Antiferromagnets and compensated ferrimagnets offer opportunities to investigate spin dynamics in the 'terahertz gap' because their resonance modes lie in the 0.3 THz to 3 THz range. Despite some inherent advantages when compared to ferromagnets, these materials have not been extensively studied due to difficulties in exciting and detecting the high-frequency spin dynamics, especially in thin films. Here we show that spin-obit torque in a single layer of the highly spin-polarized compensated ferrimagnet Mn2RuxGa is remarkably efficient at generating spin-orbit fields μ_0H_eff, which approach 0.1x10-10 T m2/A in the low-current density limit -- almost a thousand times the Oersted field, and one to two orders of magnitude greater than the effective fields in heavy metal/ferromagnet bilayers. From an analysis of the harmonic Hall effect which takes account of the thermal contributions from the anomalous Nernst effect, we show that the antidamping component of the spin-orbit torque is sufficient to sustain self-oscillation. Our study demonstrates that spin electronics has the potential to underpin energy-frugal, chip-based solutions to the problem of ultra high-speed information transfer.
The spin-orbit torque switching of ferrimagnetic Gd$_x$(Fe$_{90}$Co$_{10}$)$_{100-x}$ films was studied for both transition metal (TM)-rich and rare earth (RE)-rich configurations. The spin-orbit torque driven magnetization switching follows the same handedness in TM-rich and RE-rich samples with respect to the total magnetization, but the handedness of the switching is reversed with respect to the TM magnetization. This indicates that the sign of the spin-orbit-torque-driven magnetic switching follows the total magnetization, although transport based techniques such as anomalous Hall effect a…
We use micro-focus Brillouin light scattering spectroscopy to study the effects of spin-orbit torque on thermal spin waves in almost angular-momentum compensated ferrimagnetic CoGd alloy films. The spin-orbit torque is produced by the electric current flowing in the Pt layer adjacent to CoGd. Both the ferromagnetic and the exchange modes are detected in our measurements. The intensity and the linewidth of the ferromagnetic mode are modified by the spin-orbit torque. In contrast, the properties of the exchange mode are unaffected by the spin-orbit torque. We also find that the frequencies and t…
So far, studies of spin-orbit torques (SOT) in ferromagnets with perpendicular magnetic anisotropy (PMA) have been restricted to ultra thin samples, while a systematic study of its thickness dependence is still lacking in literature. In this article we discuss the thickness dependence of SOT in GdFeCo samples with bulk PMA. We show that the effective SOT fields are decreasing inversely as a function of thickness while the spin-Hall angle stays constant, as expected from angular momentum conservation. Further we show that even 30nm thick GdFeCo samples can be switched with SOT. This has importa…
Magnetic skyrmionium is a skyrmion-like spin texture with nanoscale size and high mobility. It is a topologically trivial but dynamically stable structure, which can be used as a non-volatile information carrier for next-generation spintronic storage and computing devices. Here, we study the dynamics of a skyrmionium driven by the spin torque in a ferrimagnetic nanotrack. It is found that the direction of motion is jointly determined by the internal configuration of a skyrmionium and the spin polarization vector. Besides, the deformation of a skyrmionium induced by the intrinsic skyrmion Hall …
A theory of magnetization dynamics in ferrimagnetic materials with antiparallel aligned spin sub-lattices under action of spin-transfer torques (STT) is developed. We consider magnetization dynamics in GdFeCo layers in two cases of magnetic anisotropy: easy plane and easy axis. We demonstrate that, (i) for the easy plane anisotropy the precession of the Néel vector is conical and the cone angle depends on the STT strength and the value of spin non-compensation, while the frequency of precession can reach sub-THz frequencies; (ii) for the easy axis anisotropy two regimes are possible: determini…
The manipulation of mesoscale domain wall phenomena has emerged as a powerful strategy for designing ferroelectric responses in functional devices, but its full potential has not yet been realized in the field of magnetism. We show that mechanically strained samples of Mn$_3$O$_4$ and MnV$_2$O$_4$ exhibit a stripe-like patterning of the bulk magnetization below known magnetostructural transitions, similar to the structural domains reported in ferroelectric materials. Building off our previous magnetic force microscopy data, we use small angle neutron scattering to show that these patterns exte…
Current-induced spin-orbit torques (SOTs) are of interest for fast and energy-efficient manipulation of magnetic order in spintronic devices. To be deterministic, however, switching of perpendicularly magnetized materials by SOT requires a mechanism for in-plane symmetry breaking. Existing methods to do so involve the application of an in-plane bias magnetic field, or incorporation of in-plane structural asymmetry in the device, both of which can be difficult to implement in practical applications. Here, we reported bias-field-free SOT switching in a single perpendicular CoTb layer with an eng…
The fascinating high-speed field-driven domain wall (DW) motion along ferrimagnetic nanowires near the angular momentum compensation point (AMCP) is solved based on the generic ferrimagnetic dynamics. The physics of the absences of precessional torque and infinite high Walker breakdown field at the AMCP is proved under general conditions. Based on the energy conservation principle, an almost exact DW velocity formula, valid beyond the Walker breakdown field, is obtained. Our results agree with all existing experiments and simulations. This theory provides useful guidances to DW manipulation.
