We report on the experimental observation of coherent cavity soliton frequency combs in silica microspheres. Specifically, we demonstrate that careful alignment of the microsphere relative to the coupling fiber taper allows for the suppression of higher-order spatial modes, reducing mode interactions and enabling soliton formation. Our measurements show that the temporal cavity solitons have sub-100-fs durations, exhibit considerable Raman self-frequency shift, and generally come in groups of three or four, occasionally with equidistant spacing in the time domain. RF amplitude noise measurements and spectral interferometry confirm the high coherence of the observed soliton frequency combs, and numerical simulations show good agreement with experiments.
We demonstrated the tuning of whispering gallery modes (WGMs) of a silica microsphere during optical levitation through the annealing process. We determined the annealing temperature from the power balance between the CO2 laser light heating and several cooling processes. Cooling caused by heat conduction through the surrounding air molecules is the dominant process. We achieved a blue shift of the WGMs as large as 1 \%, which was observed in the white-light scattering spectrum from the levitated microsphere.
We experimentally demonstrate controlled polarization-selective phenomena in a whispering gallery mode resonator. We observed efficient ($\approx 75 %$) polarization conversion of light in a silica microsphere coupled to a tapered optical fiber with proper optimization of the polarization of the propagating light. A simple model treating the microsphere as a ring resonator provides a good fit to the observed behavior.
A tunable, all-optical, coupling method has been realized for a high-\textit{Q} silica microsphere and an optical waveguide. By means of a novel optical nanopositioning method, induced thermal expansion of an asymmetric microsphere stem for laser powers up to 171~mW has been observed and used to fine tune the microsphere-waveguide coupling. Microcavity displacements ranging from (0.612~$\pm$~0.13) -- (1.5 $\pm$ 0.13) $μ$m and nanometer scale sensitivities varying from (2.81 $\pm$ 0.08) -- (7.39 $\pm$ 0.17) nm/mW, with an apparent linear dependency of coupling distance on stem laser heating, we…
The scattering and absorption suppression of the silica microspheres is experimentally achieved by semicontinuous gold shell synthesized on the silica microspheres. These fractal gold shells on the silica spheres are shown to have significant extinction in the visible and mid-infrared spectral range. It is found that the silica scattering peak in the visible and the relative contribution of the vibrational stretching band in the infrared gradually decreases with increasing of the gold coverage.
Dissipative optomechanics has some advantages in cooling compared to the conventional dispersion dominated systems. Here, we study the optical response of a cantilever-like, silica, microsphere pendulum, evanescently coupled to a fiber taper. In a whispering gallery mode resonator the cavity mode and motion of the pendulum result in both dispersive and dissipative optomechanical interactions. This unique mechanism leads to an experimentally observable, asymmetric response function of the transduction spectrum which can be explained using coupled-mode theory. The optomechanical transduction, an…
Robust Radiative Cooling in Functionalizable Silica Microsphere Paints
Instituto de Ciencia de Materiales de Madrid (ICMM), Consejo Superior de Investigaciones Científicas (CSIC)（马德里材料科学研究所（ICMM），西班牙国家研究委员会（CSIC））；Cooling Photonics Sociedad Limitada（冷却光子学有限公司）；Universitat Politècnica de Catalunya（加泰罗尼亚理工大学）
Quantitative measurements of the vibrational eigenmodes in ultra-high-Q silica microspheres are reported. The modes are efficiently excited via radiation-pressure induced dynamical back-action of light confined in the optical whispering-gallery modes of the microspheres (i.e. via the parametric oscillation instability). Two families of modes are studied and their frequency dependence on sphere size investigated. The measured frequencies are in good agreement both with Lamb's theory and numerical finite element simulation and are found to be proportional to the sphere's inverse diameter.
We have tuned the whispering gallery modes of a fused silica microresonator over nearly 1 nm at 800 nm, i.e. over 0.5 FSR or 10^6 linewidths of the resonator. This has been achieved by a new method based on the stretching of a two-stem microsphere. The devices described below will permit new Cavity-QED experiments with this high-Q optical resonator when it is desirable to optimize its coupling to emitters with given transition frequencies. The tuning capability demonstrated here is compatible with both UHV and low temperature operation, which should be useful for future experiments with laser …
Accurate calculation of internal and surface scattering losses in fused silica microspheres is done. We show that in microspheres internal scattering is partly inhibited as compared to losses in the bulk material. We pay attention on the effect of frozen thermodynamical capillary waves on surface roughness. We calculate also the value of mode splitting due to backscattering and other effects of this backscattering.
