Motivated by recent developments in magnetic materials, frustrated nanoarrays and cold atomic systems, we investigate the behaviour of dipolar spins on the frustrated two-dimensional kagome lattice. By combining the Luttinger-Tisza approach, numerical energy minimization, spin-wave analysis and parallel tempering Monte-Carlo, we study long-range ordering and finite-temperature phase transitions for a Hamiltonian containing both dipolar and nearest-neighbor interactions. For both weak and moderate dipolar interactions, the system enters a three-sublattice long-range ordered state, with each triangle having vanishing dipole and quadrupole moments; while for dominating dipolar interactions we uncover ferrimagnetic three-sublattice order. These are also the ground states for XY spins. We discuss excitations of, as well as phase transitions into, these states. We find behaviour consistent with Ising criticality for the 120-degree state, while the ferrimagnetic state appears to be associated with drifting exponents. The celebrated flat band of zero-energy excitations of the kagome nearest-neighbour Heisenberg model is lifted to finite energies but acquires only minimal dispersion as dipolar interactions are added.
The $S=1/2$ kagome- and triangular-lattice Heisenberg antiferromagnets are investigated using the numerical exact diagonalization and the finite-size scaling analysis. The behaviour of the field derivative at zero magnetization is examined for both systems. The present result indicates that the spin excitation is gapless for each system.
The effect of the quenched bond-randomness on the ordering of the $S=1/2$ antiferromagnetic Heisenberg model on the kagome lattice is investigated by means of an exact-diagonalization method. When the randomness exceeds a critical value, the ground state of the model exhibits a transition within the non-magnetic state into the randomness-relevant gapless spin-liquid state. Implications to the S=1/2 kagome-lattice antiferromagnet herbertsmithite is discussed.
We have studied the ground state of the classical Kagome antiferromagnet NaBa$_{2}$Mn$_{3}$F$_{11}$. Strong magnetic Bragg peaks observed in the $d$-spacing shorter than 6.0 Å were indexed by the propagation vectors of $\boldsymbol{k}_{0} = (0,0,0)$. Additional peaks with weak intensities in the range of the $d$-spacing longer than 8.0 Å were indexed by the incommensurate vectors of $\boldsymbol{k}_{1}=(0.3209(2),0.3209(2),0)$ and $\boldsymbol{k}_{2}=(0.3338(4),0.3338(4),0)$. Magnetic structure analysis exhibits that the 120$^{\circ}$ structure with the {\it tail-chase} geometry having $\bolds…
We present an extensive quantum Monte Carlo study of a nearest-neighbor, singlet-projection model on the kagome lattice that exhibits SO($N$) symmetry and is sign-problem-free. We find that in contrast to the previously studied SU($N$) variations of this model, the non-bipartite lattices appear to harbor spin-liquid phases for intermediate values of $N$, a result also seen on the triangular lattice with this same model. Unlike the triangular lattice, however, the kagome lattice appears to admit no valence bond solid (VBS) phase for large $N$, instead remaining a spin-liquid. We also observe th…
Using an advanced Monte Carlo algorithm and high precision spin dynamics simulation, we investigated the dynamical behavior of the Heisenberg antiferromagnet on a kagome lattice at extremely low temperatures. We demonstrate that the detection and correct identification of propagating excitations depends crucially on the choice of coordinates and we show how modes are displaced in Fourier space if a single, global Cartesian coordinate system is chosen.
We consider the thermodynamic properties of the quasi-two-dimensional spin-half Heisenberg ferromagnet on the stacked square and the stacked kagomé lattices by using the spin-rotation-invariant Green's function method. We calculate the critical temperature $T_C$, the uniform static susceptibility $χ$, the correlation lengths $ξ_ν$ and the magnetization $M$ and investigate the short-range order above $T_C$. We find that $T_C$ and $M$ at $T>0$ are smaller for the stacked kagomé lattice which we attribute to frustration effects becoming relevant at finite temperatures.
