Superconductivity is a quantum phenomenon caused by bound pairs of electrons. In diverse families of strongly correlated electron systems, the electron pairs are not bound together by phonon exchange but instead by some other kind of bosonic fluctuations. In these systems, superconductivity is often found near a magnetic quantum critical point (QCP) where a magnetic phase vanishes in the zero-temperature limit. Moreover, the maximum of superconducting transition temperature Tc frequently locates near the magnetic QCP, suggesting that the proliferation of critical spin fluctuations emanating from the QCP plays an important role in Cooper pairing. In cuprate superconductors, however, the superconducting dome is usually separated from the antiferromagnetic phase and Tc attains its maximum value near the verge of enigmatic pseudogap state that appears below doping-dependent temperature T*. Thus a clue to the pairing mechanism resides in the pseudogap and associated anomalous transport properties. Recent experiments suggested a phase transition at T*, yet, most importantly, relevant fluctuations associated with the pseudogap have not been identified. Here we report on direct observations of enhanced nematic fluctuations in (Bi,Pb)2Sr2CaCu2O8+d by elastoresistance measurements, which couple to twofold in-plane electronic anisotropy, i.e. electronic nematicity. The nematic susceptibility shows Curie-Weiss-like temperature dependence above T*, and an anomaly at T* evidences a second-order transition with broken rotational symmetry. Near the pseudogap end point, where Tc is not far from its peak in the superconducting dome, nematic susceptibility becomes singular and divergent, indicating the presence of a nematic QCP. This signifies quantum critical fluctuations of a nematic order, which has emerging links to the high-Tc superconductivity and strange metallic behaviours in cuprates.
During the last decade, translational and rotational symmetry-breaking phases -- density wave order and electronic nematicity -- have been established as generic and distinct features of many correlated electron systems, including pnictide and cuprate superconductors. However, in cuprates, the relationship between these electronic symmetry-breaking phases and the enigmatic pseudogap phase remains unclear. Here, we employ resonant x-ray scattering in a cuprate high-temperature superconductor La$_{1.6-x}$Nd$_{0.4}$Sr$_{x}$CuO$_{4}$ (Nd-LSCO) to navigate the cuprate phase diagram, probing the rel…
A central issue in the quest to understand the superconductivity in cuprates is the nature and origin of the pseudogap state, which harbours anomalous electronic states such as Fermi arc, charge density wave (CDW), and $d$-wave superconductivity. A fundamentally important, but long-standing controversial problem has been whether the pseudogap state is a distinct thermodynamic phase characterized by broken symmetries below the onset temperature $T^*$. Electronic nematicity, a fourfold ($C_4$) rotational symmetry breaking, has emerged as a key feature inside the pseudogap regime, but the presenc…
The pseudogap phenomenon in cuprates is the most mysterious puzzle in the research of high-temperature superconductivity. In particular, whether the pseudogap is associated with a crossover or phase transition has been a long-standing controversial issue. The tetragonal cuprate HgBa$_2$CuO$_{4+δ}$, with only one CuO$_2$ layer per primitive cell, is an ideal system to tackle this puzzle. Here, we measure the anisotropy of magnetic susceptibility within the CuO$_2$ plane with exceptionally high-precision magnetic torque experiments. Our key finding is that a distinct two-fold in-plane anisotropy…
Within the Landau paradigm of continuous phase transitions, ordered states of matter are characterized by a broken symmetry. Although the broken symmetry is usually evident, determining the driving force behind the phase transition is often a more subtle matter due to coupling between otherwise distinct order parameters. In this paper we show how measurement of the divergent nematic susceptibility of an iron pnictide superconductor unambiguously distinguishes an electronic nematic phase transition from a simple ferroelastic distortion. These measurements also reveal an electronic nematic quant…
Starting from a microscopic itinerant model, we derive and analyze the effective low-energy model for collective magnetic excitations in the iron pnictides. We show that the stripe magnetic order is generally preempted by an Ising-nematic order which breaks $C_{4}$ lattice symmetry but preserves O(3) spin-rotational symmetry. This leads to a rich phase diagram as function of doping, pressure, and elastic moduli, displaying split magnetic and nematic tri-critical points. The nematic transition may instantly bring the system to the verge of a magnetic transition, or it may occur first, being fol…
The nature of the pseudogap and its relationship with superconductivity are one of the central issues of cuprate superconductors. Recently, a possible scenario has been proposed that the pseudogap state is a distinct phase characterized by spontaneous rotational symmetry breaking called "nematicity" based on transport and magnetic susceptibility measurements, where the symmetry breaking was observed below the pseudogap temperature $T^*$. Here, we report a temperature-dependent ARPES study of nematicity in slightly overdoped Bi${}_{1.7}$Pb${}_{0.5}$Sr${}_{1.9}$CaCu${}_2$O${}_{8+δ}$ triggered by…
We present a model for the combined nematic and `smectic' or stripe-like orders seen in recent scanning tunneling microscopy (STM) experiments in cuprates. We model the stripe order as an electronic charge density wave with associated Peierls distortion -- a `Pomeranchuk wave'. Disorder restricts this primary order to nanoscale domains, while secondary coupling to strain generates nematic order with considerably longer range.
