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arXiv 1206.4392cond-mat.str-el
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磁亚晶格稀释对CeNiGe3和UNiSi2中磁序的影响

The influence of magnetic sublattice dilution on magnetic order in CeNiGe3 and UNiSi2

Adam P. Pikul

摘要:

用X射线粉末衍射、宽温区磁化强度和比热测量等方法研究了Y稀释反铁磁体CeNiGe_3(T_N = 5.5K)和Th稀释反铁磁体UNiSi_2(T_C = 95 K)的多晶样品。Ce_(1-x)Y_xNiGe_3合金的晶格常数随Y含量的增加而线性减小,而U_(1-x)Th_xNiSi_2合金的晶胞体积随Th含量的增加而线性增大。系统的有序化温度随x的增加单调下降,在Ce0.4Y0.6NiGe3和U0.3Th0.7NiSi2中分别为1.2 K和26 K,在它们的磁相图上形成了一个长程磁有序的圆顶。磁有序的抑制与合金化引起的晶体无序引起的T_N,C处的异常明显展宽有关。在Ce基合金和U基合金的磁逾渗阈值xc分别为0.68和0.75以下,长程磁序平滑地演变成短程磁序,在磁相图上形成尾部。所观察到的行为Ce_(1-x)Y_xNiGe_3和U_(1-x)Th_xNiSi_2是稀磁合金的特征。(c)2012 IOP出版有限公司

英文摘要:

Polycrystalline samples of the Y-diluted antiferromagnet CeNiGe3 (T_N = 5.5 K) and Th-diluted ferromagnet UNiSi2 (T_C = 95 K) were studied by means of x-ray powder diffraction, magnetization and specific heat measurements performed in a wide temperature range. The lattice parameters of the Ce1-xYxNiGe3 alloys decrease linearly with increasing the Y content, while the unit cell volume of U1-xThxNiSi2 increases linearly with rising the Th content. The ordering temperatures of the systems decrease monotonically with increasing x down to about 1.2 K in Ce0.4Y0.6NiGe3 and 26 K in U0.3Th0.7NiSi2, forming a dome of a long-range magnetic order on their magnetic phase diagrams. The suppression of the magnetic order is associated with distinct broadening of the anomalies at T_N,C due to crystallographic disorder being a consequence of the alloying. Below the magnetic percolation threshold xc of about 0.68 and 0.75 in the Ce- and U-based alloys, respectively, the long-range magnetic order smoothly evolves into a short-range one, forming a tail on the magnetic phase diagrams. The observed behaviour Ce1-xYxNiGe3 and U1-xThxNiSi2 is characteristic of diluted magnetic alloys. (c) 2012 IOP Publishing Ltd.

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