A fractionally quantized Berry phase is examined numerically in an anisotropic spin-1/2 XXZ model on the Kagome lattice. It is shown that the Berry phase has a fractionally quantized and non-zero value when an anisotropy is increased, which is consistent with the emergence of the tripartite entangled plaquette phase discussed by J. Carrasquilla et al. [Phys. Rev. B96, 054405 (2017)].
An effective-field theory based on the single-spin cluster has been used to study of a diluted spin-$1/2$ Ising antiferromagnet on the Kagome lattice with nearest-neighbor interactions. We observe five plateaus in the magnetization curve of the diluted antiferromagnet when a magnetic field is applied which is in agreement with Monte Carlo calculation. The effect of the site-dilution on the magnetic susceptibility is also investigated and discussed. In particular, we have found that the frustrated Kagome lattice inverse susceptibility fall to zero at $0$K.
We find an exact spin liquid state without time reversal symmetry on the kagome lattice with odd number of electrons per unit cell and explicit wave functions for all eigenstates. We also obtain that all spin-spin correlations are zero except trivial cases. We then show that there are anyonic excitations in our model. Finally, we demonstrate the existence of ground state degeneracy and gapless edge states indicating nontrivial topological order in our model. We also label all eiginstates on torus by local and global string operators.
We discuss the ground state and the low-lying excitations of the spin-half Heisenberg antiferromagnet on the two-dimensional square-kagome lattice. This magnetic system belongs to the class of highly frustrated spin systems with an infinite non-trivial degeneracy of the classical ground state as it is known also for the Heisenberg antiferromagnet on the kagome and on the star lattice. The quantum ground state of the spin-half system is a quantum paramagnet likely with a finite spin gap and with a large number of non-magnetic excitations within this gap. The magnetization versus field curve sho…
We study the ground-state properties of the S=1/2 Heisenberg models on the quasi-onedimensional kagome strip lattices by the exact diagonalization and density matrix renormalization group methods. The models with two different strip widths share the same lattice structure in their inner part with the spatially anisotropic two-dimensional kagome lattice. When there is no magnetic frustration, the well-known Lieb-Mattis ferrimagnetic state is realized in both models. When the strength of magnetic frustration is increased, on the other hand, the Lieb-Mattis-type ferrimagnetism is collapsed. We fi…
We compute specific heat of the antiferromagnetic spin-1/2 Heisenberg model on the kagome lattice. We use a recently introduced technique to analyze high-temperature series expansion based on the knowledge of high-temperature series expansions, the total entropy of the system and the low-temperature expected behavior of the specific heat as well as the ground-state energy. In the case of kagome-lattice antiferromagnet, this method predicts a low-temperature peak at T/J<0.1.
The magnetization process of the spin-1/2 antiferromagnetic Heisenberg model on two-dimensional square-kagome lattice is studied theoretically. The metamagnetic jumps exist in the magnetization process at the higher edge of the 1/3 and 2/3 plateaus. The parameter-dependencies of the critical field and the magnitude of the magnetization jump at the higher edge of the 1/3 plateau are obtained by using the approximated state in the unit cell and compared with the nu- merical results of the exact diagonalization of 42 sites.
We investigate the ground-state phase diagram of the Kondo lattice model with classical localized spins on triangular-to-kagome lattices by using a variational calculation. We identify the parameter regions where a four-sublattice noncoplanar order is stable with a finite spin scalar chirality while changing the lattice structure from triangular to kagome continuously. Although the noncoplanar spin states appear in a wide range of parameters, the spin configurations on the kagome network become coplanar as approaching the kagome lattice; eventually, the scalar chirality vanishes for the kagome…
We investigate the $S=1/2$ quantum spin antiferromagnets on the triangular and Kagome lattices in magnetic field, using the numerical exact diagonalization. Particularly we focus on an anomalous magnetization behavior of each system at 1/3 of the saturation magnetization. The critical exponent analyses suggest that it is a conventional magnetization plateau on the triangular lattice, while an unconventional phenomenon, called the magnetization ramp, on the Kagome lattice.