In the present paper II, we will gain an understanding of the nematicity, insulating ground state (IGS), nematicity to stripe phase transition, Fermi pockets evolution, and resistivity temperature upturn, as to be metal - insulator (fermion-boson)- crossover (MIC) phenomena for the pseudogap (PG) region of cuprates. While in the paper I [1], we obtained an understanding of the observed heat conductivity downturn, anomalous Lorentz ratio, insulator resistivity boundary, nonlinear entropy as manifestations of the same MIC. The recently observed nematicity and hidden magnetic order are related to…
Using Monte Carlo simulations with a tunable uniaxial strain, for the first time the nematic susceptibility of a model for the pnictides is calculated. The results are in good agreement with the experiments by J-H. Chu {\it et al.}, Science {\bf 337}, 710 (2012). Via a Ginzburg-Landau analysis, our study suggests a nematicity in pnictides primarily originating on magnetism, but with the lattice/orbital boosting up critical temperatures and separating the structural $T_S$ and Néel $T_N$ transitions. At $T>T_S$, Curie-Weiss behavior is observed with the characteristic temperature $T^*$ unveiled …
Experiments that have been interpreted as providing evidence that the pseudogap phase in cuprates is an electronic nematic are discussed from the point of view of lattice structure. We conclude that existing experiments are not sufficient to prove a nematic origin of the pseudogap in underdoped cuprates.
Establishing the presence and the nature of a quantum critical point in their phase diagram is a central enigma of the high-temperature superconducting cuprates. It could explain their pseudogap and strange metal phases, and ultimately their high superconducting temperatures. Yet, while solid evidences exist in several unconventional superconductors of ubiquitous critical fluctuations associated to a quantum critical point, in the cuprates they remain undetected until now. Here using symmetry-resolved electronic Raman scattering in the cuprate Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$, we report the obser…
Nematicity has emerged as a key feature of cuprate superconductors, but its link to other fundamental properties such as superconductivity, charge order and the pseudogap remains unclear. Here we use measurements of transport anisotropy in YBa$_2$Cu$_3$O$_y$ to distinguish two types of nematicity. The first is associated with short-range charge-density-wave modulations in a doping region near $p = 0.12$. It is detected in the Nernst coefficient, but not in the resistivity. The second type prevails at lower doping, where there are spin modulations but no charge modulations. In this case, the on…
Recent observations of broken symmetries have partly demystified the pseudogap phase. Here we review evidence for long-range intra-unit-cell(IUC) nematic order and its unexpectedly strong coupling to the phase of the fluctuating stripes in the pseudogap states of underdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. In particular, we focus on the analysis techniques that reveal this evidence in scanning tunneling spectroscopy data, the definition of the extracted IUC nematic order parameter, and a phenomenological theory of the coupling between the IUC nematic order and the previously reported coexisting …
Overshadowing the superconducting dome in hole-doped cuprates, the pseudogap state is still one of the mysteries that no consensus can be achieved. It has been suggested that the rotational symmetry is broken in this state and may result in a nematic phase transition, whose temperature seems to coincide with the onset temperature of the pseudogap state $T^*$ around optimal doping level, raising the question whether the pseudogap results from the establishment of the nematic order. Here we report results of resistivity measurements under uniaxial pressure on several hole-doped cuprates, where t…
