We calculate the phonon, electron and magnon temperature profiles in yttrium iron garnet/platinum bilayers by diffusive theory with appropriate boundary conditions, in particular taking into account interfacial thermal resistances. Our calculations show that in thin film hybrids, the interface magnetic heat conductance qualitatively affects the magnon temperature. Based on published material parameters we assess the degree of non-equilibrium at the yttrium iron garnet/platinum interface. The magnitude of the spin Seebeck effect derived from this approach compares well with experimental results for the longitudinal spin Seebeck effect. Additionally we address the temperature profiles in the transverse spin Seebeck effect.
We theoretically investigate the spin--wave spin current induced by the spin Seebeck effect in magnonic spin tunneling junctions (MSTJs) for arbitrary magnetization directions. We show that the MSTJ functions as a \textit{tunable} spin Seebeck diode in which the tunneling spin current can be turned on and off with high efficiency by controlling the magnetization direction.
The tunnel magneto-Seebeck effect is the dependence of the thermopower of magnetic tunnel junctions on the magnetic configuration. It is conventionally interpreted in terms of a thermoelectric generalization of the tunnel magnetoresistance. Here, we investigate the heat-driven electron transport in these junctions associated with electron-magnon scattering, using stochastic Landau-Lifshitz phenomenology and quantum kinetic theory. Our findings challenge the widely accepted single-electron picture of the tunneling thermopower in magnetic junctions.
In the absence of an external magnetic field and a spin-polarized charge current, an antiferromagnetic system supports two degenerate magnon modes. An applied thermal bias activates the magnetic dynamics, leading to a magnon flow from the hot to the cold edge (magnonic spin Seebeck current). Both degenerate bands contribute to the magnon current but the orientations of the magnetic moments underlying the magnons are opposite in different bands. Therefore, while the magnon current is nonzero, the net spin current is zero.
Recent experimental evidence points to low-energy magnons as the primary contributors to the spin Seebeck effect. This spectral dependence is puzzling since it is not observed on other thermocurrents in the same material. Here, we argue that the physical origin of this behavior is the magnon-magnon scattering mediated by phonons, in a process which conserves the number of magnons. To assess the importance and features of this kind of scattering, we derive the effective magnon-phonon interaction from a microscopic model, including band energy, a screened electron-electron interaction and the el…
Our joint theoretical and computer experimental study of heat-to-spin conversion reveals that noncollinear antiferromagnetic insulators are promising materials for generating magnon spin currents upon application of a temperature gradient: they exhibit spin Seebeck and spin Nernst effects. Using Kubo theory and spin dynamics simulations, we explicitly evaluate these effects in a single kagome sheet of potassium iron jarosite, KFe$_3$(OH)$_6$(SO$_4$)$_2$, and predict a spin Seebeck conversion factor of $0.2 μ\mathrm{V}/\mathrm{K}$ at a temperature of $20 \mathrm{K}$.
