Quantum metrology utilizes nonclassical states to improve the precision of measurement devices. In this context, strongly squeezed vacuum states of light have proven to be a useful resource. They are typically produced by spontaneous parametric down-conversion, but have not been generated at shorter wavelengths so far, as suitable nonlinear materials do not exist. Here, we report on the generation of strongly squeezed vacuum states at 532 nm with 5.5 dB noise suppression by means of frequency up-conversion from the telecommunication wavelength of 1550 nm. The up-converted states are employed in a model Mach-Zehnder interferometer to illustrate their use in quantum metrology.
We study the quantum correlations induced by spontaneous parametric down-conversion (SPDC) of a frequency comb. We derive a theoretical method to find the output state corresponding to a pump with an arbitrary spectral profile. After applying it to the relevant example of a spectrally chirped pump, we run an optimization algorithm to numerically find the pump profiles maximizing some target functions. These include the number of independently squeezed modes and the variances of nullifiers defining cluster states used in many continuous-variable quantum information protocols. To assess the adva…
Quantum frequency conversion, the process of shifting the frequency of an optical quantum state while preserving quantum coherence, can be used to produce non-classical light at otherwise unapproachable wavelengths. We present experimental results based on highly efficient sum-frequency generation (SFG) between a vacuum squeezed state at 1064 nm and a tunable pump source at 850 nm $\pm$ 50 nm for the generation of bright squeezed light at 472~nm $\pm$ 4~nm, currently limited by the phase-matching of the used nonlinear crystal. We demonstrate that the SFG process conserves part of the quantum c…
We investigate the effects of a squeezed pump on the quantum properties and conversion efficiency of the light produced in single-pass second harmonic generation. Using stochastic integration of the two-mode equations of motion in the positive-P representation, we find that larger violations of continuous-variable harmonic entanglement criteria are available for lesser effective interaction strengths than with a coherent pump. This enhancement of the quantum properties also applies to violations of the Reid-Drummond inequalities used to demonstrate a harmonic version of the Einstein-Podolsky-R…
Continuous-wave (cw) squeezed states of light have applications in sensing, metrology and secure communication. In recent decades their efficient generation has been based on parametric down-conversion, which requires pumping by externally generated pump light of twice the optical frequency. Currently, there is immense effort in miniaturizing squeezed-light sources for chip-integration. Designs that require just a single input wavelength are favored since they offer an easier realization. Here we report the first observation of cw squeezed states generated by self-phase modulation caused by su…
In this paper we experimentally study the statistical properties of a bright squeezed vacuum state containing up to 10^13 photons per mode (10 uJ per pulse), produced via high gain parametric down conversion (PDC). The effects of bunching and superbunching of photons were observed for a single mode PDC radiation by second-order intensity correlation function measurements with analog detectors.
We have considered theoretically the feasibility of the broadband quantum memory based on the resonant tripod-type atomic configuration. In this case, the writing of a signal field is carried out simultaneously into two channels, and characterized by an excitation of two spin waves of the atomic ensemble. With simultaneous read out from both channels quantum properties of the original signal are mapped on the retrieval pulse no worse than in the case of memory based on Lambda-type atomic configuration. At the same time new possibilities are opened up for manipulation of quantum states associat…
The two modes of the Einstein-Podolsky-Rosen quadrature entangled state generated by parametric down-conversion interfere on a beam splitter of variable splitting ratio. Detection of a photon in one of the beam splitter output channels heralds preparation of a signal state in the other, which is characterized using homodyne tomography. By controlling the beam splitting ratio, the signal state can be chosen anywhere between the single-photon and squeezed state.