A general model is presented for coupling of high-$Q$ whispering-gallery modes in optical microsphere resonators with coupler devices possessing discrete and continuous spectrum of propagating modes. By contrast to conventional high-Q optical cavities, in microspheres independence of high intrinsic quality-factor and controllable parameters of coupling via evanescent field offer variety of regimes earlier available in RF devices. The theory is applied to the earlier-reported data on different types of couplers to microsphere resonators and complemented by experimental demonstration of enhanced…
Daytime radiative cooling has attracted considerable attention recently due to its tremendous potential for passively exploiting the coldness of deep-sky as clean and renewable energy. Many advanced materials with novel photonic micro-nanostructures have already been developed to enable highly efficient daytime radiative coolers, among which the flexible hierarchical porous coatings (HPCs) are a more distinguished category. However, it is still hard to precisely control the size distribution of the randomized pores within the HPCs, usually resulting in a deficient solar reflection at the near-…
We investigate the feasibility of activating coherent mechanical oscillations in lasing microspheres by modulating the laser emission at a mechanical eigenfrequency. To this aim, 1.5% Nd3+:Barium-Titanium-Silicate microspheres with diameters around 50 μm were used as high quality factor (Q>10^6) whispering gallery mode lasing cavities. We have implemented a pump-and-probe technique in which the pump laser used to excite the Nd3+ ions is focused on a single microsphere with a microscope objective and a probe laser excites a specific optical mode with the evanescent field of a tapered fibre. The…
We report the direct observation of the electromagnetic-field distribution of whispering?gallery modes in silica microcavities (spheres and toroids). It is revealed by their excitation efficiency with a tapered fiber coupler swept along the meridian. The originality of this method lies in the use of the coupler itself for the near field mapping, eliminating the need of additional tools used in previous work. This method is successfully applied to microspheres and microtoroids
A high sensitivity force sensor based on dielectric microspheres in vacuum, optically trapped by a single, upward-propagating laser beam, is described. Off-axis parabolic mirrors are used both to focus the 1064~nm trapping beam and to recollimate it to provide information on the horizontal position of the microsphere. The vertical degree of freedom is readout by forming an interferometer between the light retroreflected by the microsphere and a reference beam, hence eliminating the need for auxiliary beams. The focus of the trapping beam has a 1/e$^2$ radius of 3.2~$μ$m and small non-Gaussian …
We report narrow linewidth optomechanical oscillation of a silica microsphere immersed in a buffer solution. Through a novel optomechanical transduction sensing approach, single 10-nm-radius silica beads and Bovine serum albumin (BSA) protein molecules with a molecular weight of 66 kDalton were detected. This approach predicts the detection of 3.9 kDalton single molecules at a signal-to-noise ration above unity.
We report a weighing metrology experiment of a single silica microsphere optically trapped and immersed in air. Based on fluctuations about thermal equilibrium, three different mass measurements are investigated, each arising from one of two principle methods. The first method is based on spectral analysis and enables simultaneous extraction of various system parameters. Additionally, the spectral method yields a mass measurement with systematic relative uncertainty of 3.0\% in 3~s and statistical relative uncertainty of 0.9\% across several trapping laser powers. Parameter values learned from…
Herein, we report sub-wavelength propagation and directional out-coupling of whispering gallery modes (WGMs) of a fluorescent silica microsphere resonator mediated via plasmon polaritons in a single crystalline silver nanowire. Fluorescent spectral signatures of emission from the nanowire ends confirm efficient guiding of WGMs via nanowire plasmons. By employing Fourier plane optical microscopy, we reveal and quantify the directional fluorescence emission of WGMs from the ends of the nanowire. Given that the discussed geometry is self-assembled from a solution-phase, our results will find rele…
Coherent inter-conversion between an optical and a mechanical excitation in an optomechanical resonator can be used for the storage of an optical pulse as an excitation in a mechanical oscillator. This optomechanical light storage is enabled by external writing and readout pulses at one mechanical frequency below the optical resonance. In this paper, we expand an earlier experimental study [Phys. Rev. Lett. 107, 133601 (2011)] on storing an optical pulse as a radial breathing mode in a silica microsphere. We show that the heterodyne beating between a readout pulse and the corresponding retriev…
In whispering gallery mode resonator sensing applications, the conventional way to detect a change in the parameter to be measured is by observing the steady state transmission spectrum through the coupling waveguide. Alternatively, cavity ring-up spectroscopy (CRUS) sensing can be achieved transiently. In this work, we investigate CRUS using coupled mode equations and find analytical solutions with a large spectral broadening approximation of the input pulse. The relationships between the frequency detuning, coupling gap and ring-up peak height are determined and experimentally verified using…
