Single-photon sources that emit photons at the same energy play a key role in the emerging concepts of quantum information, such as entanglement swapping, quantum teleportation and quantum networks. They can be realized in a variety of systems, where semiconductor quantum dots, or 'artificial atoms', are arguably among the most attractive. However, unlike 'natural atoms', no two artificial atoms are alike. This peculiarity is a serious hurdle for quantum information applications that require photonic quantum states with identical energies. Here we demonstrate a single artificial atom that generates photons with an absolute energy that is locked to an optical transition in a natural atom. Furthermore, we show that our system is robust and immune to drifts and fluctuations in the environment of the emitter. Our demonstration is crucial for realization of a large number of universally-indistinguishable solid-state systems at arbitrary remote locations, where frequency-locked artificial atoms might become fundamental ingredients.
We experimentally study the phase stabilization of a semiconductor double quantum dot (DQD) single atom maser by injection locking. A voltage-biased DQD serves as an electrically tunable microwave frequency gain medium. The statistics of the maser output field demonstrate that the maser can be phase locked to an external cavity drive, with a resulting phase noise of -99 dBc/Hz at a frequency offset of 1.3 MHz. The injection locking range, and the phase of the maser output relative to the injection locking input tone are in good agreement with Adler's theory. Furthermore, the electrically tunab…
Atomic systems display a rich variety of quantum dynamics due to the different possible symmetries obeyed by the atoms. These symmetries result in selection rules that have been essential for the quantum control of atomic systems. Superconducting artificial atoms are mainly governed by parity symmetry. Its corresponding selection rule limits the types of quantum systems that can be built using electromagnetic circuits at their optimal coherence operation points ("sweet spots"). Here, we use third-order nonlinear coupling between the artificial atom and its readout resonator to drive transition…
We present experiments on the driven dynamics of a two-level superconducting artificial atom. The driving strength reaches 4.78 GHz, significantly exceeding the transition frequency of 2.288 GHz. The observed dynamics is described in terms of quasienergies and quasienergy states, in agreement with Floquet theory. In addition, we observe the role of pulse shaping in the dynamics, as determined by non-adiabatic transitions between Floquet states, and we implement subnanosecond single-qubit operations. These results pave the way to quantum control using strong driving with applications in quantum…
Rabi oscillations of a two-level atom appear as a quantum interference effect between the amplitudes associated to atomic superpositions, in analogy with the classic double-slit experiment which manifests a sinusoidal interference pattern. By extension, through direct detection of time-resolved resonance fluorescence from a quantum-dot neutral exciton driven in the Rabi regime, we experimentally demonstrate triple-slit-type quantum interference via quantum erasure in a V-type three-level artificial atom. This result is of fundamental interest in the experimental studies of the properties of V-…
We have investigated the cross Kerr phase shift of propagating microwave fields strongly coupled to an artificial atom. The artificial atom is a superconducting transmon qubit in an open transmission line. We demonstrate average phase shifts of 11 degrees per photon between two coherent microwave fields both at the single-photon level. At high control power, we observe phase shifts up to 30 degrees. Our results provide an important step towards quantum gates with propagating photons in the microwave regime.
We present experimental observation of electromagnetically induced transparency (EIT) on a single macroscopic artificial "atom" (superconducting quantum system) coupled to open 1D space of a transmission line. Unlike in a optical media with many atoms, the single atom EIT in 1D space is revealed in suppression of reflection of electromagnetic waves, rather than absorption. The observed almost 100 % modulation of the reflection and transmission of propagating microwaves demonstrates full controllability of individual artificial atoms and a possibility to manipulate the atomic states. The system…
In traditional quantum optics, where the interaction between atoms and light at optical frequencies is studied, the atoms can be approximated as point-like when compared to the wavelength of light. So far, this relation has also been true for artificial atoms made out of superconducting circuits or quantum dots, interacting with microwave radiation. However, recent and ongoing experiments using surface acoustic waves show that a single artificial atom can be coupled to a bosonic field at several points wavelengths apart. Here, we theoretically study this type of system. We find that the multip…
The NSF AI Institute for Artificial Intelligence and Fundamental Interactions（美国国家科学基金会人工智能与基本相互作用人工智能研究所）；Massachusetts Institute of Technology（麻省理工学院）；Harvard University（哈佛大学）
Moiré engineering in atomically thin van der Waals heterostructures creates artificial quantum materials with designer properties. We solve the many-body problem of interacting electrons confined to a moiré superlattice potential minimum (the moiré atom) using a 2D fermionic neural network. We show that strong Coulomb interactions in combination with the anisotropic moiré potential lead to striking ``Wigner molecule" charge density distributions observable with scanning tunneling microscopy.
