ranging from radio to optical frequencies.
Expressions corresponding to the transmission of a uniaxial optically active crystal platelet are provided for an optical axis parallel and perpendicular to the plane of interface. The optical activity is taken into account by a consistent multipolar expansion of the crystal medium response due to the path of an electromagnetic wave. Numerical examples of the effect of the optical activity are given for quartz platelets of chosen thicknesses. The optical activity's effects on the variations of the transmission of quartz platelets as a function of the angle of incidence is also investigated.
Electromagnetically induced transparency has the unique ability to optically control transparency windows with low light in atomic systems. However, its practical applications in quantum physics and information science are limited due to rigid experimental requirements. Here, we demonstrate a new mechanism of optically induced transparency in a micro-cavity by introducing a four-wave mixing gain to nonlinearly couple two separated resonances of the micro-cavity in an ambient environment. A signature Fano-like resonance was observed owing to the nonlinear interference of the two coupled resonan…
From Newtons third law, the principle of actio et reactio, we expect the forces between interacting particles to be equal and opposite. However, non-reciprocal forces can arise. Specifically, this has recently been shown theoretically in the interaction between dissimilar optically trapped particles mediated by an external field. As a result, despite the incident external field not having a transverse component of momentum, the particle pair experiences a force in a direction transverse to the light propagation direction. In this letter, we directly measure the net non-reciprocal force in elec…
An optical signal that propagates along a conventional waveguide is back reflected at waveguide terminations. If the waveguide permits only one-way propagation, this back reflection cannot take place; the optical signal undergoes a nearly 100% conversion to radiation modes. Hence, a terminated one-way waveguide may serve as a matched nano-antenna with a natural guiding and feeding mechanism. We examine the termination effect in a recently suggested nano-scale one-way plasmonic waveguide, and its properties as a matched nano antenna are shown. Since one-way structures are inherently non-recipro…
The realization of optical non-reciprocity is crucial for many device applications, and also of fundamental importance for manipulating and protecting the photons with desired time-reversal symmetry. Recently, various new mechanisms of magnetic-free non-reciprocity have been proposed and implemented, avoiding the limitation of the strong magnetic field imposed by the Faraday effect. However, due to the difficulties in suppressing the drive and its induced noises, these devices exhibit limited isolation performances and leave the quantum noise properties rarely studied. Here, we demonstrate a n…
We investigate the rotation of the polarization of a light ray propagating in the gravitational field of a circularly polarized laser beam. The rotation consists of a reciprocal part due to gravitational optical activity, and a non-reciprocal part due to the gravitational Faraday effect. We discuss how to distinguish the two effects: Letting light propagate back and forth between two mirrors, the rotation due to gravitational optical activity cancels while the rotation due to the gravitational Faraday effect accumulates. In contrast, the rotation due to both effects accumulates in a ring cavit…
We describe a new approach for on-chip optical non-reciprocity which makes use of strong optomechanical interaction in microring resonators. By optically pumping the ring resonator in one direction, the optomechanical coupling is only enhanced in that direction, and consequently, the system exhibits a non-reciprocal response. For different configurations, this system can function either as an optical isolator or a coherent non-reciprocal phase shifter. We show that the operation of such a device on the level of single-photon could be achieved with existing technology.
In this article the concept of enantiomorphism is developed in terms of topological, rather than geometrical, concepts. Chirality is to be associated with enantiomorphic pairs which induce Optical Activity, while Helicity is to be associated enantiomorphic pairs which induce a Faraday effect. Experimentally, the existence of enantiomorphic pairs is associated with the lack of a center of symmetry, which is also serves as a necessary condition for Optical Activity. However, Faraday effects may or may not require a lack of a center of symmetry. The two species of enantiomorphic pairs are distinc…
Optically active artificial structures have attracted tremendous research attention. Such structures must meet two requirements: Lack of spatial inversion symmetries and, a condition usually not explicitly considered, the structure shall preserve the helicity of light, which implies that there must be a vanishing coupling between the states of opposite polarization handedness among incident and scattered plane waves. Here, we put forward and demonstrate that a unit cell made from chiraly arranged electromagnetically dual scatterers serves exactly this purpose. We prove this by demonstrating op…
Optical activity (OA), also called circular birefringence, is known for two hundred years, but its applications for topological photonics remain unexplored. Unlike the Faraday effect, OA provokes rotation of the linear polarization of light without magnetic effects, thus preserving the time-reversal symmetry. Here, we report a direct measurement of the Berry curvature and quantum metric of the photonic modes of a planar cavity containing an optically active organic microcrystal (perylene). Photonic spin-orbit-coupling induced by the cavity results in the action of a non-Abelian gauge field on …
Light is generally expected to travel through isotropic media independent of its direction. This makes it challenging to develop non-reciprocal optical elements like optical diodes or circulators, which currently rely on magneto-optical effects and birefringent materials. Here we present measurements of non-reciprocal transmission and spontaneous symmetry breaking between counter-propagating light in dielectric microresonators. The symmetry breaking corresponds to a resonance frequency splitting that allows only one of two counter-propagating (but otherwise identical) light waves to circulate …
Advanced photonic nanostructures have enabled the maximization of synthetic chiroptic activities. The unique structuring of these building blocks has empowered chiral selective interactions with electromagnetic waves in plasmonic structures and dielectric media. Given the repertoire of optimized chiral surfaces in the literature and the ubiquity of chirality in the organic realm, the natural direction to consider is the operation of these devices in larger optical systems much like their chiral organic counterparts. In this review, we recapitulate advances in active and nonlinear chiral metama…
Prospects of using metal hole arrays for the enhanced optical detection of molecular chirality in nanosize volumes are investigated. Light transmission through the holes filled with an optically active material is modeled and the activity enhancement by more than an order of magnitude is demonstrated. The spatial resolution of the chirality detection is shown to be of a few tens of nanometers. From comparing the effect in arrays of cylindrical holes and holes of complex chiral shape, it is concluded that the detection sensitivity is determined by the plasmonic near field enhancement. The intri…
Dirac points, new photonic band gaps and effect of magnetically induced transparency in dichroic cholesteric liquid crystals with wavelength dependent magnetooptical activity parameter
The basic principles of classical and semi-classical theories of molecular optical activity are discussed. These theories are valid for dilute solutions of optically active organic molecules. It is shown that all phenomena known in the classical theory of molecular optical activity can be described with the use of one pseudo-scalar which is a uniform function of the incident light frequency $ω$. The relation between optical rotation and circular dichroism is derived from the basic Kramers-Kronig relations. In our discussion of the general theory of molecular optical activity we introduce the t…
Silicon films doped with Er and O were prepared by techniques of physical vapor deposition on crystalline silicon, ion beam mixing and oxygen incorporation through Ar+ and O2+ implantation, and thermal annealing. Processing steps were tailored to be compatible with standard CMOS and to be of notably low cost to fabricate optically active media for silicon-based infrared emitters. The Si:Er:O films exhibit strong photoluminescence at room temperature that is analogous to Stark-split Er+3 ion 1.55-micron bands in fiber-optic materials. Concentration distributions were determined by Rutherford ba…
We demonstrate an optically controlled waveplate at ~1323 nm using the 5S1/2-5P1/2-6S1/2 ladder transition in a Rb vapor cell. The lower leg of the transitions represents the control beam, while the upper leg represents the signal beam. We show that we can place the signal beam in any arbitrary polarization state with a suitable choice of polarization of the control beam. Specifically, we demonstrate a differential phase retardance of ~180 degrees between the two circularly polarized components of a linearly polarized signal beam. We also demonstrate that the system can act as a Quarter Wave p…
