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arXiv 1407.2018cond-mat.str-el
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有限系统Anderson杂质模型的推广:磁矩的带隙控制

Extension of the Anderson impurity model for finite systems: Band gap control of magnetic moments

Konstantin Hirsch, Julian Tobias Lau, Bernd von Issendorff

摘要:

我们研究了嵌入有限尺寸非磁性带隙基质中的单个杂质的自旋磁矩。使用紧束缚模型哈密顿量进行计算。安德森杂质模型中给出的磁性到非磁性转变的简单判据在这些情况下失效。我们展示了如何自旋磁矩的杂质,通常会被淬灭后,可以恢复在费米能级的主机态密度的间隙。杂质自旋磁矩的大小与带隙的大小单调成比例。这种观察甚至适用于具有强离散态密度的主体材料。因此,应该可以通过改变掺杂纳米颗粒的尺寸并由此改变其带隙来调节掺杂纳米颗粒的磁矩。

英文摘要:

We study the spin magnetic moment of a single impurity embedded in a finite-size non-magnetic host exhibiting a band gap. The calculations were performed using a tight-binding model Hamiltonian. The simple criterion for the magnetic to non-magnetic transition as given in the Anderson impurity model breaks down in these cases. We show how the spin magnetic moment of the impurity that normally would be quenched can be restored upon introducing a gap at the Fermi level in the host density of states. The magnitude of the impurity spin magnetic moment scales monotonically with the size of the band gap. This observation even holds for a host material featuring a strongly discretized density of states. Thus, it should be possible to tune the magnetic moment of doped nano-particles by varying their size and thereby their band gap.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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