We performed inelastic neutron scattering measurements on a polycrystalline sample of a classical kagome antiferromagnet NaBa$_{2}$Mn$_{3}$F$_{11}$ to investigate the possibility of a dispersionless zero-energy excitation associated with rotation of spins along the chains. The observed spectra indeed exhibit such an excitation with strong intensity at low energy, as well as dispersive excitations with weak intensity at high energy. Combining the measurements with calculations from linear spin-wave theory reveals that NaBa$_{2}$Mn$_{3}$F$_{11}$ is a good realization of the classical kagome anti…
Saturation field entropies of antiferromagnetic Ising models on quasi one-dimensional lattices (ladders) and the kagome lattice are calculated. The former is evaluated exactly by constructing the corresponding transfer matrices, while the latter calculation uses Binder's algorithm for efficiently and exactly computing the partition function of over 1300 spins to give, in Boltzmann's units, S = 0.393589(6). We comment on the relation of the kagome lattice to the experimental situation in the spin-ice compound dysprosium titanium oxide.
The recently discovered natural minerals Cu3Zn(OH)6Cl2 and Cu3Mg(OH)6Cl2 are spin 1/2 systems with an ideal kagome geometry. Based on electronic structure calculations, we develop a realistic model which includes couplings across the kagome hexagons beyond the original kagome model that are intrinsic in real kagome materials. Exact diagonalization studies for the derived model reveal a strong impact of these couplings on the magnetic ground state. Our predictions could be compared to and supplied with neutron scattering, thermodynamic and NMR data.
A brief review is provided of earlier work on the low temperature phases of $S=1$ kagome and triangular lattice antiferromagnets in which there is sufficiently strongly single-ion anisotropy $D$ that dominates over the antiferromagnetic exchange $J$.
Recent experimental discovery of several families of kagome-lattice materials has boosted the interest in electronic correlations on kagome lattice. As an initial step to understand the observed complex phenomena, it is helpful to know the correspondence between simple forms of interactions and the induced correlated states on kagome lattice. Considering the lack of such studies, here we systematically investigate the attractive kagome-lattice Hubbard model using the mean-field approach and determinant quantum Monte Carlo (DQMC). A charge-density-wave order satisfying the triangle rule is pred…
We study the Heisenberg model on the pinwheel distorted kagome lattice as observed in the material Rb_2Cu_3SnF_12. Experimentally relevant thermodynamic properties at finite temperatures are computed utilizing numerical linked-cluster expansions. We also develop a Lanczos-based, zero-temperature, numerical linked cluster expansion to study the approach of the pinwheel distorted lattice to the uniform kagome-lattice Heisenberg model. We find strong evidence for a phase transition before the uniform limit is reached, implying that the ground state of the kagome-lattice Heisenberg model is likely…
We consider the effects of doping the S=3/2 kagome lattice with static, nonmagnetic impurities. By exact diagonalization calculations on small clusters we deduce the local spin correlations and magnetization distribution around a vacancy. As in the S=1/2 kagome lattice, in the vicinity of the impurity we find an extended region where the spin correlations are altered as a consequence of frustation relief, and no indications for the formation of local moments. We discuss the implications of our results for local probe measurements on S=3/2 kagome materials.
Motivated by a recent experiment on Rb2Cu3SnF12, where spin-1/2 Cu2+ moments reside on the layers of Kagome-like lattices, we investigate quantum ground states of the antiferromagnetic Heisenberg model on a series of deformed Kagome lattices. The deformation is characterized by a weaker exchange coupling (alpha*J) on certain lattice links appropriate for Rb2Cu3SnF12 with alpha=1 corresponding to the ideal Kagome lattice. In particular, we study possible valence bond solid phases using the perturbation theory around isolated dimer limits, dimer series expansion, and self-consistent bond operato…
We use $^{79}$Br nuclear quadrupole resonance (NQR) to demonstrate that ultra slow lattice dynamics set in below the temperature scale set by the Cu-Cu super-exchange interaction $J$~($\simeq160$~K) in the kagome lattice Heisenberg antiferromagnet Zn-barlowite. The lattice completely freezes below 50~K, and $^{79}$Br NQR lineshapes become twice broader due to increased lattice distortions. Moreover, the frozen lattice exhibits an oscillatory component in the transverse spin echo decay, a typical signature of pairing of nuclear spins by indirect nuclear spin-spin interaction. This indicates tha…
We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide an unambiguous assignment of infrared-active lattice vibrations involving in-plane and out-of-plane atom displacements in the kagome layers. Upon cooling, non-thermal red-shifts and broadening appear specifically for modes that deform the kagome layer or affect the Cu-O-Cu bond angles, thus creating pronounced modifications of the antiferromagnetic exchange c…
The magnetization process of the spin-S Heisenberg antiferromagnet on the kagome lattice is studied by the numerical-diagonalization method. Our numerical-diagonalization data for small finite-size clusters with S=1, 3/2, 2, and 5/2 suggest that a magnetization plateau appears at one-third of the height of the saturation in the magnetization process irrespective of S. We discuss the S dependences of the edge fields and the width of the plateau in comparison with recent results obtained by real-space perturbation theory.
