Narrowband Biphotons: Generation, Manipulation, and Applications
Chih-Sung Chuu, Shengwang Du
备注：
to appear as a book chapter in a compilation "Engineering the Atom-Photon Interaction" published by Springer in 2015, edited by A. Predojevic and M. W. Mitchell
In this chapter, we review recent advances in generating narrowband biphotons with long coherence time using spontaneous parametric interaction in monolithic cavity with cluster effect as well as in cold atoms with electromagnetically induced transparency. Engineering and manipulating the temporal waveforms of these long biphotons provide efficient means for controlling light-matter quantum interaction at the single-photon level. We also review recent experiments using temporally long biphotons and single photons.
We describe and demonstrate a quantum state tomography for measuring the complex temporal waveform of narrowband biphotons. Through six sets of two-photon interference measurements projected in different polarization subspaces, we can construct the time-frequency entangled two-photon joint amplitude and phase functions in continuous-variable time domain. For the first time, we apply this technique to experimentally determine the temporal quantum states of narrowband biphotons generated from spontaneous four-wave mixing in cold atoms, and fully confirm the theoretical predictions.
We demonstrate the generation of narrowband biphotons with polarization-frequency coupled hy- perentanglement from spontaneous four-wave mixing in cold atoms. The coupling between polariza- tion and frequency is realized through a frequency shifter and linear optics. When the polarization- frequency degrees of freedom are decoupled, it is robust to create polarization and frequency Bell states, confirmed by the polarization quantum-state tomography and the two-photon temporal quan- tum beating. Making use of the polarization-frequency coupling to transfer polarization phase retard to the entan…
We study the generation of paired photons due to the effect of four-wave mixing in an ensemble of pumped two-level systems that decay via an intermediate metastable state. The slow population relaxation of the metastable state to the ground state is utilized to create long-lived coherent population oscillation, leading to narrowband nonlinear response of the medium. The biphotons have a narrow bandwidth, long coherence time and length, which can be controlled by the pump field. In addition, the biphotons are antibunched, with antibunching period determined by the dephasing time. During this pe…
We report the direct characterization of energy-time entanglement of narrowband biphotons produced from spontaneous four-wave mixing in cold atoms. The Stokes and anti-Stokes two-photon temporal correlation is measured by single-photon counters with nano second temporal resolution, and their joint spectrum is determined by using a narrow linewidth optical cavity. The energy-time entanglement is verified by the joint frequency-time uncertainty product of 0.063 +/- 0.0044, which does not only violate the separability criterion but also satisfies the continuous variable Einstein-Podolsky-Rosen st…
Nonclassical photon sources of high brightness are key components of quantum communication technologies. We here demonstrate the generation of narrowband, nonclassical photon pairs by employing spontaneous four-wave mixing in an optically-dense ensemble of cold atoms within a hollow-core fiber. The brightness of our source approaches the limit of achievable generated spectral brightness at which successive photon pairs start to overlap in time. For a generated spectral brightness per pump power of up to $2\times 10^{9} \ \textrm{pairs/(s MHz mW)}$ we observe nonclassical correlations at pump p…
We study narrow-band biphoton generation from spontaneous four-wave mixing with electromagnetically induced transparency in a laser cooled atomic ensemble. We compare two formalisms in the interaction and Heisenberg pictures, and find that they agree in the low gain regime but disagree in the high gain regime. We extend both formalisms accounting the non-uniformity in atomic density and the driving laser fields. We find that for a fixed optical depth and a weak and far-detuned pump laser beam, the two-photon waveform is independent of the atomic density distribution. However, the spatial profi…
Interference between an unknown two-photon state (a "biphoton") and the two-photon component of a reference state gives a phase-sensitive arrival-time distribution containing full information about the biphoton temporal wave function. Using a coherent state as a reference, we observe this interference and reconstruct the wave function of single-mode biphotons from a low-intensity narrowband squeezed vacuum state.
