Pillar microcavities are excellent light-matter interfaces providing an electromagnetic confinement in small mode volumes with high quality factors. They also allow the efficient injection and extraction of photons, into and from the cavity, with potentially near-unity input and output-coupling efficiencies. Optimizing the input and output coupling is essential, in particular, in the development of solid-state quantum networks where artificial atoms are manipulated with single incoming photons. Here we propose a technique to accurately measure input and output coupling efficiencies using polarization tomography of the light reflected by the cavity. We use the residual birefringence of pillar microcavities to distinguish the light coupled to the cavity from the uncoupled light: the former participates to rotating the polarization of the reflected beam, while the latter decreases the polarization purity. Applying this technique to a micropillar cavity, we measure a $53 \pm2 \% $ output coupling and a $96 \pm 1\%$ input coupling with unprecedented precision.
The relaxation of a quantum field stored in a high-$Q$ superconducting cavity is monitored by non-resonant Rydberg atoms. The field, subjected to repetitive quantum non-demolition (QND) photon counting, undergoes jumps between photon number states. We select ensembles of field realizations evolving from a given Fock state and reconstruct the subsequent evolution of their photon number distributions. We realize in this way a tomography of the photon number relaxation process yielding all the jump rates between Fock states. The damping rates of the $n$ photon states ($0\leq n \leq 7$) are found …
A polarization degenerate microcavity containing charge-controlled quantum dots (QDs) enables equal coupling of all polarization degrees of freedom of light to the cavity QED system, which we explore through resonant laser spectroscopy. We first measure interference of the two fine-split neutral QD transitions and find very good agreement of this V-type three-level system with a coherent polarization dependent cavity QED model. We also study a charged QD that suffers from decoherence, and find also in this case that availability of the full polarization degrees of freedom is crucial to reveal …
We study broadband polarization entangled states generated within the line width of type-II Spontaneous Parametric Down Conversion (SPDC). Applying a complete quantum polarization tomography protocol at arbitrary combination of frequency and angular sideband modes we reveal a complex structure of non-degenerate non-collinear polarization entangled states generated within the SPDC line width. It is demonstrated that simultaneous compensation of longitudinal and transverse walk off leads to homogenizing the structure of polarization entanglement.
The polarization properties of macroscopic Bell states are characterized using three-dimensional quantum polarization tomography. This method utilizes three-dimensional inverse Radon transform to reconstruct the polarization quasiprobability distribution function of a state from the probability distributions measured for various Stokes observables. The reconstructed 3D distributions obtained for the macroscopic Bell states are compared with those obtained for a coherent state with the same mean photon number. The results demonstrate squeezing in one or more Stokes observables.
We propose and demonstrate a method for quantum-state tomography of qudits encoded in the quantum polarization of $N$-photon states. This is achieved by distributing $N$ photons nondeterministically into three paths and their subsequent projection, which for $N=1$ is equivalent to measuring the Stokes (or Pauli) operators. The statistics of the recorded $N$-fold coincidences determines the unknown $N$-photon polarization state uniquely. The proposed, fixed setup manifestly rules out any systematic measurement errors due to moving components and allows for simple switching between tomography of…
We experimentally study the phase space distribution (PSD) of a mechanical resonator that is simultaneously coupled to two electromagnetic cavities. The first one, operating in the microwave band, is employed for inducing either cooling or self-excited oscillation, whereas the second one, operating in the optical band, is used for displacement detection. A tomography technique is employed for extracting the PSD from the signal reflected by the optical cavity. Measurements of PSD are performed in steady state near the threshold of self-excited oscillation while sweeping the microwave cavity det…
Polarization-sensitive quantum optical coherence tomography (PS-QOCT) makes use of a Type-II twin-photon light source for carrying out optical sectioning with polarization sensitivity. A BBO nonlinear optical crystal pumped by a Ti:sapphire psec-pulsed laser is used to confirm the theoretical underpinnings of this imaging paradigm. PS-QOCT offers even-order dispersion cancellation with simultaneous access to the group-velocity dispersion characteristics of the interstitial medium between the reflecting surfaces of the sample.
In this work we demonstrate the use of stimulated emission tomography to characterize a hyper-entangled state generated by spontaneous parametric down-conversion in a CW-pumped source. In particular, we consider the generation of hyper-entangled states consisting of photon pairs entangled in polarisation and path. These results extend the capability of stimulated emission tomography beyond the polarisation degree of freedom, and demonstrate the use of this technique to study states in higher dimension Hilbert spaces.