The magnetization process of the isotropic Heisenberg antiferromagnet on the kagome lattice is studied. Data obtained from the numerical-diagonalization method are reexamined from the viewpoint of the derivative of the magnetization with respect to the magnetic field. We find that the behavior of the derivative at approximately one-third of the height of the magnetization saturation is markedly different from that for the cases of typical magnetization plateaux. The magnetization process of the kagome-lattice antiferromagnet reveals a new phenomenon, which we call the "magnetization ramp".
We study the system size dependence of the singlet-triplet excitation gap in the $S=1/2$ kagome-lattice Heisenberg antiferromagnet by numerical diagonalization. We successfully obtain a new result of a cluster of 42 sites. The two sequences of gaps of systems with even-number sites and that with odd-number sites are separately analyzed. Careful examination clarifies that there is no contradiction when we consider the system to be gapless.
We study a model of strongly correlated spinless fermions on a kagome lattice at 1/3 filling, with interactions described by an extended Hubbard Hamiltonian. An effective Hamiltonian in the desired strong correlation regime is derived, from which the spectral functions are calculated by means of exact diagonalization techniques. We present our numerical results with a view to discussion of possible signatures of confinement/deconfinement of fractional charges.
We study the spin-1/2 Heisenberg model in a lattice that interpolates between the triangular and the kagome lattices. The exchange interaction along the bonds of the kagome lattice is J, and the one along the bonds connecting kagome and non-kagome sites is J', so that J'=J corresponds to the triangular limit and J'=0 to the kagome one. We use variational and exact diagonalization techniques. We analyze the behavior of the order parameter for the antiferromagnetic phase of the triangular lattice, the spin gap, and the structure of the spin excitations as functions of J'/J. Our results indicate …
A quantum dimer model (QDM) on the kagome lattice with an extensive ground-state entropy was recently introduced [Phys. Rev. B 67, 214413 (2003)]. The ground-state energy of this QDM in presence of one and two static holes is investigated by means of exact diagonalizations on lattices containing up to 144 kagome sites. The interaction energy between the holes (at distances up to 7 lattice spacings) is evaluated and the results show no indication of confinement at large hole separations.
Magnetization plateaus in quantum spin systems emerges in two-dimensional frustrated systems such as kagome lattice. The spin-1/2 antiferromagnetic Heisenberg model on square-kagome lattice is also appropriate for the study of magnetization plateau. Motivated by recent experimental finding of such a square-kagome lattice with nonequivalent three bonds, we investigate the phase diagrams and magnetization plateaus of the lattice by the exact diagonalization method. In addition to previously reported the 1/3 and 2/3 plateaus in the model with two equivalent bonds, we find a new 2/3 plateau whose …
In spin-charge coupled systems, geometrical frustration of underlying lattice structures can give rise to nontrivial magnetic orders and electronic states. Here we explore such a possibility in the Kondo lattice model with classical localized spins on a triangular lattice by using a variational calculation and simulated annealing. We find that the system exhibits a four-sublattice collinear ferrimagnetic phase at 5/8 filling for a large Hund's-rule coupling. In this state, the system spontaneously differentiates into the up-spin kagome network and the isolated down-spin sites, which we call th…
In order to study the magnetic properties of frustrated metallic systems, we present Quantum Monte Carlo data on the magnetic susceptibility of the Hubbard model on triangular and Kagome lattices. We show that the underlying lattice structure is important, and determines the nature and the doping dependence of the magnetic fluctuations. In particular, in the doped Kagome case we find strong short-range magnetic correlations, which makes the metallic Kagome systems a promising field for studies of superconductivity.