Strongly interacting electrons can exhibit novel collective phases, among which the electronic nematic phases are perhaps the most surprising as they spontaneously break rotational symmetry of the underlying crystal lattice. The electron nematicity has been recently observed in the iron-pnictide and cuprate high-temperature superconductors. Whether such a tendency of electrons to self-organise unidirectionally has a common feature in these superconductors is, however, a highly controversial issue. In the cuprates, the nematicity has been suggested as a possible source of the pseudogap phase, w…
This article is devoted to a discussion of stripe and electron-nematic order and their connection to electronic properties in the pseudogap regime of copper-oxide superconductors. We review basic properties of these symmetry-breaking ordering phenomena as well as proposals which connect them to quantum-oscillation measurements. Experimental data indicate that these orders are unlikely to be the cause of the pseudogap phenomenon, implying that they occur on top of the pseudogap state which itself is of different origin. Specifically, we discuss the idea that the non-superconducting pseudogap gr…
Using a dynamic cluster quantum Monte Carlo approximation, we study a two-dimensional Hubbard model with a small orthorhombic distortion in the nearest neighbor hopping integrals. We find a large nematic response in the low-frequency single-particle scattering rate which develops with decreasing temperature and doping as the pseudogap region is entered. At the same time, the d-wave superconducting gap function develops an s-wave component and its amplitude becomes anisotropic. The strength of the pairing correlations, however, is found to be unaffected by the strong anisotropy, indicating that…
We report Raman scattering measurement of charge nematic fluctuations in the tetragonal phase of BaFe$_2$As$_2$ and Sr(Fe$_{1-x}$Co$_x$)$_2$As$_2$ (x=0.04) single crystals. In both systems, the observed nematic fluctuations are found to exhibit divergent Curie-Weiss like behavior with very similar characteristic temperature scales, indicating a universal tendency towards charge nematic order in 122 iron-based superconductors.
We analyze how thermal fluctuations near a finite temperature nematic phase transition affect the spectral function $A({\bf k},ω)$ for single-electron excitations in a two-dimensional metal. Perturbation theory yields a splitting of the quasi-particle peak with a d-wave form factor, reminiscent of a pseudogap. We present a resummation of contributions to all orders in the Gaussian fluctuation regime. Instead of a splitting, the resulting spectral function exhibits a pronounced broadening of the quasi-particle peak, which varies strongly around the Fermi surface and vanishes upon approaching th…
Recently, complex phase transitions accompanied by the rotational symmetry breaking have been discovered experimentally in cuprate superconductors. To find the realized order parameters, we study various charge susceptibilities in an unbiased way, by applying the functional-renormalization-group method to the realistic $d$-$p$ Hubbard model. Without assuming the wavevector of the order parameter, we reveal that the most dominant instability is the uniform ($q = 0$) charge modulation on the $p_x$ and $p_y$ orbitals, which possesses the d-symmetry. This uniform nematic order triggers another nem…
Unconventional symmetry-breaking phenomena due to nontrivial order parameters attract increasing attention in strongly correlated electron systems. Here, we predict theoretically the occurrence of nanoscale spontaneous spin-current, called the spin loop-current (sLC) order, as a promising origin of the pseudogap and electronic nematicity in cuprates. We reveal that the sLC is driven by the odd-parity electron-hole condensation that are mediated by transverse spin fluctuations around the pseudogap temperature $T^*$. At the same temperature, odd-parity magnon pair condensation occurs. The sLC or…
Perspective on S. Mukhopadhyay, et al. Evidence for a vestigial nematic state in the cuprate pseudogap phase, PNAS 116, 13249 (2019); arXiv:1904.00915.
