Unconventional Josephson junctions with topological Kondo insulator weak links
Xuecheng Ye, Jacob Cook, Erik D. Huemiller, Aaron D. K. Finck, Pouyan Ghaemi, Thomas Vojta, Vivekananda Adiga, Shanta R. Saha, Johnpierre Paglione, Cihan Kurter
Proximity-induced superconductivity in three dimensional (3D) topological insulators forms a new quantum phase of matter and accommodates exotic quasiparticles such as Majorana bound states. One of the biggest drawbacks of the commonly studied 3D topological insulators is the presence of conducting bulk that obscures both surface states and low energy bound states. Introducing superconductivity in topological Kondo insulators such as SmB$_6$, however, is promising due to their true insulating bulk at low temperatures. In this work, we develop an unconventional Josephson junction by coupling superconducting Nb leads to the surface states of a SmB$_6$ crystal. We observe a robust critical current at low temperatures that responds to the application of an out-of-plane magnetic field with significant deviations from usual Fraunhofer patterns. The appearance of Shaphiro steps under microwave radiation gives further evidence of a Josephson effect. Moreover, we explore the effects of Kondo breakdown in our devices, such as ferromagnetism at the surface and anomalous temperature dependence of supercurrent. Particularly, the magnetic diffraction patterns show an anomalous hysteresis with the field sweep direction suggesting the coexistence of magnetism with superconductivity at the SmB$_6$ surface. The experimental work will advance the current understanding of topologically nontrivial superconductors and emergent states associated with such unconventional superconducting phases.
We present the theoretical approach to study the unconventional Josephson junction (uJJ) made by putting the non-superconduncting strip on the top of superconducting strip. We work in the framework of the Ginzburg-Landau, Bogoliubov de Gennes and Usadel formalisms. We solve the non-linear parital differential equations numerically for few simple cases. We obtaine the eigenenergies of the uJJ by means of combined GL and BdGe method. cases. We predict the occurence of the physical effect, which we call the topological Meissner effect. Basing on the obtained results and current knowledge on Josep…
We have contacted single wall carbon nanotubes grown by chemical vapor deposition to superconducting Ti/Al/Ti electrodes. The device, we here report on is in the Kondo regime exhibiting a four-fold shell structure, where a clear signature of the superconducting electrodes is observed below the critical temperature. Multiple Andreev reflections are revealed by sub-gap structure and a narrow peak in the differential conductance around zero bias is seen depending on the shell filling. We interpret the peak as a proximity induced supercurrent and examine its interplay with Kondo resonances.
We measure the non-dissipative supercurrent in a single InAs self-assembled quantum dot (QD) coupled to superconducting leads. The QD occupation is both tuned by a back-gate electrode and lateral side-gate. The geometry of the side-gate allows tuning of the QD-lead tunnel coupling in a region of constant electron number with appropriate orbital state. Using the side-gate effect we study the competition between Kondo correlations and superconducting pairing on the QD, observing a decrease in the supercurrent when the Kondo temperature is reduced below the superconducting energy gap in qualitati…
We report on transport properties of Josephson junctions in hybrid superconducting-topological insulator devices, which show two striking departures from the common Josephson junction behavior: a characteristic energy that scales inversely with the width of the junction, and a low characteristic magnetic field for suppressing supercurrent. To explain these effects, we propose a phenomenological model which expands on the existing theory for topological insulator Josephson junctions.
We study a Majorana island coupled to a bulk superconductor via a Josephson junction and to multiple external normal leads. In the absence of the Josephson coupling, the system displays a topological Kondo state, which had been largely studied recently. However, we find that this state is unstable even to small Josephson coupling, which instead leads at low temperature $T$ to a new fixed point. Most interesting is the case of three external leads, forming a minimal electronic realization of the long sought two-channel Kondo effect. While the $T=0$ conductance corresponds to simple resonant And…
Josephson effect in junctions between unconventional superconductors is studied theoretically within the model describing the effects of interface roughness. The particularly important issue of applicability of the frequently used Sigrist-Rice formula for Josephson current in d-wave superconductor / insulator / d-wave superconductor junctions is addressed. We show that although the SR formula is not applicable in the ballistic case, it works well for rough interfaces when the diffusive normal metal regions exist between the d-wave superconductor and the insulator. It is shown that the SR appro…
We show that the non-local polarization response in a multimode circuit-QED setup, devised from a Cooper pair box coupled to a long chain of Josephson junctions, provides an alternative route to access the elusive Kondo screening cloud. For moderate circuit impedance, we compute analytically the universal lineshape for the decay of the charge susceptibility along the circuit, that relates to spatial entanglement between the qubit and its electromagnetic environment. At large circuit impedance, we numerically find further spatial correlations that are specific to a true many-body state.
