We considered the two-photon adiabatic rapid passage excitation of a single atom from the ground to a Rydberg state. Three schemes were analyzed: both pump and Stokes fields chirped and pulsed, only the pump field is chirped, and only the pump field is pulsed and chirped while the Stokes field is continuous wave (CW). In all three cases high transfer efficiencies $>99\%$ were achieved for the experimentally realizable Rabi frequencies and the pulse durations of the fields.
We review methods for coherently controlling Rydberg quantum states of atomic ensembles using Adiabatic Rapid Passage and Stimulated Raman Adiabatic Passage. These methods are commonly used for population inversion in simple two-level and three-level systems. We show that adiabatic techniques allow us to control population and phase dynamics of complex entangled states of mesoscopic atomic ensembles for quantum information processing with Rydberg atoms. We also propose several schemes of single-qubit and two-qubit gates based on adiabatic passage, Rydberg blockade and Förster resonances in Ryd…
In an atomic ensemble, quantum information is typically carried as single collective excitations. It is very advantageous if the creation of single excitations is efficient and robust. Rydberg blockade enables deterministic creation of single excitations via collective Rabi oscillation by precisely controlling the pulse area, being sensitive to many experimental parameters. In this paper, we implement the adiabatic rapid passage technique to the Rydberg excitation process in a mesoscopic atomic ensemble. We make use of a two-photon excitation scheme with an intermediate state off-resonant and …
Rydberg blockaded gate is a fundamental ingredient for scalable quantum computation with neutral Rydberg atoms. However the fidelity of such a gate is intrinsically limited by a blockade error coming from a Rydberg level shift that forbids its extensive use. Based on a dark-state adiabatic passage, we develop a novel protocol for realizing a two-atom blockade-error-free quantum gate in a hybrid system with simultaneous van der Waals (vdWsI) and resonant dipole-dipole interactions (DDI). The basic idea relies on converting the roles of two interactions, which is, the DDI serves as one time-depe…
We analyze neutral atom Rydberg $C_Z$ gates based on adiabatic pulses applied symmetrically to both atoms. Analysis with smooth pulse shapes and Cs atom parameters predicts the gates can create Bell states with fidelity ${\mathcal F}>0.999$ using adiabatic rapid passage (ARP) pulses. With globally optimized adiabatic pulse shapes, in a two-photon excitation process, we generate Bell states with fidelity ${\mathcal F}=0.997$. The analysis fully accounts for spontaneous emission from intermediate and Rydberg states, including the Rydberg lifetime in a room temperature environment, but does not i…
We analyze excitation of two ground state atoms to a double Rydberg state by a two-photon chirped optical pulse in the regime of adiabatic rapid passage. For intermediate Rydberg-Rydberg interaction strengths, relevant for atoms separated by $\sim$ten $μ$m, adiabatic excitation can be achieved at experimentally feasible Rabi frequencies and chirp rates of the pulses, resulting in high transfer efficiencies. We also study the adiabatic transfer between ground and Rydberg states as a means to realize a controlled phase gate between atomic qubits.