It has been predicted that transverse spin current can propagate coherently (without dephasing) over a long distance in antiferromagnetically ordered metals. Here, we estimate the dephasing length of transverse spin current in ferrimagnetic CoGd alloys by spin pumping measurements across the compensation point. A modified drift-diffusion model, which accounts for spin-current transmission through the ferrimagnet, reveals that the dephasing length is about 4-5 times longer in nearly compensated CoGd than in ferromagnetic metals. This finding suggests that antiferromagnetic order can mitigate sp…
Non-uniform magnetic structures produce emergent electromagnetic phenomena such as the topological Hall effect and the spin-motive force (SMF). The experimental reports on the SMF, however, are very few and the relationship between the SMF and material parameters is still unclear. In this study, we investigated the SMF in ferrimagnetic GdFeCo alloy films using the spin-torque-induced ferromagnetic resonance method and clarified the relationship. The amplitude of the detected SMF becomes larger than that of the transition metal alloy FeCo by the Gd doping and reaches the maximum near a Gd compo…
The discovery of spin torque transfer (STT) has lead to a significant advance in the development of spintronic devices. Novel structures and materials have been studied in order to improve the performance of the magnetic tunnel junctions (MTJs) performances and understand the fundamental physics in spin torque transfer. The adiabatic spin torque effect, which is due to the spatial non-uniformity of magnetic properties, has been predicted in theory and demonstrated experimentally in magnetic nanowires. However, this important spin torque has been rarely concerned in the magnetic tunnel junction…
We report on the combination of current-induced spin-orbit torques and giant magnetoresistance in a single device to achieve all-electrical write and read out of the magnetization. The device consists of perpendicularly magnetized TbCo and Co layers separated by a Pt or Cu spacer. Current injection through such layers exerts spin-orbit torques and switches the magnetization of the Co layer while the TbCo magnetization remains fixed. Subsequent current injection of lower amplitude senses the relative orientation of the magnetization of the Co and TbCo layers, which results in two distinct resis…
We report a giant spin Hall effect (SHE) in β-W thin films. Using spin torque induced ferromagnetic resonance with a β-W/CoFeB bilayer microstrip we determine the spin Hall angle to be |θ|=0.30\pm0.02, large enough for an in-plane current to efficiently reverse the orientation of an in-plane magnetized CoFeB free layer of a nanoscale magnetic tunnel junction adjacent to a thin β-W layer. From switching data obtained with such 3-terminal devices we independently determine |θ|=0.33\pm0.06. We also report variation of the spin Hall switching efficiency with W layers of different resistivities and…
We report a giant spin Hall effect (SHE) in β-Ta that generates spin currents intense enough to induce efficient spin-transfer-torque switching of ferromagnets, thereby providing a new approach for controlling magnetic devices that can be superior to existing technologies. We quantify this SHE by three independent methods and demonstrate spin-torque (ST) switching of both out-of-plane and in-plane magnetized layers. We implement a three-terminal device that utilizes current passing through a low impedance Ta-ferromagnet bilayer to effect switching of a nanomagnet, with a higher-impedance magne…
We report on first-principles calculations of spin-transfer torque (STT) in epitaxial magnetic tunnel junctions (MTJs) based on ferrimagnetic tetragonal Mn$_3$Ga electrodes, both as analyzer in an Fe/MgO stack, and also in an analogous stack with a second Mn$_3$Ga electrode (instead of Fe) as polarizer. Solving the ballistic transport problem (NEGF + DFT) for the nonequilibrium spin density in a scattering region extended to over 7.6 nm into the Mn$_3$Ga electrode, we find long-range spatial oscillations of the STT decaying on a length scale of a few tens of angstroms, both in the linear respo…