The polarizing multi-photon quantum states tomography with non-unit quantum efficiency of detectors is considered. A new quantum tomography protocol is proposed. This protocol considers events of losing photons of multi-photon quantum state in one or more channels among with n-fold coincidence events. The advantage of the proposed protocol compared with the standard n-fold coincidence protocol is demonstrated using the methods of statistical analysis.
We set forth a polarization-sensitive quantum-optical coherence tomography (PS-QOCT) technique that provides axial optical sectioning with polarization-sensitive capabilities. The technique provides a means for determining information about the optical path length between isotropic reflecting surfaces, the relative magnitude of the reflectance from each interface, the birefringence of the interstitial material, and the orientation of the optical axis of the sample. PS-QOCT is immune to sample dispersion and therefore permits measurements to be made at depths greater than those accessible via o…
The standard description of cavity-modified molecular reactions typically involves a single (resonant) mode, while in reality the quantum cavity supports a range of photon modes. Here we demonstrate that as more photon modes are accounted for, physico-chemical phenomena can dramatically change, as illustrated by the cavity-induced suppression of the important and ubiquitous process of proton-coupled electron-transfer. Using a multi-trajectory Ehrenfest treatment for the photon-modes, we find that self-polarization effects become essential, and we introduce the concept of self-polarization-modi…
We report on the experimental implementation of a polarimeter based on a scheme known to be optimal for obtaining the polarization vector of ensembles of spin-1/2 quantum systems, and the alignment procedure for this polarimeter is discussed. We also show how to use this polarimeter to estimate the polarization state for identically prepared ensembles of single photons and photon pairs and extend the method to obtain the density matrix for generic multi-photon states. State reconstruction and performance of the polarimeter is illustrated by actual measurements on identically prepared ensembles…
We reconstruct the polarization sector of a bright polarization squeezed beam starting from a complete set of Stokes measurements. Given the symmetry that underlies the polarization structure of quantum fields, we use the unique SU(2) Wigner distribution to represent states. In the limit of localized and bright states, the Wigner function can be approximated by an inverse three-dimensional Radon transform. We compare this direct reconstruction with the results of a maximum likelihood estimation, finding an excellent agreement.
We introduce a self-consistent tomography for arbitrary quantum non-demolition (QND) detectors. Based on this, we build a complete physical characterization of the detector, including the measurement processes and a quantification of the fidelity, ideality, and back-action of the measurement. This framework is a diagnostic tool for the dynamics of QND detectors, allowing us to identify errors, and to improve their calibration and design. We illustrate this on a realistic Jaynes-Cummings simulation of superconducting qubit readout. We characterize non-dispersive errors, quantify the back-action…
We propose a cavity-QED scheme that can deterministically generate Einstein-Podosky-Rosen polarization-entangled photon pairs. A four-level tripod atom successively couples to two high-Q optical cavities possessing polarization degeneracy, assisted by a classical $π$-polarized pump field. The stimulated Raman adiabatic passage process in the atom-cavity system is used to produce the polarization-entangled photon pairs. The proposal is particularly robust against atomic spontaneous decay, which should have potential applications in quantum information processing.
We present a complete polarization characterization of any quantum state of two orthogonal polarization modes, and give a systematic measurement procedure to collect the necessary data. Full characterization requires measurements of the photon number in both modes and linear optics. In the situation where only the photon-number difference can be determined, a limited but useful characterization is obtained. The characteristic Stokes moment profiles are given for several common quantum states.