We investigate the Josephson coupling between two superconductors mediated through an infinite U Anderson impurity, adapting a variational wavefunction approach which has proved successful for the Kondo model. Unlike the Kondo problem, however, a crossing of singlet and doublet state energies may be produced by varying the ratio of Kondo energy to superconducting gap, in agreement with recent work of Clerk and Ambegaokar. We construct the phase diagram for the junction and discuss properties of different phases. In addition, we find the singlet and doublet state energies within a slave boson m…
We study a spin-1/2 Kondo impurity coupled to an unconventional host in which the density of band states vanishes either precisely at (``gapless'' systems) or on some interval around the Fermi level (``gapped''systems). Despite an essentially nonlinear band dispersion, the system is proven to exhibit hidden integrability and is diagonalized exactly by the Bethe ansatz.
We apply a Gutzwiller-like variational technique to study Josephson conduction across a quantum dot with an odd number of electrons connected to two superconducting leads. Our method projects out all states on the dot but the Kondo singlet and is valid when Kondo correlations are dominant and no Andreev bound states localized at the dot are available for Kondo screening. In these conditions superconducting pairing is a competing effect and the junction is $π-$like, to optimize antiferromagnetic correlations on the dot. As the superconducting gap increases, the Josephson current also increases,…
Josephson effect in junctions of quasi one-dimensional triangular lattice superconductors is discussed, where the theoretical model corresponds to organic superconductors (TMTSF)_2PF_6. We assume the quarter-filling electron band and p, d and f wave like pairing symmetries in organic superconductors. To realize the electronic structures in organic superconductors, we introduce the asymmetric hopping integral, (t') among second nearest lattice sites. At t'=0, the Josephson current in the d wave symmetry saturates in low temperatures, whereas those in the p and the f wave symmetries show the low…
We study the Josephson current 0-$π$ transition of a quantum dot tuned to the Kondo regime. The physics can be quantitatively captured by the numerically exact continuous time quantum Monte Carlo method applied to the single-impurity Anderson model with BCS superconducting leads. For a comparison to an experiment the tunnel couplings are determined by fitting the normal-state linear conductance. Excellent agreement for the dependence of the critical Josephson current on the level energy is achieved. For increased tunnel couplings the Kondo scale becomes comparable to the superconducting gap an…
For certain orientations of Josephson junctions between two p_x-wave or two d-wave superconductors, the subgap Andreev bound states produce a 4pi-periodic relation between the Josephson current I and the phase difference phi: I ~ sin(phi/2). Consequently, the ac Josephson current has the fractional frequency eV/h, where V is the dc voltage. In the tunneling limit, the Josephson current is proportional to the first power (not square) of the electron tunneling amplitude. Thus, the Josephson current between unconventional superconductors is carried by single electrons, rather than by Cooper pairs…
A junction between two topological superconductors containing a pair of Majorana fermions exhibits a `fractional' Josephson effect, $4π$ periodic in the superconductors' phase difference. An additional fractional Josephson effect, however, arises when the Majoranas are spatially separated by a superconducting barrier. This new term gives rise to a set of Shapiro steps which are essentially absent without Majorana modes and therefore provides a unique signature for these exotic states.