General conditions in which disordered, spin liquid, and valence-bond ordered phases occur in quantum Ising antiferromagnets are studied using the prototype Kagome lattice spin models. A range of quantum dynamical processes in the Ising model, with and without total Ising spin conserved, are analytically shown to yield all three characteristic quantum paramagnetic phases in the Kagome system. Special emphasis is given to the XXZ model that can be sensibly compared to the Kagome lattice Heisenberg antiferromagnet. It is explicitly demonstrated that the total-spin-conserving dynamics can yield a…
Numerical investigation on the thermodynamic properties of an Ising spin Kondo lattice model on a kagome lattice is reported. By using Monte Carlo simulation, we investigated the magnetic phases at 1/3-filling. We identified two successive transitions from high-temperature paramagnetic state to a Kosterlitz-Thouless-like phase in an intermediate temperature range and to a partially disordered phase at a lower temperature. The partially disordered state is characterized by coexistence of antiferromagnetic hexagons and paramagnetic sites with period $\sqrt3 \times \sqrt3$. We compare the results…
We investigate the connection between highly frustrated kagome based Hamiltonians and a recently synthesized family of materials containing Ti3+ S=1/2 ions. Employing a combination of all electron density functional theory and numerical diagonalization techniques, we establish the Heisenberg Hamiltonians for the distorted kagome antiferromagnets Rb2NaTi3F12, Cs2NaTi3F12 and Cs2KTi3F12. We determine magnetization curves in excellent agreement with experimental observations. Our calculations successfully clarify the relationship between the experimental observations and the magnetization-plateau…
Unconventional features of the magnetization curve at zero temperature such as plateaus or jumps are a hallmark of frustrated spin systems. Very little is known about their behavior at non-zero temperatures. Here we investigate the temperature dependence of the magnetization curve of the kagome lattice antiferromagnet in particular at 1/3 of the saturation magnetization for large lattice sizes of up to N=48 spins. We discuss the phenomenon of asymmetric melting and trace it back to a combined effect of unbalanced magnetization steps on either side of the investigated plateau as well as on the …
We demonstrate that interactions can substantially undermine the free-particle description of magnons in ferromagnets on geometrically frustrated lattices. The anharmonic coupling, facilitated by the Dzyaloshinskii-Moriya interaction, and a highly-degenerate two-magnon continuum yield a strong, non-perturbative damping of the high-energy magnon modes. We provide a detailed account of the effect for the $S=1/2$ ferromagnet on the kagomé lattice and propose further experiments.
The spin wave excitations of the ideal S=5/2 Kagome lattice antiferromagnet KFe3(OH)6(SO4)2 have been measured using high-resolution inelastic neutron scattering. We directly observe a flat mode which corresponds to a lifted "zero energy mode," verifying a fundamental prediction for the Kagome lattice. A simple Heisenberg spin Hamiltonian provides an excellent fit to our spin wave data. The antisymmetric Dzyaloshinskii-Moriya interaction is the primary source of anisotropy and explains the low temperature magnetization and spin structure.
