Non-thermalization in trapped atomic ion spin chains
P. W. Hess, P. Becker, H. B. Kaplan, A. Kyprianidis, A. C. Lee, B. Neyenhuis, G. Pagano, P. Richerme, C. Senko, J. Smith, W. L. Tan, J. Zhang, C. Monroe
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14 pages, 5 figures, submitted for edition of Phil. Trans. R. Soc. A on "Breakdown of ergodicity in quantum systems"
Linear arrays of trapped and laser cooled atomic ions are a versatile platform for studying emergent phenomena in strongly-interacting many-body systems. Effective spins are encoded in long-lived electronic levels of each ion and made to interact through laser mediated optical dipole forces. The advantages of experiments with cold trapped ions, including high spatiotemporal resolution, decoupling from the external environment, and control over the system Hamiltonian, are used to measure quantum effects not always accessible in natural condensed matter samples. In this review we highlight recent work using trapped ions to explore a variety of non-ergodic phenomena in long-range interacting spin-models which are heralded by memory of out-of-equilibrium initial conditions. We observe long-lived memory in static magnetizations for quenched many-body localization and prethermalization, while memory is preserved in the periodic oscillations of a driven discrete time crystal state.
We studied a single atom trapped in an optical tweezer interacting with a thermal bath of ultracold atoms of a different species. Because of the collisions between the trapped atom and the bath atoms, the trapped atom undergoes changes in its vibrational states occupation to reach thermal equilibrium with the bath. By using Monte Carlo simulations, we characterized the single atom's thermalization process, and we studied how this can be used for cooling. Our simulations demonstrate that, within known experimental limitations, it is feasible to cool a trapped single atom with a thermal bath.
We have studied the role of thermalization in lifetime reduction of quantum memory based on multi-atomic ensembles. Herein, it is shown to be impossible to remove the thermaization-caused decoherence in such systems using the methods of dynamical decoupling. We have analyzed the existing models of the thermalization and have proposed a new understanding of the thermalization as a result of the internal processes which are not described in the unitary quantum dynamics formalism. The possible ways for reducing the negative influence of thermalization on the quantum memory lifetime are also discu…
We study how the thermalization time of a single radiation cavity-field mode changes drastically depending on the type of the atomic reservoir it interacts. Temporal evolution of the field is analyzed within the micromaser scheme, where each atomic reservoir is modeled as a beam of atoms crossing an electromagnetic cavity in which they weakly interact with the field. The cavity-field thermalizes when we consider either multi-atom or multi-level atom reservoirs. We found that each atomic reservoir generates a different scaling law in the thermalization time of the cavity-field. Such scaling law…
Experiments with trapped atomic gases have opened novel possibilities for studying the evolution of nonequilibrium finite quantum systems, which revived the necessity of reconsidering and developing the theory of such processes. This review analyzes the basic approaches to describing the phenomena of equilibration, thermalization, and decoherence in finite quantum systems. Isolated, nonisolated, and quasi-isolated quantum systems are considered. The relations between equilibration, decoherence, and the existence of time arrow are emphasized. The possibility for the occurrence of rare events, p…
Atomic collisions are included in an interacting system of optical fields and trapped atoms allowing field amplification. We study the effects of collisions on the system stability. Also a study of the degree of entanglement between atomic and optical fields is made. We found that, for an atomic field initially in a vacuum state and optical field in a coherent state, the degree of entanglement does not depend on the optical field intensity or phase. We show that in conditions of exponential instability the system presents at long times two distinct stationary degree of entanglement with collis…
We use trapped atomic ions forming a hybrid Coulomb crystal, and exploit its phonons to study an isolated quantum system composed of a single spin coupled to an engineered bosonic environment. We increase the complexity of the system by adding ions and controlling coherent couplings and, thereby, we observe the emergence of thermalization: Time averages of spin observables approach microcanonical averages while related fluctuations decay. Our platform features precise control of system size, coupling strength, and isolation from the external world to explore the dynamics of equilibration and t…
Ordered atomic arrays trapped in the vicinity of nanoscale waveguides offer original light-matter interfaces, with applications to quantum information and quantum non-linear optics. Here, we study the decay dynamics of a single collective atomic excitation coupled to a waveguide in different configurations. The atoms are arranged as a linear array and only a segment of them is excited to a superradiant mode and emits light into the waveguide. Additional atomic chains placed on one or both sides play a passive role, either reflecting or absorbing this emission. We show that when varying the geo…
Distribution of the entangled state of trapped atomic ions to long distance using quantum repeater protocol is considered. Indeed, the long distance is divided into short parts, and then using entanglement generation and entanglement swapping techniques in optomechanical cavities, the entanglement is distributed. To do the task, we perform interaction between trapped atomic ions in optomechanical cavities, operate proper measurements on trapped ions and also make Bell state measurement as a well-known way to swap the entanglement. Accordingly, the entanglement is distributed between target ion…
We study semi-classical slow light propagation in trapped two level atomic quantum gases. The temperature dependent behaviors of both group velocity and transmissions are compared for low temperature Bose, Fermi, and Boltzman gases within the local density approximation for their spatial density profile.
