Magnetic field tuning of exciton polaritons in a semiconductor microcavity
B. Pietka, D. Zygmunt, M. Krol, J. Szczytko, J. Lusakowski, M. R. Molas, A. A. L. Nicolet, P. Stepnicki, P. Zieba, I. Tralle, F. Morier-Genoud, M. Matuszewski, … 展开作者
B. Pietka, D. Zygmunt, M. Krol, J. Szczytko, J. Lusakowski, M. R. Molas, A. A. L. Nicolet, P. Stepnicki, P. Zieba, I. Tralle, F. Morier-Genoud, M. Matuszewski, M. Potemski, B. Deveaud
We detail the influence of a magnetic field on exciton-polaritons inside a semiconductor microcavity. Magnetic field can be used as a tuning parameter for exciton and photon resonances. We discuss the change of the exciton energy, the oscillator strength and redistribution of the polariton density along the dispersion curves due to the magnetically-induced detuning. We have observed that field-induced shrinkage of the exciton wave function has a direct influence not only on the exciton oscillator strength, which is observed to increase with the magnetic field, but also on the polariton linewidth. We discuss the effect of the Zeeman splitting on polaritons which magnitude changes with the exciton Hopfield coefficient and can be modelled by independent coupling of the two spin components of excitons with cavity photons.
The spin Hall effect for polaritons (SHEP) in a transition metal dichalcogenides (TMDC) monolayer embedded in a microcavity is predicted. We demonstrate that two counterpropagating laser beams incident on a TMDC monolayer can deflect a superfluid polariton flow due to the generation the effective gauge vector and scalar potentials. The components of polariton conductivity tensor for both non-interacting polaritons without Bose-Einstein condensation (BEC)and for weakly-interacting Bose gas of polaritons in the presence of BEC and superfluidity are obtained. It is shown that the polariton flows …
We have developed a model of the nonlinear polariton dynamics in realistic 3D non-planar microcavity wires in the driven-dissipative regime. We find that the typical microcavity optical bistability evolves into multistability upon variation of the model parameters. The origin of the multistability is discussed in detail. We apply linear perturbation analysis to modulational instabilities, and identify conditions for localisation of composite multi-mode polariton solitons in the triggered parametric oscillator regime. Further, we demonstrate stable polariton soliton propagation in tilted and ta…
We present a precise calculation of spatially-indirect exciton states in semiconductor coupled quantum wells and polaritons formed from their coupling to the optical mode of a microcavity. We include the presence of electric and magnetic fields applied perpendicular to the quantum well plane. Our model predicts the existence of polaritons which are in the strong coupling regime and at the same time possess a large static dipole moment. We demonstrate, in particular, that a magnetic field can compensate for the reduction in light-matter coupling that occurs when an electric field impresses a di…
We describe exciton-polariton modes formed by the interaction between excitons in a 2D layer of a transition metal dichalcogenide embedded in a cylindrical microcavity and the microcavity photons. For this, an expression for the excitonic susceptibility of a semiconductor disk placed in the symmetry plane perpendicular to the axis of the microcavity is derived. Semiclassical theory provides dispersion relations for the polariton modes, while the quantum-mechanical treatment of a simplified model yields the Hopfield coefficients, measuring the degree of exciton-photon mixing in the coupled mode…
We present a systematic investigation of two-photon excitation processes in a GaAs-based microcavity in the strong-coupling regime. We observe second harmonic generation resonant to the upper and lower polariton level, which exhibits a strong dependence on the photonic fraction of the corresponding polariton. In addition we have performed two-photon excitation spectroscopy to identify $2p$ exciton states which are crucial for the operation as a terahertz lasing device, which was suggested recently [A. V. Kavokin et al., Phys. Rev. Lett. \textbf{108}, 197401 (2012)]. However, no distinct signat…
We study the polarization optical properties of microcavities with embedded (110)-oriented quantum wells. The spin dynamics of exciton polaritons in such structures is governed by the interplay of the spin-orbit splitting of exciton states, which is odd in the in-plane momentum, and the longitudinal-transverse splitting of cavity modes, which is even in the momentum. We demonstrate the generation of polariton spin currents by linearly polarized optical pump and analyze the arising polariton spin textures in the cavity plane. Tuning the excitation spot size, which controls the polariton distrib…
We study tunable polaritons in monolayers of silicene, germanene, and stanene (Xenes) via an external electric field in an open optical microcavity whose length can be adjusted. An external electric field applied perpendicular to the plane of the Xene monolayer simultaneously changes the band gap and the exciton binding energy, while the variable length of the open microcavity allows one to keep the exciton and cavity photon modes in resonance. First, the Schrödinger equation for an electron and hole in an Xene monolayer is solved, yielding the eigenergies and eigenfunctions of the exciton as …