Circuit quantum electrodynamics systems are typically built from resonators and two-level artificial atoms, but the use of multi-level artificial atoms instead can enable promising applications in quantum technology. Here we present an implementation of a Josephson junction circuit dedicated to operate as a V-shape artificial atom. Based on a concept of two internal degrees of freedom, the device consists of two transmon qubits coupled by an inductance. The Josephson nonlinearity introduces a strong diagonal coupling between the two degrees of freedom that finds applications in quantum non-dem…
An atom in open space can be detected by means of resonant absorption and reemission of electromagnetic waves, known as resonance fluorescence, which is a fundamental phenomenon of quantum optics. We report on the observation of scattering of propagating waves by a single artificial atom. The behavior of the artificial atom, a superconducting macroscopic two-level system, is in a quantitative agreement with the predictions of quantum optics for a pointlike scatterer interacting with the electromagnetic field in one-dimensional open space. The strong atom-field interaction as revealed in a high…
We show conduction bands of artificial gauge field assisted atom flow in triangle optical lattice. The conduction bands are result from periodicity boundary condition of artificial magnetic flux induced phases of atoms. The positions of conduction bands depend on geometry of the atom trajectory. We consider a cell of the triangle optical lattice which is a opened system connected to its environment of Fermion atom clouds. The chemical potentials of the atom clouds are the same and the atom flow is absolutely created by a clock laser induced spin-orbit coupling. Our results are important for th…
A single superconducting artificial atom provides a unique basis for coupling electromagnetic fields and photons hardly achieved with a natural atom. Bringing a pair of harmonic oscillators into resonance with transitions of the three-level atom converts atomic spontaneous processes into correlated emission dynamics. We demonstrate two-mode correlated emission lasing on harmonic oscillators coupled via the fully controllable three-level artificial atom. Correlation of two different color emissions reveals itself as equally narrowed linewiths and quench of their mutual phase-diffusion. The mutu…
We address the recent advances on microwave quantum optics with artificial atoms. This field relies on the fact that the coupling between a superconducting artificial atom and propagating microwave photons in a 1D open transmission line can be made strong enough to observe quantum coherent effects, without using any cavity to confine the microwave photons. We investigate the scattering properties in such a system with resonant coherent microwaves. We observe the strong nonlinearity of the artificial atom and under strong driving we observe the Mollow triplet. By applying two resonant tones, we…
In this work, robustness of controlled density of optical states in doubly driven artificial atoms is studied under phonon dissipation. By using both perturbative and polaron approaches, we investigate the influence of carrier-phonon interactions on the emission properties of a two-level solid-state emitter, simultaneously coupled to two intense distinguishable lasers. Phonon decoherence effects on the emission spectra are found modest up to neon boiling temperatures ($\sim 30$ K), as compared with photon generation at the Fourier transform limit obtained in absence of lattice vibrations (zero…
We investigate photovoltaic effect of atomtronics induced by artificial gauge field in four optical potentials. Effective magnetic flux gives rise to polarization of atom occupation probability which creates current of atomtronics. The relation between atomic current and magnetic flux behaves like the current-phase property in Josephson junction. The photovoltaic cell is well defined by the atomic opened system which have effective voltage and two different poles that correspond to two internal states of atomtronics. The atom flow is controllable by changing the direction of incident light and…
The electronic properties of nanoscale quantum dots are reviewed. The similarities and differences between these `artificial atoms' and real atoms are discussed and, in particular, the effect of electron correlations is examined. It is shown that for (semiconductor) quantum dots, with only a few electrons, electron correlations can give rise to important new physics which is absent in their true atomic counterparts.
We study dynamics of an artificial two-level atom in an open 1D space by measuring evolution of its coherent and incoherent emission. States of the atom -- a superconducting flux qubit coupled to a transmission line -- are fully controlled by resonant excitation microwave pulses. The coherent emission -- a direct measure of superposition in the atom -- exhibits decaying oscillations shifted by $π/2$ from oscillations of the incoherent emission, which, in turn, is proportional to the atomic population. The emission dynamics provides information about states and properties of the atom. By measur…
The spectra of quantum dots of different geometry (``quantum ring'', ``quantum cylinder'', ``spherical square-well'' and ``parabolic confinement'') are studied. The stochastic variational method on correlated Gaussian basis functions and a large scale shell-model approach have been used to investigate these ``artificial'' atoms and their properties in magnetic field. Accurate numerical results are presented for $N$=2-8 electron systems.