We experimentally verify the quantum non-Gaussian character of a conditionally generated noisy squeezed single-photon state with positive Wigner function. Employing an optimized witness based on probabilities of squeezed vacuum and squeezed single-photon states we prove that the state cannot be expressed as a mixture of Gaussian states. In our experiment, the non-Gaussian state is generated by conditional subtraction of a single photon from squeezed vacuum state. The state is probed with a homodyne detector and the witness is determined by averaging a suitable pattern function over the measure…
Bright squeezed vacuum, a promising tool for quantum information, can be generated by high-gain parametric down-conversion. However, its frequency and angular spectra are typically quite broad, which is undesirable for applications requiring single-mode radiation. We tailor the frequency spectrum of high-gain parametric down-conversion using an SU(1,1) interferometer consisting of two nonlinear crystals with a dispersive medium separating them. The dispersive medium allows us to select a narrow band of the frequency spectrum to be exponentially amplified by high-gain parametric amplification. …
Although squeezed states are nonclassical states, so far, their nonclassicality could not be demonstrated by negative quasiprobabilities. In this work we derive pattern functions for the direct experimental determination of so-called nonclassicality quasiprobabilities. The negativities of these quantities turn out to be necessary and sufficient for the nonclassicality of an arbitrary quantum state and are therefore suitable for a direct and general test of nonclassicality. We apply the method to a squeezed vacuum state of light that was generated by parametric down-conversion in a second-order…
We propose to produce pulses of strongly squeezed light by Raman scattering of a strong laser pulse on a spin squeezed atomic sample. We prove that the emission is restricted to a single field mode which perfectly inherits the quantum correlations of the atomic system.
In this Letter we experimentally demonstrate the generation of squeezed, bright twin beams which arise due to competing gain and absorption, in a medium that is overall transparent. To accomplish this, we make use of a non-degenerate four-wave mixing process in warm potassium vapor, such that one of the twin beams experiences strong on-resonant absorption. At room temperature and above, due to Doppler broadening and smaller frequency detunings compared to other schemes, the ground state hyperfine splittings used in the present double-$Λ$ setup are completely overlapped. We show that despite th…
We report on the generation of a stable continuous-wave low-frequency squeezed vacuum field with a squeezing level of $3.8\pm0.1$ dB at 1064 nm, the wavelength at which laser interferometers for gravitational wave (GW) detection operate, using periodically poled KTiOPO$_4$ (PPKTP) in a sub-threshold optical parametric oscillator. PPKTP has the advantages of higher nonlinearity, smaller intra-crystal and pump-induced seed absorption, user-specified parametric down-conversion temperature, wider temperature tuning range, and lower susceptibility to thermal lensing over alternative nonlinear mater…
We study the spatial properties of high-gain parametric down-conversion (PDC). From the Hamiltonian we find the Schmidt modes, apply the Bloch-Messiah reduction, and calculate analytically the measurable quantities, such as the angular distributions of photon numbers and photon-number correlations. Our approach shows that the Schmidt modes of PDC radiation can be considered the same as for the low-gain (biphoton) case while the Schmidt eigenvalues strongly depend on the parametric gain. Its validity is confirmed by comparison with several experimental results, obtained by us and by other group…
We propose a method for generation of a single-cycle squeezed light by parametric down-conversion in a chirped quasi-phase-matched nonlinear crystal. We find an exact quantum solution for this process valid for an arbitrary parametric gain, and discover an ultrabroadband squeezing in the down-converted light with flat squeezing spectrum comprising the full optical octave. We describe a scheme for observation of this kind of squeezing using second-harmonic generation as an ultrafast correlator.
We report a scheme for generation of high-order vortex states using two-mode photon-number squeezed states, generated via the non-linear process of Spontaneous Parametric Down Conversion. By applying a parametric rotation in quadrature space $(X,Y)$, using a $ϕ$ converter, the Gaussian quadrature profile of the photon-number squeezed input state can be mapped into a superposition of Laguerre-Gauss modes with $N$ vortices or singularities, for an input state containing $N$ photons, thus mapping photon-number fluctuations to interference effects in quadrature space. Our scheme has the potential …
We propose an experimental scheme to generate, in a heralded fashion, arbitrary quantum superpositions of two-mode optical states with a fixed total photon number $n$ based on weakly squeezed two-mode squeezed state resources (obtained via weak parametric down conversion), linear optics, and photon detection. Arbitrary $d$-level (qudit) states can be created this way where $d=n+1$. Furthermore, we experimentally demonstrate our scheme for $n=2$. The resulting qutrit states are characterized via optical homodyne tomography. We also discuss possible extensions to more than two modes concluding t…
In this letter we present a scheme for the implementation of frequency up- and down-conversion operations in two-mode cavity quantum electrodynamics (QED). This protocol for engineering bilinear two-mode interactions could enlarge perspectives for quantum information manipulation and also be employed for fundamental tests of quantum theory in cavity QED. As an application we show how to generate a two-mode squeezed state in cavity QED (the original entangled state of Einstein-Podolsky-Rosen).
