Carbon based optoelectronic devices promise to revolutionize modern integrated circuits by combining outstanding electrical and optical properties into a unified technology. By coupling nanoelectronic devices to nanophotonic structures functional components such as nanoscale light emitting diodes, narrow-band thermal emitters, cavity controlled detectors and wideband electro optic modulators can be realized for chipscale information processing. These devices not only allow the light-matter interaction of low-dimensional systems to be studied, but also provide fundamental building blocks for high bandwidth on-chip communication. Here we demonstrate how light from an electrically-driven carbon-nanotube can be coupled directly into a photonic waveguide architecture. We realize wafer scale, broadband sources integrated with nanophotonic circuits allowing for propagation of light over centimeter distances. Moreover, we show that the spectral properties of the emitter can be controlled directly on chip with passive devices using Mach-Zehnder interferometers and grating structures. The direct, near-field coupling of electrically generated light into a waveguide, opposed to far-field fiber coupling of external light sources, opens new avenues for compact optoelectronic systems in a CMOS compatible framework.
Electrically-driven light emission from carbon nanotubes could be exploited in nano-scale lasers and single-photon sources, and has therefore been the focus of much research. However, to date, high electric fields and currents have been either required for electroluminescence, or have been an undesired side effect, leading to high power requirements and low efficiencies. In addition, electroluminescent linewidths have been broad enough to obscure the contributions of individual optical transitions. Here, we report electrically-induced light emission from individual carbon nanotube p-n diodes. …
We demonstrate an individual single-walled carbon nanotube light emitter integrated onto a microcavity and a waveguide operating in the telecom wavelength regime. Light emission from the carbon nanotube is enhanced at the cavity resonance and is efficiently extracted from the waveguide facet. We have transferred carbon nanotubes to a nanobeam cavity with a dry process, ensuring that an individual carbon nanotube is used. The guided light emission from a chirality-identified single carbon nanotube has a narrow linewidth of less than 1.3 nm and an off-resonance rejection of $\sim$17 dB. The wave…
Semiconducting single-walled carbon nanotubes show extraordinary electronic and optical properties, such as high charge carrier mobilities and diameter-dependent near-infrared photoluminescence. The introduction of sp3 defects in the carbon lattice of these nanotubes creates new electronic states that result in even further red-shifted photoluminescence with longer lifetimes and higher photoluminescence yield. These luminescent defects or organic color centers can be tuned chemically by controlling the precise binding configuration and the electrostatic properties of the attached substituents.…
We demonstrate with a quantum-mechanical approach that carbon nanotubes are excellent spin-current waveguides and are able to carry information stored in a precessing magnetic moment for long distances with very little dispersion and with tunable degrees of attenuation. Pulsed magnetic excitations are predicted to travel with the nanotube Fermi velocity and are able to induce similar excitations in remote locations. Such an efficient way of transporting magnetic information suggests that nanotubes are promising candidates for memory devices with fast magnetization switchings.