A theoretical model for describing the emission spectra of microsphere cavities is presented, and its prediction of detailed lineshapes of emission spectra associated with whispering gallery modes (WGMs) of various orders in ZnO microspheres (MSs) are verified experimentally by photoluminescence (PL) spectroscopy. The interplay of Purcell effect, quality factor, and leaky modes in spontaneous and stimulated emission spectra related to WGMs of all orders is revealed. The key success of the theory is based on the expansion of the full Green function of the MS in terms of all possible resonance m…
We theoretically and experimentally investigated the transition between modulation instability and Raman gain in a small silica microcavity with a large free-spectral range (FSR), which reveals that we can selectively switch from a four-wave mixing dominant state to a stimulated Raman scattering dominant state. Both the theoretical analysis and the experiment show that a Raman-dominant region is present between transitions of Kerr combs with different free-spectral range spacings. We can obtain a stable Kerr comb and a stable Raman state selectively by changing the driving power, coupling betw…
A high-Q silica whispering-gallery mode microresonator is an attractive platform on which to demonstrate a broad and phase-locked Raman comb in various wavelength regimes. Raman combs can be used for applications such as compact pulse laser sources, sensors, optical clocks, and coherence tomography. However, the formation dynamics of a Raman comb has not been well exploited. Here we study the dynamics of the Raman comb formation in silica rod microresonators, which have cavity free spectral ranges in microwave rates. We generated a Raman comb with a smooth spectral envelope and also observed t…
The influence of Raman scattering and higher order dispersions on solitons and frequency comb generation in silica microring resonators is investigated. The Raman effect introduces a threshold value in the resonator quality factor above which the frequency locked solitons can not exist and, instead, a rich dynamics characterized by generation of self-frequency shift- ing solitons and dispersive waves is observed. A mechanism of broadening of the Cherenkov radiation through Hopf instability of the frequency locked solitons is also reported.
We report on the use of 4.7-$μ$m-diameter, optically levitated, charged microspheres to image the three-dimensional force field produced by charge distributions on an Au-coated, microfabricated Si beam in vacuum. An upward-propagating, single-beam optical trap, combined with an interferometric imaging technique, provides optimal access to the microspheres for microscopy. In this demonstration, the Au-coated surface of the Si beam can be brought as close as ${\sim}10~μ$m from the center of the microsphere while forces are simultaneously measured along all three orthogonal axes, fully mapping th…
To date there are extensive studies of optical nonlinearities in whispering gallery resonators (WGRs) in the near and mid-infrared wavelengths. Pushing this research into the visible region is equally valuable. Here, we demonstrate a Kerr frequency comb and Raman lasing at 462 nm in an SiO2 WGR. Notably, due to the high optical intensities achieved, photodarkening is unavoidable and can quickly degrade the optical quality of both the coupling optical nanofiber and the microcavity even at very low pump powers. Nonetheless, stable stimulated Raman scattering (SRS) and hyper-parametric oscillatio…
By combining detailed imaging measurements at different tilt angles with simulations of ray emission from prolate deformed lasing micro-droplets, we conclude that the probability density for the lasing modes in a three-dimensional dielectric microcavity must reside in the chaotic region of the ray phase space. In particular, maximum emission from such chaotic lasing modes is not from tangent rays emerging from the highest curvature part of the rim. The laser emission is observed and calculated to be non-tangent and displaced from the highest curvature due to the presence of stable orbits. In t…
Frequency comb generation in microresonators at visible wavelengths has found applications in a variety of areas such as metrology, sensing, and imaging. To achieve Kerr combs based on four-wave mixing in a microresonator, dispersion must be in the anomalous regime. In this work, we demonstrate dispersion engineering in a microbubble resonator (MBR) fabricated by a two-CO$_2$ laser beam technique. By decreasing the wall thickness of the MBR down to 1.4 $μ$m, the zero dispersion wavelength shifts to values shorter than 764 nm, making phase matching possible around 765 nm. With the optical \text…
We fabricated polygonal silica toroidal microcavities to achieve stable mechanical coupling with an evanescent coupler such as a tapered fiber. The polygonal cavity was fabricated by using a combination of isotropic etching, anisotropic etching and laser reflow. It offers both high and low coupling efficiencies with the cavity mode even when the coupler is in contact with the cavity, which offers the possibility of taking the device outside the laboratory. A numerical simulation showed that an octagonal silica toroidal microcavity had an optical quality factor of 8.8\times10^6.
Multi-gigahertz mechanical vibrations stemming from interactions between light fields and matter, also known as acoustic phonons, have long been a subject of study. In recent years, specially designed functional devices have been developed to enhance the light-matter interaction strength, since the excitation of acoustic phonons by a continuous wave laser alone is insufficient. However, with such structure-dependent enhancements, the strength of the interaction cannot be aptly and instantly controlled. We propose a new technique to control the effective interaction strength, which is not via t…
