We employ the R-matrix with time-dependence method to investigate extreme-ultraviolet-initiated high-harmonic generation (XIHHG) in Ar$^{+}$. Using a combination of extreme-ultraviolet (XUV, $92\textrm{ nm}$, $3\times 10^{12}\,\textrm{Wcm}^{-2}$) and time-delayed, infrared (IR, $800\textrm{ nm}$, $3\times 10^{14}\,\textrm{Wcm}^{-2}$) laser pulses, we demonstrate that control over both the mechanism, and timing, of ionization can afford significant enhancements in the yield of plateau, and sub-threshold, harmonics alike. The presence of the XUV pulse is also shown to alter the relative contribution of different electron emission pathways. Manifestation of the Ar$^{+}$ electronic structure is found in the appearance of a pronounced Cooper minimum. Interferences amongst the outer-valence $3p$, and inner-valence $3s$, electrons are found to incur only a minor suppression of the harmonic intensities, at least for the present combination of XUV and IR laser light. Additionally, the dependence of the XIHHG efficiency on time delay is discussed, and rationalized with the aid of classical trajectory simulations.
We report spectroscopic measurements of highly charged samarium and erbium performed at the National Institute of Standards and Technology (NIST) Electron Beam Ion Trap (EBIT). These measurements are in the extreme ultraviolet (EUV) range, and span electron beam energies from 0.98 keV to 3.00 keV. We observed 71 lines from Kr-like Sm$^{26+}$ to Ni-like Sm$^{34+}$, connecting 83 energy levels, and 64 lines from Rb-like Er$^{32+}$ to Ni-like Er$^{40+}$, connecting 78 energy levels. Of these lines, 64 in Sm and 60 in Er are new. Line identifications are performed using collisional-radiative model…
Coherent sources of attosecond extreme ultraviolet (XUV) radiation present many challenges if their full potential is to be realized. While many applications benefit from the broadband nature of these sources, it is also desirable to produce narrow band XUV pulses, or to study autoionizing resonances in a manner that is free of the broad ionization background that accompanies above-threshold XUV excitation. Here we demonstrate a method for controlling the coherent XUV free induction decay that results from using attosecond pulses to excite a gas, yielding a fully functional modulator for XUV w…
We report on the experimental observation of strong-field dressing of an autoionizing two-electron state in helium with intense extreme-ultraviolet laser pulses from a free-electron laser. The asymmetric Fano line shape of this transition is spectrally resolved, and we observe modifications of the resonance asymmetry structure for increasing free-electron-laser pulse energy on the order of few tens of $μ$J. A quantum-mechanical calculation of the time-dependent dipole response of this autoionizing state, driven by classical extreme-ultraviolet (XUV) electric fields, reveals a direct link betwe…
We present a comprehensive experimental and theoretical study on superfluorescence in the extreme ultraviolet wavelength regime. Focusing a high-intensity free-electron laser pulse in a cell filled with Xe or Kr gas, the medium is quasi instantaneously population-inverted by inner-shell ionization on the giant resonance followed by Auger decay. On the timescale of 100 ps a macroscopic polarization builds up in the medium, resulting in superfluorescent emission of several Xe and Kr lines in the forward direction. As the number of emitters in the system is increased by either raising the pressur…
X-ray and extreme-ultraviolet spectra from collisions of Ar$^{18+}$ and O$^{8+}$ ions with neutrals
Max-Planck-Institut für Kernphysik（马克斯·普朗克核物理研究所）；NASA Goddard Space Flight Center（美国国家航空航天局戈达德太空飞行中心）；Johns Hopkins University（约翰斯·霍普金斯大学）；Helmholtz-Institut Jena（亥姆霍兹耶拿研究所）；GSI Helmholtzzentrum für Schwerionenforschung（GSI重离子研究中心）；University of California（加利福尼亚大学）；SRON, Space Research Organisation Netherlands（荷兰空间研究组织）
In this study the generation of energetic coherent extreme ultraviolet (XUV) radiation with controlled polarization, is reported. The XUV radiation results from the process of high harmonic generation (HHG), in a gas phase atomic medium, driven by an intense two-color circularly polarized counter-rotating laser field, under loose focusing geometry conditions. The energy of the XUV radiation emitted per laser pulse is found to be of the order of ~100 nJ with the spectrum spanning from 17 to 26 eV. The demonstrated energy values along with tight focusing geometries is sufficient to induce nonlin…
Interferometric pump-probe experiments in the extreme ultraviolet (XUV) domain are experimentally very challenging due to the high phase stability required between the XUV pulses. Recently, an efficient phase stabilization scheme was introduced for seeded XUV free electron lasers (FELs) combining shot-to-shot phase modulation with lock-in detection. This method stabilized the seed laser beampath on the fundamental ultraviolet wavelength to a high degree. Here, we extend this scheme including the stabilization of the XUV beampath, incorporating phase fluctuations from the FEL high gain harmonic…