Spintronics provides an efficient platform for realizing non-volatile memory and logic devices. In these systems, data is stored in the magnetization of magnetic materials, and magnetization is switched in the writing process. In conventional spintronic devices, ferromagnetic materials are used which have a magnetization dynamics timescale of around the nanoseconds, setting a limit for the switching speed. Increasing the magnetization switching speed has been one of the challenges in spintronic research. In this work we take advantage of the ultrafast magnetization dynamics in ferrimagnetic ma…
We report on first-principles spin-polarised quantum transport calculations (from NEGF+DFT) in MgO-spaced magnetic tunnel junctions (MTJs) based on two different Mn-based Heusler ferrimagnetic metals, namely Mn$_3$Al and Mn$_3$Ga in their tetragonal DO$_{22}$ phase. The former is a fully compensated half-metallic ferrimagnet, while the latter is a low-moment high-spin-polarisation ferrimagnet, both with a small lattice mismatch from MgO. In identical symmetric and asymmetric interface reconstructions across a 3-monolayer thick MgO barrier for both ferrimagets, the linear response (low-voltage)…
Modern spintronics relies on the generation of spin currents through spin-orbit coupling. The spin-current generation has been believed to be triggered by current-induced orbital dynamics, which governs the angular momentum transfer from the lattice to the electrons in solids. The fundamental role of the orbital response in the angular momentum dynamics suggests the importance of the orbital counterpart of spin currents: orbital currents. However, evidence for its existence has been elusive. Here, we demonstrate the generation of giant orbital currents and uncover fundamental features of the o…
A microscopic calculation is presented for the spin-transfer torques (STT) and damping torques in metallic antiferromagnets (AF). It is found that the sign of the STT is opposite to that in ferromagnets because of the AF transport character, and the current-to-STT conversion factor is enhanced near the AF gap edge. The dissipative torque parameter $β_n$ and the damping parameter $α_n$ for the Néel vector arise from spin relaxation of electrons. Physical consequences are demonstrated for the AF domain wall motion using collective coordinates, and some similarities to the ferromagnetic case are …
Harnessing Native Chromium Oxidation for Giant Orbital Torque and Field-Free Magnetization Switching in NiFe/Cr Bilayers
Indian Institute of Technology Ropar（印度理工学院罗帕尔分校）；Indian Institute of Technology Mandi（印度理工学院曼迪分校）；Indian Institute of Technology Bhubaneswar（印度理工学院布巴内斯瓦尔分校）；Virginia Commonwealth University（弗吉尼亚联邦大学）；Jaypee Institute of Information Technology（贾伊皮信息技术学院）
Control of magnetic domain wall movement by the spin-polarized current looks promising for creation of a new generation of magnetic memory devices. A necessary condition for this is the domain wall shift by a low-density current. Here I show that a strongly anisotropic exchange interaction between mobile heavy holes and localized magnetic moments enormously increases the current-induced torque on the domain wall as compared to systems with isotropic exchange. This enables one to control the domain wall motion by current density 10^4 A/cm^2 in ferromagnet/semiconductor hybrids. The experimental…
The current-driven domain wall dynamics along ferrimagnetic systems are here theoretically analyzed as a function of the temperature by means of micromagnetic simulations and a one dimensional model. Contrarily to conventional effective approaches, our model takes into account the two coupled ferromagnetic sublattices forming the ferrimagnetic system. Although the model is suitable for systems with asymmetric exchange interaction and spin-orbit coupling effects due to adjacent heavy metal layers, we here focus our attention on the case of single-layer ferrimagnetic strips where domain walls ad…
Spin waves in ferrimagnetic yttrium iron garnet (YIG) films with ultralow magnetic damping are relevant for magnon-based spintronics and low-power wave-like computing. The excitation frequency of spin waves in YIG is rather low in weak external magnetic fields because of its small saturation magnetization, which limits the potential of YIG films for high-frequency applications. Here, we demonstrate how exchange-coupling to a CoFeB film enables efficient excitation of high-frequency perpendicular standing spin waves (PSSWs) in nanometer-thick (80 nm and 295 nm) YIG films using uniform microwave…
