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arXiv 1202.4492cond-mat.str-elcond-mat.mtrl-scicond-mat.supr-con
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超导Ba(Fe $_{1-x}$ Ir $_x$)$_2$ As $_2$中Ir掺杂原子的磁极化

Magnetically polarized Ir dopant atoms in superconducting Ba(Fe$_{1-x}$Ir$_x$)$_2$As$_2$

M. P. M. Dean, M. G. Kim, A. Kreyssig, J. W. Kim, X. Liu, P. J. Ryan, A. Thaler, S. L. Bud'ko, W. Strassheim, P. C. Canfield, J. P. Hill, A. I. Goldman

摘要:

利用Ir $L_3$边缘X射线共振磁散射(XRMS)研究了磷属元素超导体Ba(Fe $_{1-x}$ Ir $_x$)$_2$ As $_2$ with $x=0.027(2)$中Ir $5d$掺杂态的磁极化.尽管掺杂部分抑制反铁磁过渡的事实,我们发现,磁秩序的生存周围的Ir掺杂剂的网站。的Ir状态的磁极化与相称的条纹状反铁磁秩序和长的相关长度,$ξ_{\text{mag}}>$ 2800和$>$ 850,在$ab$平面和沿c轴,分别由它们的相互作用与Fe自旋。这种Ir磁序一直持续到大多数Fe自旋在$T_N=74(2)$ K下的Néel跃迁。在5 K时,我们发现Ba(Fe $_{1-x}$ Ir $_x$)$_2$ As $_2$中微观上的磁有序与超导电性共存。通过Ir $L_3$边缘的XRMS的能量依赖性示出了非洛伦兹线形,我们解释在Ir共振散射和Fe非共振磁散射之间的干涉。

英文摘要:

We investigate the magnetic polarization of the Ir $5d$ dopant states in the pnictide superconductor Ba(Fe$_{1-x}$Ir$_x$)$_2$As$_2$ with $x=0.027(2)$ using Ir $L_3$ edge x-ray resonant magnetic scattering (XRMS). Despite the fact that doping partially suppresses the antiferromagnetic transition, we find that magnetic order survives around the Ir dopant sites. The Ir states are magnetically polarized with commensurate stripe-like antiferromagnetic order and long correlations lengths, $ξ_{\text{mag}}>$ 2800 and $>$850 Å, in the $ab$-plane and along the c-axis, respectively, driven by their interaction with the Fe spins. This Ir magnetic order persists up to the Néel transition of the majority Fe spins at $T_N=74(2)$ K. At 5 K we find that magnetic order co-exists microscopically with superconductivity in Ba(Fe$_{1-x}$Ir$_x$)$_2$As$_2$. The energy dependence of the XRMS through the Ir $L_3$ edge shows a non-Lorentzian lineshape, which we explain in terms of interference between Ir resonant scattering and Fe non-resonant magnetic scattering.

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