Magnetically polarized Ir dopant atoms in superconducting Ba(Fe$_{1-x}$Ir$_x$)$_2$As$_2$
M. P. M. Dean, M. G. Kim, A. Kreyssig, J. W. Kim, X. Liu, P. J. Ryan, A. Thaler, S. L. Bud'ko, W. Strassheim, P. C. Canfield, J. P. Hill, A. I. Goldman
利用Ir $L_3$边缘X射线共振磁散射(XRMS)研究了磷属元素超导体Ba(Fe $_{1-x}$ Ir $_x$)$_2$ As $_2$ with $x=0.027(2)$中Ir $5d$掺杂态的磁极化.尽管掺杂部分抑制反铁磁过渡的事实,我们发现,磁秩序的生存周围的Ir掺杂剂的网站。的Ir状态的磁极化与相称的条纹状反铁磁秩序和长的相关长度,$ξ_{\text{mag}}>$ 2800和$>$ 850,在$ab$平面和沿c轴,分别由它们的相互作用与Fe自旋。这种Ir磁序一直持续到大多数Fe自旋在$T_N=74(2)$ K下的Néel跃迁。在5 K时,我们发现Ba(Fe $_{1-x}$ Ir $_x$)$_2$ As $_2$中微观上的磁有序与超导电性共存。通过Ir $L_3$边缘的XRMS的能量依赖性示出了非洛伦兹线形,我们解释在Ir共振散射和Fe非共振磁散射之间的干涉。
英文摘要:
We investigate the magnetic polarization of the Ir $5d$ dopant states in the pnictide superconductor Ba(Fe$_{1-x}$Ir$_x$)$_2$As$_2$ with $x=0.027(2)$ using Ir $L_3$ edge x-ray resonant magnetic scattering (XRMS). Despite the fact that doping partially suppresses the antiferromagnetic transition, we find that magnetic order survives around the Ir dopant sites. The Ir states are magnetically polarized with commensurate stripe-like antiferromagnetic order and long correlations lengths, $ξ_{\text{mag}}>$ 2800 and $>$850 Å, in the $ab$-plane and along the c-axis, respectively, driven by their interaction with the Fe spins. This Ir magnetic order persists up to the Néel transition of the majority Fe spins at $T_N=74(2)$ K. At 5 K we find that magnetic order co-exists microscopically with superconductivity in Ba(Fe$_{1-x}$Ir$_x$)$_2$As$_2$. The energy dependence of the XRMS through the Ir $L_3$ edge shows a non-Lorentzian lineshape, which we explain in terms of interference between Ir resonant scattering and Fe non-resonant magnetic scattering.
对Cu_(1-x)Zn_xGeO_3(0<= x <= 0.045)单晶的极化非弹性光散射实验表明,当x<>0时,在自旋Peierls跃迁以下的单重态响应能量的近一半处出现了一个新的模式。这种模式的温度,磁场,极化,和掺杂的依赖性是类似的单重束缚态。的自旋辅助光散射过程中的数据进行解释。峰的位置和形状为Cu_(1-x)Zn_xGeO_3中掺杂剂束缚的自旋子的存在提供了有力的证据。
Magnetic Brightening and Nanoscale Imaging of Spin-Polarized Helical Edge Modes
Ames National Laboratory(艾姆斯国家实验室);Department of Physics and Astronomy, Iowa State University(爱荷华州立大学物理与天文系);Condensed Matter Physics and Materials Sciences Department, Brookhaven National Laboratory(布鲁海文国家实验室凝聚态物理与材料科学系);Department of Physics and Astronomy, Stony Brook University(石溪大学物理与天文系)
Approaching the Ground State of Frustrated A-site Spinels: A Combined Magnetization and Polarized Neutron Scattering Study
我们重新研究磁阻挫,{ \it金刚石晶格反铁磁体}尖晶石FeAl $_2$ O $_4$和MnAl $_2$ O $_4$使用磁化测量和极化中子的漫散射。在FeAl $_2$ O $_4$中,宏观测量证实了在13 K附近零场冷却磁化率的“尖点”。动态磁化率和{ \it记忆效应}实验提供的结果不符合该材料中的典型自旋玻璃情形。通过极化中子散射研究,证实了FeAl $_2$ O $_4$在低至4~K的温度范围内不存在长程磁序。通过模拟粉末平均微分磁中子散射截面,我们估计,在这种化合物中的自旋-自旋相关延伸到第三个最近邻壳。Landé $g$因子的估计值指向Fe $^{2+}$的轨道贡献。这也得到了居里-外斯磁化率分析的支持。而MnAl $_2$ O $_4$在低于$\approx$ 40~K时发生磁相变,进入长程有序态,这一点得到了宏观测量和极化中子衍射的证实。然而,极化中子研究揭示了显著的自旋涨落与长程反铁磁有序共存的存在。磁扩散强度表明与FeAl $_2$ O $_4$类似的短程有序。本工作的结果支持自旋自旋相关性的重要性,在理解磁响应的挫折磁铁一样,$A$网站尖晶石具有主导的短程自旋相关性,让人想起“自旋液体”状态。
Magnetic order and excitations in the magnetically intercalated van der Waals material Cr$_{\frac{1}{4}}$NbSe$_2$
The Institute for Solid State Physics, University of Tokyo(东京大学固体离子体研究所);Department of Applied Physics, University of Tokyo(东京大学应用物理系);Institute of Materials Structure Science, High Energy Accelerator Research Organization(高能加速器研究机构物质结构科学研究所);Neutron Scattering Division, Oak Ridge National Laboratory(橡树岭国家实验室中子散射部);College of Engineering, Shibaura Institute of Technology(芝浦工业大学工程学院);Research Center for Advanced Science and Technology, University of Tokyo(东京大学先端科学技术研究中心)