We propose inducing Bose-Einstein condensation of magnons in a magnetic insulator by a heat flow oriented toward its boundary. At a critical heat flux, the oversaturated thermal gas of magnons accumulated at the boundary precipitates the condensate, which then grows gradually as the thermal bias is dialed up further. The thermal magnons thus pumped by the magnonic bulk (spin) Seebeck effect must generally overcome both the local Gilbert damping associated with the coherent magnetic dynamics as well as the radiative spin-wave losses toward the magnetic bulk, in order to achieve the threshold of…
A non-uniform temperature profile may generate a pure spin current in magnetic films, as observed for instance in the spin Seebeck effect. In addition, thermally induced elastic deformations may set in that could affect the spin current. A self-consistent theory of the magnonic spin Seebeck effect including thermally activated magneto-elastic effects is presented and analytical expressions for the thermally activated deformation tensor and dispersion relations for coupled magneto-elastic modes are obtained. We derived analytical results for bulk (3D) systems and thin magnetic (2D) films. We ob…
We report the observation of magnon spin currents generated by the Spin Seebeck effect (SSE) in a bulk single crystal of the easy-plane antiferromagnet NiO. A magnetic field induces a non-degeneracy and thereby an imbalance in the population of magnon modes with opposite spin. A temperature gradient then gives rise to a non-zero magnon spin current. This SSE is measured both in a local and a non-local geometry at 5$\,$K in bulk NiO. The magnetic field dependence of the obtained signal is modelled by magnetic field splitting of the low energy magnon modes, affecting the spin Seebeck coefficient…
Following the theoretical approach by Xiao et al [Phys. Rev. B 81, 214418 (2010)] to the spin Seebeck effect, we calculate the mean value of the total spin current flowing through a normalmetal/ ferromagnet interface. The spin current emitted from the ferromagnet to the normal metal is evaluated in the framework of the Fokker-Planck approach for the stochastic Landau-Lifshitz-Gilbert equation. We show that the total spin current depends not only on the temperature difference between the electron and the magnon baths, but also on the external magnetic field and magnetic anisotropy. Apart from t…
We develop a Boltzmann transport theory of coupled magnon-phonon transport in ferromagnetic insulators. The explicit treatment of the magnon-phonon coupling within the Boltzmann approach allows us to calculate the low-temperature magnetic-field dependence of the spin-Seebeck voltage. Within the Boltzmann theory we find that this magnetic field dependence shows similar features as found by Flebus et al. [Phys. Rev. B 95, 144420 (2017)] for a strongly coupled magnon phonon system that forms magnon-polarons, and consistent with experimental findings in yttrium iron garnet by Kikkawa et al. [Phys.…
The determination of the magnon diffusion length (MDL) is important for increasing the efficiency of spin Seebeck effect (SSE) based devices utilising non-metallic magnets. We extract the MDL at $50$ and $300\,\rm{K}$ in an $\rm{Fe}_{3}\rm{O}_{4}$ single crystal from the magnon dispersion obtained using inelastic neutron scattering (INS) and find them to be equal within error. We then measure the heat flux normalised SSE responses and in-plane magnetization of $\rm{Fe}_{3}\rm{O}_{4}$ thin films and normalise by the static magnetization contribution to the SSE before determining the MDLs from a…
The impact of the longitudinal spin Seebeck effect (LSSE) on the magnon damping in magnetic-insulator/nonmagnetic-metal bilayers was recently discussed in several reports. However, results of those experiments can be blurred by multimode excitation within the measured linewidth. In order to avoid possible intermodal interference, we investigated the damping of a single magnon group in a platinum covered Yttrium Iron Garnet (YIG) film by measurement of the threshold of its parametric excitation. Both dipolar and exchange spin-wave branches were probed. It turned out that the LSSE-related modifi…
We have studied thermally driven magnon spin transport (spin Seebeck effect, SSE) in heterostructures of antiferromagnetic $α$-$\mathrm{Cr_2O_3}$ and Pt at low temperatures. Monitoring the amplitude of the local and nonlocal SSE signals as a function of temperature, we found that both decrease with increasing temperature and disappear above 100 K and 20 K, respectively. Additionally, both SSE signals show a tendency to saturate at low temperatures. The nonlocal SSE signal decays exponentially for intermediate injector-detector separation, consistent with magnon spin current transport in the re…
We study the nonequilibrium transport for the asymmetric and negative differential magnon tunneling driven by temperature bias. We demonstrate that the many-body magnon interaction that makes the magnonic spectrum temperature-dependent is the crucial factor for the emergence of rectification and negative differential spin Seebeck effects in magnon tunneling junctions. When magnonic junctions have temperature-dependent density of states, reversing the temperature bias is able to give asymmetric spin currents and increasing temperature bias could give an anomalously decreasing magnonic spin curr…
We studied the transient behavior of the spin current generated by the longitudinal spin Seebeck effect (LSSE) in a set of platinum-coated yttrium iron garnet (YIG) films of different thicknesses. The LSSE was induced by means of pulsed microwave heating of the Pt layer and the spin currents were measured electrically using the inverse spin Hall effect in the same layer. We demonstrate that the time evolution of the LSSE is determined by the evolution of the thermal gradient triggering the flux of thermal magnons in the vicinity of the YIG/Pt interface. These magnons move ballistically within …
Based on the relaxation time approximation, the mean collision time for magnon scattering $τ_c(T)$ is computed from the experimental spin Seebeck coefficient of a bulk YIG / Pt bilayer. The scattering results to be composed by two processes: the low temperature one, with a $T^{-1/2}$ dependence, is attributed to the scattering by defects and provides a mean free path around 10 $μ$m; the high temperature one, depending on $T^{-4}$, is associated to the scattering by other magnons. The results are employed to predict the thickness dependence of the spin Seebeck coefficient for thin films.