Quantum fluctuations in an anharmonic superconducting circuit enable frequency conversion of individual incoming photons. This effect, linear in the photon beam intensity, leads to ramifications for the standard input-output circuit theory. We consider an extreme case of anharmonicity in which photons scatter off a small set of weak links within a Josephson junction array. We show that this quantum impurity displays Kondo physics and evaluate the elastic and inelastic photon scattering cross sections. These cross sections reveal many-body properties of the Kondo problem that are hard to access…
Inspired by the recent experimental evidence of antiferromagnetism and superconductivity coexistence in heavy fermion CeRhIn$_5$, we propose a fully microscopic approach based on the idea of real space pairing within the Anderson-Kondo lattice model. We present an overall phase diagram incorporating the emergence of a quantum critical point, where Kondo insulating (KI), antiferromagnetic (AF) and superconducting (SC) phases meet. We also obtain the Kondo insulating state with totally compensated magnetic moments as the parental state for the emerging SC phases. Furthermore, the coexistent (AF+…
Orbital degrees of freedom of a Cooper pair play an important role in the unconventional superconductivity. To elucidate the orbital effect in the Kondo problem, we investigated a single magnetic impurity coupled to Cooper pairs with a $p_x +i p_y$ ($d_{x^2-y^2}+id_{xy}$) symmetry using the numerical renormalization group method. It is found that the ground state is always a spin doublet. The analytical solution for the strong coupling limit explicitly shows that the orbital dynamics of the Cooper pair generates the spin 1/2 of the ground state.
A new type of Kondo effect peculiar to unconventional superconductors is studied theoretically by using the Wilson's numerical renormalization group method. In this case, an angular momentum of a Cooper pair plays an important role in the Kondo effect. It produces multichannel exchange couplings with a local spin. Here we focus on a $p_x +i p_y$-wave state which is a full gap system. The calculated impurity susceptibility shows that the local spin is almost quenched by the Kondo effect in the strong coupling region ($T_{\rm K}/Δ\to \infty$), while the ground state is always a spin doublet over…
Junction systems of odd-frequency (OF) superconductors are investigated based on a mean-field Hamiltonian formalism. One-dimensional two-channel Kondo lattice (TCKL) is taken as a concrete example of OF superconductors. Properties of normal and Andreev reflections are examined in a normal metal/superconductor junction. Unlike conventional superconductors, normal reflection is always present due to the normal self energy that necessarily appears in the present OF pairing state. The conductance reflects the difference between repulsive and attractive potentials located at the interface, which is…
We study large arrays of mesoscopic junctions between gapless superconductors where the tunneling processes of both, particle-hole and Cooper, pairs give rise to a strongly retarded effective action which, contrary to the standard case, can not be readily characterized in terms of a local Josephson energy. This complexity is expected to arise in, e.g., the grain boundary and c-axis junctions in layered high-T_c superconductors. A new representation for describing collective phenomena in this system is introduced, and its phase diagram is discussed, alongside the electrical conductivity.
The explanation of heavy-fermion superconductivity is a long-standing challenge to theory. It is commonly thought to be connected to non-local fluctuations of either spin or charge degrees of freedom and therefore of unconventional type. Here we present results for the Kondo-lattice model, a paradigmatic model to describe heavy-fermion compounds, obtained from dynamical mean-field theory which captures local correlation effects only. Unexpectedly, we find robust s-wave superconductivity in the heavy-fermion state. We argue that this novel type of pairing is tightly connected to the formation o…
The Kondo effect in superconductors is frequently investigated using the local quasiparticle density of states as sole bath characteristics, i.e., the presence of anomalous propagators is ignored. Here we point out that this treatment is exact for a number of situations, including point-like impurities in d-wave superconductors. We comment on recent investigations [M. Matsumoto and M. Koga, J. Phys. Soc. Jpn. 70, 2860 (2001), cond-mat/0011256, and Phys. Rev. B 65, 024508 (2002), cond-mat/0103053] which reached different conclusions: while their numerical results are likely correct, their inter…
The nature of unconventional superconductivity is intimately linked to the microscopic nature of the pairing interactions. In this work, motivated by cubic heavy fermion compounds with embedded multipolar moments, we theoretically investigate superconducting instabilities instigated by multipolar Kondo interactions. Employing multipolar fluctuations (mediated by RKKY interaction) coupled to conduction electrons via two-channel Kondo and novel multipolar Kondo interactions, we uncover a variety of superconducting states characterized by higher-angular momentum Cooper pairs, $J=0,1,2,3$. We demo…
