arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 1901.07580cond-mat.mes-hallcond-mat.mtrl-sci
收藏

时间分辨光电发射测量中的相干激子量子拍

Coherent Excitonic Quantum Beats in Time-Resolved Photoemission Measurements

Avinash Rustagi, Alexander F. Kemper

摘要:

通过超快激光脉冲对材料的相干激发在时间分辨光电发射测量中可以具有有趣的、可观察的动力学。超快抽运脉冲的宽光谱宽度可以相干激发多个激子能级。当这种相干激发态通过光电子能谱探测时,不同激子能级的偏振之间的干涉可以导致可观察到的相干激子拍频。本文提出了计算相干激发激子态的时间和角度分辨光电子能谱的理论方法。随后,我们应用我们的形式主义一个简单的模型例子类氢激子能级,以确定控制量子拍频的依赖关系。我们的研究结果表明,相干量子激子拍频的最明显的效果是看到中间的激发激子能级和泵浦脉冲的中心能量提供这种效果的可调谐性。

英文摘要:

Coherent excitation of materials via ultrafast laser pulses can have interesting, observable dynamics in time-resolved photoemission measurements. The broad spectral width of ultrafast pump pulses can coherently excite multiple exciton energy levels. When such coherently excited states are probed by means of photoemission spectroscopy, interference between the polarization of different exciton levels can lead to observable coherent exciton beats. Here, we present the theoretical formalism for evaluating the Time- and Angle- Resolved Photoemission Spectra (tr-ARPES) arising from the coherently excited exciton states. We subsequently apply our formalism to a simple model example of hydrogenic exciton energy levels to identify the dependencies that control the quantum beats. Our findings indicate that the most pronounced effect of coherent quantum excitonic beats is seen midway between the excited exciton energy levels and the central energy of the pump pulse provides tunability of this effect.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

↑