A thermoelectric effect of the noncentrosymmetric electron-phonon coupled system is proposed, in which a temperature difference between electrons and phonons, instead of a spatial temperature gradient, induces an electric current. This is a realization of Seebeck ratchet in solids with the asymmetric energy dispersion of electrons, and the dynamical phonons act as the fluctuation of the scalar potential and induce the dc current. Possible realizations of this mechanism are also discussed.
We study the transport of thermally excited non-equilibrium magnons through the ferrimagnetic insulator YIG using two electrically isolated Pt strips as injector and detector. The diffusing magnons induce a non- local inverse spin Hall voltage in the detector corresponding to the so-called non-local spin Seebeck effect (SSE). We measure the non-local SSE as a function of temperature and strip separation. In experiments at room temperature we observe a sign change of the non-local SSE voltage at a characteristic strip separation d0, in agreement with previous investigations. At lower temperatur…
Spin Seebeck effect (SSE) holds promise for new spintronic devices with low-energy consumption. The underlying physics, essential for a further progress, is yet to be fully clarified. This study of the time resolved longitudinal SSE in the magnetic insulator yttrium iron garnet (YIG) concludes that a substantial contribution to the spin current stems from small wave-vector subthermal exchange magnons. Our finding is in line with the recent experiment by S. R. Boona and J. P. Heremans, Phys. Rev. B 90, 064421 (2014). Technically, the spin-current dynamics is treated based on the Landau-Lifshitz…
Using a simplified microscopic model of coupled spin and lattice excitations in a ferromagnetic insulator we evaluate the magnetic-field dependence of the spin Seebeck effect at low temperatures. The model includes Heisenberg exchange coupling, a harmonic lattice potential, and a pseudo-dipolar exchange interaction. Our approach goes beyond previous work [Phys. Rev. B 98, 134421 (2018)] in that it does not rely on the a priori assumption of a fast equilibration of the magnon and phonon distributions. Our theory shows that singular features in the magnetic-field dependence of the spin Seebeck e…
We study magnon hybridization in a ferrimagnetic heterostructure consisting of ultrathin gadolinium iron garnet and yttrium iron garnet layers and show the localized and extended spatial profiles of the magnon modes with different polarizations. These modes are expected to have distinct thermal excitation properties in the presence of a temperature gradient across the heterostructure. From a quantitative analysis of their consequences on longitudinal spin Seebeck effect, we predict an observable shift of the sign-changing temperature with respect to the one previously observed in gadolinium ir…
Efficient generation of spin polarization is the central focus of spintronics. In magnetic materials, spin currents can arise from heat currents by the conventional spin Seebeck effect. Recently, chiral phonons with definite handedness and angular momenta have also produced profound impacts on multiple research fields. In this paper, starting with nonequilibrium distribution of chiral phonons under temperature gradient, we find a new spin selectivity effect - chiral phonon activated spin Seebeck (CPASS) effect, in chiral materials without magnetic order nor spin-orbit coupling. With both phono…
Thermal-bias-induced spin angular momentum transfer between a paramagnetic metal and ferromagnetic insulator is studied theoretically based on the stochastic Landau-Lifshitz-Gilbert (LLG) phenomenology. Magnons in the ferromagnet establish a nonequilibrium steady state by equilibrating with phonons via bulk Gilbert damping and electrons in the paramagnet via spin pumping, according to the fluctuation-dissipation theorem. Subthermal magnons and the associated spin currents are treated classically, while the appropriate quantum crossover is imposed on high-frequency magnetic fluctuations. We ide…
