We observe a spontaneous parity breaking bifurcation to a ferromagnetic state in a spatially trapped exciton-polariton condensate. At a critical bifurcation density under nonresonant excitation, the whole condensate spontaneously magnetizes and randomly adopts one of two elliptically polarized (up to 95% circularly-polarized) states with opposite handedness of polarization. The magnetized condensate remains stable for many seconds at 5 K, but at higher temperatures it can flip from one magnetic orientation to another. We optically address these states and demonstrate the inversion of the magnetic state by resonantly injecting 100-fold weaker pulses of opposite spin. Theoretically, these phenomena can be well described as spontaneous symmetry breaking of the spin degree of freedom induced by different loss rates of the linear polarizations.
We report on spinor polariton interactions in GaAs based microcavities. This investigation is carried out by means of heterodyne polarized pump-probe spectroscopy. We show the dependence of the energy renormalization of the lower and upper polariton resonances with cavity detuning for different polariton densities. We use the exciton-photon based Gross-Pitaevskii equation to model the experiment for both lower and upper polariton modes. The theoretical results reproduce qualitatively the experimental observations revealing the magnitude and the sign of the parallel and anti-parallel spin inter…
We show that recent paper by Flayac et al. [Phys. Rev. B 81, 045318 (2010) and arXiv:0911.1650] is misleading. We demonstrate the existence of static half-quantum vortices in exciton-polariton condensates and calculate the warping of their polarization texture produced by TE-TM splitting of polariton band.
We realise bistability in the spinor of polariton condensates under non-resonant optical excitation and in the absence of biasing external fields. Numerical modelling of the system using the Ginzburg-Landau equation with an internal Josephson coupling between the two spin components of the condensate qualitatively describes the experimental observations. We demonstrate that polariton spin bistability persists for sweep times in the range of $[10 μsec,1 sec]$ offering a promising route to spin switches and spin memory elements.
We consider half-integer topological defects in a spinor Bose-Einstein condensate of exciton-polaritons. We show that they accelerate under the effect of an in-plane effective magnetic field, like regular electric charges in the electric field. The trajectories of these analogues of magnetic monopoles are derived analytically and checked by numerical simulations. We show that these "magnetic charges" propagate at large in-plane velocities and remain stable up to a critical magnetic field, thanks to the unique spin-anisotropy of polariton interactions.
We propose a new system for the study of event horizons and black holes - a Bose-Einstein condensate of exciton-polaritons. Hawking radiation from a closed horizon in 2D is observed in numerical experiments. We simulate inter-Universe and intra-Universe wormholes capitalizing on the spinor nature of polariton condensates and on the spin dependence of polariton-polariton interactions.
We consider theoretically one-dimensional polariton ring accounting for both longitudinal-transverse (TE-TM) and Zeeman splitting of spinor polariton states and spin dependent polariton-polariton interactions. We present the novel class of solutions in the form of the localized defects rotating with constant angular velocity and analyze their properties for realistic values of the parameters of the system. We show that the effects of the geometric phase arising from the interplay between external magnetic field and TE-TM splitting introduce chirality in the system and make solitons propagating…
Recently, split-ring bosonic condensates of exciton polaritons have been proposed for realisation of qubits. We formulate an analytical model of a polariton condensate in a one-dimensional ring split by a delta-function potential. The persistent current is stopped by the potential defect embedded in a scalar condensate of non-interacting particles, however, it reappears in the presence of an up-critical non-linearity. The nonlinear supercurrents are characterised by fractional orbital momenta while their eigenfunctions may feature grey or dark solitons. The coupling between the spin and the or…
We consider effective interactions in a 2D hybrid polariton- electron system and calculate dispersion of elementary excitations accounting the spin degree of freedom of the particles. Due to the crucial role played by the exchange term in polariton- electron interactions the dispersions of this system become spin- dependent and show unusual behavior. The coupling of the excitations of the condensate with 2D plasmon can result in appearence of roton minimum in the dispersion and destruction of the condensate for close enough situated quantum wells with electrons and excitons.
We theoretically demonstrate the generation of dark solitons trains in a one-dimensional exciton- polariton condensate within an experimentally trivial scheme. In particular we show that the fre- quency of the train can be finely tuned either electrically of fully optically to provide a stable and efficient output signal modulation. Taking the polarization degree of freedom into account we elucidate the possibility to additionally form on-demand half-solitons trains.
