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arXiv 1601.06012physics.atom-phphysics.atm-clus
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光电子反作用于电离态$H_2^+$的电子定域

Electron localization in dissociating $H_2^+$ by retroaction of a photoelectron onto its source

M. Waitz, D. Aslitürk, N. Wechselberger, H. K. Gill, J. Rist, F. Wiegandt, C. Goihl, G. Kastirke, M. Weller, T. Bauer, D. Metz, F. P. Sturm, J. Voigtsberger, S.… 展开作者

M. Waitz, D. Aslitürk, N. Wechselberger, H. K. Gill, J. Rist, F. Wiegandt, C. Goihl, G. Kastirke, M. Weller, T. Bauer, D. Metz, F. P. Sturm, J. Voigtsberger, S. Zeller, F. Trinter, G. Schiwietz, T. Weber, J. B. Williams, M. S. Schöffler, L. Ph. H. Schmidt, T. Jahnke, R. Dörner

摘要:

我们调查的解离$H_2^+$成一个质子和$H^0$单电离后的能量接近阈值的光子。发现当$H_2^+$沿$1sσ_g$基态解离时,$p^+$和$H^0$并不对称出现.相反,可以观察到$p^+$在逃逸光电子的方向上的优先喷射。这种对称性破缺在电子能量很小的情况下是最强的。我们的实验与Serov和Kheietov最近的预测一致[Phys.Rev.A89,031402(2014)]。在他们的模型中,经典地处理光电子,对称性破缺是由长程库仑势对离解的$H_2^+$的反作用引起的。

英文摘要:

We investigate the dissociation of $H_2^+$ into a proton and a $H^0$ after single ionization with photons of an energy close to the threshold. We find that the $p^+$ and the $H^0$ do not emerge symmetrically in case of the $H_2^+$ dissociating along the $1sσ_g$ ground state. Instead, a preference for the ejection of the $p^+$ in the direction of the escaping photoelectron can be observed. This symmetry breaking is strongest for very small electron energies. Our experiment is consistent with a recent prediction by Serov and Kheifets [Phys. Rev. A 89, 031402 (2014)]. In their model, which treats the photoelectron classically, the symmetry breaking is induced by the retroaction of the long range Coulomb potential onto the dissociating $H_2^+$.

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