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arXiv 1707.04834cond-mat.str-el
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阻挫磁体$\mathrm{Ca}_{10}\mathrm{Cr}_{7}\mathrm{O}_{28}$类液体行为的半经典理论

Semiclassical theory for liquid-like behaviour of the frustrated magnet $\mathrm{Ca}_{10}\mathrm{Cr}_{7}\mathrm{O}_{28}$

Sounak Biswas, Kedar Damle

摘要:

我们确定的低能量有效的哈密顿量,预计将描述的受抑磁体$\mathrm{Ca}_{10}\mathrm{Cr}_{7}\mathrm{O}_{28}$的低温性能。由于这种有效哈密顿量具有$S=3/2$有效矩作为其自由度,我们利用半经典自旋波理论研究了这种有效模型的$T=0$物理,并认为奇异自旋波涨落破坏了这种有效哈密顿量的交换耦合所支持的螺旋序.我们还使用经典的蒙特卡罗模拟和分子动力学,以及分析近似的组合,研究在低,非零温度的物理。这些非零温度计算的结果捕获了在最近的实验所访问的温度范围内观察到的类液体结构因子。此外,在更低的温度下,他们预测,在键能中的一个过渡到π阶反映了自己在自旋通道中的形式交叉到一个政权与大,但有限的相关长度的螺旋自旋相关和相应的自旋动力学减慢。

英文摘要:

We identify the low energy effective Hamiltonian that is expected to describe the low temperature properties of the frustrated magnet $\mathrm{Ca}_{10}\mathrm{Cr}_{7}\mathrm{O}_{28}$. Motivated by the fact that this effective Hamiltonian has $S=3/2$ effective moments as its degrees of freedom, we use semiclassical spinwave theory to study the $T=0$ physics of this effective model and argue that singular spinwave fluctuations destabilize the spiral order favoured by the exchange couplings of this effective Hamiltonian. We also use a combination of classical Monte-Carlo simulations and molecular dynamics, as well as analytical approximations, to study the physics at low, nonzero temperatures. The results of these nonzero temperature calculations capture the liquid-like structure factors observed in the temperature range accessed by recent experiments. Additionally, at still lower temperatures, they predict that a transition to nematic order in the bond energies reflects itself in the spin channel in the form of a crossover to a regime with large but finite correlation length for spiral spin correlations and a corresponding slowing down of spin dynamics.

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