High-fidelity entangled Bell states are of great interest in quantum physics. Entanglement of ultracold neutral atoms in two spatially separated optical dipole traps is promising for implementation of quantum computing and quantum simulation and for investigation of Bell states of material objects. We propose a new method to entangle two atoms via long-range Rydberg-Rydberg interaction. Alternatively to previous approaches, based on Rydberg blockade, we consider radiofrequency-assisted Stark-tuned Förster resonances in Rb Rydberg atoms. To reduce the sensitivity of the fidelity of Bell states …
We develop a scheme for deterministic generation of an entangled state between two atoms on different Rydberg states via a chirped adiabatic passage, which directly connects the initial ground and target entangled states and also does not request the normally needed blockade effect. The occupancy of intermediate states suffers from a strong reduction via two pulses with proper time-dependent detunings and the electromagnetically induced transparency condition. By solving the analytical expressions of eigenvalues and eigenstates of a two-atom system, we investigate the optimal parameters for gu…
We propose schemes of controlled-Z and controlled-NOT gates with ultracold neutral atoms based on deterministic phase accumulation during double adiabatic passage of the Stark-tuned Förster resonance of Rydberg states. The effect of deterministic phase accumulation during double adiabatic passage in a two-level quantum system has been analyzed in detail. Adiabatic rapid passage using nonlinearly chirped pulses with rectangle intensity profile has been discussed. Nonlinear time dependence of the energy detuning from the Förster resonance is used to achieve a high fidelity of population transfer…
Entangled states are crucial for modern quantum enabled technology which makes their creation key for future developments. In this paper, a robust quantum control methodology is presented to create entangled states of two typical classes, the W and the Greenberger-Horne-Zeilinger (GHZ). It was developed from the analysis of a chain of alkali atoms $^{87}Rb $ interaction with laser pulses, which lead to the two-photon transitions from the ground to the Rydberg states with a predetermined magnetic quantum number. The methodology is based on the mechanism of two-photon adiabatic passage using ove…
We implement high-efficiency coherent excitation to a Rydberg state using stimulated Raman adiabatic passage in a cold atom electron and ion source. We achieve an efficiency of 60% averaged over the laser excitation volume with a peak efficiency of 82%, a 1.6 times improvement relative to incoherent pulsed-laser excitation. Using pulsed electric field ionization of the Rydberg atoms we create electron bunches with durations of 250 ps. High-efficiency excitation will increase source brightness, crucial for ultrafast electron diffraction experiments, and coherent excitation to high-lying Rydberg…
We study angular-momentum couplings in $^{87}$Rb$_2$ Rydberg molecules formed between Rydberg and 5S$_{1/2}$ ground-state atoms. We use a Fermi model that includes S-wave and P-wave singlet and triplet scattering of the Rydberg electron with the 5S$_{1/2}$ atom, along with the fine structure coupling of the Rydberg atom and hyperfine structure coupling of the 5S$_{1/2}$ atom. We discuss the effects of these couplings on the adiabatic molecular potentials. We obtain bound-state energies, lifetimes, and electric and magnetic dipole moments for the vibrational ground states of the $^{87}$Rb$(n$D$…
Ultralong-range Rydberg molecules provide an exciting testbed for molecular physics at exaggerated scales. In the so-called trilobite and butterfly Rydberg molecules, the Born-Oppenheimer approximation can fail due to strong non-adiabatic couplings arising from the combination of radial oscillations and rapid energy variations in the adiabatic potential energy curves. We utilize an accurate coupled-channel treatment of the vibronic system to observe the breakdown of Born-Oppenheimer physics, such as non-adiabatic trapping and decay of molecular states found near pronounced avoided crossings in…
We discuss three proposed schemes of initializing circular-state Rydberg atoms via optical couplings provided by the ponderomotive effect in contrast to the current circularization methods that utilize electric-dipole interactions. In our first proposed method, a radial optical trap consisting of two Laguerre-Gaussian beams of opposite winding numbers transfers orbital angular momentum to the Rydberg atom, providing a first-order coherent coupling between an F-state and a circular state. Additionally, we propose a one-dimensional ponderomotive optical lattice modulated at rf frequencies, provi…
Motivated by recent progress in the experimental manipulation of cold atoms in optical lattices, we study three different protocols for non-adiabatic quantum state preparation and state transport in chains of Rydberg atoms. The protocols we discuss are based on the blockade mechanism between atoms which, when excited to a Rydberg state, interact through a van der Waals potential, and rely on single-site addressing. Specifically, we discuss protocols for efficient creation of an antiferromagnetic GHZ state, a class of matrix product states including a so-called Rydberg crystal and for the state…