Due to its transverse nature, spin Hall effects (SHE) provide the possibility to excite and detect spin currents and magnetization dynamics even in magnetic insulators. Magnetic insulators are outstanding materials for the investigation of nonlinear phenomena and for novel low power spintronics applications because of their extremely low Gilbert damping. Here, we report on the direct imaging of electrically driven spin-torque ferromagnetic resonance (ST-FMR) in the ferrimagnetic insulator Y$_3$Fe$_5$O$_{12}$ based on the excitation and detection by SHEs. The driven spin dynamics in Y$_3$Fe$_5$…
The interface between a ferro-/ferrimagnetic insulator and a normal metal can support spin currents polarized collinear with and perpendicular to the magnetization direction. The flow of angular momentum perpendicular to the magnetization direction ("transverse" spin current) takes place via spin torque and spin pumping. The flow of angular momentum collinear with the magnetization ("longitudinal" spin current) requires the excitation of magnons. In this article we extend the existing theory of longitudinal spin transport [Bender and Tserkovnyak, Phys. Rev. B 91, 140402(R) (2015)] in the zero-…
Magnetic skyrmions are compact chiral spin textures that exhibit a rich variety of topological phenomena and hold potential for developing high-density memory devices and novel computing schemes driven by spin currents. Here, we demonstrate room temperature interfacial stabilization and current-driven control of skyrmion bubbles in the ferrimagnetic insulator Tm3Fe5O12 (TmIG) coupled to Pt. We track the current-induced motion of individual skyrmion bubbles. The ferrimagnetic order of the crystal together with the interplay of spin-orbit torques and pinning determine the skyrmion dynamics in Tm…
Magnetic damping is a key metric for emerging technologies based on magnetic nanoparticles, such as spin torque memory and high-resolution biomagnetic imaging. Despite its importance, understanding of magnetic dissipation in nanoscale ferromagnets remains elusive, and the damping is often treated as a phenomenological constant. Here we report the discovery of a giant frequency-dependent nonlinear damping that strongly alters the response of a nanoscale ferromagnet to spin torque and microwave magnetic field. This novel damping mechanism originates from three-magnon scattering that is strongly …
We study the Casimir torque between two metallic one-dimensional gratings rotated by an angle $θ$ with respect to each other. We find that, for infinitely extended gratings, the Casimir energy is anomalously discontinuous at $θ=0$, due to a critical zero-order geometric transition between a 2D- and a 1D-periodic system. This transition is a peculiarity of the grating geometry and does not exist for intrinsically anisotropic materials. As a remarkable practical consequence, for finite-size gratings, the torque per area can reach extremely large values, increasing without bounds with the size of…
The ability of spin-orbit interactions to convert charge current into spin current, most often in the bulk of heavy metal thin films, has been the hallmark of spintronics in the last decade. In this study, we demonstrate how the insertion of light metal element interface profoundly affects both the nature of spin-orbit torque and its efficiency in terms of damping-like ($H_{\text{DL}}$) and field-like ($H_{\text{FL}}$) effective fields in ultrathin Co ferromagnet. Indeed, we measure unexpectedly large $H_{\text{FL}}$/$H_{\text{DL}}$ ratio ($\sim$2.5) upon inserting a 1.4 nm thin Al layer in Pt…
Spin-orbit torque nano-oscillators based on bilayers of ferromagnetic (FM) and nonmagnetic (NM) metals are ultra-compact current-controlled microwave signal sources. They serve as a convenient testbed for studies of spin-orbit torque physics and are attractive for practical applications such as microwave assisted magnetic recording, neuromorphic computing, and chip-to-chip wireless communications. However, a major drawback of these devices is low output microwave power arising from the relatively small anisotropic magnetoresistance (AMR) of the FM layer. Here we experimentally show that the ou…