Diazonium reactions with carbon nanotubes form optical $sp^3$ defects that can be used in optical and electrical circuits. We investigate a direct on-device reaction supported by confined laser irradiation and present a technique where an arbitrary carbon nanotube can be preferentially functionalized within a device by matching the light frequency with its transition energy. An exemplary reaction was carried out between (9,7) nanotube and 4-bromobenzenediazonium tetrafluoroborate. The substrate supported nanotubes of multiple semiconducting chiralities were locally exposed to laser light while…
We propose an experimentally viable setup for the realization of one-dimensional ultracold atom gases in a nanoscale magnetic waveguide formed by single doubly-clamped suspended carbon nanotubes. We show that all common decoherence and atom loss mechanisms are small guaranteeing a stable operation of the trap. Since the extremely large current densities in carbon nanotubes are spatially homogeneous, our proposed architecture allows to overcome the problem of fragmentation of the atom cloud. Adding a second nanowire allows to create a double-well potential with a moderate tunneling barrier whic…
The propagation of azimuthally symmetric guided waves in multiwalled carbon nanotubes (MWCNTs) was analyzed theoretically in the mid-infrared and the visible regimes. The MWCNTs were modeled as ensembles of concentric, cylindrical, conducting shells. Slightly attenuated guided waves and antenna resonances due to the edge effect exist for not-too-thick MWCNTs in the far- and mid-infrared regimes. Interband transitions hinder the propagation of guided waves and have a deleterious effect on the performance of a finite-length MWCNT as an antenna. Propagation of surface-plasmon waves along an MWCNT…
Graphene with its dispersion relation resembling that of photons offers ample opportunities for applications in electron optics. The spacial variation of carrier density by external gates can be used to create electron waveguides, in analogy to optical fiber, with additional confinement of the carriers in bipolar junctions leading to the formation of few transverse guiding modes. We show that waveguides created by gating graphene with carbon nanotubes (CNTs) allow obtaining sharp conductance plateaus, and propose applications in the Aharonov-Bohm and two-path interferometers, and a pointlike s…
Molybdenum rhenium alloy thin films can exhibit superconductivity up to critical temperatures of $T_c=15\mathrm{K}$. At the same time, the films are highly stable in the high-temperature methane / hydrogen atmosphere typically required to grow single wall carbon nanotubes. We characterize molybdenum rhenium alloy films deposited via simultaneous sputtering from two sources, with respect to their composition as function of sputter parameters and their electronic dc as well as GHz properties at low temperature. Specific emphasis is placed on the effect of the carbon nanotube growth conditions on…
The in-place growth of suspended carbon nanotubes facilitates the observation of both unperturbed electronic transport spectra and high-Q vibrational modes. For complex structures integrating, e.g., superconducting rf elements on-chip, selection of a chemically and physically resistant material that survives the chemical vapor deposition (CVD) process provides a challenge. We demonstrate the implementation of molybdenum-rhenium coplanar waveguide resonators that exhibit clear resonant behaviour at cryogenic temperatures even after having been exposed to nanotube growth conditions. The properti…
Relativistic massless charged particles in a two-dimensional conductor can be guided by a one-dimensional electrostatic potential, in an analogous manner to light guided by an optical fiber. We use a carbon nanotube to generate such a guiding potential in graphene and create a single mode electronic waveguide. The nanotube and graphene are separated by a few nanometers and can be controlled and measured independently. As we charge the nanotube, we observe the formation of a single guided mode in graphene that we detect using the same nanotube as a probe. This single electronic guided mode in g…
Carbon Nanotubes (CNs) are made of tubular graphite layers. These macromolecules have interesting features which are generally introduced in the first chapter of the thesis. In the rest of the thesis, the light conduction in metallic CNs is investigated. In chapter 2, by modeling metallic single-wall CNs as 2D free electron gas layers, we find the density of electrons on a 2D electron gas and solve the Maxwell's equations for these cylindrical waveguides. We assume the same time-dependency or frequency for the electrons oscillations on the 2D gas layers and the propagating electromagnetic wave…