We study the ground state of a spin-half Heisenberg antiferromagnet on the stacked kagome lattice by using a spin-rotation-invariant Green's-function method. Since the pure two-dimensional kagome antiferromagnet is most likely a magnetically disordered quantum spin liquid, we investigate the question whether the coupling of kagome layers in a stacked three-dimensional system may lead to a magnetically ordered ground state. We present spin-spin correlation functions and correlation lengths. For comparison we apply also linear spin wave theory. Our results provide strong evidence that the system…
Determining ground states of correlated electron systems is fundamental to understanding novel phenomena in condensed matter physics. A difficulty, however, arises in a geometrically frustrated system in which the incompatibility between the global topology of an underlying lattice and local spin interactions gives rise to macroscopically degenerate ground states, potentially prompting the emergence of quantum spin states, such as resonating valence bond (RVB) and valence bond solid (VBS). Although theoretically proposed to exist in a kagome lattice -- one of the most highly frustrated lattice…
Spin-1/2 magnets with kagome geometry, being for years a generic object of theoretical investigations, have few real material realizations. Recently, a DFT-based microscopic model for two such materials, kapellasite Cu3Zn(OH)6Cl2 and haydeeite Cu3Mg(OH)6Cl2, was presented [O. Janson, J. Richter and H. Rosner, arXiv:0806.1592]. Here, we focus on the intrinsic properties of real spin-1/2 kagome materials having influence on the magnetic ground state and the low-temperature excitations. We find that the values of exchange integrals are strongly dependent on O--H distance inside the hydroxyl group…
Kagome lattices host flat bands due to their frustrated lattice geometry, which leads to destructive quantum interference of electron wave functions. Here, we report imaging of the kagome flat band localization in real-space using scanning tunneling microscopy. We identify both the Fe3Sn kagome lattice layer and the Sn2 honeycomb layer with atomic resolution in kagome antiferromagnet FeSn. On the Fe3Sn lattice, at the flat band energy determined by the angle resolved photoemission spectroscopy, tunneling spectroscopy detects an unusual state localized uniquely at the Fe kagome lattice network.…
In the theory of quantum spin liquids, gauge fluctuations are emergent excitations at low energy. The gauge magnetic field is proportional to the scalar spin chirality, S1.(S2xS3). It is therefore highly desirable to measure the fluctuation spectrum of the scalar spin chirality. We show that in the Kagome lattice with a Dzyaloshinskii-Moriya term, the fluctuation in Sz which is readily measured by neutron scattering contains a piece which is proportional to the chirality fluctuation.
We consider the Kondo-lattice model on the kagome lattice and study its weak-coupling instabilities at band filling fractions for which the Fermi surface has singularities. These singularites include Dirac points, quadratic Fermi points in contact with a flat band, and Van Hove saddle points. By combining a controlled analytical approach with large-scale numerical simulations, we demonstrate that the weak-coupling instabilities of the Kondo-lattice model lead to exotic magnetic orderings. In particular, some of these magnetic orderings produce a spontaneous quantum anomalous Hall state.
We study the phase diagram of the extended Hubbard model on the kagome lattice at 1/3 filling. By combining a configuration interaction approach to an unrestricted Hartree-Fock, we construct an effective hamiltonian which takes the correlations back on top of the mean-field solution. We obtain a rich phase diagram with, in particular, the presence of two original phases. The first one consists of polarized droplets of metal standing on the hexagons of the lattice, and an enlarged kagome charge order, inversely polarized, on the remaining sites. The second, obeying a local ice-rule type constra…
The hole-doped kagome lattice of Cu2+ ions in LaCuO2.66 was investigated by nuclear quadrupole resonance (NQR), electron spin resonance (ESR), electrical resistivity, bulk magnetization and specific heat measurements. For temperatures above ~180 K, the spin and charge properties show an activated behavior suggestive of a narrow-gap semiconductor. At lower temperatures, the results indicate an insulating ground state which may or may not be charge ordered. While the frustrated spins in remaining patches of the original kagome lattice might not be directly detected here, the observation of coexi…
We introduce quantum dimer models on lattices made of corner-sharing triangles. These lattices includes the kagome lattice and can be defined in arbitrary geometry. They realize fully disordered and gapped dimer-liquid phase with topological degeneracy and deconfined fractional excitations, as well as solid phases. Using geometrical properties of the lattice, several results are obtained exactly, including the full spectrum of a dimer-liquid. These models offer a very natural - and maybe the simplest possible - framework to illustrate general concepts such as fractionalization, topological ord…
We construct a phenomenological Z_2 lattice gauge theory to describe the spin-liquid state of the S=1/2 kagome Heisenberg antiferromagnet in the sector with zero total spin. The model is a natural generalization of the Misguich-Serban-Pasquier Hamiltonian with added interactions that are strongly constrained by lattice symmetries. We are able to reproduce qualitatively many of the characteristic features observed in recent numerical studies. We also make connections to the previous works along similar lines.
