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arXiv 1206.4464cond-mat.mes-hall
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分子量子点非平衡电荷输运的双稳态特征

Bistability signatures in nonequilibrium charge transport through molecular quantum dots

Klaus Ferdinand Albrecht, Haobin Wang, Lothar Muehlbacher, Michael Thoss, Andreas Komnik

摘要:

研究了在有限电压作用下,与内部振动自由度强耦合的分子结的瞬态非平衡动力学。使用两种不同的,数值精确的技术,图解Monte Carlo和多层多组态时间依赖性Hartree方法,我们表明,通过结的稳态电流可能依赖于敏感的系统的初始准备,从而揭示了签名的双稳态。分析了偏置电压和瞬态动力学对双稳态现象的影响。此外,在nanoelectromecanical器件中的随机开关现象的可能关系进行了讨论。

英文摘要:

We investigate the transient nonequilibrium dynamics of a molecular junction biased by a finite voltage and strongly coupled to internal vibrational degrees of freedom. Using two different, numerical exact techniques, diagrammatic Monte Carlo and the multilayer multiconfiguration time-dependent Hartree method, we show that the steady state current through the junction may depend sensitively on the initial preparation of the system, thus revealing signatures of bistability. The influence of the bias voltage and the transient dynamics on the phenomenon of bistability is analyzed. Furthermore, a possible relation to the phenomenon of stochastic switching in nanoelectromecanical devices is discussed.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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