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arXiv 1211.7233nlin.CDcond-mat.stat-mechphysics.flu-dyn
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稀释反应-平流系统中湮灭过程$A + A \to \varnothing$的有效速率

Effective rates in dilute reaction-advection systems for the annihilation process $A + A \to \varnothing$

Giorgio Krstulovic, Massimo Cencini, Jeremie Bec

摘要:

考虑了由流体流动输送的反应颗粒的稀体系。当粒子在有限的相互作用半径内时,它们以给定的速率作为$A + A \to \varnothing$反应。该系统中描述的联合n点的数量的空间密度,它是服从一个层次的传输方程。通过使用拉格朗日方法,其中沿非反应轨迹执行统计平均,在稀或长时间限制中获得解析解。在这个限制,它表明,粒子数的时刻有一个指数衰减,而不是代数预测的标准平均场方法。有效的反应速率,然后相关的拉格朗日对统计的大偏差原则。引入一个唯象模型来研究有效速率作为相互作用长度、动力学的混沌程度和载流子流的可压缩性的函数的定性行为。精确的计算,通过费曼-卡茨的方法,在一个光滑的,可压缩的,随机增量相关的时间高斯速度场支持所提出的启发式方法。

英文摘要:

A dilute system of reacting particles transported by fluid flows is considered. The particles react as $A + A \to \varnothing$ with a given rate when they are within a finite radius of interaction. The system is described in terms of the joint n-point number spatial density that it is shown to obey a hierarchy of transport equations. An analytic solution is obtained in either the dilute or the long-time limit by using a Lagrangian approach where statistical averages are performed along non- reacting trajectories. In this limit, it is shown that the moments of the number of particles have an exponential decay rather than the algebraic prediction of standard mean-field approaches. The effective reaction rate is then related to Lagrangian pair statistics by a large-deviation principle. A phenomenological model is introduced to study the qualitative behavior of the effective rate as a function of the interaction length, the degree of chaoticity of the dynamics and the compressibility of the carrier flow. Exact computations, obtained via a Feynman-Kac approach, in a smooth, compressible, random delta-correlated-in-time Gaussian velocity field support the proposed heuristic approach.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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