The pseudogap regime of the cuprate high-temperature superconductors is characterized by a variety of competing orders, the nature of which are still widely debated. Recent experiments have provided evidence for electron nematic order, in which the electron fluid breaks rotational symmetry while preserving translational invariance. Raman spectroscopy, with its ability to symmetry resolve low energy excitations, is a unique tool that can be used to assess nematic fluctuations and nematic ordering tendencies. Here, we compare results from determinant quantum Monte Carlo simulations of the Hubbar…
The individual k\parallel and k\perp stripe excitations in fluctuating spin-charge stripes have not been observed yet. In Raman scattering if we set, for example, incident and scattered light polarizations to two possible stripe directions, we can observe the fluctuating stripe as if it is static. Using the different symmetry selection rule between the B1g two-magnon scattering and the B1g and B2g isotropic electronic scattering, we succeeded to obtain the k\parallel and k\perp strip magnetic excitations separately in La2-xSrxCuO4. Only the k\perp stripe excitations appear in the wide-energy i…
The intra-unit-cell nematic phase is studied within the three-band Emery model of the cuprates with the use of the approach based on the diagrammatic expansion of the Gutzwiller wave function (DE-GWF). According to our analysis the spontaneous $C_4$ symmetry breaking of the electronic wave function, leading to the nematic behavior, can appear due to electron correlations induced mainly by the onsite Coulomb repulsion, even in the absence of the corresponding intersite oxygen-oxygen repulsion term. The latter has been considered as the triggering factor of the nematic state formation in a numbe…
Charge stripe order has recently been established as an important ingredient of the physics of cuprate high-T$_c$ superconductors. However, due to the complex interplay between competing phases and the influence of disorder, it is unclear how it emerges from the parent metallic state. Here we report on the discovery of an unconventional electronic ordered phase between charge-stripe order and (pseudogapped) metal in the cuprate La$_{2-x-y}$Eu$_{y}$Sr$_x$CuO$_4$ with $y = 0.2$ (LESCO). The peculiar properties of the intermediate phase are revealed through three complementary experiments: nuclea…
We analyze fermionic spectral function in the spin-density-wave (SDW) phase of quasi-2D cuprates at small but finite T. We use a non-perturbative approach and sum up infinite series of thermal self-energy terms, keeping at each order nearly-divergent (T/J) |log epsilon| terms, where epsilon is a deviation from a pure two-dimensionality, and neglecting regular T/J corrections. We show that, as SDW order decreases, the spectral function in the antinodal region acquires peak/hump structure: the coherent peak position scales with SDW order parameter, while the incoherent hump remains roughly at th…
We investigate how emergent nematic order and nematic fluctuations affect several macroscopic properties of both the normal and superconducting states of the iron pnictides. Due to its magnetic origin, long-range nematic order enhances magnetic fluctuations, leaving distinctive signatures in the spin-lattice relaxation rate, the spin-spin correlation function, and the uniform magnetic susceptibility. This enhancement of magnetic excitations is also manifested in the electronic spectral function, where a pseudogap can open at the hot spots of the Fermi surface. In the nematic phase, electrons a…
We derive the fermionic contribution to the longitudinal and Hall conductivities within a Kubo formalism, using a phenomenological Greens function which has been previously developed to describe photoemission data in the pseudogap phase of the cuprates. We find that the in-plane electrical and thermal conductivities are metallic-like, showing a universal limit behavior characteristic of a d-wave spectrum as the scattering rate goes to zero. In contrast, the c-axis resistivity and the Hall number are insulating-like, being divergent in the same limit. The relation of these results to transport …
An unusual noise component is found near and below about 250 K in the normal state of underdoped YBCO and Ca-YBCO films. This noise regime, unlike the more typical noise above 250 K, has features expected for a symmetry-breaking collective electronic state. These include large individual fluctuators, a magnetic sensitivity, and aging effects. A possible interpretation in terms of fluctuating charge nematic order is presented.