Ion traps are often loaded from atomic beams produced by resistively heated ovens. We demonstrate an atomic oven which has been designed for fast control of the atomic flux density and reproducible construction. We study the limiting time constants of the system and, in tests with $^{40}\textrm{Ca}$, show we can reach the desired level of flux in 12s, with no overshoot. Our results indicate that it may be possible to achieve an even faster response by applying an appropriate one-off heat treatment to the oven before it is used.
We theoretically study trapped ions that are immersed in an ultracold gas of Rydberg-dressed atoms. By off-resonant coupling on a dipole-forbidden transition, the adiabatic atom-ion potential can be made repulsive. We study the energy exchange between the atoms and a single trapped ion and find that Langevin collisions are inhibited in the ultracold regime for these repulsive interactions. Therefore, the proposed system avoids recently observed ion heating in hybrid atom-ion systems caused by coupling to the ion's radio frequency trapping field and retains ultracold temperatures even in the pr…
We demonstrate how to use feedback to control the internal states of trapped coherent ensembles of two-level atoms, and to protect a superposition state against the decoherence induced by a collective noise. Our feedback scheme is based on weak optical measurements with negligible back-action and coherent microwave manipulations. The efficiency of the feedback system is studied for a simple binary noise model and characterized in terms of the trade-off between information retrieval and destructivity from the optical probe. We also demonstrate the correction of more general types of collective …
Using trapped ions in an entangled state we propose detecting a magnetic dipole of a single atom at distance of a few $μ$m. This requires a measurement of the magnetic field gradient at a level of about 10$^{-13}$ Tesla/$μ$m. We discuss applications e.g. in determining a wide variation of ionic magnetic moments, for investigating the magnetic substructure of ions with a level structure not accessible for optical cooling and detection,and for studying exotic or rare ions, and molecular ions. The scheme may also be used for measureing spin imbalances of neutral atoms or atomic ensembles trapped …
To facilitate quantum simulation of open quantum systems at finite temperatures, an important ingredient is to achieve thermalization on a given time-scale. We consider a Rydberg aggregate (an arrangement of Rydberg atoms that interact via long-range interactions) embedded in a laser-driven atomic environment. For the smallest aggregate (two atoms), suitable laser parameters can be found by brute force scanning of the four tunable laser parameters. For more atoms, however, such parameter scans are too computationally costly. Here we apply Gaussian processes to predict the thermalization perfor…
We study a hybrid quantum system composed of an ion and an electric dipole. We show how a trapped ion can be used to measure the small electric field generated by a classical dipole. We discuss the application of this scheme to measure the electric dipole moment of cold polar molecules, whose internal state can be controlled with ultrafast laser pulses, by trapping them in the vicinity of a trapped ion.
We construct a connection of the ultracold atomic system in a harmonic trap with Raman-induced spin-orbit coupling to the quantum Rabi-like model. By mapping the trapped atomic system to a Rabi-like model, we can get the exact solution of the Rabi-like model following the methods to solve the quantum Rabi model. The existence of such a mapping implies that we can study the basic model in quantum optics by using trapped atomic gases with spin-orbit coupling.