We present a quantum theory of parametric down-conversion of light in chirped quasi-phase-matched second-order nonlinear crystals with undepleted quasi-monochromatic pump. This theory allows us to consider generation of ultrabroadband squeezed states of light and is valid for arbitrary, sufficiently slowly-varying nonlinear poling profiles. Using a first-order approximate quantum solution for the down-converted light field, we calculate the squeezing spectra and the characteristic squeezing angles. We compare the approximate solutions with the exact and numerical ones and find a very good agre…
The LIGO-II gravitational-wave interferometers (ca. 2006--2008) are designed to have sensitivities at about the standard quantum limit (SQL) near 100 Hz. This paper describes and analyzes possible designs for subsequent, LIGO-III interferometers that can beat the SQL. These designs are identical to a conventional broad-band interferometer (without signal recycling), except for new input and/or output optics. Three designs are analyzed: (i) a "squeezed-input interferometer" (conceived by Unruh based on earlier work of Caves) in which squeezed vacuum with frequency-dependent (FD) squeeze angle i…
The squeezed cat state, an essential quantum resource, can be used for quantum error correction and slowing decoherence of the optical cat state. However, preparing a squeezed cat state with high generation rate, and effectively manipulating it, remain challenging. In this work, a high-performance all-optical in-line squeezer is developed to prepare a squeezed cat state and manipulate the phase of the quadrature squeezing. This scheme has the advantages that the phase of the quadrature squeezing of the squeezed cat state can be manipulated by changing the working condition of the squeezer, and…
Bright squeezed vacuum, a macroscopic nonclassical state of light, can be obtained at the output of a strongly pumped non-seeded traveling-wave optical parametric amplifier (OPA). By constructing the OPA of two consecutive crystals separated by a large distance we make the squeezed vacuum spatially single-mode without a significant decrease in the brightness or squeezing.
In recent development of quantum technologies, a frequency conversion of quantum signals has been studied widely. We investigate the optic-microwave entanglement that is generated by applying an electro-optomechanical frequency conversion scheme to one mode in an optical two-mode squeezed vacuum state. We quantify entanglement of the converted two-mode Gaussian state, where surviving entanglement of the state is analyzed with respect to the parameters of the electro-optomechanical system. Furthermore, we show that there exists an upper bound for the entanglement that survives after the convers…
Control over the spectral properties of the bright squeezed vacuum (BSV), a highly multimode non-classical macroscopic state of light that can be generated through high-gain parametric down conversion, is crucial for many applications. In particular, in several recent experiments BSV is generated in a strongly pumped SU(1,1) interferometer to achieve phase supersensitivity, perform broadband homodyne detection, or tailor the frequency spectrum of squeezed light. In this work, we present an analytical approach to the theoretical description of BSV in the frequency domain based on the Bloch-Mess…
We analyze the long-time quantum dynamics of degenerate parametric down-conversion from an initial sub-harmonic vacuum (spontaenous down-conversion). Standard linearization of the Heisenberg equations of motions fails in this case, since it is based on an expansion around an unstable classical solution and neglects pump depletion. Introducing a mean-field approximation we find a periodic exchange of energy between the pump and subharmonic mode goverened by an anharmonic pendulum equation. From this equation the optimum interaction time or crystal length for maximum conversion can be determined…
In a strongly pumped non-degenerate traveling-wave OPA, we produce two-color squeezed vacuum with up to millions of photons per pulse. Our approach to registering this macroscopic quantum state is direct detection of a large number of transverse and longitudinal modes, which is achieved by making the detection time and area much larger than the coherence time and area, respectively. Using this approach, we obtain a record value of twin-beam squeezing for direct detection of bright squeezed vacuum. This makes direct detection of macroscopic squeezed vacuum a practical tool for quantum informati…
Intermittency in Quantum Graviton-Phonon Conversion
Ecole Normale Supérieure - PSL（巴黎高等师范学院-PSL）；Kobe University（神户大学）；Kyushu University（九州大学）；Quantum and Spacetime Research Institute, Kyushu University（九州大学量子与时空研究所）
The role of the spatiotemporal degrees of freedom in the preparation and observation of squeezed photonic states, produced by parametric down-conversion, is investigated. The analysis is done with the aid of a functional approach under the semi-classical approximation and the thin-crystal approximation. It is found that the squeezed state loses its minimum uncertainty property as the efficiency of down-conversion is increased, in a way that depends on the conditions of the homodyne measurements with which the amount of squeezing is determined.