We propose a pump-probe set-up to analyse the properties of the collective excitation spectrum of a spinor polariton fluid. By using a linear response approximation scheme, we carry on a complete classification of all excitation spectra, as well as their intrinsic degree of polarisation, in terms of two experimentally tunable parameters only, the mean-field polarisation angle and a rescaled pump detuning. We evaluate the system response to the external probe, and show that the transmitted light can undergo a spin rotation along the dispersion for spectra that we classify as diffusive-like. We …
In this work I introduce a powerful analytical method to analyze states of non-equilibrium polariton Bose-Einstein condensates (BEC). It is shown that the condensate wave functions carrying dark solitons and half-dark solitons can be expressed in terms of the natural parameters of the non-equilibrium system, i.e. the growth and decay rates and the interaction parameters. The derivation is based on a non-conservative Lagrangian formalism, which provides ordinary differential equations for the parameters of the dark soliton solutions in their dynamic environment. Explicit expressions for the sta…
We investigate the spin dynamics of half-solitons in polariton Bose-Einstein condensates. Half-solitons, which behave as magnetic monopoles, can be accelerated in the presence of the effective magnetic field of the microcavity. We study the generation of DC magnetic currents in a gas of half-solitons. At low densities, the current is suppressed due to the dipolar oscillations. At moderate densities, a magnetic current is recovered as a consequence of the collisions between the carriers. We show a deviation from Ohm's law due to the competition between magnetic dipoles and monopoles.
We theoretically explore nonresonantly pumped polaritonic graphene, a system consisting of a honeycomb lattice of micropillars in the regime of strong light-matter coupling. We demonstrate that, depending on the parameters of the structure, such as intensity of the pump and coupling strength between the pillars, the system shows rich variety of macroscopic ordering, including analogs of ferromagnetic, antiferromagnetic, and resonant valence bond phases. Transitions between these phases are associated with dramatic reshaping of the spectrum of the system connected with spontaneous appearance of…
In a recent work [H. Flayac, I.A. Shelykh, D.D. Solnyshkov and G. Malpuech, Phys. Rev. B 81, 045318 (2010)], we have analyzed the effect of the TE-TM splitting on the stability of the exciton-polariton vortex states. We considered classical vortex solutions having cylindrical symmetry and we found that the so-called half-vortex states [Yu. G. Rubo, Phys. Rev. Lett. 99, 106401 (2007)] are not solutions of the stationary Gross-Pitaevskii equation. In their Comment [M. Toledo Solano, Yu.G. Rubo, Phys. Rev. B 82, 127301 (2010)], M. Toledo Solano and Yuri G. Rubo claim that this conclusion is misle…
We report on the observation of spin whirls in a radially expanding polariton condensate formed under non-resonant optical excitation. Real space imaging of polarization- and time-resolved photoluminescence reveal a spiralling polarization pattern in the plane of the microcavity. Simulations of the spatiotemporal dynamics of a spinor condensate reveal the crucial role of polariton interactions with a spinor exciton reservoir. Harnessing spin dependent interactions between the exciton reservoir and polariton condensates allows for the manipulation of spin currents and the realization of dynamic…
First order coherence measurements of a polariton condensate, reveal a regime where the condensate pseudo-spin precesses persistently within the driving optical pulse. Within a single 20 $μ$s optical pulse the condensate pseudo-spin performs over $10^5$ precessions with striking frequency stability. The condensate maintains its phase coherence even after a complete precession of the spin vector, making the observed state by a definition a spin coherent state. The emergence of the precession is traced to the polariton interactions that give rise to a self-induced out-of-plane magnetic field tha…
Subcritical bifurcation and on-off bistability in ballistic polariton condensates
Korea Advanced Institute of Science and Technology (KAIST)（韩国科学技术院）；Institute for Basic Science (IBS)（基础科学研究院）；St. Petersburg State University（圣彼得堡国立大学）；Moscow Institute of Physics and Technology（莫斯科物理技术学院）；ITMO University（ITMO大学）
We investigate an optically trapped exciton-polariton condensate and observe temporal coherence beyond 1~ns duration. Due to the reduction of the spatial overlap with the thermal reservoir of excitons, the coherence time of the trapped condensate is more than an order of magnitude longer than that of an untrapped condensate. This ultralong coherence enables high precision spectroscopy of the trapped condensate, and we observe periodic beats of the field correlation function due to a fine energy splitting of two polarization modes of the condensate. Our results are important for realizing polar…