We collect the fluorescence from two trapped atomic ions, and measure quantum interference between photons emitted from the ions. The interference of two photons is a crucial component of schemes to entangle atomic qubits based on a photonic coupling. The ability to preserve the generated entanglement and to repeat the experiment with the same ions is necessary to implement entangling quantum gates between atomic qubits, and allows the implementation of protocols to efficiently scale to larger numbers of atomic qubits.
We study the complex quantum dynamics of a system of many interacting atoms in an elongated anharmonic trap. The system is initially in a Bose-Einstein condensed state, well described by Thomas-Fermi profile in the elongated direction and the ground state in the transverse directions. After a sudden quench to a coherent superposition of the ground and lowest energy transverse modes, quantum dynamics starts. We describe this process employing a three-mode many-body model. The experimental realization of this system displays decaying oscillations of the atomic density distribution. While a mean-…
We discuss cooling efficiency for different-species Fermi-Bose mixtures in magnetic traps. A better heat capacity matching between the two atomic species is achieved by a proper choice of the Bose cooler and the magnetically trappable hyperfine states of the mixture. When a partial spatial overlap between the two species is also taken into account, the deepest Fermi degeneracy is obtained for an optimal value of the trapping frequency ratio. This can be achieved by assisting the magnetic trap with a deconfining light beam, as shown in the case of fermionic 6Li mixed with 23Na, 87Rb, and 133Cs,…
We investigate theoretical decoherence effects of the motional degrees of freedom of a single trapped atomic/ionic electronically coded qubit. For single bit rotations from a resonant running wave laser field excitation, we found the achievable fidelity to be determined by a single parameter characterized by the motional states. Our quantitative results provide a useful realistic view for current experimental efforts in quantum information and computing.
We experimentally demonstrate a method to determine the temperature of trapped ions which is suitable for monitoring fast thermalization processes. We show that observing and analyzing the lineshape of dark resonances in the fluorescence spectrum provides a temperature measurement which accurate over a large dynamic range, applied to single ions and small ion crystals. Laser induced fluorescence is detected over a time of only $20\,μ$s allowing for rapid determination of the ion temperature. In the measurement range of $10^{-1}-10^{+2}\,$mK we reach better than $15\,\%$ accuracy. Tuning the co…
It has been proposed to use magnetically trapped atomic ensembles to enhance the interrogation time in microwave clocks. To mitigate the perturbing effects of the magnetic trap, near-magic-field configurations are employed, where the involved clock transition becomes independent of the atom's potential energy to first order. Still, higher order effects are a dominating source for dephasing, limiting the performance of this approach. Here we propose a simple method to cancel the energy dependence to both first and second order, using weak radio-frequency dressing. We give values for dressing fr…
We propose an implementation for quantum logic and computing using trapped atomic spins of two different species, interacting via direct magnetic spin-spin interaction. In this scheme, the spins (electronic or nuclear) of distantly spaced trapped neutral atoms serve as the qubit arrays for quantum information processing and storage, and the controlled interaction between two spins, as required for universal quantum computing, is implemented in a three step process that involves state swapping with a movable auxiliary spin.
Trapped atomic ensembles are convenient systems for quantum information storage in the long-lived sublevels of the electronic ground state and its conversion to propagating optical photons via stimulated Raman processes. Here we investigate a phase-matched emission of photons from a coherently prepared atomic ensemble. We consider an ensemble of cold atoms in an elongated harmonic trap with normal density distribution, and determine the parameters of paraxial optics to match the mode geometry of the emitted radiation and optimally collect it into an optical waveguide.