We present an experimental realization of resonance fluorescence in squeezed vacuum. We strongly couple microwave-frequency squeezed light to a superconducting artificial atom and detect the resulting fluorescence with high resolution enabled by a broadband traveling-wave parametric amplifier. We investigate the fluorescence spectra in the weak and strong driving regimes, observing up to 3.1 dB of reduction of the fluorescence linewidth below the ordinary vacuum level and a dramatic dependence of the Mollow triplet spectrum on the relative phase of the driving and squeezed vacuum fields. Our r…
We address the security of continuous-variable quantum key distribution with squeezed states upon realistic conditions of noisy and lossy environment and limited reconciliation efficiency. Considering the generalized preparation scheme and clearly distinguishing between classical and quantum resources, we investigate the effect of finite squeezing on the tolerance of the protocol to untrusted channel noise. For a long-distance strongly attenuating channel and the consequent low reconciliation efficiency, we show that feasible limited squeezing is surprisingly sufficient to provide the security…
We study the properties of bi-squeezed tripartite Gaussian states created by two spontaneous parametric down-conversion processes that share a common idler. We give a complete description of the quantum correlations across of all partitions, as well as of the genuine multipartite entanglement, obtaining analytical expressions for most of the quantities of interest. We find that the state contains genuine tripartite entanglement, in addition to the bipartite entanglement among the modes that are directly squeezed. We also investigate the effect of homodyne detection of the photons in the common…
We propose a method to obtain a regular arrangement of two-level atoms in a three-dimensional optical lattice with unit filling, where all the atoms share internal state coherence and metrologically useful quantum correlations. Such a spin-squeezed atomic crystal is obtained by adiabatically raising an optical lattice in an interacting two-component Bose-Einstein condensate. The scheme could be directly implemented on a microwave transition with state-of-the art techniques and used in optical-lattice atomic clocks with bosonic atoms to strongly suppress the collisional shift and benefit from t…
Universal quantum computing with continuous variables requires non-Gaussian resources, in addition to a Gaussian set of operations. A known resource enabling universal quantum computation is the cubic phase state, a non-Gaussian state whose experimental implementation has so far remained elusive. In this paper, we introduce two Gaussian conversion protocols that allow for the conversion of a non-Gaussian state that has been achieved experimentally, namely the trisqueezed state [Sandbo Changet al., Phys. Rev. X10, 011011 (2020)],to a cubic phase state. The first protocol is deterministic and it…
We present a single-pass source of broadband multimode squeezed light with potential application in quantum information and quantum metrology. The source is based on a type I parametric down-conversion (PDC) process inside a bulk nonlinear crystal in a non-collinear configuration. The generated squeezed light exhibits a spatiotemporal multimode behavior that is probed using a homodyne measurement with a local oscillator shaped both spatially and temporally. Finally we follow a covariance matrix based approach to reveal the distribution of the squeezing among several independent temporal and sp…
Multimode Squeezed State for Reconfigurable Quantum Networks at Telecommunication Wavelengths
ICFO - Instituto de Ciencias Fotonicas, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科学技术研究所）；Laboratoire Kastler Brossel, Sorbonne Université, ENS-Université PSL, CNRS, Collège de France（卡斯勒布罗塞尔实验室，索邦大学，巴黎文理研究大学，法国国家科学研究中心，法兰西公学院）；Sorbonne Université, LIP6, CNRS（索邦大学，LIP6实验室，法国国家科学研究中心）
Strongly squeezed light finds many important applications within the fields of quantum metrology, quantum communication and quantum computation. However, due to the bulkiness and complexity of most squeezed light sources of today, they are still not a standard tool in quantum optics labs. We have taken the first steps in realizing a compact, high-performance 1550 nm squeezing source based on commercially available fiber components combined with a free-space double-resonant parametric down-conversion source. The whole setup, including single-pass second-harmonic generation in a waveguide, fits …
We propose an efficient scheme for generating spin-squeezed states at steady state in a spin-mechanical hybrid system, where an ensemble of SiV centers are coupled to a strongly damped nanomechanical resonator. We show that,there exists a collective steady state in the system, which is exactly formed by the collective spin states plus the zero excitation state of the mechanical mode. The generation of the steady spin-squeezed state is based on a dissipative quantum dynamical process in which the mechanical dissipation plays a positive role but without destroying the target state. We demonstrat…
