含辐射衰变的多尺度非绝热动力学:稀有气体四聚体电离后碎裂的个例研究
Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers
摘要:
在这份补充材料中,为了读者的方便,我们选择了建议的多尺度模型的一般方案(第二节)。1),以及用于试点研究的方法的基本信息:相互作用模型的详细描述(第2节)。2)和用于暗动力学步骤的动力学方法(Sec. 3)在之前的两项研究中报道过[1,2]。此外,还详细描述了辐射过程的处理(第二节)。4)。
英文摘要:
In this supplementary material, we recollect, for reader's convenience, the general scheme of suggested multiscale model (Sec. 1), and basic informations about approaches used for pilot study: a detailed description of the interaction model (Sec. 2) and dynamical methods used for the dark dynamics step (Sec. 3) reported previously in two preceding studies [1, 2]. In addition, a detailed description of the treatment of radiative processes is also given (Sec. 4).
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