The origin of the suppression of the longitudinal spin Seebeck effect by applied magnetic fields is studied. We perform numerical simulations of the stochastic Landau-Lifshitz-Gilbert equation of motion for an atomistic spin model and calculate the magnon accumulation in linear temperature gradients for different strengths of applied magnetic fields and different length scales of the temperature gradient. We observe a decrease of the magnon accumulation with increasing magnetic field and we reveal that the origin of this effect is a field dependent change of the frequency distribution of the p…
The spin diffusion length for thermally excited magnon spins is measured by utilizing a non-local spin-Seebeck effect measurement. In a bulk single crystal of yttrium iron garnet (YIG) a focused laser thermally excites magnon spins. The spins diffuse laterally and are sampled using a Pt inverse spin Hall effect detector. Thermal transport modeling and temperature dependent measurements demonstrate the absence of spurious temperature gradients beneath the Pt detector and confirm the non-local nature of the experimental geometry. Remarkably, we find that thermally excited magnon spins in YIG tra…
We investigated the effect of an external magnetic field on the diffusive spin transport by magnons in the magnetic insulator yttrium iron garnet (YIG), using a non-local magnon transport measurement geometry. We observed a decrease in magnon spin diffusion length $λ_m$ for increasing field strengths, where $λ_m$ is reduced from 9.6$\pm1.2$ $μ$m at 10 mT to 4.2$\pm0.6$ $μ$m at 3.5 T at room temperature. In addition, we find that there must be at least one additional transport parameter that depends on the external magnetic field. Our results do not allow us to unambiguously determine whether t…
The nonlocal transport of thermally generated magnons not only unveils the underlying mechanism of the spin Seebeck effect, but also allows for the extraction of the magnon relaxation length ($λ_m$) in a magnetic material, the average distance over which thermal magnons can propagate. In this study, we experimentally explore in yttrium iron garnet (YIG)/platinum systems much further ranges compared with previous investigations. We observe that the nonlocal SSE signals at long distances ($d$) clearly deviate from a typical exponential decay. Instead, they can be dominated by the nonlocal genera…
We theoretically investigate the fluctuation of a pure spin current induced by the spin Seebeck effect and spin pumping in a normal metal (NM)/ferromagnet (FM) bilayer system. Starting with a simple FI--NM interface model with both spin-conserving and spin-non-conserving processes, we derive general expressions of the spin current and the spin-current noise at the interface within second-order perturbation of the FI--NM coupling strength, and estimate them for an yttrium iron garnet (YIG) --platinum interface. We show that the spin-current noise can be used to determine the effective spin carr…
We studied the nonlocal transport behavior of both electrically and thermally excited magnons in yttrium iron garnet (YIG) as a function of its thickness. For electrically injected magnons, the nonlocal signals decrease monotonically as the YIG thickness increases. For the nonlocal behavior of the thermally generated magnons, or the nonlocal spin Seebeck effect (SSE), we observed a sign reversal which occurs at a certain heater-detector distance, and it is influenced by both the opacity of the YIG/heater interface and the YIG thickness. Our nonlocal SSE results can be qualitatively explained b…