We probe the high frequency emission of a carbon nanotube based Josephson junction and compare it to its DC Josephson current. The AC emission is probed by coupling the carbon nanotube to an on-chip detector (a Superconductor-Insulator-Superconductor junction), via a coplanar waveguide resonator. The measurement of the photo-assisted current of the detector gives direct access to the signal emitted by the carbon nanotube. We focus on the gate regions that exhibit Kondo features in the normal state and demonstrate that when the DC supercurrent is enhanced by the Kondo effect, the AC Josephson e…
A single-wall carbon nanotube possesses two different types of plasmons specified by the wavenumbers in the azimuthal and axial directions. The azimuthal plasmon that is caused by interband transitions has been studied, while the effect of charge doping is unknown. In this paper, we show that when nanotubes are heavily doped, intraband transitions cause the azimuthal plasmons to appear as a plasmon resonance in the near-infrared region of the absorption spectra, which is absent for light doping due to the screening effect. The axial plasmons that are inherent in the cylindrical waveguide struc…
Hybrid circuit quantum electrodynamics (QED) involves the study of coherent quantum physics in solid state systems via their interactions with superconducting microwave circuits. Here we present an implementation of a hybrid superconducting qubit that employs a carbon nanotube as a Josephson junction. We realize the junction by contacting a carbon nanotube with a superconducting Pd/Al bi-layer, and implement voltage tunability of the qubit frequency using a local electrostatic gate. We demonstrate strong dispersive coupling to a coplanar waveguide resonator via observation of a resonator frequ…
In a recent paper Liang {\it et al.} [Nature {\bf 411}, 665 (2001)] showed experimentally, that metallic nanotubes, strongly coupled to external electrodes, may act as coherent molecular waveguides for electronic transport. The experimental results were supported by theoretical analysis based on the scattering matrix approach. In this paper we analyze theoretically this problem using a real-space approach, which makes it possible to control quality of interface contacts. Electronic structure of the nanotube is taken into account within the tight-binding model. External electrodes and the centr…
We show that a single quantum emitter can efficiently couple to the tunable plasmons of a highly doped single-wall carbon nanotube (SWCNT). Plasmons in these quasi-one-dimensional carbon structures exhibit deep subwavelength confinement that pushes the coupling efficiency close to 100% over a very broad spectral range. This phenomenon takes place for distances and tube diameters comprising the nanometer and micrometer scales. In particular, we find a beta factor ~1 for QEs placed 1-100 nm away from SWCNTs that are just a few nanometers in diameter, while the corresponding Purcell factor exceed…
Nanomechanical devices can operate at much higher speeds than their macroscopic analogues, due to low inertia. For example, peak speeds >100m/s have been predicted for carbon nanotube devices. This stimulates our interest in the atomic-scale physics of friction at high velocity. Here we study a model nanosystem consisting of a graphene flake moving freely on a graphite substrate at >100m/s. Using molecular dynamics we discover that ultra-low friction, or superlubricity, is punctuated by high-friction transients as the flake rotates through successive crystallographic alignments with the substr…
Nonreciprocal plasmons in one-dimensional carbon nanostructures
Max-Born-Institut（马克斯·玻恩研究所）；Center for Nanophotonics, NWO Institute AMOLF（纳米光子学中心，NWO AMOLF研究所）；ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科学技术研究所）；ICREA-Institució Catalana de Recerca i Estudis Avançats（ICREA-加泰罗尼亚研究高级学院）；POLIMA—Center for Polariton-driven Light–Matter Interactions, University of Southern Denmark（POLIMA-极化激元驱动光物质相互作用中心，南丹麦大学）；Danish Institute for Advanced Study, University of Southern Denmark（丹麦高等研究院，南丹麦大学）
Taming quantum interference: a route to high electrical conductance in carbon nanotube assemblies
University of Warsaw（华沙大学）；Warsaw University of Technology（华沙理工大学）；University of Cambridge（剑桥大学）；University of Cincinnati（辛辛那提大学）；Air Force Research Laboratory（空军研究实验室）；Cranfield University（克兰菲尔德大学）；Los Alamos National Laboratory（洛斯阿拉莫斯国家实验室）；CIC nanoGUNE（nanoGUNE研究中心）；Simune Atomistics（Simune原子模拟公司）；Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC and BIST（加泰罗尼亚纳米科学与纳米技术研究所（ICN2），西班牙国家科学研究委员会和巴塞罗那自治大学系统）；Center for Terahertz Research and Applications - Centera 2, Centre for Advanced Materials and Technologies (CEZAMAT), Warsaw University of Technology（太赫兹研究与应用技术中心 - Centera 2，先进材料与技术中心（CEZAMAT），华沙理工大学）；Wroclaw University of Science and Technology（弗罗茨瓦夫科技大学）；University of Regensburg（雷根斯堡大学）；Ikerbasque, Basque Foundation for Science（伊克尔巴斯基，巴斯克科学基金会）