In cavity quantum electrodynamics, the multiple reflections of a photon between two mirrors defining a cavity is exploited to enhance the light-coupling of an intra-cavity atom. We show that this paradigm for enhancing the interaction of a flying particle with a localized object can be generalized to spintronics based on van der Waals 2D magnets. Upon tunneling through a magnetic bilayer, we find the spin transfer torques per electron incidence can become orders of magnitude larger than $\hbar/2$, made possible by electron's multi-reflection path through the ferromagnetic monolayers as an inte…
Spin-polarized charge-currents induce magnetic tunnel junction (MTJ) switching by virtue of spin-transfer-torque (STT). Recently, by taking advantage of the spin dependent thermoelectric properties of magnetic materials, novel means of generating spin-currents from temperature gradients, and their associated thermal spin torques (TSTs) have been proposed, but so far these TSTs have not been large enough to influence MTJ switching. Here we demonstrate significant TSTs in MTJs by generating large temperature gradients across ultrathin MgO tunnel barriers that considerably affect the switching fi…
Topological insulators (TIs) with spin momentum locked topological surface states (TSS) are expected to exhibit a giant spin-orbit torque (SOT) in the TI/ferromagnet systems. To date, the TI SOT driven magnetization switching is solely reported in a Cr doped TI at 1.9 K. Here, we directly show giant SOT driven magnetization switching in a Bi2Se3/NiFe heterostructure at room temperature captured using a magneto-optic Kerr effect microscope. We identify a large charge to spin conversion efficiency of ~1-1.75 in the thin TI films, where the TSS is dominant. In addition, we find the current densit…
The orbital Hall effect provides an alternative means to the spin Hall effect to convert a charge current into a flow of angular momentum. Recently, compelling signatures of orbital Hall effects have been identified in 3d transition metals. Here, we report a systematic study of the generation, transmission, and conversion of orbital currents in heterostructures comprising 3d, 5d, and 4f metals. We show that the orbital Hall conductivity of Cr reaches giant values of the order of 5*10^5 Ohm^{-1} m^{-1} and that Pt presents a strong orbital Hall effect in addition to the spin Hall effect. Measur…
The spin-orbit torque (SOT) arising from materials with large spin-orbit coupling promises a path for ultra-low power and fast magnetic-based storage and computational devices. We investigated the SOT from magnetron-sputtered BixSe(1-x) thin films in BixSe(1-x)/CoFeB heterostructures by using a dc planar Hall method. Remarkably, the spin Hall angle (SHA) was found to be as large as 18.83, which is the largest ever reported at room temperature (RT). Moreover, switching of a perpendicular CoFeB multilayer using SOT from the BixSe(1-x) has been observed with the lowest-ever switching current dens…
Heavy metal/ferromagnet interfaces feature emergent spin-orbit effects absent in the bulk materials. Because of their inherent strong coupling between spin, charge and orbital degrees of freedom, such systems provide a platform for technologically sought-after spin-orbit torques (SOTs). However, the microscopic origin of purely interfacial antidamping SOT, especially in the ultimate atomically thin limit, has proven elusive. Here, using two-dimensional (2D) van der Waals materials as a testbed for interfacial phenomena, we address this problem by means of a microscopic framework accounting for…
Efficient generation of spin-orbit torques (SOTs) is central for the exciting field of spin-orbitronics. Platinum, the archetypal spin Hall material, has the potential to be an outstanding provider for spin-orbit torques due to its giant spin Hall conductivity, low resistivity, high stabilities, and the ability to be compatible with CMOS circuits. However, pure clean-limit Pt with low resistivity still provides a low damping-like spin-orbit torque efficiency, which limits its practical applications. The efficiency of spin-orbit torque in Pt-based magnetic heterostructures can be improved consi…