In several Fe-based superconductors, slight $C_4$ symmetry breaking occurs at $T^*$, which is tens of Kelvin higher than the structural transition temperature $T_S$. In this "hidden" nematic state at $T_S<T<T^*$, the orthorhombicity is tiny [$ϕ=(a-b)/(a+b) \ll 0.1$%], but clear evidences of bulk phase transition have been accumulated. To explain this long-standing mystery, we propose the emergence of antiferro-bond (AFB) order with the antiferro wavevector ${\bf q}=(0,π)$ at $T=T^*$, by which the characteristic phenomena below $T^*$ are satisfactorily explained. This AFB order originates from …
The nature of the pseudogap phase is a central problem in the quest to understand high-Tc cuprate superconductors. A fundamental question is what symmetries are broken when that phase sets in below a temperature T*. There is evidence from both polarized neutron diffraction and polar Kerr effect measurements that time- reversal symmetry is broken, but at temperatures that differ significantly. Broken rotational symmetry was detected by both resistivity and inelastic neutron scattering at low doping and by scanning tunnelling spectroscopy at low temperature, but with no clear connection to T*. H…
Nematicity in the heavily hole-doped iron pnictide superconductors remains controversial. Sizeable nematic fluctuations and even nematic orders far from a magnetic instability were declared in RbFe$_2$As$_2$ and its sister compounds. Here we report a systematic elastoresistance study of series of isovalent- and electron-doped KFe$_2$As$_2$ crystals. We found divergent elastoresistance upon cooling for all the crystals along their [110] direction. The amplitude of elastoresistivity diverges if K is substituted with larger ions or if the system is driven towards a Lifshitz transition. However, w…
We investigate temperature and fluence dependent dynamics of the photoexcited quasi-particle relaxation and low-energy electronic structure in electron-doped 1111-structure Sm(Fe_{0.93}Co_{0.07})AsO single crystal. We find that the behavior is qualitatively identical to the 122-structure Ba(Fe,Co)_{2}As_{2} including the presence of a normal state pseudogap and a marked 2-fold symmetry breaking in the tetragonal phase that we relate to the electronic nematicity. The 2-fold symmetry breaking appears to be a general feature of the electron doped iron pnictides.
The pseudogap (PG) state and its related intra-unit-cell symmetry breaking remain the focus in the research of cuprate superconductors. Although the nematicity has been studied in Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$, especially underdoped samples, its behavior in other cuprates and different doping regions is still unclear. Here we apply a scanning tunneling microscope to explore an overdoped (Bi, Pb)$_2$Sr$_2$CuO$_{6+δ}$ with a large Fermi surface (FS). The establishment of a nematic order and its real-space distribution is visualized as the energy scale approaches the PG.
Unveiling the driving force for a phase transition is normally difficult when multiple degrees of freedom are strongly coupled. One example is the nematic phase transition in iron-based superconductors. Its mechanism remains controversial due to a complex intertwining among different degrees of freedom. In this paper, we report a method for measuring the nematic susceptibly of FeSe$_{0.9}$S$_{0.1}$ using angle-resolved photoemission spectroscopy (ARPES) and an $in$-$situ$ strain-tuning device. The nematic susceptibility is characterized as an energy shift of band induced by a tunable uniaxial …
The most intriguing observation of cuprate experiments is most likely the metal-insulator-crossover (MIC), seen in the underdome region of the temperature-doping phase diagram of copper-oxides under a strong magnetic field, when the superconductivity is suppressed. This MIC, which results in such phenomena as heat conductivity downturn, anomalous Lorentz ratio, nonlinear entropy, insulating ground state, nematicity- and stripe-phases and Fermi pockets, reveals the nonconventional dielectric property of the pseudogap-normal phase. Since conventional superconductivity appears from a conducting n…
Experimental studies of the pairing state of cuprate superconductors reveal asymmetric behaviors of the hole-doped (p-type) and electron-doped (n-type) cuprates. The pairing symmetry, pseudogap phenomenon, low-energy spin excitations and the spatial homogeneity of the superconducting order parameter appear to be non-universal among the cuprates, which may be attributed to competing orders. We propose that the non-universal pseudogap and nano-scale variations in the quasiparticle spectra may be the result of a charge nematic (CN) phase stabilized by disorder in highly two-dimensional (2D) p-typ…