We study the formation of chaos and strange attractors in the order parameter space of a system of two coupled, non-resonantly driven exciton-polariton condensates. The typical scenario of bifurcations experienced by the system with increasing external pumping consists of (i) formation of $π$-synchronized condensates at low pumping, (ii) symmetry breaking pitchfork bifurcation leading to unequal occupations of the condensates with non-trivial phase difference between them, (iii) loss of the stability of all fixed points in the system resulting in chaotic dynamics, (iv) limit cycle dynamics of …
We generalize the spin Meissner effect for exciton-polariton condensate confined in annular geometries to the case of non-trivial topology of the condensate wavefunction. In contrast to the conventional spin Meissner state, topological spin Meissner states can in principle be observed at arbitrary high magnetic field not limited by the critical magnetic field value for the condensate in a simply-connected geometry. One special example of the topological Meissner states are half-vortices. We show that in the absence of magnetic field half-vortices in a ring exist in a form of superposition of e…
Collective (elementary) excitations of quantum bosonic condensates, including condensates of exciton polaritons in semiconductor microcavities, are a sensitive probe of interparticle interactions. In anisotropic microcavities with momentum-dependent TE-TM splitting of the optical modes, the excitations dispersions are predicted to be strongly anisotropic, which is a consequence of the synthetic magnetic gauge field of the cavity, as well as the interplay between different interaction strengths for polaritons in the singlet and triplet spin configurations. Here, by directly measuring the disper…
We demonstrate that multiply-coupled spinor polariton condensates can be optically tuned through a sequence of spin-ordered phases by changing the coupling strength between nearest neighbors. For closed 4-condensate chains these phases span from ferromagnetic (FM) to antiferromagnetic (AFM), separated by an unexpected crossover phase. This crossover phase is composed of alternating FM-AFM bonds. For larger 8 condensate chains, we show the critical role of spatial inhomogeneities and demonstrate a scheme to overcome them and prepare any desired spin state. Our observations thus demonstrate a fu…
Nonlinear interactions in coherent gases are not only at the origin of of bright and dark solitons and superfluids. At the same time, they give rise to phenomena such as multistability, which hold great promise for the development of advanced photonic and spintronic devices. In particular, spinor multistability in strongly-coupled semiconductor microcavities shows that the spin of hundreds of exciton-polaritons can be coherently controlled, opening the route to spin-optronic devices such as ultrafast spin memories, gates or even neuronal communication schemes. Here, we demonstrate that switchi…
We determine experimentally the spinor interaction constants of lower-polaritons $α_1$ and $α_2$ using resonant pump-probe spectroscopy with a spectrally narrow pump pulse. Our experimental findings are analyzed with the Bogoliubov-like theory and mean-field two channel model based on the lower-polariton and biexciton basis. We find an enhancement of the attractive interaction and dissipative nonlinearity of lower-polaritons with anti-parallel spins in the vicinity of the biexciton resonance when the energy of two lower-polaritons approaches energetically that of the biexciton. These observati…
We calculate the dispersion of spinor exciton-polaritons in a planar microcavity with its active region containing a single Transitional Metal Dichalcogenide (TMD) monolayer, taking into account excitonic and photonic spin-orbit coupling. We consider the radial propagation of polaritons in presence of disorder. We show that the reduction of the disorder scattering induced by the formation of polariton states allows to observe an optical Valley Hall effect, namely the coherent precession of the locked valley and polarization pseudospins leading to the formation of spatial valley-polarized domai…
The formation of nonlinear Bloch states in open driven-dissipative system of exciton-polaritons loaded into a weak-contrast 1D periodic lattice is studied numerically and analytically. The condensate is described within the framework of mean-field theory by the coupled equations for the order parameter and for the density of incoherent excitons. The stationary nonlinear solutions having the structure of Bloch waves are studied in detail. It is shown that there is a bifurcation leading to the appearance of a family of essentially nonlinear states. The special feature of these solutions is that …
We report on noise-induced-spin-ordering in a collective quasipaticle system: spinor stochastic resonance. Synergetic interplay of a polarization-modulated signal and a polarization-noise allows us to switch coherently between the two metastable states of a microcavity-polariton spin bistable system. Spinor stochastic resonance is demonstrated in a zero-dimensional GaAs based microcavity. The resonance behavior of both the spin amplification and the signal-to-noise ratio are experimentally evidenced as a function of the noise strength for different amplitude modulations. They are theoretically…