Within the t-J model, we study the electronic properties of the doped antiferromagnet on the kagome lattice based on the framework of the self-consistent mean-field theory. At the half-filling, the spin-liquid ground-state energy per site of the kagome antiferromagnet is Eg/NJ=-0.859, which is in very good agreement with the numerical estimates. Away from the half-filling, the electron photoemission spectroscopy and density of states are discussed, and the results indicate that there is a gap in the normal-state of the system.
Quantum materials with tunable correlated and/or topological electronic states, such as the electronic Kagome lattice, provide an ideal platform to study the exotic quantum properties. However, the real-space investigations on the correlated electronic Kagome lattice have been rarely reported. Herein, we report on the electronic Kagome lattice emerging in the correlated charge-density-wave (CDW) state of 1T-TaS$_2$ at ~200 K via variable-temperature scanning tunneling microscopy (VT-STM). This emergent Kagome lattice can be considered a fractional electron-filling superstructure with reduced t…
Motivated by the recent discovery of metallic kagome lattice materials, AV$_{3}$Sb$_{5}$ (A=K, Rb, Cs), we investigate the ground state of the half-filled kagome lattice Hubbard model by employing the density-matrix renormalization group (DMRG) method. We identify a metal-insulator transition around $U \thicksim U_{c1}$ and four distinct phases as a function of $U/t$ on narrower cylinders, including a metallic phase at $U < U_{c1}$, two insulating intermediate phases: a translational symmetry breaking phase at $U_{c1} < U < U_{c2}$ and a quantum spin liquid phase at $U_{c2} < U < U_{c3}$, and …
We investigate the stability and the nature of the chiral spin liquids which were recently uncovered in extended Heisenberg models on the kagome lattice. Using a Gutzwiller projected wave function approach -- i.e. a parton construction -- we obtain large overlaps with ground states of these extended Heisenberg models. We further suggest that the appearance of the chiral spin liquid in the time-reversal invariant case is linked to a classical transition line between two magnetically ordered phases.
Signatures of field-induced multi-color kagome spin liquids in the dipole-octupole pyrochlore $\mathrm{Ce_2Hf_2O_7}$
Université Paris-Saclay, CNRS, Laboratoire de Physique des Solides（巴黎萨克雷大学，法国国家科学研究中心，固体物理实验室）；The Institute for Solid State Physics, The University of Tokyo（东京大学固体物质研究所）；Institut für Theoretische Physik and Würzburg-Dresden Cluster of Excellence ctd.qmat, Technische Universität Dresden（德累斯顿工业大学理论物理研究所及维尔茨堡-德累斯顿卓越集群ctd.qmat）；Department of Physics, The University of Tennessee（田纳西大学物理系）；Institute for Advanced Study, Chengdu University（成都大学高等研究院）；Department of Physics and Astronomy, McMaster University（麦克马斯特大学物理与天文学系）；Brockhouse Institute for Materials Research, McMaster University（麦克马斯特大学布罗克豪斯材料研究所）；Département de Physique, Université（大学物理系）
A novel cuprate Volborthite, Cu3V2O7(OH)2-2H2O, containing an S-1/2 (Cu 2+ spin) kagome-like lattice is studied by magnetic susceptibility, specific heat, and 51 V NMR measurements. Signs for neither long-range order nor spin-gapped singlet ground states are detected down to 1.8 K, in spite of large antiferromagnetic couplings of ~100 K between Cu spins forming a two-dimensional kagome-like network. It is suggested that Volborthite represents a system close to a quantum critical point between classical long-range ordered and quantum disordered phases.
We study strongly correlated electrons on a kagome lattice at 1/6 and 1/3 filling. They are described by an extended Hubbard Hamiltonian. We are concerned with the limit |t|<<V<<U with hopping amplitude t, nearest-neighbor repulsion V and on-site repulsion U. We derive an effective Hamiltonian and show, with the help of the Perron-Frobenius theorem, that the system is ferromagnetic at low temperatures. The robustness of ferromagnetism is discussed and extensions to other lattices are indicated.