Terahertz emission between exciton-polariton branches in semiconductor microcavities is expected to be strongly stimulated in the polariton laser regime, due to the high density of particles in the lower state (final state stimulation effect). However, non-radiative scattering processes depopulate the upper state and greatly hinder the efficiency of such terahertz sources. In this work, we suggest a new scheme using multiple microcavities and exploiting the transition between two interband polariton branches located below the exciton level. We compare the non-radiative processes loss rates in …
We report an extended family of spin textures in coexisting modes of zero-dimensional polariton condensates spatially confined in tunable open microcavity structures. The coupling between photon spin and angular momentum, which is enhanced in the open cavity structures, leads to new eigenstates of the polariton condensates carrying quantised spin vortices. Depending on the strength and anisotropy of the cavity confinement potential and the strength of the spin-orbit coupling, which can be tuned via the excitonic/photonic fractions, the condensate emissions exhibit either spin-vortex-like patte…
Monolayer transition metal dichalcogenides, known for exhibiting strong excitonic resonances, constitute a very interesting and versatile platform for investigation of light-matter interactions. In this work we report on a strong coupling regime between excitons in monolayer WSe2 and photons confined in an open, voltage-tunable dielectric microcavity. The tunability of our system allows us to extend the exciton-polariton state over a wide energy range and, in particular, to bring the excitonic component of the lower polariton mode into resonance with other excitonic transitions in monolayer WS…
We investigate the statistics of microcavity polariton Bose-Einstein condensation by measuring photoluminescence dynamics from a GaAs microcavity excited by single laser excitation pulses. We directly observe fluctuations (jitter) of the polariton condensation onset time and model them using a master equation for the occupancy probabilities. The jitter of the condensation onset time is an inherent property of the condensate formation and its magnitude is approximately equal to the rise time of the condensate density. We investigate temporal correlations between the emission of condensate in op…
The formation and propagation of a polariton condensate under tightly focused excitation is investigated in a ZnO microcavity both experimentally and theoretically. 2D near-field and far-field images of the condensate are measured under quasi-continuous non-resonant excitation. The corresponding spatial profiles are compared to a model based on the Gross-Pitaevskii equation under cylindrical geometry. This work allows to connect the experiments performed with a small excitation laser spot and the previous kinetic models of condensation in a 2D infinite microcavity, and to determine the relevan…
We present a theoretical model that allows us to describe the dynamics of exciton polaritons in the strong-coupling regime in a monolayer WS2 based semiconductor microcavity. Numerical simulations using Boltzmann equations give an overall description of polariton kinetics over a temperature range of 130-230K, under nonresonant excitation. Here, only the scattering rate via optical phonons (LO) from the upper (UP) towards lower (LP) polariton branches is considered. According this model we show the importance of the radiative lifetime of the polaritonic states relative to polariton relaxation r…
We present an experimental study on the ignition and decay of a polariton optical parametric oscillator (OPO) in a semiconductor microcavity pillar. The combination of a continuous wave laser pump, under quasi-phase matching conditions, and a non-resonant, 2 ps-long pulse probe allows us to obtain the full dynamics of the system. The arrival of the probe induces a blue-shift in the polariton emission, bringing the OPO process into resonance with the pump, which triggers the OPO-process. We time-resolve the polariton OPO signal emission for more than 1 nanosecond in both real and momentum-space…
Electrical control over the energy exchange between exciton states mediated by cavity-polaritons at room temperature is demonstrated. Spatially separated field effect transistors based on monolayers of WS$_2$ and MoS$_2$ are placed in a tuneable Fabry-Pérot microcavity. This device is specially designed for the formation of exciton-polaritons that combine the two exciton species and a tuneable cavity mode. It is further shown that the tuning of the free carrier density in the WS$_2$ film leads to a strong modulation of the Rabi splitting that modifies the excitonic and photonic nature of excit…
Based on the studies of propagation of an exciton-polariton condensate in a patterned optical microcavity with an embedded graphene layer, we propose a design of a Y-shaped electrically-controlled optical switch. The polaritons are driven by a time-independent force due to the microcavity wedge shape and by a time-dependent drag force owing to the interaction of excitons in graphene and the electric current running in a neighboring quantum well. It is demonstrated that one can control the polariton flow direction by changing the direction of the electric current. The simulations also show that…
We are interested in the emission characteristics of an atom interacting with the polaritonic excitations of a semiconductor or insulator embedded in a one-mode cavity. Since polaritons inside of the cavity exhibit intrinsic squeezing, we discuss how the squeezed polariton ground state modifies the atomic emission and how an indirect evidence of polariton squeezing outside of he cavity may be obtained.