Half-vortices have been recently shown to be the elementary topological defects supported by a spinor cavity exciton-polaritons condensates with spin anisotropic interactions (Y. G. Rubo, Phys. Rev. Lett. 99, 106401 (2007)). A half vortex is composed by an integer vortex for one circular component of the condensate, whereas the other component remain static. We analyze theoretically the effect of the splitting between TE and TM polarized eigen modes on the structure of the vortices in this system. For TE and TM modes, the polarization states depend on the direction of propagations of particles…
We investigate, through polarization-resolved spectroscopy, the spin transport by propagating polariton condensates in a quasi one-dimensional microcavity ridge along macroscopic distances. Under circularly polarized, continuous-wave, non-resonant excitation, a sinusoidal precession of the spin in real space is observed, whose phase depends on the emission energy. The experiments are compared with simulations of the spinor-polariton condensate dynamics based on a generalized Gross-Pitaevskii equation, modified to account for incoherent pumping, decay and energy relaxation within the condensate…
An infinite chain of driven-dissipative condensate spins with uniform nearest-neighbor coherent coupling is solved analytically and investigated numerically. Above a critical occupation threshold the condensates undergo spontaneous spin bifurcation (becoming magnetized) forming a binary chain of spin-up or spin-down states. Minimization of the bifurcation threshold determines the magnetic order as a function of the coupling strength. This allows control of multiple magnetic orders via adiabatic (slow ramping of) pumping. In addition to ferromagnetic and anti-ferromagnetic ordered states we sho…
We present a comprehensive theoretical description of quantum well exciton-polaritons imbedded in a planar semiconductor microcavity. The exact non-local dielectric response of the quantum well exciton is treated in detail. The 4-spinor structure of the hole subband in the quantum well is considered, including the pronounced band mixing effect. The scheme is self-contained and can be used to treat different semiclassical aspects of the microcavity properties. As an example, we analyze the "selection" rules for the exciton-cavity mode coupling for different excitons.
We present a model for theoretical description of the dynamics of a system of spinor cavity polaritons in real space and time accounting for all relevant types of the interactions and effective magnetic fields. We apply our general formalism for the consideration of the polarization dynamics of the coherently driven one dimensional polariton channel. We investigate effect of the temperature and the longitudinal-transverse splitting on the spin (polarization) multistability and hysteresis arising from the polarization-dependent polariton-polariton interaction. We show that the effect of the pha…
We study, theoretically and numerically, the onset and development of modulational instability in an incoherently pumped spatially homogeneous polariton condensate. Within the framework of mean-field theory, we identify regimes of modulational instability in two cases: 1) Strong feedback between the condensate and reservoir, which may occur in scalar condensates, and 2) Parametric scattering in the presence of polarization splitting in spinor condensates. In both cases we investigate the instability induced textures in space and time including non-equilibrium dynamics of phase dislocations and…
We predict the spontaneous modulated emission from a pair of exciton-polariton condensates due to coherent (Josephson) and dissipative coupling. We show that strong polariton-polariton inter- action generates complex dynamics in the weak-lasing domain way beyond Hopf bifurcations. As a result, the exciton-polariton condensates exhibit self-induced oscillations and emit an equidistant frequency comb light spectrum. A plethora of possible emission spectra with asymmetric peak dis- tributions appears due to spontaneously broken time-reversal symmetry. The lasing dynamics is affected by the shot n…
We address evolution of a spinor polariton condensate in radially periodic potentials. Such potentials allow for the observation of novel nonlinear excitations and support a variety of dynamically stable soliton states never demonstrated before in polariton condensates, including ring-like solitons with density peaks located in different radial minima of the potential and extended dynamically stable multiring patterns. Among the advantages of the system is that azimuthal modulational instabilities are suppressed due to dominating repulsive interactions between polaritons with the same spin, th…
For dipole-carrying excitations observed in a high-quality resonator, strong-coupling modes can appear as composite bosons with the spontaneous formation of quantized vortices in the condensed phase of a polariton fluid. In exciton-polaritons, in particular, it leads to sustained trapping of the emitted photon. In this paper, we show that magnon-polaritons can be realized due to magnon condensation caused by magnetic dipole-dipole interaction. In a quasi-2D ferrite disk placed in a microwave cavity, one observes quantum confinement effects of magnetic-dipolar-mode (MDM) oscillations. These mod…
