We predict several effects associated with the optical response of systems prepared in a nonequilibrium state by impulsive optical excitations. The linear response depends on the phase of the electric field even if the initial nonequilirbium state has only populations, no coherences. Initial quantum coherences induce additional phase dependence which also shows new resonances in nonlinear wave mixing. In systems strongly driven by an external optical field, the field frequency generates a phase dependent probe absorption. This gives further control to manipulate the relative contribution to the linear signal due to initial populations and coherences.
Quantum probes are atomic-sized devices mapping information of their environment to quantum mechanical states. By improving measurements and at the same time minimizing perturbation of the environment, they form a central asset for quantum technologies. We realize spin-based quantum probes by immersing individual Cs atoms into an ultracold Rb bath. Controlling inelastic spin-exchange processes between probe and bath allows mapping motional and thermal information onto quantum-spin states. We show that the steady-state spin-population is well suited for absolute thermometry, reducing temperatur…
We study the role of excited phonon populations in the relaxation rates of nonequilibrium electrons using a nonequilibrium Green's function formalism. The transient modifications in the phononic properties are accounted for by self-consistently solving the Dyson equation for the electron and phonon Green's functions. The pump induced changes manifest in both the electronic and phononic spectral functions. We find that the excited phonon populations suppress the decay rates of nonequilibrium electrons due to enhanced phonon absorption. The increased phonon occupation also sets the nonequilibriu…
We characterize photonic transport in a boundary driven array of nonlinear optical cavities. We find that the output field suddenly drops when the chain length is increased beyond a threshold. After this threshold a highly chaotic and unstable regime emerges, which marks the onset of a super-diffusive photonic transport. We show the scaling of the threshold with pump intensity and nonlinearity. Finally, we address the competition of disorder and nonlinearity presenting a diffusive-insulator phase transition.
We report a theoretical non-equilibrium description of polaritonics and we propose ultrafast all- optical switching due to highly nonlinear polaritonics. The electronic band structure within gold (Au) nano grains is modified by external laser light. The Au grains are coupled to a single mode photonic waveguide and we derive a strong transmission reduction of switching originating from the establishd quantum interference with a finite lifetime.
We study quantum dynamics in the framework of repeated interactions between a system and a stream of identical probes. We present a coarse-grained master equation that captures the system's dynamics in the natural regime where interactions with different probes do not overlap, but is otherwise valid for arbitrary values of the interaction strength and mean interaction time. We then apply it to some specific examples. For probes prepared in Gibbs states, such channels have been used to describe thermalisation: while this is the case for many choices of parameters, for others one finds out-of-eq…
We show that inflationary cosmology may be used to test the statistical predictions of quantum theory at very short distances and at very early times. Hidden-variables theories, such as the pilot-wave theory of de Broglie and Bohm, allow the existence of vacuum states with non-standard field fluctuations ('quantum nonequilibrium'). We show that inflationary expansion can transfer microscopic nonequilibrium to macroscopic scales, resulting in anomalous power spectra for the cosmic microwave background. The conclusions depend only weakly on the details of the de Broglie-Bohm dynamics. We discuss…
Symmetries play a crucial role in ubiquitous systems found in Nature. In this work, we propose an elegant approach to detect symmetries by measuring quantum currents. Our detection scheme relies on initiating the system in an anti-symmetric initial condition, with respect to the symmetric sites, and using a probe that acts like a local noise. Depending on the position of the probe the currents exhibit unique signatures such as a quasi-stationary plateau indicating the presence of meta-stability and multi-exponential decays in case of multiple symmetries. The signatures are sensitive to the pro…
What is the minimum time required to take a temperature? In this paper, we solve this question for a large class of processes where temperature is inferred by measuring a probe (the thermometer) weakly coupled to the sample of interest, so that the probe's evolution is well described by a quantum Markovian master equation. Considering the most general control strategy on the probe (adaptive measurements, arbitrary control on the probe's state and Hamiltonian), we provide bounds on the achievable measurement precision in a finite amount of time, and show that in many scenarios these fundamental…
We explore the quantum metrology in an optical molecular system coupled to two environments with different temperatures, using a quantum master equation beyond secular approximation. We discover that the steady-state coherence originating from and sustained by the nonequilibrium condition can enhance quantum metrology. We also study the quantitative measures of the nonequilibrium condition in terms of the curl flux, heat current and entropy production at the steady state. They are found to grow with temperature difference. However, an apparent paradox arises considering the contrary behaviors …