Efficient detection of magnetic fields is central to many areas of research and has important practical applications ranging from materials science to geomagnetism. High sensitivity detectors are commonly built using direct current-superconducting quantum interference devices (DC-SQUIDs) or atomic systems. Here we use a single artificial atom to implement an ultrahigh sensitivity magnetometer with a size in the micron range. The artificial atom is a superconducting two-level system at low temperatures, operated in a way similar to atomic magnetometry. The high sensitivity results from quantum …
Virtual photons can mediate interaction between atoms, resulting in an energy shift known as a collective Lamb shift. Observing the collective Lamb shift is challenging, since it can be obscured by radiative decay and direct atom-atom interactions. Here, we place two superconducting qubits in a transmission line terminated by a mirror, which suppresses decay. We measure a collective Lamb shift reaching 0.8% of the qubit transition frequency and exceeding the transition linewidth. We also show that the qubits can interact via the transmission line even if one of them does not decay into it.
We propose a feasible experimental test of a 1-D version of the Fermi problem using superconducting qubits. We give an explicit non-perturbative proof of strict causality in this model, showing that the probability of excitation of a two-level artificial atom with a dipolar coupling to a quantum field is completely independent of the other qubit until signals from it may arrive. We explain why this is in perfect agreement with the existence of nonlocal correlations and previous results which were used to claim apparent causality problems for Fermi's two-atom system.
We show that the physics underlying the dynamical Casimir effect may generate multipartite quantum correlations. To achieve it, we propose a circuit quantum electrodynamics (cQED) scenario involving superconducting quantum interference devices (SQUIDs), cavities, and superconducting qubits, also called artificial atoms. Our results predict the generation of highly entangled states for two and three superconducting qubits in different geometric configurations with realistic parameters. This proposal paves the way for a scalable method of multipartite entanglement generation in cavity networks t…
We propose an approach for cooling both an artificial atom (e.g., a flux qubit) and its neighboring quantum system, the latter modeled by either a quantum two-level system or a quantum resonator. The flux qubit is cooled by manipulating its states, following an inverse process of state population inversion, and then the qubit is switched on to resonantly interact with the neighboring quantum system. By repeating these steps, the two subsystems can be simultaneously cooled. Our results show that this cooling is robust and effective, irrespective of the chosen quantum systems connected to the qu…
The requirements of quantum computations impose high demands on the level of qubit protection from perturbations; in particular, from those produced by the environment. Here we propose a superconducting flux qubit design that is naturally protected from ambient noise. This decoupling is due to the qubit interacting with the electromagnetic field only through its toroidal moment, which provides an unusual qubit-field interaction.
The strength of radiative transitions in atoms is governed by selection rules. Spectroscopic studies of allowed transitions in hydrogen and helium provided crucial evidence for the Bohr's model of an atom. Forbidden transitions, which are actually allowed by higher-order processes or other mechanisms, indicate how well the quantum numbers describe the system. We apply these tests to the quantum states in semiconductor quantum dots (QDs), which are regarded as artificial atoms. Electrons in a QD occupy quantized states in the same manner as electrons in real atoms. However, unlike real atoms, t…
We study strongly correlated states in triangular artificial atoms. Symmetry-driven orbital degeneracy of the single particle states can give rise to an SU(4) Kondo state with entangled orbital and spin degrees of freedom, and a characteristic phase shift $δ= π/4$. Upon application of a Zeeman field, a purely orbital Kondo state is formed with somewhat smaller Kondo temperature and a fully polarized current through the device. The Kondo temperatures are in the measurable range. The triangular atom also provides a tool to systematically study the singlet-triplet transitions observed in recent e…
Using a realistic quantum master equation we show that the resonance fluorescence spectra of a two-level artificial atom (quantum dot) can be tuned by adjusting its photonic local density of states via biasing of one or more graphene monolayers. The structured photon reservoir is included using a photon Green function theory which fully accounts for the loss and dispersion. The field-driven Mollow triplet spectrum can be actively controlled by the graphene bias in the THz frequency regime. We also consider the effect of a dielectric support environment, and multiple graphene layers, on the emi…
The phonon-induced dephasing dynamics in optically excited semiconductor quantum dots is studied within the frameworks of the independent Boson model and optimal control. We show that appropriate tailoring of laser pulses allows a complete control of the optical excitation despite the phonon dephasing, a finding in marked contrast to other environment couplings.