We experimentally demonstrate that a non-classical state prepared in an atomic memory can be efficiently transferred to a single mode of free-propagating light. By retrieving on demand a single excitation from a cold atomic gas, we realize an efficient source of single photons prepared in a pure, fully controlled quantum state. We characterize this source using two detection methods, one based on photon-counting analysis, and the second using homodyne tomography to reconstruct the density matrix and Wigner function of the state. The latter technique allows us to completely determine the mode o…
A scheme is discussed for measuring Nth-order coherences of two orthogonally polarized light fields in a single spatial mode at very limited experimental cost. To implement the scheme, the only measurements needed are the Nth-order intensity moments after the light beam has passed through two quarter-wave plates, one half-wave plate, and a polarizing beam splitter for specific settings of the wave plates. It is shown that this method can be applied for arbitrarily large N. A set of explicit values is given for the settings of the wave plates, constituting an optimal measurement of the Nth-orde…
We study the optical properties of coupled quantum dot-microcavity systems with elliptical cross section. First, we develop an analytic model that describes the spectrum of the cavity modes that are split due to the reduced symmetry of the resonator. By coupling the QD emission to the polarized fundamental cavity modes, we observe the vectorial nature of the Purcell enhancement, which depends on the intrinsic polarization of the quantum dot and its relative alignment with respect to the cavity axis. The variable interaction strength of the QD with the polarized cavity modes leads to the observ…
We utilize high-bandwidth phase quadrature homodyne measurement of the light transmitted through a Fabry-Perot cavity, driven strongly and on resonance, to detect excess phase noise induced by a single intracavity atom. We analyze the correlation properties and driving-strength dependence of the atom-induced phase noise to establish that it corresponds to the long-predicted phenomenon of spontaneous dressed-state polarization. Our experiment thus provides a demonstration of cavity quantum electrodynamics in the strong driving regime, in which one atom interacts strongly with a many-photon cavi…
A single photon has many physical degrees of freedom (DOF) that can carry the state of a high-dimensional quantum system. Nevertheless, only a single DOF is usually used in any specific demonstration. Furthermore, when more DOF are being used, they are analyzed and measured one at a time. We introduce a two-qubit information system, realized by two degrees of freedom of a single photon: polarization and time. The photon arrival time is divided into two time-bins representing a qubit, while its polarization state represents a second qubit. The time difference between the two time-bins is create…
In this work we present an algorithm of building an adequate model of polarizing quantum state measurement. This model takes into account chromatic aberration of the basis change transformation caused by the parasitic dispersion of the wave plates crystal and finite radiation spectral bandwidth. We show that the chromatic aberration reduces the amount of information in the measurements results. Using the information matrix approach we estimate the impact of this effect on the qubit state reconstruction fidelity for different values of sample size and spectral bandwidth. We also demonstrate tha…
Experiments in the field of optomechanics do not yet fully exploit the photon polarization degree of freedom. Here experimental results for an optomechanical interaction in a polarization nondegenerate system are presented and schemes are proposed for how to use this interaction to perform accurate side-band thermometry and to create novel forms of photon-phonon entanglement. The experimental system utilizes the compressive force in the mirror attached to a mechanical resonator to create a micro-mirror with two radii of curvature which leads, when combined with a second mirror, to a significan…
We further elaborate the theory of quantum fluctuations in vertical-cavity surface-emitting lasers (VCSELs), developed in Ref. \cite{Hermier02}. In particular, we introduce the quantum Stokes parameters to describe the quantum self- and cross-correlations between two polarization components of the electromagnetic field generated by this type of lasers. We calculate analytically the fluctuation spectra of these parameters and discuss experiments in which they can be measured. We demonstrate that in certain situations VCSELs can exhibit polarization squeezing over some range of spectral frequenc…
We have generated a new type of biphoton state by cavity-enhanced down-conversion in a type-II phase-matched, periodically-poled KTiOPO_4 (PPKTP) crystal. By introducing a weak intracavity birefringence, the polarization-entangled output was modulated between the singlet and triplet states according to the arrival-time difference of the signal and idler photons. This cavity-enhanced biphoton source is spectrally bright, yielding a single-mode fiber-coupled coincidence rate of 0.7 pairs/s per mW of pump power per MHz of down-conversion bandwidth. Its novel biphoton behavior may be utilized in s…
We study the dynamics of a general quartic interaction Hamiltonian under the influence of dissipation and non-classical driving. We show that this scenario could be realised with a cascaded superconducting cavity-qubit system in the strong dispersive regime in a setup similar to recent experiments. In the presence of dissipation, we find that an effective Hartree-type decoupling with a Fokker-Planck equation yields a good approximation. We find that the stationary state is approximately a squeezed vacuum, which is enhanced by the $Q$-factor of the cavity but conserved by the interaction. The q…
We present two cavity quantum electrodynamics proposals that, sharing the same basic elements, allow for the deterministic generation of entangled photons pairs by means of a three-level atom successively coupled to two single longitudinal mode high-Q optical resonators presenting polarization degeneracy. In the faster proposal, the three-level atom yields a polarization entangled photon pair via two truncated Rabi oscillations, whereas in the adiabatic proposal a counterintuitive Stimulated Raman Adiabatic Passage process is considered. Although slower than the former process, this second met…
We have performed the first experimental tomographic reconstruction of a three-photon polarization state. Quantum state tomography is a powerful tool for fully describing the density matrix of a quantum system. We measured 64 three-photon polarization correlations and used a "maximum-likelihood" reconstruction method to reconstruct the GHZ state. The entanglement class has been characterized using an entanglement witness operator and the maximum predicted values for the Mermin inequality was extracted.