We perform Ramsey spectroscopy on the ground state of ultra-cold 87Rb atoms magnetically trapped on a chip in the Knudsen regime. Field inhomogeneities over the sample should limit the 1/e contrast decay time to about 3 s, while decay times of 58 s are actually observed. We explain this surprising result by a spin self-rephasing mechanism induced by the identical spin rotation effect originating from particle indistinguishability. We propose a theory of this synchronization mechanism and obtain good agreement with the experimental observations. The effect is general and susceptible to appear i…
We study the ground state properties of trapped atomic condensates with electric field induced dipole-dipole interactions. A rigorous method for constructing the pseudo potential in the spirit of ladder approximation is developed for general non-spherical (polarized) particles interacting anisotropically. We discuss interesting features not previously considered for currently available alkali condensates. In addition to provide a quantitative assessment for controlling atomic interactions with electric fields, our investigation may also shed new light into the macroscopic coherence properties …
We present quantitative predictions for quantum simulator experiments on Ising models from trapped ions to Rydberg chains and show how the thermalization, and thus decoherence times, can be controlled by considering common, independent, and end-cap couplings to the bath. We find (i) independent baths enable more rapid thermalization in comparison to a common one; (ii) the thermalization timescale depends strongly on the position in the Ising phase diagram; (iii) for a common bath larger system sizes show a significant slow down in the thermalization process; and (iv) finite-size scaling indica…
For an atomic condensate in an axially symmetric magnetic trap, the sum of the axial components of the orbital angular momentum and the hyperfine spin is conserved. Inside an Ioffe-Pritchard trap (IPT) whose magnetic field (B-field) is not axially symmetric, the difference of the two becomes surprisingly conserved. In this paper we investigate the relationship between the values of the sum/difference angular momentums for an atomic condensate inside a magnetic trap and the associated gauge potential induced by the adiabatic approximation. Our result provides significant new insight into the vo…
We describe a simple approach to the problem of incorporating the response time of an atom or ion being Doppler-cooled into the theory of the cooling process. The system being cooled does not in general respond instantly to the changing laser frequencies it experiences in its rest frame, and this "dynamic effect" can affect significantly the temperatures attainable. It is particularly important for trapped ions when there is a slow decay out of the cooling cycle requiring the use of a repumping beam. We treat the cases of trapped ions with two and three internal states, then apply the theory t…
In ergodic many-body quantum systems, locally encoded quantum information becomes, in the course of time evolution, inaccessible to local measurements. This concept of "scrambling" is currently of intense research interest, entailing a deep understanding of many-body dynamics such as the processes of chaos and thermalization. Here, we present first experimental demonstrations of quantum information scrambling on a 10-qubit trapped-ion quantum simulator representing a tunable long-range interacting spin system, by estimating out-of-time ordered correlators (OTOCs) through randomized measurement…
We experimentally and theoretically investigate the lowest-lying axial excitation of an atomic Bose-Einstein condensate in a cylindrical box trap. By tuning the atomic density, we observe how the nature of the mode changes from a single-particle excitation (in the low-density limit) to a sound wave (in the high-density limit). Throughout this crossover the measured mode frequency agrees with Bogoliubov theory. Using approximate low-energy models we show that the evolution of the mode frequency is directly related to the interaction-induced shape changes of the condensate and the excitation. Fi…
A single laser-cooled and trapped 9Be+ ion is used to investigate methods of coherent quantum-state synthesis and quantum logic. We create and characterize nonclassical states of motion including "Schroedinger-cat" states. A fundamental quantum logic gate is realized which uses two states of the quantized ion motion and two ion internal states as qubits. We explore some of the applications for, and problems in realizing, quantum computation based on multiple trapped ions.
Scrambling of quantum information is the process by which information initially stored in the local degrees of freedom of a quantum many-body system spreads over its many-body degrees of freedom, becoming inaccessible to local probes and thus apparently lost. Scrambling and entanglement are key concepts reconciling seemingly unrelated behaviors including thermalization of isolated quantum systems and information loss in black holes, and have revolutionized our understanding of non-equilibrium phenomena. Here, we demonstrate that a family of fidelity out-of-time-order correlators (FOTOCs), rece…
The method of phenomenological damping developed by Pitaevskii for superfluidity near the $λ$ point is simulated numerically for the case of a dilute, alkali, inhomogeneous Bose-condensed gas near absolute zero. We study several features of this method in describing the damping of excitations in a Bose-Einstein condensate. In addition, we show that the method may be employed to obtain numerically accurate ground states for a variety of trap potentials.