We study the formation of molecular states in a two-electron quantum dot as a function of the barrier potential dividing the dot. The increasing barrier potential drives the two electron system from an artificial helium atom to an artificial hydrogen molecule. To study this strongly coupled regime, we introduce variational wavefunctions which describe accurately two electrons in a single dot, and then study their mixing induced by the barrier. The evolution of the singlet-triplet gap with the barrier potential and with an external magnetic field is analyzed.
We present a new model to realize artificial 2D lattices with cold atoms investigating the atomic artificial graphene: a 2D-confined matter wave is scattered by atoms of a second species trapped around the nodes of a honeycomb optical lattice. The system allows an exact determination of the Green function, hence of the transport properties. The inter-species interaction can be tuned via the interplay between scattering length and confinements. Band structure and density of states of a periodic lattice are derived for different values of the interaction strength. Emergence and features of Dirac…
We study a superconducting artificial atom which is represented by a single Josephson junction or a Josephson junction chain, capacitively coupled to a coherently driven transmission line, and which contains exactly one residual quasiparticle (or up to one quasiparticle per island in a chain). We study the dissipation in the atom induced by the quasiparticle tunneling, taking into account the quasiparticle heating by the drive. We calculate the transmission coefficient in the transmission line for drive frequencies near resonance and show that, when the artificial atom spectrum is nearly harmo…
Spin-dependent electrical injection has found useful applications in storage devices, but fully operational spin-dependent semiconductor electronics remain a challenging task because of weak spin-orbit couplings and/or strong spin relaxations. These limitations are lifted considering atoms instead of electrons or holes as spin carriers. In this emerging field of atomtronics, we demonstrate the equivalent of a Datta-Das transistor using a degenerate Fermi gas of strontium atoms as spin carriers in interaction with a tripod laser-beams scheme. We explore the dependence of spin rotation, and we i…
We determine the contributions from the direct Coulomb and exchange interactions to the total interaction in semiconductor artificial atoms. We tune the relative strengths of the two interactions and measure them as a function of the number of confined electrons. We find that electrons tend to have parallel spins when they occupy nearly degenerate single-particle states. We use a magnetic field to adjust the single-particle state degeneracy, and find that the spin-configurations in an arbitrary magnetic field are well explained in terms of two-electron singlet and triplet states.
We present linear ensembles of dangling bond chains on a hydrogen terminated Si(100) surface, patterned in the closest spaced arrangement allowed by the surface lattice. Local density of states maps over a range of voltages extending spatially over the close-coupled entities reveal a rich energetic and spatial variation of electronic states. These artificial molecules exhibit collective electronic states resulting from covalent interaction of the constituent atoms. A pronounced electrostatic perturbation of dangling bond chain structure is induced by close placement of a negatively dangling bo…
We report two-photon resonance fluorescence of an individual semiconductor artificial atom. By non-linearly driving a single quantum dot via a two-photon transition, we probe the linewidth of the two-photon processes and show that, similar to their single-photon counterparts, they are close to being Fourier limited at low temperatures. The evolution of the population of excitonic states with the Rabi frequency exhibits a clear s-shaped behavior, indicative of the non-linear response via the two-photon excitation process. We model the non-linear response using a 4-level atomic system representi…
Low-dimensional electron systems fabricated from quantum matter have in recent years become available and are being explored with great intensity. This article gives an overview of the fundamental properties of such systems and summarizes the state of the field. We furthermore present and consider the concept of artificial atoms fabricated from quantum materials, anticipating remarkable scientific advances and possibly important applications of this new field of research. The surprising properties of these artificial atoms and of molecules or even of solids assembled from them are presented an…
We consider two-dimensional (2D) "artificial atoms" confined by an axially symmetric potential $V(ρ)$. Such configurations arise in circular quantum dots and other systems effectively restricted to a 2D layer. Using the semiclassical method, we present the first fully self-consistent and analytic solution yielding equations describing the density distribution, energy, and other quantities for any form of $V(ρ)$ and an arbitrary number of confined particles. An essential and nontrivial aspect of the problem is that the 2D density of states must be properly combined with 3D electrostatics. The s…