In this work, we experimentally manipulate the spectrum and phase of a biphoton wave packet in a two-dimensional frequency space. The spectrum is shaped by adjusting the temperature of the crystal, and the phase is controlled by tilting the dispersive glass plate. The manipulating effects are confirmed by measuring the two-photon spectral intensity (TSI) and the Hong-Ou-Mandel (HOM) interference patterns. Unlike the previous independent manipulation schemes, here we perform joint manipulation on the biphoton spectrum. The technique in this work paves the way for arbitrary shaping of a multi-ph…
We report the efficient generation of subnatural-linewidth (< 6 MHz, for Rb D1/D2 lines) biphotons from a Doppler-broadened (530 MHz) hot atomic vapor cell. We use on-resonance spontaneous four-wave mixing in a hot paraffin-coated 87Rb vapor cell at 63 C to produce time-frequency entangled photon pairs with controllable bandwidth (1.9 - 3.2 MHz) and coherence time (47 - 94 ns). Our backward phase-matching scheme with optical pumping is the key to minimize the generation of uncorrelated photons from resonance fluorescence. The result paves the way toward miniature narrowband biphoton source bas…
We theoretically investigated spectrally uncorrelated biphotons generated in a counter-propagating spontaneous parametric downconversion (CP-SPDC) from periodically poled MTiOXO4 (M = K, Rb, Cs; X = P, As) crystals. By numerical calculation, it was found that the five crystals from the KTP family can be used to generate heralded single photons with high spectral purity and wide tunability. Under the type-0 phase-matching condition, the purity at 1550 nm was between 0.91 and 0.92, and the purity can be maintained over 0.90 from 1500 nm to 2000 nm wavelength. Under the type-II phase-matching con…
Bell states are a fundamental resource in photonic quantum information processing. These states have been generated successfully in many photonic degrees of freedom. Their manipulation, however, in the momentum space remains challenging. Here, we present a scheme for engineering the symmetry of two-photon states entangled in the transverse momentum degree of freedom through the use of a spatially variable phase object. We demonstrate how a Hong-Ou-Mandel interferometer must be constructed to verify the symmetry in momentum entanglement via photon "bunching"/"anti-bunching" observation. We also…
The robust generation and manipulation of entangled multiphoton states on-chip has an essential role in quantum computation and communication. Lattice topology has emerged as a means of protecting photonic states from disorder but entanglement across different topologies remained unexplored. We report biphoton entanglement between topologically distinct spatial modes in a bipartite array of silicon waveguides. The results highlight topology as an additional degree of freedom for entanglement and open avenues for investigating information teleportation between trivial and topological modes.
We use a single trapped 40Ca+ ion as a resonant, polarization-sensitive absorber to detect and characterize the entanglement of tunable narrowband photon pairs from a spontaneous parametric down-conversion source. Single-photon absorption is marked by a quantum jump in the ion and heralded by coincident detection of the partner photon. For three polarization basis settings of absorption and detection of the herald, we find maximum coincidences always for orthogonal polarizations. The polarization entanglement is further evidenced by tomographic reconstruction of the biphoton quantum state.
The possibility to manipulate the wavepackets of single photons or biphotons has enriched quantum optics and quantum information science, with examples ranging from faithful quantum-state mapping and high-efficiency quantum memory to the purification of single photons. Here we demonstrate another fascinating use of wavepacket manipulation on restoring quantum interference. By modulating the photons' temporal wavepacket, we observe the revival of post-selected entanglement that would otherwise be degraded or lost due to poor quantum interference. Our study shows that the amount of the restored …
Efficient heralded generation of entanglement together with its manipulation is of great importance for quantum communications. In addition, states generated with bandwidths naturally compatible with atomic transitions allow a more efficient mapping of light into matter which is an essential requirement for long distance quantum communications. Here we propose a scheme where the indistinguishability between two spontaneous four-wave mixing processes is engineered to herald generation of single-photon frequency-bin entangled states, i.e., single-photons shared by two distinct frequency modes. W…
A silicon quantum photonic circuit was proposed and demonstrated as an integrated quantum light source for telecom band polarization entangled Bell state generation and dynamical manipulation. Biphoton states were firstly generated in four silicon waveguides by spontaneous four wave mixing. They were transformed to polarization entangled Bell states through on-chip quantum interference and quantum superposition, and then coupled to optical fibers. The property of polarization entanglement in generated photon pairs was demonstrated by two-photon interferences under two non-orthogonal polarizati…
Plenty of quantum information protocols are enabled by manipulation and detection of photonic spectro-temporal degrees of freedom via light-matter interfaces. While present implementations are well suited for high-bandwidth photon sources such as quantum dots, they lack the high resolution required for intrinsically narrow-band light-atom interactions. Here, we demonstrate far-field temporal imaging based on ac-Stark spatial spin-wave phase manipulation in a multimode gradient echo memory. We achieve spectral resolution of 20 kHz with MHz-level bandwidth and ultra-low noise equivalent to 0.023…
Counter-propagating parametric conversion processes in non-linear bulk crystals have been shown to feature unique properties for efficient narrowband frequency conversion. In quantum optics, the generation of photon pairs with a counter-propagating parametric down-conversion process (PDC) in a waveguide, where signal and idler photons propagate in opposite directions, offers unique material-independent engineering capabilities. However, realizing counter-propagating PDC necessitates quasi-phase-matching (QPM) with extremely short poling periods. Here, we report on the generation of counter-pro…
We demonstrate the storage and manipulation of narrowband heralded single photons from a cavity-enhanced spontaneous parametric downconversion (SPDC) source in the atomic quantum memory based on electromagnetically induced transparency. We show that nonclassical correlations are preserved between the heralding and the retrieved photons after storage process. By varying the intensity of the coupling field during retrieval process, we further demonstrate that the waveform or bandwidth of the single photons can be manipulated and the nonclassical correlation between the photon pairs can be even e…