In this letter, we show that Giant Spin Hall Effect (GSHE) MRAM can enable better energy- delay and voltage performance than traditional MTJ based spin torque devices at scaled nanomagnet dimensions (10-30 nm). Firstly, we derive the effect of dimensional scaling on spin injection efficiency, voltage-delay and energy-delay of spin torque switching using MTJs and GSHE and identify the optimum electrode geometry for low operating voltage (<0.1 V), high speed (>10 GHz) operation. We show that effective spin injection efficiency >100 % can be obtained using optimum spin hall electrode thickness fo…
Two-dimensional electron gas (2DEG) formed at the interface between SrTiO3 (STO) and LaAlO3 (LAO) insulating layer is supposed to possess strong Rashba spin-orbit coupling. To date, the inverse Edelstein effect (i.e. spin-to-charge conversion) in the 2DEG layer is reported. However, the direct effect of charge-to-spin conversion, an essential ingredient for spintronic devices in a current induced spin-orbit torque scheme, has not been demonstrated yet. Here we show, for the first time, a highly efficient spin generation with the efficiency of ~6.3 in the STO/LAO/CoFeB structure at room tempera…
We investigate ferrimagnetic domain wall dynamics induced by circularly polarized spin waves theoretically and numerically. We find that the direction of domain wall motion depends on both the circular polarization of spin waves and the sign of net spin density of ferrimagnet. Below the angular momentum compensation point, left- (right-) circularly polarized spin waves push a domain wall towards (away from) the spin-wave source. Above the angular momentum compensation point, on the other hand, the direction of domain wall motion is reversed. This bidirectional motion originates from the fact t…
Microwave detectors based on the spin-transfer torque diode effect are among the key emerging spintronic devices. By utilizing the spin of electrons in addition to charge, they have the potential to overcome the theoretical performance limits of their semiconductor (Schottky) counterparts, which cannot operate at low input power. Here, we demonstrate nanoscale microwave detectors exhibiting record-high detection sensitivity of 75400 mV mW$^{-1}$ at room temperature, without any external bias fields, for input microwave power down to 10 nW. This sensitivity is 20x and 6x larger than state-of-th…
Despite their great promise for providing a pathway for very efficient and fast manipulation of magnetization at the nanoscale, spin-orbit torque (SOT) operations are currently energy inefficient due to a low damping-like SOT efficiency per unit current bias, and/or the very high resistivity of the spin Hall materials. Here, we report an advantageous spin Hall material, Pd1-xPtx, which combines a low resistivity with a giant spin Hall effect as evidenced through the use of three independent SOT ferromagnetic detectors. The optimal Pd0.25Pt0.75 alloy has a giant internal spin Hall ratio of >0.4…
The ferrimagnets, such as GdxFeCo(1-x), can produce ultrafast magnetic switching and oscillation due to the strong exchange field. The two-sublattices macrospin model has been widely used to explain the experimental results. However, it fails in describing the spatial nonuniform magnetic dynamics which gives rises to many important phenomenons such as the domain walls and skyrmions. Here we develop the two-dimensional atomistic model and provide a torque analysis method to study the ferrimagnetic oscillation. Under the spin-transfer torque, the magnetization oscillates in the exchange mode or …
One fundamental obstacle to efficient ferromagnetic spintronics is magnetic precession, which intrinsically limits the dynamics of magnetic textures, We demonstrate that the domain wall precession fully vanishes with a record mobility when the net angular momentum is compensated (TAC) in DWs driven by spin-orbit torque in a ferrimagnetic GdFeCo/Pt track. We use transverse in-plane fields to reveal the internal structure of DWs and provide a robust and parameter-free measurement of TAC. Our results highlight the mechanism of faster and more efficient dynamics in materials with multiple spin lat…