In the present work we report on the current progress of the recently constructed GW attosecond extreme ultraviolet (XUV) source developed at the Institute of Electronic Structure and Laser of the Foundation for Research and Technology-Hellas (I.E.S.L-FO.R.T.H.). By the implementation of a compact-collinear polarization gating arrangement, the generation of a broadband, coherent XUV quasi-continuum produced by the interaction of a many-cycle infrared field with a gas phase medium is achieved. The spectral width of the XUV emission generated in Xenon, is spanning in the range of 17-32 eV and ca…
The development of schemes for coherent nonlinear time-domain spectroscopy in the extreme-ultraviolet regime (XUV) has so far been impeded by experimental difficulties that arise at these short wavelengths. In this work we present a novel experimental approach, which facilitates the timing control and phase cycling of XUV pulse sequences produced by harmonic generation in rare gases. The method is demonstrated for the generation and high spectral resolution characterization of narrow-bandwidth harmonics ($\approx14\,$eV) in argon and krypton. Our technique simultaneously provides high phase st…
Femtosecond induced transparency and absorption in the extreme ultraviolet by coherent coupling of the He 2s2p (1P0) and 2p2 (1Se) double excitation states with 800 nm light
Many atomic and molecular systems of fundamental interest possess resonance frequencies in the extreme ultraviolet (XUV) where laser technology is limited and radiation sources have traditionally lacked long-term phase coherence. Recent breakthroughs in XUV frequency comb technology have demonstrated spectroscopy with unprecedented resolution at the megahertz level, but even higher resolutions are desired for future applications in precision measurement. By characterizing heterodyne beats between two XUV comb sources, we demonstrate the capability for sub-hertz spectral resolution. This corres…
After decades of supremacy of the Titanium:Sapphire technology, Ytterbium-based high-order harmonic sources are emerging as an interesting alternative for experiments requiring high flux of ultrashort extreme ultraviolet (XUV) radiation. In this article we describe a versatile experimental setup delivering XUV photons in the 10-50 eV range. The use of cascaded high-harmonic generation enables us to reach 1.8 mW of average power at 18 eV. Several spectral focusing schemes are presented, to select either a single harmonic or group of high-harmonics and thus an attosecond pulse train. In the pers…
High-intensity laser pulses covering the ultraviolet to terahertz spectral regions are nowadays routinely generated in a large number of laboratories. In contrast, intense extreme-ultraviolet (XUV) pulses have only been demonstrated using a small number of sources including free-electron laser facilities [1-3] and long high-harmonic generation (HHG) beamlines [4-9]. Here we demonstrate a concept for a compact intense XUV source based on HHG that is focused to an intensity of $2 \times 10^{14}$ W/cm$^2$, with a potential increase up to $10^{17}$ W/cm$^2$ in the future. Our approach uses tight f…
Refraction is a well-known optical phenomenon that alters the direction of light waves propagating through matter. Microscopes, lenses and prisms based on refraction are indispensable tools for controlling the properties of light beams at visible, infrared, ultraviolet and X-ray wavelengths. The large absorption of extreme-ultraviolet (XUV) radiation in matter, however, hinders the development of refractive lenses and prisms in this spectral region. Here, we demonstrate control over the refraction of XUV radiation by using a gas jet with a density gradient across the XUV beam profile. A gas ph…
Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates, $f_{rep}\lesssim$100 kHz, where phase-matched frequency conversion into the XUV is readily achieved. However, there are many applications that demand the improved counting statistics or frequency-comb precision afforded by operation at high repetition rates, $f_{rep}$ > 10 MHz. Unfortunately, at such high $f_{rep}$, phase matching is prevented by the accumulated stead…
We demonstrate time-resolved nonlinear extreme-ultraviolet absorption spectroscopy on multiply charged ions, here applied to the doubly charged neon ion, driven by a phase-locked sequence of two intense free-electron laser pulses. Absorption signatures of resonance lines due to 2$p$--3$d$ bound--bound transitions between the spin-orbit multiplets $^3$P$_{0,1,2}$ and $^3$D$_{1,2,3}$ of the transiently produced doubly charged Ne$^{2+}$ ion are revealed, with time-dependent spectral changes over a time-delay range of $(2.4\pm0.3)\,\text{fs}$. Furthermore, we observe 10-meV-scale spectral shifts o…
Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet (XUV) light have previously been limited by either space-charge effects, low photon flux, or limited tuning range. In this article, we describe space-charge-free XUV photoelectron spectroscopy experiments with up to 5 nA of average sample current using a tunable cavity-enhanced high-harmonic source operating at 88 MHz repetition rate. The source delivers $ …