The first generation of quantum computers are on the horizon, fabricated from quantum hardware platforms that may soon be able to tackle certain tasks that cannot be performed or modelled with conventional computers. These quantum devices will not likely be universal or fully programmable, but special-purpose processors whose hardware will be tightly co-designed with particular target applications. Trapped atomic ions are a leading platform for first generation quantum computers, but are also fundamentally scalable to more powerful general purpose devices in future generations. This is because…
Atomic ensembles have many potential applications in quantum information science. Owing to collective enhancement, working with ensembles at high densities increases the overall efficiency of quantum operations, but at the same time also increases the collision rate and leads to faster decoherence. Here we report on experiments with optically trapped 87Rb atoms demonstrating a 20-fold increase of the coherence time when a dynamical decoupling sequence with more than 200 pi-pulses is applied. We perform quantum process tomography and demonstrate that using the decoupling scheme a dense ensemble…
Methods for, and limitations to, the generation of entangled states of trapped atomic ions are examined. As much as possible, state manipulations are described in terms of quantum logic operations since the conditional dynamics implicit in quantum logic is central to the creation of entanglement. Keeping with current interest, some experimental issues in the proposal for trapped-ion quantum computation by I. Cirac and P. Zoller (University of Innsbruck) are discussed. Several possible decoherence mechanisms are examined and what may be the more important of these are identified. Some potential…
We report on ground state laser cooling of single 111Cd+ ions confined in radio-frequency (Paul) traps. Heating rates of trapped ion motion are measured for two different trapping geometries and electrode materials, where no effort was made to shield the electrodes from the atomic Cd source. The low measured heating rates suggest that trapped 111Cd+ ions may be well-suited for experiments involving quantum control of atomic motion, including applications in quantum information science.
We numerically show that a topologically nontrivial 3D Skyrmion can be energetically stable in a trapped two-component atomic Bose-Einstein condensate, for the parameters of Rb-87 condensate experiments. The separate conservation of the two atomic species can stabilize the Skyrmion against shrinking to zero size, while drift of the Skyrmion due to the trap-induced density gradient can be prevented by rotation or by a laser potential.
We have studied the atomic density of a cloud confined in an isotropic harmonic trap at the vicinity of the Bose-Einstein transition temperature. We show that, for a non-interacting gas and near this temperature, the ground-state density has the same order of magnitude as the excited states density at the centre of the trap. This holds in a range of temperatures where the ground-state population is negligible compared to the total atom number. We compare the exact calculations, available in a harmonic trap, to semi-classical approximations. We show that these latter should include the ground-s…
We describe an entanglement purification protocol (EPP) for multipartite three-level atomic entangled pair using photonic Faraday rotation. In this EPP, the multipartite atomic entangled state can be purified with the help of some single photons. This protocol resorts to the photonic Faraday rotation to realize the function of the controlled-Not (CNOT) gate. The purified multipartite atomic entangled state can be retained and to be repeated to reach a higher fidelity.