In this paperwe propose two theoretical schemes for implementation of quantum phase gates by engineering the phase-sensitive dark state of two atoms subjected to Rydberg-Rydberg interaction. Combining the conventional adiabatic techniques and currently developed approaches of phase control, a feasible proposal for implementation of a geometric phase gate is presented, where the conditional phase shift (Berry phase) is achieved by adiabatically and cyclically changing the parameters of the driving fields. Here we find that the geometric phase acquired is related to the way how the relative phas…
One scheme is presented to construct the robust multi-qubit arbitrary-phase controlled-phase gate (CPG) with one control and multiple target qubits in Rydberg atoms using the Lewis-Riesenfeld (LR) invariant method. The scheme is not limited by adiabatic condition while preserves the robustness against control parameter variations of adiabatic evolution. Comparing with the adiabatic case, our scheme does not require very strong Rydberg interaction strength. Taking the construction of two-qubit $π$ CPG as an example, our scheme is more robust against control parameter variations than non-adiabat…
A semiclassical, four-level model of a nanosecond, chirped pulse interacting with all optically accessible hyperfine states in the ultracold Rb atom is analyzed aiming at population inversion within $5S_{1/2}$ electronic state. The nature of two-photon adiabatic passage performed by such a single pulse having a bandwidth smaller than the hyperfine splitting of $5S_{1/2}$ state is investigated in the framework of the dressed state picture. It is shown that two dressed states are involved in the adiabatic dynamics of population inversion. The excited state manifold appeared to play an important …
The Stimulated Raman Adiabatic Passage (STIRAP) procedure is a robust and complete population transfer method which have various application in chemistry and atomic physics. Here, we study the effects of one-photon detuning, transition time, pulse width, and pulse delay parameters on the population transfer via STIRAP and b-STIRAP techniques. Moreover, the impact of the field amplitude which decreases the population transfer has been analyzed and it is shown that in b-STIRAP, the robustness of the complete transition can be improved by decreasing the field amplitude in the single-photon resona…
We present a robust protocol for implementing high-fidelity multiqubit controlled phase gates $(C^kZ)$ on neutral atom qubits coupled to highly excited Rydberg states. Our approach is based on extending adiabatic rapid passage to two-photon excitation via a short-lived intermediate excited state common to alkali-atom Rydberg experiments, accounting for the full impact of spontaneous decay and differential AC Stark shifts from the complete manifold of hyperfine excited states. We evaluate and optimize gate performance, concluding that for Cs and currently available laser frequencies and powers,…
We propose a directional coupler exploiting the framework of adiabatic passage for two level atomic systems with configuration dependent Allen-Eberly scheme. Recently developed shortcut to adiabatic passage method (STA), which uses transitionless quantum driving algorithm, is applied to the coupler. The study shows that it is possible to reduce the device length significantly using STA, keeping the efficiency of power transfer100%.Shortcut approach shows much superiority in terms of robustness and fidelity in power switching compared to the adiabatic one.
We provide a theoretical analysis for a recently demonstrated cooling method. Two-level particles undergo successive adiabatic transfers upon interaction with counter-propagating laser beams that are repeatedly swept over the transition frequency. We show that particles with narrow linewidth transitions can be cooled to near the recoil limit. This cooling mechanism has a reduced reliance on spontaneous emission compared to Doppler cooling, and hence shows promise for application to systems lacking closed cycling transitions, such as molecules.
The development of advanced quantum technologies and the quest for a deeper understanding of many-particle quantum mechanics requires control over the quantum state of interacting particles to a high degree of fidelity. However, the quickly increasing density of the spectrum, together with the appearance of crossings in time-dependent processes, makes any effort to control the system hard and resource intensive. Here we show that in trapped systems regimes can exist, in which isolated energy bands appear that allow to easily generalize known single-particle techniques. We demonstrate this for …
We study a scheme for implementing a controlled-Z (CZ) gate between two neutral-atom qubits based on the Rydberg blockade mechanism in a manner that is robust to errors caused by atomic motion. By employing adiabatic dressing of the ground electronic state, we can protect the gate from decoherence due to random phase errors that typically arise because of atomic thermal motion. In addition, the adiabatic protocol allows for a Doppler-free configuration that involves counterpropagating lasers in a $σ_+/σ_-$ orthogonal polarization geometry that further reduces motional errors due to Doppler shi…