Nonlinear relaxation between spin waves (magnons) and the crystal lattice (phonons) in an insulating ferromagnet is investigated theoretically. Magnons and phonons are described by the equilibrium Bose-Einstein distributions with different temperatures. The nonlinear heat current from magnons to phonons is calculated microscopically in terms of the Cherenkov radiation of phonons by magnons. The results are discussed in comparison with the well-known theoretical results on the nonlinear electron-phonon relaxation in metals [Kaganov, Lifshitz, Tanatarov, J. Exp. Theor. Phys. 31, 232 (1956)]. The…
We theoretically investigate the energy relaxation rate of magnons and phonons near the resonance points to clarify the underlying mechanism of heat transport in ferromagnetic materials. We find that the simple two-temperature model is valid for the one-phonon/one-magnon process, as the rate of energy exchange between magnons and phonons is proportional to the temperature difference between them, and it is independent of temperature in the high temperature limit. We found that the magnon-phonon relaxation time due to the one-phonon/one-magnon interaction could be reduced to 1.48 $μs$ at the re…
Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect, i.e. measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1-x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi e…
We investigate both theoretically and experimentally a gigantic enhancement of the spin Seebeck effect in a prototypical magnet LaY$_2$Fe$_5$O$_{12}$ at low temperatures. Our theoretical analysis sheds light on the important role of phonons; the spin Seebeck effect is enormously enhanced by nonequilibrium phonons that drag the low-lying spin excitations. We further argue that this scenario gives a clue to understand the observation of the spin Seebeck effect that is unaccompanied by a global spin current, and predict that the substrate condition affects the observed signal.
The magnonic spin Seebeck effect is a key element of spin caloritronic, a field that exploits thermal effects for spintronic applications. Early studies were focused on investigating the steady-state nonequilibrium magnonic spin Seebeck current, and the underlying physics of the magnonic spin Seebeck effect is now relatively well established. However, the initial steps of the formation of the spin Seebeck current are in the scope of recent interest. To address this dynamical aspect theoretically we propose here a new approach to the time-resolved spin Seebeck effect. Our method exploits the su…
D-Wave Phonon Angular Momentum Texture in Altermagnets by Magnon-Phonon Hybridization
Institute of Physics, Martin Luther University Halle-Wittenberg and Halle-Berlin-Regensburg Cluster of Excellence “Center for Chiral Electronics”（马丁·路德哈雷-维滕贝格大学物理研究所）；Institute of Physics, Otto von Guericke University Magdeburg（奥托·冯·格里克马格德堡大学物理研究所）；Institute of Solid State Theory, University of Münster（明斯特大学固体理论研究所）；Institute of Physics, Johannes Gutenberg University Mainz（约翰内斯·古腾堡美因茨大学物理研究所）
Bilayer Heisenberg ferromagnetic insulators hold degenerate terahertz Dirac magnon modes associated with two opposite valleys of the hexagonal Brillouin zone. We show that this energy degeneracy can be removed by breaking of the inversion symmetry (I), leading to a topological magnon valley current. We show furthermore that this current leads to valley Seebeck effect for magnons and is thereby detectable. We perform calculations in the specific example of bilayer CrBr3, where I can be broken by electrostatic doping.
We report time-resolved magneto-optic Kerr effect measurements of the longitudinal spin Seebeck effect driven by an interfacial temperature difference between itinerant electrons and magnons. The measured time-evolution of spin accumulation induced by laser-excitation indicates transfer of angular momentum across Au/Y$_3$Fe$_5$O$_{12}$ and Cu/Y$_3$Fe$_5$O$_{12}$ interfaces on a picosecond time-scale. The product of spin-mixing conductance and interfacial spin Seebeck coefficient determined is of the order of $10^8$ A m$^{-2}$ K$^{-1}$.