We systematically investigate the photoexcited (PE) quasi-particle (QP) relaxation and low-energy electronic structure in electron doped Ba(Fe_{1-x}Co_{x})_{2}As_{2} single crystals as a function of Co doping, 0<= x <=0.11. The evolution of the photoinduced reflectivity transients with $x$ proceeds with no abrupt changes. In the orthorhombic spin-density-wave (SDW) state a bottleneck associated with a partial charge-gap opening is detected, similar to previous results in different SDW iron-pnictides. The relative charge gap magnitude decreases with increasing x. In the superconducting (SC) sta…
Compton scattering provides invaluable information on the underlying Fermi surface (FS) and is a powerful tool complementary to angle-resolved photoemission spectroscopy and quantum oscillation measurements. Here we perform high-resolution Compton scattering measurements for La_{2-x}Sr_{x}CuO_{4} with x=0.08 (Tc=20K) at 300K and 150K, and image the momentum distribution function in the two-dimensional Brillouin zone. We find that the observed images cannot be reconciled with the conventional hole-like FS believed so far. Instead, our data imply that the FS is strongly deformed by the underlyin…
We study the crystal structure of the tetragonal iron selenide FeSe and its nematic phase transition to the low-temperature orthorhombic structure using synchrotron x-ray and neutron scattering analyzed in both real and reciprocal space. We show that in the local structure the orthorhombic distortion associated with the electronically driven nematic order is more pronounced at short length scales. It also survives up to temperatures above 90 K where reciprocal-space analysis suggests tetragonal symmetry. Additionally, the real-space pair distribution function analysis of the synchrotron x-ray …
The nematic-superconductor state is an example of a quantum liquid crystal that breaks gauge as well as rotation invariance. It was conjectured to exist in the pseudogap regime of the cuprates high $T_c$ superconductors. The nematic-superconductor state is characterized by two complex order parameters: one of them is related with superconductivity and the other one describes a nematic order. It supports two main classes of topological defects: half-vortices and disclinations. In this paper we present a Ginzburg-Landau approach to study the structure of these topological defects. Due to a geome…
The main features in iron-based superconductors would be (i) the orthorhombic transition accompanied by remarkable softening of shear modulus, (ii) high-Tc superconductivity close to the orthorhombic phase, and (iii) nematic transition in the tetragonal phase. In this paper, we present a unified explanation for them, based on the orbital fluctuation theory, considering both the e-ph and the Coulomb interaction. It is found that a small e-ph coupling constant ($λ~ 0.2$) is enough to produce large orbital (=charge quadrupole $O_{xz/yz}$) fluctuations, which causes the s-wave superconductivity wi…
We survey the use of spectroscopic imaging STM to probe the electronic structure of underdoped cuprates. Two distinct classes of electronic states are observed in both the d-wave superconducting (dSC) and the pseudogap (PG) phases. The first class consists of the dispersive Bogoliubov quasiparticle excitations of a homogeneous d-wave superconductor, existing below a lower energy scale E=Delta0. We find that the Bogoliubov quasiparticle interference signatures of delocalized Cooper pairing are restricted to a k-space arc which terminates near the lines connecting k=\pm(pi/a0,0) to k=\pm(pi/a0).…
Among all experimental observations of cuprate physics, the metal-insulator-crossover (MIC), seen in the pseudogap (PG) region of the temperature-doping phase diagram of copper-oxides under a strong magnetic field, when the superconductivity is suppressed, is most likely the most intriguing one. Since it was expected that the PG-normal state for these materials, as for conventional superconductors, is conducting. This MIC, revealed in such phenomena as heat conductivity downturn, anomalous Lorentz ratio, insulator resistivity boundary, nonlinear entropy, resistivity temperature upturn, insulat…
One of the key motivations for the development of atomically resolved spectroscopic imaging STM (SI-STM) has been to probe the electronic structure of cuprate high temperature superconductors. In both the d-wave superconducting (dSC) and the pseudogap (PG) phases of underdoped cuprates, two distinct classes of electronic states are observed using SI-STM. The first class consists of the dispersive Bogoliubov quasiparticles of a homogeneous d-wave superconductor. These are detected below a lower energy scale |E|=Δ0 and only upon a momentum space (k-space) arc which terminates near the lines conn…
We investigated the form of the orbital ordering in the electronic nematic phase of the Iron-based superconductors by applying a group theoretical analysis on a realistic five-band model. We find the orbital order can be either of the inter-orbital s-wave form or the intra-orbital d-wave form. From the comparison with existing ARPES measurements of band splitting, we find the orbital ordering in the 122 system is dominated by an intra-orbital d-wave component, while that in the 111 system is dominated by an inter-orbital s-wave component. We find both forms of orbital order are strongly entang…