The newly discovered valley degree of freedom in atomically thin two-dimensional transition metal dichalcogenides (TMD) offers a promising platform to explore rich nonlinear physics, such as spinor Bose-Einstein condensate (BEC) and novel valleytronics applications. However, the critical nonlinear effect, such as valley polariton bosonic stimulation, has long remained an unresolved challenge due to the generation of limited polariton ground state densities necessary to induce the stimulated scattering of polaritons in specific valleys. Here, we report the self-induced valley bosonic stimulatio…
We analyse nonequilibrium phase transitions in microcavity polariton condensates trapped in optically induced annular potentials. We develop an analytic model for annular optical traps, which gives an intuitive interpretation for recent experimental observations on the polariton spatial mode switching with variation of the trap size. In the vicinity of polariton lasing threshold we then develop a nonlinear mean-field model accounting for interactions and gain saturation, and identify several bifurcation scenarios leading to formation of high angular momentum quantum vortices. For experimentall…
We studied optical response of microcavity non-equilibrium exciton-polariton Bose-Einstein condensate with saturable nonlinearity under simultaneous resonant and non-resonant pumping. We demonstrated the emergence of multistabile behavior due to the satutration of the excitonic absorbtion. Stable periodic Rabi- type oscillations of the excitonic and photonic condensate components in the regime of the stationary pump and their transition to the chaotic dynamics through the cascade of Hopf bifurcations by tuning of the electrical pump are revealed.
Hidden chirality and half-vortex formation in exciton-polariton condensates
School of Physics and Engineering, ITMO University（ITMO大学物理与工程学院）；Hybrid Photonics Laboratory, Skolkovo Institute of Science and Technology（斯科尔科沃科学技术学院混合光子学实验室）
The phase and the frequency of an exciton polariton condensate excited by a nonresonant pump can be efficiently manipulated by an external coherent light. Being tuned close to the resonance with the condensate eigenfrequency, the external laser light imposes its frequency to the condensate and locks its phase, thereby manifesting a synchronization effect. The conditions of formation of the phase synchronized regime are determined. The synchronization of a couple of closely spaced polariton condensates by a spatially uniform coherent light is examined. At the moderate strength of the coherent d…
Theoretical study is performed of a single-mode polariton system with linear coupling of spin components. When combined with an ordinary two-particle interaction, the spin coupling involves a spontaneous symmetry breaking accompanied by a switch from linear to circular polarization under resonant driving. The asymmetric steady states can also lose stability, giving way to oscillatory and chaotic dynamics. Here, we explore a continuous transformation between the multistable regime, where the system is steady and locked in phase to the pump but has a broken spin symmetry, and full-span oscillati…
Exciton polaritons in semiconductor microcavities exhibit many fundamental physical effects, with some of them amenable to being controlled by external fields. The polariton transport is affected by the polaritonic spin-orbit interaction, which is caused by the splitting of transverse-electric and transverse-magnetic (TE-TM) modes. This is the basis for a polaritonic Hall effect, called optical spin Hall effect (OSHE), which is related to the formation of spin/polarization textures in momentum space, determining anisotropic ballistic transport, as well as related textures in real space. Owing …
We consider dark solitons and their stability in spin-orbit coupled polariton condensates. The system supports spinor solitons of two types: conventional (symmetric) dark solitons and asymmetric half-dark solitons. They demonstrate essentially different behavior upon variation of the strength of spin-orbit coupling. One-dimensional spin-orbit coupled dark solitons are usually unstable, while half-dark solitons can be stable. Two-dimensional dark solitons at early stages of the development of transverse instabilities turn into asymmetric snaking patterns and later into sets of vortex-antivortex…
We study Bogoliubov excitations of a spinor Bose Einstein condensate in a honeycomb periodic potential, in the presence of a Zeeman field and of a spin-orbit coupling specific for photonic systems, which is due to the energy splitting between TE and TM polarized eigenstates. We also consider spin-anisotropic interactions typical for cavity polaritons. We show that the non-trivial topology of the single particle case is also present for the interacting system. At low condensate density, the topology of the single-particle bands is transferred to the bogolon dispersion. At a critical value, the …