Reliable generation and measurement of triphoton states has yet to be achieved in laboratory. We give an overview of the problems in generating and measuring triphoton quantum states and analyze several protocols of quantum measurements, which allow for high precision of reconstruction when sizes of available statistical data samples are limited. The tomography procedure under investigation is based on root approach to state estimation. In particular, we use the generalized Fisher information matrix to assess the accuracy of the quantum state parameters measurement. We use tomographic protocol…
Chiral-induced spin selectivity (CISS) is a phenomenon in which electron spins are polarized as they are transported through chiral molecules, and the spin polarization depends on the handedness of the chiral molecule. In this study, we show that spin selectivity can be realized in achiral materials by coupling electrons to a single mode of a chiral optical cavity. By investigating spin-dependent electron transport using the nonequilibrium Green's function approach, the spin polarization in a two-terminal setup is demonstrated to approach unity if the rate of dephasing is sufficiently small an…
We propose and demonstrate cavity-enhanced polarization-rotation measurement as a means to detect magnetic effects in transparent media with greater sensitivity at equal optical disturbance to the medium. Using the Jones calculus, we compute the effective polarization rotation effect in a Fabry-Perot cavity containing a magnetic medium, including losses due to enclosure windows or other sources. The results show that when measuring polarization rotation, collecting the transmitted light has advantages in simplicity and linearity relative to collecting the reflected light. We demonstrate the te…
We report the implementation of projective measurement on a single 1/2 nuclear spin of the 171Yb atom by measuring the polarization of cavity-enhanced fluorescence. To obtain cavity-enhanced fluorescence having a nuclear-spin-dependent polarization, we construct a two-mode cavity QED system, in which two cyclic transitions are independently coupled to each of the orthogonally polarized cavity modes, by manipulating the energy level of 171Yb. This system can associate the nuclear spin degrees of freedom with the polarization of photons, which will facilitate the development of hybrid quantum sy…
We show that the coupling between a qubit and a single mode cavity can be estimated from the process tomography data for the qubit alone. All the parameters of the coupling Hamiltonian between the qubit and the cavity mode can be obtained from observations on the qubit. We also show that the variance matrix and the photon number statistics of the single mode cavity can be reconstructed. Our results provide an alternate means of obtaining the coupling and reconstructing the state of the cavity mode in comparison with the techniques presently used.
We theoretically investigate polarization-entangled photon generation by using a semiconductor quantum dot embedded in a microcavity. The entangled states can be produced by the application of two cross-circularly polarized laser fields. The quantum dot nanostructure is considered as a four-level system (ground, two excitons and bi-exciton states) and the theoretical study relies on the dressed states scheme. The quantum correlations, reported in terms of the entanglement of formation, are extensively studied for several values of the important parameters of the quantum dot system as the bi-ex…
Optically-active spin systems coupled to photonic cavities with high cooperativity can generate strong light-matter interactions, a key ingredient in quantum networks. But obtaining high cooperativities for quantum information processing often involves the use of photonic crystal cavities that feature a poor optical access from the free space, especially to circularly polarized light required for the coherent control of the spin. Here, we demonstrate coupling with cooperativity as high as $8$ of an InAs/GaAs quantum dot to a fabricated bullseye cavity that provides nearly degenerate and Gaussi…
We investigate the effects of the electron-hole spin dynamics on the polarization fluctuations in the light emitted from a vertical cavity surface emitting laser (VCSEL). The Langevin equations are derived based on a rate equation model including birefringence, dichroism, and two carrier density pools seperately coupled to right and left circular polarization. The results show that the carrier dynamics phase lock the polarization fluctuations to the laser mode. This is clearly seen in the difference between fluctuations in ellipticity and fluctuations in polarization direction. Seperate measur…
Polarization quasi-probability distribution (PQPD) is defined in the Stokes space, and it enables the calculation of mean values and higher-order moments for polarization observables using simple algebraic averaging. It can be reconstructed with the help of polarization quantum tomography and provides a full description of the polarization properties of quantum states of light. We show here that, due to its definition in terms of the discrete-valued Stokes operators, polarization quasi-probability distribution has singularities and takes negative values at integer values of the Stokes observab…