We study transport phenomena cross-correlated among the heat and electric currents of magnons and Dirac electrons on the surface of ferromagnetic topological insulators. For a perpendicular magnetization, we calculate magnon- (electron-) drag anomalous Nernst/Seebeck (anomalous Ettingshausen/Peltier) effects and magnon-/electron-drag thermal Hall effects. The magnon-drag thermoelectric effects are interpreted to be caused by magnon-induced electromotive force. When the magnetization has in-plane components, there arise thermal/thermoelectric analogs of anisotropic magnetoresistance (AMR). In t…
Tripartite Phonon-Magnon-Plasmon Coupling, Parametric Amplification, and Formation of a Phonon-Magnon-Plasmon Polariton in a Two-Dimensional Periodic Array of Magnetostrictive/Plasmonic Bilayered Nanodots
The plethora of recent discoveries in the field of topological electronic insulators has inspired a search for boson systems with similar properties. There are predictions that ferromagnets on a two-dimensional honeycomb lattice may host chiral edge magnons. In such systems, we theoretically study how magnons and phonons couple. We find topological magneto-polarons around the avoided crossings between phonons and topological magnons. Exploiting this feature along with our finding of Rayleigh edge phonons in armchair ribbons, we demonstrate the existence of chiral edge modes with a phononic cha…
While recent experiments on the spin Seebeck effect have revealed the decisive role of the magnon contribution to the heat current $Q$ in hybrid systems containing thin ferromagnetic layers, the available acoustic mismatch theory does not account for their magnetic properties. Here, we analyze theoretically the heat transfer through an insulating ferromagnet (F) sandwiched between two insulators (I). Depending on the relation between the F thickness, $d$, and the mean free path of phonons generated by magnons, $l_{ls}$, we reveal two qualitatively different regimes in the nonlinear heat transp…
We theoretically study the Berry curvature of the magnon induced by the hybridization with the acoustic phonons via the spin-orbit and dipolar interactions. We first discuss the magnon-phonon hybridization via the dipolar interaction, and show that the dispersions have gapless points in momentum space, some of which form a loop. Next, when both spin-orbit and dipolar interactions are considered, we show anisotropic texture of the Berry curvature and its divergence with and without gap-closing. Realistic evaluation of the consequent anomalous velocity is given for yttrium iron garnet.
We derive thermomagnonic torque and its "$β$-type" dissipative correction from the stochastic Landau-Lifshitz-Gilbert equation. The "$β$-type" dissipative correction describes viscous coupling between magnetic dynamics and magnonic current and it stems from spin mistracking of the magnetic order. We show that thermomagnonic torque is important for describing temperature gradient induced motion of skyrmions in helical magnets while dissipative correction plays an essential role in generating transverse Magnus force. We propose to detect such skyrmionic motion by employing the transverse spin Se…
We investigate thermoelectric transport through interfaces with inelastic scatterings by developing a quantum theory, which has been extensively validated by existing theories. We find that under temperature bias, while a two-terminal conductor-insulator interface behaves only as a thermal resistor, a three-terminal conductor-insulator-conductor interface can function as an electricity generator caused by phonon-mediated electron scatterings with heat-charge current separation. Unlike conventional thermoelectrics which is a property of a bulk caused by the Seebeck effect, this thermoelectric b…
We investigate the rectification and negative differential effects of full-counting statistics of conjugate thermal spin transport in a spin Seebeck engine. The engine is made by an electron/magnon interface diode driven by a temperature bias, of which the scaled cumulant generating function is formulated in the framework of nonequilibrium Green's function. The strongly fluctuating interfacial electron density of states induced by quantum dot is responsible for these intriguing properties. This work is relevant for designing efficient spin caloritronic engine and can broaden our view in nonequ…
We propose a new mechanism for the thermal Hall effect in exchange spin-wave systems, which is induced by the magnon-phonon interaction. Using symmetry arguments, we first show that this effect is quite general, and exists whenever the mirror symmetry in the direction of the magnetization is broken. We then demonstrate our result in a collinear ferromagnet on a square lattice, with perpendicular easy-axis anisotropy and Dzyaloshinskii-Moriya interaction from mirror symmetry breaking. We show that the thermal Hall conductivity is controlled by the resonant contribution from the anti-crossing po…