We propose and analyse a cascaded optical parametric system which involves three interacting modes across two octaves of frequency difference. Our system, combining degenerate optical parametric oscillation (OPO) with second harmonic generation (SHG), promises to be a useful source of squeezed and entangled light at three differing frequencies. We show how changes in damping rates and the ratio of the two concurrent nonlinearities affect the quantum correlations in the output fields. We analyse the threshold behaviour, showing how the normal OPO threshold is changed by the addition of the SHG …
Parametric down-conversion (PDC) is the established standard for the practical generation of a multiplicity of quantum optical states. These include two-mode squeezed vacuum, heralded non-Gaussian states and entangled photon pairs. Detailed theoretical studies provide insight into the time-frequency (TF) structure of PDC, which are governed by the complex-valued joint spectral amplitude (JSA) function. However in experiments, the TF structure of PDC is mostly characterised by intensity measurementsthat forbid access to the important phase of the JSA. In this paper, we present an amplitude-sens…
A quantum internet connects remote quantum processors that need interact and exchange quantum signals over a long distance through photonic channels. However, these quantum nodes are usually composed of quantum systems with emitted photons unsuitable for long-distance transmission. Therefore, quantum wavelength conversion to telecom is crucial for long-distance quantum networks based on optical fiber. Here we propose wavelength conversion devices for single-photon polarization qubits using continuous variable quantum teleportation, which can efficiently convert qubits between near-infrared (78…
Boson sampling is a simple model for non-universal linear optics quantum computing using far fewer physical resources than universal schemes. An input state comprising vacuum and single photon states is fed through a Haar-random linear optics network and sampled at the output using coincidence photodetection. This problem is strongly believed to be classically hard to simulate. We show that an analogous procedure implements the same problem, using photon-added or -subtracted squeezed vacuum states (with arbitrary squeezing), where sampling at the output is performed via parity measurements. Th…
Engineering quantum states of light represents a crucial task in the vast majority of photonic quantum technology applications. Direct manipulation of the number of photons in the light signal, such as single-photon subtraction and addition, proved to be an efficient strategy for the task. Here we propose an adaptive multi-photon subtraction scheme where a particular subtraction task is conditioned by all previous subtraction events in order to maximize the probability of successful subtraction. We theoretically illustrate this technique on the model example of conversion of Fock states via ph…
We present an experimental method for the generation of amplitude squeezed high-order vector beams. The light is modified twice by a spatial light modulator such that the vector beam is created by means of a collinear interferometric technique. A major advantage of this approach is that it avoids systematic losses, which are detrimental as they cause decoherence in continuous-variable quantum systems. The utilisation of a spatial light modulator (SLM) gives the flexibility to switch between arbitrary mode orders. The conversion efficiency with our setup is only limited by the efficiency of the…
Squeezed light is a key quantum resource that enables quantum advantages for sensing, networking, and computing applications. The scalable generation and manipulation of squeezed light with integrated platforms are highly desired for the development of quantum technology with continuous variables. In this letter, we demonstrate squeezed light generation with thin-film lithium niobate integrated photonics. Para-metric down-conversion is realized with quasi-phase matching using ferroelectric domain engineering. With sub-wavelength mode confinement, efficient nonlinear processes can be observed w…
In this paper, we theoretically investigate the displacement and momentum fluctuations spectra of the movable mirror in a standard optomechanical system driven by a finite bandwidth squeezed vacuum light accompanying a coherent laser field. Two cases in which the squeezed vacuum is generated by degenerated and non-degenerate parametric oscillators (DPO and NDPO) are considered. We find that for the case of finite bandwidth squeezed vacuum injection, the two spectra exhibit unique features, which strongly differ from those of broadband squeezing excitation. In particular, the spectra exhibit a …
High-order correlations and ultrafast Wigner negativities in bright-squeezed-vacuum-driven high-harmonic generation
Max Planck Institute for the Structure and Dynamics of Matter（马普固体与结构研究所）；Guangdong Technion-Israel Institute of Technology（广东以色列理工学院）；Technion–Israel Institute of Technology（以色列理工学院）；Initiative for Computational Catalysis (ICC), Flatiron Institute（Flatiron研究所计算催化倡议）