Semiconductor quantum dots are probably the preferred choice for interfacing anchored, matter spin qubits and flying photonic qubits. While full tomography of a flying qubit or light polarization is in general straightforward, matter spin tomography is a challenging and resource-consuming task. Here we present a novel all-optical method for conducting full tomography of quantum-dot-confined spins. Our method is applicable for electronic spin configurations such as the conduction-band electron, the valence-band hole, and for electron-hole pairs such as the bright and the dark exciton. We excite…
Spontaneous emission can create coherences in a multilevel atom having close lying levels, subject to the condition that the atomic dipole matrix elements are non-orthogonal. This condition is rarely met in atomic systems. We report the possibility of bypassing this condition and thereby creating coherences by letting the atom with orthogonal dipoles to interact with the vacuum of a pre-selected polarized cavity mode rather than the free space vacuum. We derive a master equation for the reduced density operator of a model four level atomic system, and obtain its analytical solution to describe…
We discuss a cavity-QED scheme to deterministically generate entangled photons pairs by using a three-level atom successively coupled to two single longitudinal mode high-Q cavities presenting polarization degeneracy. The first cavity is prepared in a well defined Fock state with two photons with opposite circular polarizations while the second cavity remains in the vacuum state. A half-of-a-resonant Rabi oscillation in each cavity transfers one photon from the first to the second cavity, leaving the photons entangled in their polarization degree of freedom. The feasibility of this implementat…
Single-acquisition tomography of photonic qubits with structured media
University of Ottawa（渥太华大学）；Università degli Studi di Napoli Federico II（那不勒斯费德里科二世大学）；National Research Council of Canada（加拿大国家研究委员会）；McGill University（麦吉尔大学）；Chapman University（查普曼大学）
We address the experimental determination of entropic quantum discord for systems made of a pair of polarization qubits. We compare results from full and partial tomography and found that the two determinations are statistically compatible, with partial tomography leading to a smaller value of discord for depolarized states. Despite the fact that our states are well described, in terms of fidelity, by families of depolarized or phase-damped states, their entropic discord may be largely different from that predicted for these classes of states, such that no reliable estimation procedure beyond …
We compute the photon creation inside a perfectly conducting, three dimensional oscillating cavity, taking the polarization of the electromagnetic field into account. As the boundary conditions for this field are both of Dirichlet and (generalized) Neumann type, we analyze as a preliminary step the dynamical Casimir effect for a scalar field satisfying generalized Neumann boundary conditions. We show that particle production is enhanced with respect to the case of Dirichlet boundary conditions. Then we consider the transverse electric and transverse magnetic polarizations of the electromagneti…
We report an experimental realization of a narrow-band polarization-entangled photon source with a linewidth of 9.6 MHz through cavity-enhanced spontaneous parametric down-conversion. This linewidth is comparable to the typical linewidth of atomic ensemble based quantum memories. Single-mode output is realized by setting a reasonable cavity length difference between different polarizations, using of temperature controlled etalons and actively stabilizing the cavity. The entangled property is characterized with quantum state tomography, giving a fidelity of 94% between our state and a maximally…
We present a hybrid atomic sensor that realizes radio-frequency electric field detection with intrinsic field amplification and polarization selectivity for robust high-sensitivity field measurement. The hybrid sensor incorporates a passive resonator element integrated with an atomic vapor cell that provides amplification and polarization selectivity for detection of incident radio-frequency fields. The amplified intra-cavity radio-frequency field is measured by atoms using a quantum-optical readout of AC level shifts of field-sensitive atomic Rydberg states. In our experimental demonstration,…
We present a moment expansion method for the systematic characterization of the polarization properties of quantum states of light. Specifically, we link the method to the measurements of the Stokes operator in different directions on the Poincaré sphere, and provide a method of polarization tomography without resorting to full state tomography. We apply these ideas to the experimental first- and second-order polarization characterization of some two-photon quantum states. In addition, we show that there are classes of states whose polarization characteristics are dominated not by their first-…
