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arXiv 1809.05565cond-mat.softcond-mat.dis-nncond-mat.mtrl-scicond-mat.stat-mech
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广义随机组织模型的超一致性

Hyperuniformity of generalized random organization models

Zheng Ma, Salvatore Torquato

摘要:

对单分散球形颗粒的随机组织模型的研究表明,当系统经历吸收相变到临界状态时,可以达到超均匀状态。在这里,我们调查到什么程度超均匀性被保存时,该模型被推广到粒子的尺寸分布和/或非球形形状。我们首先检查二进制磁盘在两个维度,并证明其临界状态是超均匀的两相介质,但不是超均匀的,也不是multihyperuniform的粒子质心形成的点图案。我们通过研究具有连续尺寸分布的颗粒进一步证实了我们研究结果的普遍性。最后,为了研究旋转自由度的影响,我们将我们的模型扩展到非圆形粒子,即具有各种纵横比的硬矩形,包括硬针极限。虽然这些系统只表现出短程取向秩序,超均匀性仍然保留。我们的分析表明,粒子的“质量”的重新分配,而不是粒子的质心是这个动力学过程的核心。考虑广义随机组织模型的“活性体积分数”可能有助于解决它们属于哪个普适类,从而可能导致对吸收态模型更深入的理论理解。我们的研究结果表明,随机组织的一般粒子系统可以成为一种鲁棒的方法,通过不同的粒子尺寸和形状分布调整结构来制造多种超均匀物质态。这反过来又潜在地使得能够产生具有期望的光学、传输和机械特性的多功能超均匀材料。

英文摘要:

Studies of random organization models of monodisperse spherical particles have shown that a hyperuniform state is achievable when the system goes through an absorbing phase transition to a critical state. Here we investigate to what extent hyperuniformity is preserved when the model is generalized to particles with a size distribution and/or nonspherical shapes. We begin by examining binary disks in two dimensions and demonstrate that their critical states are hyperuniform as two-phase media, but not hyperuniform nor multihyperuniform as point patterns formed by the particle centroids. We further confirm the generality of our findings by studying particles with a continuous size distribution. Finally, to study the effect of rotational degrees of freedom, we extend our model to noncircular particles, namely, hard rectangles with various aspect ratios, including the hard-needle limit. Although these systems exhibit only short-range orientational order, hyperuniformity is still preserved. Our analysis reveals that the redistribution of the "mass" of the particles rather than the particle centroids is central to this dynamical process. The consideration of the "active volume fraction" of generalized random organization models may help to resolve which universality class they belong to and hence may lead to a deeper theoretical understanding of absorbing-state models. Our results suggest that general particle systems subject to random organization can be a robust way to fabricate a wide class of hyperuniform states of matter by tuning the structures via different particle-size and -shape distributions. This in turn potentially enables the creation of multifunctional hyperuniform materials with desirable optical, transport, and mechanical properties.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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