Laser cooling of atomic motion enables a wide variety of technological and scientific explorations using cold atoms. Here we focus on the effect of laser cooling on the photons instead of on the atoms. Specifically, we show that non-interacting photons can thermalize with the atoms to a grand canonical ensemble with a non-zero chemical potential. This thermalization is accomplished via scattering of light between different optical modes, mediated by the laser cooling process. While optically thin modes lead to traditional laser cooling of the atoms, the dynamics of multiple scattering in optic…
We experimentally characterize the optical nonlinear response of a cold atomic medium placed inside an optical cavity, and excited to Rydberg states. The excitation to S and D Rydberg levels is carried out via a two-photon transition in an EIT (electromagnetically induced transparency) configuration, with a weak (red) probe beam on the lower transition, and a strong (blue) coupling beam on the upper transition. The observed optical nonlinearities induced by S states for the probe beam can be explained using a semi-classical model with van der Waals' interactions. For the D states, it appears n…
We investigate the nonlinear dissipative coherence bifurcation and population dynamics of a two-component atomic Bose-Einstein condensate coupling with a continuum. The coupling between the two-component condensates and the continuum brings effective dissipations to the two-component condensates. The steady states and the coherence bifurcation depend on both dissipation and the nonlinear interaction between condensed atoms. The coherence among condensed atoms may be even enhanced by the effective dissipations. The combination of dissipation and nonlinearity allows one to control the switching …
We describe a simple protocol for the single-step generation of $N$-body entangling interactions between trapped atomic ion qubits. We show that qubit state-dependent squeezing operations and displacement forces on the collective atomic motion can generate full $N$-body interactions. Similar to the Mølmer-Sørensen two-body Ising interaction at the core of most trapped ion quantum computers and simulators, the proposed operation is relatively insensitive to the state of motion. We show how this $N$-body gate operation allows the single-step implementation of a family of $N$-bit gate operations …
We show that certain coherences, termed as heat-exchange coherences, which contribute to the thermalization process of a quantum probe in a repeated interactions scheme, can modify the spectral response of the probe system. We suggest to use the power spectrum as a way to experimentally assess the apparent temperature of non-thermal atomic clusters carrying such coherences and also prove that it is useful to measure the corresponding thermalization time of the probe, assuming some information is provided on the nature of the bath. We explore this idea in two examples in which the probe is assu…
The coupling of atomic arrays and one-dimensional subwavelength waveguides gives rise to in- teresting photon transport properties, such as recent experimental demonstrations of large Bragg reflection and paves the way for a variety of potential applications in the field of quantum non-linear optics. Here, we present a theoretical analysis for the process of single-photon scattering in this configuration using a full microscopic approach. Based on this formalism, we analyze the spectral dependencies for different scattering channels from either ordered or disordered arrays. The de- veloped app…
We describe a scheme for producing conditional nonlinear phase shifts on two-photon optical fields using an interaction with one or more ancilla two-level atomic systems. The conditional field state transformations are induced by using high efficiency fluorescence shelving measurements on the atomic ancilla. The scheme can be nearly deterministic and is of obvious benefit for quantum information applications.
We derive exact closed form expressions for the first few terms of the short-distance Taylor expansion of the one-body correlation function of the Lieb-Liniger gas. As an intermediate result we obtain the high-p asymptotics of the momentum distribution of both free and harmonically trapped atoms and show that it obeys a universal 1/p^4 law for_all_ values of the interaction strength. We discuss the ways to observe the predicted momentum distributions experimentally, regarding them as a sensitive identifier for the Tonks-Girardeau regime of strong correlations.
We report the experimental demonstration of a quantum memory for collective atomic states in a far-detuned optical dipole trap. Generation of the collective atomic state is heralded by the detection of a Raman scattered photon and accompanied by storage in the ensemble of atoms. The optical dipole trap provides confinement for the atoms during the quantum storage while retaining the atomic coherence. We probe the quantum storage by cross-correlation of the photon pair arising from the Raman scattering and the retrieval of the atomic state stored in the memory. Non-classical correlations are ob…
We theoretically analyze the dynamics of an atomic double-well system with a single ion trapped in its center. We find that the atomic tunnelling rate between the wells depends both on the spin of the ion via the short-range spin-dependent atom-ion scattering length and on its motional state with tunnelling rates reaching hundreds of Hz. A protocol is presented that could transport an atom from one well to the other depending on the motional (Fock) state of the ion within a few ms. This phonon-atom coupling is of interest for creating atom-ion entangled states and may form a building block in …
Realizing systems that support robust, controlled interactions between individual photons is an exciting frontier of nonlinear optics. To this end, one approach that has emerged recently is to leverage atomic interactions to create strong and spatially non-local interactions between photons. In particular, effective interactions have been successfully created via interactions between atoms excited to Rydberg levels. Here, we investigate an alternative approach, in which atomic interactions arise via their common coupling to photonic crystal waveguides. This technique takes advantage of the abi…