We consider the lightly doped cuprates Y$_{0.97}$Ca$_{0.03}$BaCuO$_{6.05}$ and La$_{2-x}$Sr$_x$CuO$_4$ (with $x=0.02$,0.04), where the presence of a fluctuating nematic state has often been proposed as a precursor of the stripe (or, more generically, charge-density wave) phase, which sets in at higher doping. We phenomenologically assume a quantum critical character for the longitudinal and transverse nematic, and for the charge-ordering fluctuations, and investigate the effects of these fluctuations in Raman spectra. We find that the longitudinal nematic fluctuations peaked at zero transferre…
The key to unraveling the nature of high-temperature superconductivity (HTS) lies in resolving the enigma of the pseudogap state. The pseudogap state in the underdoped region is a distinct thermodynamic phase characterized by nematicity, temperature-quadratic resistive behavior, and magnetoelectric effects. Till present, a general description of the observed universal features of the pseudogap phase and their connection with HTS was lacking. The proposed work constructs a unifying effective field theory capturing all universal characteristics of HTS materials and explaining the observed phase …
In this supporting material for the main paper (the preceding submission), we show, in addition to the related information for the experiments, additional discussion that cannot fit in the main paper (due to the space constraint). It includes further discussion about our experimental observations, wider implications of our main findings with various reported candidates for the pseudogap order, and a simple mean-field argument that favors interpretations based on a finite-Q order (density wave) for the pseudogap seen by ARPES (whether "the pseudogap order" is a single order or contains multiple…
To capture various experimental results in the pseudogap regime of the underdoped cuprate superconductors for temperature $T<T^{*}$, we propose a four-component pair density wave (PDW) state, in which all components compete with each other. Without random field disorders (RFD), only one of the PDW components survives. If the RFD is included, this state could become phase separated and consist of short range PDW stripes, in which two PDW components coexist but differ in magnitudes, resulting in charge density waves (CDW) and a time-reversal symmetry breaking order, in the form of loop current, …
Topological states of matter are at the root of some of the most fascinating phenomena in condensed matter physics. Here we argue that skyrmions in the pseudo-spin space related to an emerging SU(2) symmetry enlighten many mysterious properties of the pseudogap phase in under-doped cuprates. We detail the role of the SU(2) symmetry in controlling the phase diagram of the cuprates, in particular how a cascade of phase transitions explains the arising of the pseudogap, superconducting and charge modulation phases seen at low temperature. We specify the structure of the charge modulations inside …
The Nernst coefficient of the cuprate superconductor YBa2Cu3Oy was recently shown to become strongly anisotropic within the basal plane when cooled below the pseudogap temperature T*, revealing that the pseudogap phase breaks the four-fold rotational symmetry of the CuO2 planes. Here we report on the evolution of this Nernst anisotropy at low temperature, once superconductivity is suppressed by a magnetic field. We find that the anisotropy drops rapidly below 80 K, to vanish in the T=0 limit. We show that this loss of anisotropy is due to the emergence of a small high-mobility electron-like po…
A spin density-wave quantum critical point (QCP) is the central organizing principle of organic, iron-pnictide, heavy-fermion and electron-doped cuprate superconductors. It accounts for the superconducting Tc dome, the non-Fermi-liquid resistivity, and the Fermi-surface reconstruction. Outside the magnetically ordered phase above the QCP, scattering and pairing decrease in parallel as the system moves away from the QCP. Here we argue that a similar scenario, based on a stripe-order QCP, is a central organizing principle of hole-doped cuprate superconductors. Key properties of Eu-LSCO, Nd-LSCO …
The coexistence and competition between superconductivity and electronic orders, such as spin or charge density waves, have been a central issue in high transition-temperature (${T_{\rm c}}$) superconductors. Unlike other iron-based superconductors, FeSe exhibits nematic ordering without magnetism whose relationship with its superconductivity remains unclear. More importantly, a pressure-induced fourfold increase of ${T_{\rm c}}$ has been reported, which poses a profound mystery. Here we report high-pressure magnetotransport measurements in FeSe up to $\sim9$ GPa, which uncover a hidden magnet…
