Niobium diselenide has long served as a prototype of two-dimensional charge ordering, believed to arise from an instability of the electronic structure analogous to the one-dimensional Peierls mechanism. Despite this, various anomalous properties have recently been identified experimentally which cannot be explained by Peierls-like weak-coupling theories. We consider instead a model with strong electron-phonon coupling, taking into account both the full momentum and orbital dependence of the coupling matrix elements. We show that both are necessary for a consistent description of the full range of experimental observations. We argue that NbSe$_2$ is typical in this sense, and that any charge-ordered material in more than one dimension will generically be shaped by the momentum and orbital dependence of its electron-phonon coupling as well as its electronic structure. The consequences will be observable in many charge-ordered materials, including cuprate superconductors.
Tunability of the magnetic properties in Ni intercalated transition metal dichalcogenide NbSe$_2$
International Research Centre Magtop, Institute of Physics, Polish Academy of Sciences(波兰科学院物理研究所磁学国际研究中心);Institute of Physics, Polish Academy of Sciences(波兰科学院物理研究所)
Metallic state in the vicinity of molecular orbital crystallization in the d$^1$ thiospinel ZnTi$_2$S$_4$ prepared via a reductive ion-exchange reaction
Orbital-Selective Spin-Orbit Mott Insulator in Fractional Valence Iridate La$_3$Ir$_3$O$_{11}$
Henan University(河南大学);Henan Academy of Sciences(河南省科学院);Westlake University(西湖大学);Shandong University(山东大学);Chinese Academy of Sciences(中国科学院);Tianjin University(天津大学);Nanjing University(南京大学);Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所);University of Chinese Academy of Sciences(中国科学院大学)
Massachusetts Institute of Technology(麻省理工学院);Flatiron Institute(平顿研究所);University of British Columbia(不列颠哥伦比亚大学);Canadian Light Source, Inc.(加拿大光源公司);Lund University(隆德大学);Brookhaven National Laboratory(布鲁克海文国家实验室);Lawrence Berkeley National Laboratory(劳伦斯伯克利国家实验室);Max Planck Institute for Solid State Research(马克斯·普朗克固态研究所);Universität Würzburg(维尔茨堡大学);Ludwig- Maximilians-Universität München(慕尼黑路德维希-马克西米利安大学);Munich Center for Quantum Science and Technology (MCQST)(慕尼黑量子科学与技术中心);Université Paris-Saclay(巴黎萨克雷大学);CNRS(法国国家科学研究中心);CEA(法国原子能和替代能源委员会);Institut de Physique Théorique(理论物理研究所);University of Tokyo(东京大学);University of Stuttgart(斯图加特大学);Collège de France(法兰西公学院);Université PSL(巴黎文理研究大学);Ecole Polytechnique(巴黎综合理工学院);IP Paris(巴黎理工学院);Université de Genève(日内瓦大学)
Dissecting superconductivity in the Ruddlesden-Popper nickelates: The role of electron correlation and interlayer magnetic exchange
Diamond Light Source(钻石光源);National Synchrotron Radiation Laboratory and School of Nuclear Science and Technology, University of Science and Technology of China(中国科学技术大学核科学与技术学院/国家同步辐射实验室);Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, School of Physics, Sun Yat-Sen University(中山大学物理学院/广东省铁电与磁器件重点实验室);Department of Physics, University of Oxford(牛津大学物理系);National Laboratory of Solid State Microstructures and Department of Physics, Nanjing University(南京大学固体微结构物理国家重点实验室/物理学院);Collaborative Innovation Center of Advanced Microstructures, Nanjing University(南京大学先进微结构协同创新中心)