We study theoretically the Josephson effect in junctions based on unconventional superconductors with diffusive barriers, using the quasiclassical Green's function formalism. Generalized boundary conditions at junction interfaces applicable to unconventional superconductors are derived by calculating a matrix current within the circuit transport theory. Applying these boundary conditions, we have calculated the Josephson current in structures with various pairing symmetries. A number of predictions are made: (a) nonmonotonic temperature dependence in d-wave superconductor/diffusive normal meta…
A mechanism of superconductivity is proposed for the Kondo lattice which has semi-metallic conduction bands with electron and hole Fermi surfaces. At high temperatures, the $f$ electron's localized spins/pseudospins are fluctuating between electron and hole Fermi surfaces to seek for a partner to couple with. This system tries to resolve this frustration at low temperatures and chooses to construct a quantum mechanically entangled state composed of the Kondo singlet with electron surface and that with hole surface, to break the U(1) gauge symmetry. The corresponding order parameter is given by…
Unconventional superconductivity and magnetism are intertwined on a microscopic level in a wide class of materials, including high-$T_c$ cuprates, iron pnictides, and heavy-fermion compounds. A new approach to this most fundamental and hotly debated subject focuses on the role of interactions between superconducting electrons and bosonic fluctuations at the interface between adjacent layers in heterostructures. A recent state-of-the-art molecular-beam-epitaxy technique has enabled us to fabricate superlattices consisting of different heavy-fermion compounds with atomic thickness. These Kondo s…
The transport properties of a topological Josephson junction fabricated from a magnetically doped topological insulator (TI) were investigated. The conductance spectra of the Nb/Fe-Bi$_2$Te$_2$Se/Nb junction below 1 K showed an unusual trident-shaped zero-bias conductance peak with a tiny peak width of $\sim$ 6 $μ$V. The central peak of the trident peak presents the dc-Josephson current, and the side peaks may reflect an induced unconventional Cooper pairing. Additionally, the critical currents followed inverse to temperature, which may also reflect the presence of an unconventional proximity …
The heavy quasiparticle bands in Kondo materials which originate in the hybridization of f- and conduction electrons exhibit numerous, sometimes coexisting, broken symmetry phases. Most notable are unconventional superconductivity, itinerant small moment antiferromagnetism and hidden order of higher order multipoles of f-electrons which all lead to a gapping of the heavy bands. In rare cases the chemical potential lies within the hybridization gap and the ground state is a Kondo semiconductor without ordering. The dynamical magnetic response of such gapped f-electron systems has been investiga…
To reveal the influence of the exchange interaction on the Josephson effect, the d.c. Josephson current in unconventional-superconductor / ferromagnet / unconventional-superconductor junctions is studied. When the two superconductors have d-wave symmetry, the Josephson current is drastically suppressed with the increase of the exchange interaction. On the other hand, when the two superconductors have different parities, e.g. s-wave and p-wave, an enhancement of the Josephson current is obtained with the increment of the exchange interaction due to the break-down of SU(2) symmetry in the spin s…
An array of resistively and capacitively shunted Josephson junctions with nonsinusoidal current-phase relation is considered for modelling the transition in high-T$_c$ superconductors. The emergence of higher harmonics, besides the simple sinusoid $I_{c}\sinϕ$, is expected for dominant \emph{d}-wave symmetry of the Cooper pairs, random distribution of potential drops, dirty grains, or nonstationary conditions. We show that additional cosine and sine terms act respectively by modulating the global resistance and by changing the Josephson coupling of the mixed superconductive-normal states. Firs…
We recently presented the first superconducting quantum interference device (SQUID) with single-walled carbon nanotube (CNT) Josephson junctions [1: J. P. Cleuziou, W. Wernsdorfer, V. Bouchiat, T. Ondarcuhu and M. Monthioux, Nature Nanotech. 1, 53, (2006).], http://www.nature.com/nnano/journal/v1/n1/pdf/nnano.2006.54.pdf . We showed that quantum confinement in each junction induces a discrete quantum dot (QD) energy level structure, which can be controlled with two lateral electrostatic gates. In addition, a backgate electrode can vary the transparency of the QD barriers, thus permitting to ch…
We present a theory for the Josephson effect in an unconventional superconductor / one-dimensional electron gas / unconventional superconductor (s/o/s) junction, where the Josephson current is carried by components injected perpendicular to the interface. When superconductors on both sides have triplet symmetries, the Josephson current is enhanced at low temperature due to the zero-energy states formed near the interface. Measuring Josephson current in this s/o/s junction, we can identify parity of the superconductor.
