We study a mesoscopic model for the flow of amorphous solids. The model is based on the key features identified at the microscopic level, namely peri- ods of elastic deformation interspersed with localised rearrangements of parti- cles that induce long-range elastic deformation. These long-range deformations are derived following a continuum mechanics approach, in the presence of solid boundaries, and are included in full in the model. Indeed, they mediate spatial cooperativity in the flow, whereby a localised rearrangement may lead a distant region to yield. In particular, we simulate a channel flow and find manifestations of spatial cooperativity that are consistent with published experimental obser- vations for concentrated emulsions in microchannels. Two categories of effects are distinguished. On the one hand, the coupling of regions subject to different shear rates, for instance,leads to finite shear rate fluctuations in the seemingly un- sheared "plug" in the centre of the channel. On the other hand, there is convinc- ing experimental evidence of a specific rheology near rough walls. We discuss diverse possible physical origins for this effect, and we suggest that it may be associated with the bumps of particles into surface asperities as they slide along the wall.
We present a two-dimensional mesoscopic model of a yield stress material that includes the possibility of local volume fluctuations coupled to shear, in such a way that the shear strength of the material decreases as the local density decreases. The model reproduces a number of effects well known in the phenomenology of this kind of materials. Particularly, we find that: the volume of the sample increases as the deformation rate increases; shear bands are no longer oriented at 45 $^\circ$ with respect to the principal axis of the applied stress (as in the absence of volume-shear coupling); hom…
Yield stress fluids display complex dynamics, in particular when driven into the transient regime between the solid and the flowing state. Inspired by creep experiments on dense amorphous materials, we implement mesocale elasto-plastic descriptions to analyze such transient dynamics in athermal systems. Both our mean-field and space-dependent approaches consistently reproduce the typical experimental strain rate responses to different applied steps in stress. Moreover, they allow us to understand basic processes involved in the strain rate slowing down (creep) and the strain rate acceleration …
Elastic consequences of a single plastic event: towards a realistic account of structural disorder and shear wave propagation in models of flowing amorphous solids
The deformation and flow of disordered solids, such as metallic glasses and concentrated emulsions, involves swift localized rearrangements of particles that induce a long-range deformation field. To describe these heterogeneous processes, elastoplastic models handle the material as a collection of 'mesoscopic' blocks alternating between an elastic behavior and plastic relaxation, when they are too loaded. Plastic relaxation events redistribute stresses in the system in a very anisotropic way. We review not only the physical insight provided by these models into practical issues such as strain…
The microscopic structure of two amorphous materials with extreme nonlinear optical properties has been studied. One of these materials exhibits second harmonic generation, while another material of similar molecular structure emits brilliant white light if being irradiated with a simple IR laser diode. Structural differences were investigated using X-ray scattering and EXAFS combined with molecular RMC. Transmission electron microscopy and scanning precession electron diffraction were used to understand specific structural differences on all length scales, from mesoscopic down to mutual molec…
We use a continuous mesoscopic model to address the yielding properties of plastic composites, formed by a host material and inclusions with different elastic and/or plastic properties. We investigate the flow properties of the composed material under a uniform externally applied deviatoric stress. We show that due to the heterogeneities induced by the inclusions, a scalar modeling in terms of a single deviatoric strain of the same symmetry than the externally applied deformation gives inaccurate results. A realistic modeling must include all possible shear deformations. Implementing this mode…