A nonequilibrium Green's functions (NEGF) approach for spatially inhomogeneous, strongly correlated artificial atoms is presented and applied to compute the time-dependent properties while starting from a (correlated) initial few-electron state at finite temperatures. In the regime of moderate to strong coupling, we consider the Kohn mode of a three-electron system in a parabolic confinement excited by a short pulsed classical laser field treated in dipole approximation. In particular, we numerically confirm that this mode is preserved within a conserving (e.g. Hartree-Fock or second Born) the…
The interaction of electrons with a periodic potential of atoms in crystalline solids gives rise to band structure. The band structure of existing materials can be measured by photoemission spectroscopy and accurately understood in terms of the tight-binding model, however not many experimental approaches exist that allow to tailor artificial crystal lattices using a bottom-up approach. The ability to engineer and study atomically crafted designer materials by scanning tunnelling microscopy and spectroscopy (STM/STS) helps to understand the emergence of material properties. Here, we use atom m…
We consider the spin and pseudospin (charge) response functions of the exactly soluble Anderson atom model. We demonstrate, in particular, that a deviation from the magnetic Curie-law behaviour, appropriate for a free spin one-half, increases with increasing asymmetry and temperature. In general, oscillator strength is transferred from the spin degrees of freedom to the pseudospin modes. We also consider the negative-U Anderson atom and demonstrate that the pseudospin modes are the relevant low-energy excitations in this case. Especially, the roles of the spin and charge excitations are interc…
Quantum information can be stored in micromechanical resonators, encoded as quanta of vibration known as phonons. The vibrational motion is then restricted to the stationary eigenmodes of the resonator, which thus serves as local storage for phonons. In contrast, we couple propagating phonons to an artificial atom in the quantum regime, and reproduce findings from quantum optics with sound taking over the role of light. Our results highlight the similarities between phonons and photons, but also point to new opportunities arising from the unique features of quantum mechanical sound. The low pr…
Using a master-equation approach for the description of coherent and incoherent dynamics in `artificial atoms and molecules', we present a theoretical analysis of situations where intense laser fields lead to pronounced renormalizations of carrier states. Such enhanced light-matter interactions allow for the solid-state implementation of effects hitherto only observable in atomic systems. Two prototypical examples will be presented: first, we show how two intense laser pulses can be exploited for a robust and high-fidelity population transfer of carrier states in coupled quantum dots; second, …
Chen, Apalkov, and Chakraborty (Phys. Rev. Lett. 98, 186803 (2007)) have computed Fock-Darwin levels of a graphene dot by including only basis states with energies larger than or equal to zero. We show that their results violate the Hellman-Feynman theorem. A correct treatment must include both positive and negative energy basis states. Additional basis states lead to new energy levels in the optical spectrum and anticrossings between optical transition lines.
Many-particle electron states in semiconductor quantum dots with carrier-mediated ferromagnetism are studied theoretically within the self-consistent Boltzmann equation formalism. Depending on the conditions, a quantum dot may contain there phases: partially spin-polarized ferromagnetic, fully spin-polarized ferromagnetic, and paramagnetic phases. The physical properties of many-body ferromagnetic confined systems come from the competing carrier-mediated ferromagnetic and Coulomb interactions. The magnetic phases in gated quantum dots with holes can be controlled by the voltage or via optical …
Current imaging scanning tunneling microscopy is used to observe the electronic wavefunctions in InAs/ZnSe core/shell nanocrystals. Images taken at a bias corresponding to the s conduction band state show that it is localized in the central core region, while images at higher bias probing the p state reveal that it extends to the shell. This is supported by optical and tunneling spectroscopy data demonstrating that the s-p gap closes upon shell growth. Shapes of the current images resemble atom-like envelope wavefunctions of the quantum dot calculated within a particle in a box model.
Achieving control over the electron spin in quantum dots (artificial atoms) or real atoms promises access to new technologies in conventional and in quantum information processing. Here we review our proposal for quantum computing with spins of electrons confined to quantum dots. We discuss the basic requirements for implementing spin-qubits, and describe a complete set of quantum gates for single- and two-qubit operations. We show how a quantum dot attached to leads can be used for spin filtering and spin read-out, and as a spin-memory device. Finally, we focus on the experimental characteriz…
We develop the stub model for the Dirac Quantum Dot, an electron confining device on a grapheme surface. Analytical results for the average conductance and the correlation functions are obtained and found in agreement with those found previously using semiclassical calculation. Comparison with available data are presented. The results reported here demonstrate the applicability of Random Matrix Theory in the case of Dirac electrons confined in a stadium.