Current Induced Hidden States in Josephson Junctions
Harvard University（哈佛大学）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理研究所）；University of Basel（巴塞尔大学）；Weizmann Institute of Science（魏茨曼科学研究所）
The simultaneous co-existence and gate-tuneability of the superconducting (SC), magnetic and topological orders in magic angle twisted bilayer graphene (MATBG) open up entirely new possibilities for the creation of complex hybrid Josephson junctions (JJ). Here we report on the creation of gate-defined, magnetic Josephson junctions in MATBG, where the weak link is gate-tuned close to the correlated state at a moiré filling factor of ν=-2. A highly unconventional Fraunhofer pattern emerges, which is phase-shifted and asymmetric with respect to the current and magnetic field directions, and shows…
The formation of electron pairs is a prerequisite of superconductivity. The fermionic nature of electrons yields four classes of superconducting correlations with definite symmetry in spin, space and time. Here, we suggest double quantum dots coupled to conventional s-wave superconductors in the presence of inhomogeneous magnetic fields as a model system exhibiting unconventional pairing. Due to their small number of degrees of freedom, tunable by gate voltages, quantum-dot systems provide an ideal tool to gain fundamental insight in unconventional pairing. We propose two detection schemes for…
We study a singlet-triplet Josephson junction between a conventional s-wave superconductor and an unconventional p$_{\rm x}$-wave superconductor. The Andreev spectrum of the junction yields a spontaneous magnetization in equilibrium. This allows manipulating the occupation of the Andreev levels using an ac Zeeman field. The induced Rabi oscillations manifest themselves as a resonance in the current-phase relation. For a circularly polarized magnetic field, we find a spin selection rule, yielding Rabi oscillations only in a certain interval of the superconducting phase difference.
We develop a theoretical description of non-adiabatic Josephson dynamics in superconducting junctions containing low energy quasiparticles. Within this approach we investigate the effects of midgap states in junctions of unconventional d-wave superconductors. We identify a reentrance effect in the transition between thermal activation and macroscopic quantum tunneling, and connect this phenomenon to the experimental observations in Phys. Rev. Lett. 94, 087003 (2005). It is also shown that nonlinear Josephson dynamics can be defined by resonant interaction with midgap states reminiscent to nonl…
The unconventional Josephson coupling in a ferromagnetic weak link between d-wave superconductors is studied theoretically. For strong ferromagnetic barrier influence, the unconventional coupling, with ground state phase difference across the link $0<ϕ_{\rm gs}\leq π$, is obtained at small crystal misorientation of the superconducting electrodes, in contrast to the case of normal metal barrier, where it appears at large misorientations. In both cases, with decreasing temperature there is an increasing range of misorientations, where $ϕ_{\rm gs}$ varies continuously between 0 and $π$. When the …
We investigate phase-coherent thermal transport in Josephson junctions made from unconventional superconductors or superfluids. The thermal conductance is evaluated for one- and two-dimensional junctions within the Bogoliubov-de Gennes formalism. We analyze three different scenarios of junctions between two triplet superconductors with (i) helical pairing, (ii) unitary chiral and (iii) nonunitary chiral pairing. We find that the phase-dependent thermal conductance allows us to distinguish the different pairings and provides insight into the formation of topologically nontrivial Andreev bound s…
We extend the Keldysh formulation to quantum spin systems and derive exact equations of motion. This allows us to explore the dynamics of single spins and of ferromagnets when these are inserted between superconducting leads. Several new effects are reported. Chief amongst these are nutations of single S=1/2 spins in Josephson junctions. These nutations are triggered by the superconducting pairing correlations in the leads. Similarly, we find that on rather universal grounds, magnets display unconventional spin wave dynamics when placed in Josephson junctions. These lead to modifications in th…