We present a microcavity structure with a shifted photonic stop-band to enable efficient non-resonant injection of a polariton condensate with spectrally broad femtosecond pulses. The concept is demonstrated theoretically and confirmed experimentally for a planar GaAs/AlGaAs multilayer heterostructure pumped with ultrashort near-infrared pulses while photoluminescence is collected to monitor the optically injected polariton density. As the excitation wavelength is scanned, a regime of polariton condensation can be reached in our structure at a consistently lower fluence threshold than in a sta…
Tamm polaritons (TPs) are formed at the interface between two semi-infinite periodic dielectric structures (Bragg mirrors) or other reflectors. Contrary to usual surface polaritons, TPs exist inside the "light cone", even though their amplitude also decreases exponentially with the distance from the interface as it is characteristic of evanescent waves. They couple to elementary excitations in the materials or structures that form the interface, such as metal plasmons or semiconductor excitons. Here we discuss the formation of TPs in the far-infrared (FIR) spectral range, in the optical-phonon…
We consider the possible phases of microcavity polaritons tuned near a bipolariton Feshbach resonance. We show that, as well as the regular polariton superfluid phase, a "molecular" superfluid exists, with (quasi-)long-range order only for pairs of polaritons. We describe the experimental signatures of this state. Using variational approaches we find the phase diagram (critical temperature, density and exciton-photon detuning). Unlike ultracold atoms, the molecular superfluid is not inherently unstable, and our phase diagram suggests it is attainable in current experiments.
Exciton-polariton modes arising from interaction between bound excitons in monolayer thin semiconductor sheets and photons in a Fabry-Perot microcavity are considered theoretically. We calculate the dispersion curves, mode lifetimes, Rabi splitting, and Hopfield coefficients of these structures for two nearly 2D semiconductor materials, MoS2 and WS2, and suggest that they are interesting for studying the rich physics associated with the Bose-Einstein condensation of exciton-polaritons. The large exciton binding energy and dipole allowed exciton transitions, in addition to the relatively easily…
Microcavity polaritons are light-matter quasiparticles that arise from the strong coupling between excitons and photons confined in a semiconductor microcavity. They typically operate at visible or near visible wavelengths. They combine the properties of confined electromagnetic fields, including a sizeable spin-orbit coupling, and the sensitivity to external magnetic fields and particle interactions inherited from their partly matter nature. These features make polaritons an excellent platform to study topological phases in photonics in one and two dimensional lattices, which band properties …
We report spin and intensity coupling of an exciton-polariton condensate to the mechanical vibrations of a circular membrane microcavity. We optically drive the microcavity resonator at the lowest mechanical resonance frequency while creating an optically-trapped spin-polarized polariton condensate in different locations on the microcavity, and observe spin and intensity oscillations of the condensate at the vibration frequency of the resonator. Spin oscillations are induced by vibrational strain driving, whilst the modulation of the optical trap due to the displacement of the membrane causes …
Exciton-polaritons are mixed light-matter quasiparticles. We have developed a statistical model describing stochastic exciton-photon transitions within a condensate of exciton polaritons. We show that the exciton-photon correlator depends on the "hidden variable" which characterizes the rate of exciton-photon transformations in the condensate. We discuss implications of this effect for the quantum statistics of photons emitted by polariton lasers.
The ultrafast scattering dynamics of intersubband polaritons in dispersive cavities embedding GaAs/AlGaAs quantum wells are studied directly within their band structure using a non-collinear pump-probe geometry with phase-stable mid-infrared pulses. Selective excitation of the lower polariton at a frequency of ~25 THz and at a finite in-plane momentum, $k_{||}$, leads to the emergence of a narrowband maximum in the probe reflectivity at $k_{||}=0$. A quantum mechanical model identifies the underlying microscopic process as stimulated coherent polariton-polariton scattering. These results mark …