We investigate the nonlinear light-matter interaction of a Bose-Einstein condensate trapped in an external periodic potential inside an optical cavity which is weakly coupled to vacuum radiation modes and driven by a transverse pump field. Based on a generalized Bose-Hubbard model which incorporates a single cavity mode, we include the collective backaction of the atoms on the cavity light field and determine the nonequilibrium quantum phases within the nonperturbative bosonic dynamical mean-field theory.With the system parameters adapted to recent experiments, we find a quantum phase transiti…
We present a theoretical approach to optical spectroscopy of open nonequilibrium systems, which generalizes traditional nonlinear optical spectroscopy tools by imposing charge and energy conservation at all levels of approximation. Both molecular and radiation field degrees of freedom are treated quantum mechanically. The formulation is based on the nonequilibrium Green's function (NEGF) approach and a double sided Feynman diagrammatic representation of the photon flux is developed. Numerical simulations are presented for a model system. Our study bridges the theoretical approaches of quantum …
We investigate the effect of many-body interactions on the optical absorption spectrum of a charge-tunable quantum dot coupled to a degenerate electron gas. A constructive Fano interference between an indirect path, associated with an intra dot exciton generation followed by tunneling, and a direct path, associated with the ionization of a valence-band quantum dot electron, ensures the visibility of the ensuing Fermi-edge singularity despite weak absorption strength. We find good agreement between experiment and renormalization group theory, but only when we generalize the Anderson impurity mo…
We study quasiparticle scattering effects on the dynamics of a homogeneous Bose-Einstein condensate of ultracold atoms coupled to a single mode of an optical cavity. The relevant excitations, which are polariton-like mixed excitations of photonic and atomic density-wave modes, are identified. All the first-order correlation functions are presented by means of the Keldysh Green's function technique. Beyond confirming the existence of the resonant enhancement of Beliaev damping, we find a very structured spectrum of fluctuations. There is a spectral hole burning at half of the recoil frequency r…
We derive universal properties of nonlinear response functions of nonequilibrium steady states. In particular, sum rules and asymptotic behaviors are derived. Their consequences are illustrated for nonlinear optical materials and nonlinear electrical conductors.
We develop an interferometric technique for making time-resolved measurements of field-quadrature operators for nonequilibrium ultracold bosons in optical lattices. The technique exploits the internal state structure of magnetic atoms to create two subsystems of atoms in different spin states and lattice sites. A Feshbach resonance turns off atom-atom interactions in one spin subsystem, making it a well-characterized reference state, while atoms in the other subsystem undergo nonequilibrium dynamics for a variable hold time. Interfering the subsystems via a second beam-splitting operation, tim…
We show how a quantum Ising spin chain in a time-dependent transverse magnetic field can be simulated and experimentally probed in the framework of circuit QED with current technology. The proposed setup provides a new platform for observing the nonequilibrium dynamics of interacting many-body systems. We calculate its spectrum to offer a guideline for its initial experimental characterization. We demonstrate that quench dynamics and the propagation of localized excitations can be observed with the proposed setup and discuss further possible applications and modifications of this circuit QED q…
Detecting nonequilibrium phase transitions via continuous monitoring of space-time trajectories and autoencoder-based clustering
Institut für Theoretische Physik, Universität Tübingen（蒂宾根大学理论物理研究所）；Université Paris Cité, CNRS, Matériaux et Phénomènes Quantiques（巴黎西岱大学、法国国家科学研究中心、物质与量子现象）；Centre for Fluid and Complex Systems, Coventry University（考文垂大学流体与复杂系统中心）；The University of Nottingham（诺丁汉大学）
We show that a hybrid atom-optomechanical quantum many-body system with two internal atom states undergoes both first- and second-order nonequilibrium quantum phase transitions. A nanomembrane is placed in a pumped optical cavity, whose outcoupled light forms a lattice for an ultracold Bose gas. By changing the pump strength, the effective membrane-atom coupling can be tuned. Above a critical intensity, a symmetry-broken phase emerges which is characterized by a sizeable occupation of the high-energy internal states and a displaced membrane. The order of this nonequilibrium quantum phase trans…
The Dicke model describes the coupling between a quantized cavity field and a large ensemble of two-level atoms. When the number of atoms tends to infinity, this model can undergo a transition to a superradiant phase, belonging to the mean-field Ising universality class. The superradiant transition was first predicted for atoms in thermal equilibrium and was recently realized with a quantum simulator made of atoms in an optical cavity, subject to both dissipation and driving. In this Progress Report, we offer an introduction to some theoretical concepts relevant to the Dicke model, reviewing t…
We perform an ab-initio comparison between nonequilibrium dynamical mean-field theory and optical lattice experiments by studying the time evolution of double occupations in the periodically driven Fermi-Hubbard model. For off-resonant driving, the range of validity of a description in terms of an effective static Hamiltonian is determined and its breakdown due to energy absorption close to resonance is demonstrated. For near-resonant driving, we investigate the response to a change in driving amplitude and discover an asymmetric excitation spectrum with respect to the detuning. In general, we…