High-fidelity multiqubit gates with Rydberg atoms via level-crossing-free Rapid adiabatic passage
College of Physics and Electronic Engineering, Shanxi University（山西大学物理电子工程学院）；Collaborative Innovation Center of Extreme Optics, Shanxi University（山西大学极端光学协同创新中心）
We study the Landau-Zener (LZ) dynamics in a setup of two Rydberg atoms with time-dependent detuning, both linear and periodic, using both the exact numerical calculations as well as the method of adiabatic impulse approximation (AIA). By varying the Rydberg-Rydberg interaction strengths, the system can emulate different three-level LZ models, for instance, bow-tie and triangular LZ models. The LZ dynamics exhibits non-trivial dependence on the initial state, the quench rate, and the interaction strengths. For large interaction strengths, the dynamics is well captured by AIA. In the end, we an…
We examine the adiabatic preparation of crystalline phases of Rydberg excitations in a one-dimensional lattice gas by frequency sweep of the excitation laser, as proposed by Pohl et al. [Phys. Rev. Lett. 104, 043002 (2010)] and recently realized experimentally by Schauß et al. [Science 347, 1455 (2015)]. We find that the preparation of crystals of a few Rydberg excitations in a unitary system of several tens of atoms requires exceedingly long times for the adiabatic following of the ground state of the system Hamiltonian. Using quantum stochastic (Monte-Carlo) wavefunction simulations, we show…
Using numerical simulations of two-photon electronic absorption with femtosecond pulses in Na$_2$ we show that: i) it is possible to avoid the characteristic saturation or dumped Rabi oscillations in the yield of absorption by time-delaying the laser pulses; ii) it is possible to accelerate the onset of adiabatic passage by using the vibrational coherence starting in a wave packet; and iii) it is possible to prepare the initial wave packet in order to achieve full state-selective transitions with broadband pulses. The findings can be used, for instance, to achieve ultrafast adiabatic passage b…
Laser excitation pulses that lead to perfect adiabatic state transfer in an ensemble of three-level ladder atoms lead to highly entangled states of many atoms if their highest excited state is subject to Rydberg blockade. Solution of the Schrödinger equation shows that it is increasingly difficult to ensure the adiabatic evolution as the number of atoms increases. A diminishing energy gap, significant variations in collective observables, and increased work fluctuations link the critical slowing down of the adiabatic evolution with a quantum phase transition-like behavior of the system.
Spatial adiabatic passage processes for ultracold atoms trapped in tunnel-coupled cylindrically symmetric concentric potentials are investigated. Specifically, we discuss the matter-wave analogue of the rapid adiabatic passage (RAP) technique for a high fidelity and robust loading of a single atom into a harmonic ring potential from a harmonic trap, and for its transport between two concentric rings. We also consider a system of three concentric rings and investigate the transport of a single atom between the innermost and the outermost rings making use of the matter-wave analogue of the stimu…
Recently, the creation of photonic Landau levels in a twisted cavity has been demonstrated in Nature \textbf{534}, 671 (2016). Here we propose a scheme to adiabatically transfer flux quanta in multiples of $3\hbar$ simultaneously to all cavity photons by coupling the photons through flux-threaded cones present in such cavity setup. The flux transfer is achieved using external light fields with orbital angular momentum and a near-resonant dense atomic medium as mediator. Furthermore, coupling the cavity fields to a Rydberg state in a configuration supporting electromagnetically induced transpar…
Spatial adiabatic passage represents a new way to design integrated photonic devices. In conventional adiabatic passage designs require smoothly varying waveguide separations. Here we show modelling of adiabatic passage devices where the waveguide separation is varied digitally. Despite digitisation, our designs show robustness against variations in the input wavelength and refractive index contrast of the waveguides relative to the cladding. This approach to spatial adiabatic passage opens new design strategies and hence the potential for new photonics devices.
Adiabatic passage employs a slowly varying time-dependent Hamiltonian to control the evolution of a quantum system along the Hamiltonian eigenstates. For processes of finite duration, the exact time evolving state may deviate from the adiabatic eigenstate at intermediate times, but in numerous applications it is observed that this deviation reaches a maximum and then decreases significantly towards the end of the process. We provide a straightforward theoretical explanation for this welcome but often unappreciated fact. Our analysis emphasizes a separate adiabaticity criterion for high fidelit…
We propose a robust scheme to prepare three-dimensional entanglement states between a single atom and a Bose-Einstein Condensate (BEC) via stimulated Raman adiabatic passage (STIRAP) techniques. The atomic spontaneous radiation, the cavity decay, and the fiber loss are efficiently suppressed by the engineering adiabatic passage. Our scheme is also robust to the variation of atom number in the BEC.
