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arXiv 1411.7858cond-mat.supr-concond-mat.str-el
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三斜晶系(CaFe $_{1-x}$ Pt $_x$ As)$_{10}$ Pt $_3$ As $_8$的超导性质和预形成库珀对的赝能隙

Superconducting properties and pseudogap from preformed Cooper pairs in the triclinic (CaFe$_{1-x}$Pt$_x$As)$_{10}$Pt$_3$As$_8$

M. A. Surmach, F. Brückner, S. Kamusella, R. Sarkar, P. Y. Portnichenko, J. T. Park, G. Ghambashidze, H. Luetkens, P. Biswas, W. J. Choi, Y. I. Seo, Y. S. Kwon,… 展开作者

M. A. Surmach, F. Brückner, S. Kamusella, R. Sarkar, P. Y. Portnichenko, J. T. Park, G. Ghambashidze, H. Luetkens, P. Biswas, W. J. Choi, Y. I. Seo, Y. S. Kwon, H. -H. Klauss, D. S. Inosov

摘要:

利用μ子自旋弛豫($μ$ SR)、非弹性中子散射(INS)和核磁共振(NMR)研究了具有三斜晶系结构的新型铁基超导体(CaFe $_{1-x}$ Pt $_x$ As)$_{10}$ Pt $_3$ As $_8$(T $_{\rm c}$ = 13 K)。从$μ$ SR弛豫率测量得到的超流密度的温度依赖性表明存在两个超导能隙,$Δ_\text{1}\ggΔ_\text{2}$。根据我们的INS测量,相称的自旋波动集中在($π$,0)波矢量,像大多数其他铁砷化物。它们的强度在T $_\text{c}$上保持不变,表明许多铁基超导体没有典型的自旋共振。相反,我们观察到的$\hslashω_0=\,$ 7毫电子伏左右的自旋激发光谱在相同的波矢,这持续高于T $_{\rm c}$和特征在于比$\hslashω_0/k_\text{B}T_\text{c}\approx\,$ 6.2,这是显着高于典型值的铁磷属元素化物的磁共振模式(~4.3)。在7毫电子伏的磁场强度的温度依赖性揭示了一个异常T* = 45 K附近的消失,这种新的模式。通过NMR观察到的自旋-晶格弛豫速率$1/T_1T$的抑制直接低于T*,在T $_{\rm c}$处没有任何明显的后续异常,表明T* 可以标记(CaFe $_{1-x}$ Pt $_x$ As)$_{10}$ Pt $_3$ As $_8$中赝能隙的开始,这可能与预先形成的库珀对的出现有关。

英文摘要:

Using a combination of muon-spin relaxation ($μ$SR), inelastic neutron scattering (INS) and nuclear magnetic resonance (NMR), we investigated the novel iron-based superconductor with a triclinic crystal structure (CaFe$_{1-x}$Pt$_x$As)$_{10}$Pt$_3$As$_8$ (T$_{\rm c}$ = 13 K), containing platinum-arsenide intermediary layers. The temperature dependence of the superfluid density obtained from the $μ$SR relaxation-rate measurements indicates the presence of two superconducting gaps, $Δ_\text{1}\ggΔ_\text{2}$. According to our INS measurements, commensurate spin fluctuations are centered at the ($π$, 0) wave vector, like in most other iron arsenides. Their intensity remains unchanged across T$_\text{c}$, indicating the absence of a spin resonance typical for many Fe-based superconductors. Instead, we observed a peak in the spin-excitation spectrum around $\hslashω_0=\,$7 meV at the same wave vector, which persists above T$_{\rm c}$ and is characterized by the ratio $\hslashω_0/k_\text{B}T_\text{c}\approx\,$6.2, which is significantly higher than typical values for the magnetic resonant modes in iron pnictides (~4.3). The temperature dependence of magnetic intensity at 7 meV revealed an anomaly around T* = 45 K related to the disappearance of this new mode. A suppression of the spin-lattice relaxation rate, $1/T_1T$, observed by NMR immediately below T* without any notable subsequent anomaly at T$_{\rm c}$, indicates that T* could mark the onset of a pseudogap in (CaFe$_{1-x}$Pt$_x$As)$_{10}$Pt$_3$As$_8$, which is likely associated with the emergence of preformed Cooper pairs.

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