Phenomenological Ginzburg-Landau theory is used to calculate the possible spontaneous vortex states that may exist at corner junctions of $d_{x^2-y^2}+ix$-wave, (where $x=s$ or $x=d_{xy}$) and s-wave superconductors. We study the magnetic flux and the critical current modulation with the junction orientation angle $θ$, the magnitude of the order parameter, and the magnetic field $H$. It is seen that the critical current $I_c$ versus the magnetic flux $Φ$ relation is symmetric / asymmetric for $x=d_{xy}/s$ when the orientation is exactly such that the lobes of the dominant $d_{x^2-y^2}$-wave or…
We analyze the impact of trap states in the oxide layer of a superconducting tunnel junctions, on the fluctuation of the Josephson critical current, thus on coherence in superconducting qubits. Two mechanisms are usually considered: the current blockage due to repulsion at the occupied trap states, and the noise from electrons hopping across a trap. We extend previous studies of noninteracting traps to the case where the traps have on-site electron repulsion inside one ballistic channel. The repulsion not only allows the appropriate temperature dependence of 1/f noise, but also is a control to…
We study the dynamics of a single spin embedded in the tunneling barrier between two superconductors. As a consequence of pair correlations in the superconducting state, the spin displays rich and unusual dynamics. To properly describe the time evolution of the spin we derive the effective Keldysh action for the spin. The superconducting correlations lead to an effective spin action, which is non-local in time, leading to unconventional precession. We further illustrate how the current is modulated by this novel spin dynamics.
We investigate the Josephson current in a graphene superconductor/normal/superconductor junction, where superconductivity is induced by means of the proximity effect from external contacts. We take into account the possibility of anisotropic pairing by also including singlet nearest-neighbor interactions, and investigate how the transport properties are affected by the symmetry of the superconducting order parameter. This corresponds to an extension of the usual on-site interaction assumption, which yields an isotropic s-wave order parameter near the Dirac points. Here, we employ a full numeri…
The predominant d-wave pairing symmetry in high temperature superconductors allows for a variety of current-phase relations in Josephson junctions, which is to a certain degree fabrication controlled. In this letter we report on direct experimental observations of the effects of a non-sinusoidal current-phase dependence in YBCO dc-SQUIDs, which agree with the theoretical description of the system.
We address the dynamics of a single spin embedded in the tunneling barrier between two superconductors. As a consequence of pair correlations in the superconducting state, the spin displays a rich and unusual dynamics. To properly describe the time evolution of the spin we find the generalized Wess-Zumino-Witten-Novikov term in the effective action for the spin on the Keldysh contour. The superconducting correlations lead to an effective spin action which is non-local in time leading to unconventional precessions. Our predictions might be directly tested for macroscopic spin clusters.
Thermodynamics and transport properties of resistance-shunted Josephson junctions are studied theoretically in the tight-binding limit E_C/E_J<<1, where E_C and E_J are a charging energy and a Josephson coupling energy respectively. Based on a phenomenological harmonic-oscillator model, weak coupling region K=R_Q/R<<1 is analytically studied, where R and R_Q=h/(2e)^2 are a shunted resistance and the quantum resistance. In addition to the effective bandwidth, we find that this multi-level system genuinely has a novel crossover at lower energy below which the density of states becomes strongly d…
We investigate the effect of unconventional density wave (UDW) condensate on an Anderson impurity using large-N technique at T=0. In accordance with previous treatments of a Kondo impurity in pseudogap phases, we find that Kondo effect occurs only in a certain range of parameters. The f-electron density of states reflects the influence of UDW at low energies and around the maximum of the density wave gap. The static spin susceptibility diverges at the critical coupling, indicating the transition from strong to weak coupling. In the dynamic spin susceptibility an additional peak appears showing…
