We have experimentally studied the magnetic-field dependence of the decay of a Bose-Einstein condensate of metastable 4He atoms confined in an optical dipole trap, for atoms in the m=+1 and m=-1 magnetic substates, and up to 450 G. Our measurements confirm long-standing calculations of the two-body loss rate coefficient that show an increase above 50 G. We demonstrate that for m=-1 atoms, decay is due to three-body recombination only, with a three-body loss rate coefficient of 6.5(0.4)(0.6)10^(-27)cm^6s^(-1), which is interesting in the context of universal few-body theory. We have also searched for a recently-predicted d-wave Feshbach resonance, but did not observe it.
We have investigated the ultracold interspecies scattering properties of metastable triplet He and Rb. We performed state-of-the-art ab initio calculations of the relevant interaction potential, and measured the interspecies elastic cross section for an ultracold mixture of metastable triplet $^4$He and $^{87}$Rb in a quadrupole magnetic trap at a temperature of 0.5 mK. Our combined theoretical and experimental study gives an interspecies scattering length $a_{4+87}=+17^{+1}_{-4}$ $a_0$, which prior to this work was unknown. More general, our work shows the possibility of obtaining accurate sc…
In an ultracold, optically trapped mixture of $^{87}$Rb and metastable triplet $^4$He atoms we have studied trap loss for different spin-state combinations, for which interspecies Penning ionization is the main two-body loss process. We observe long trapping lifetimes for the purely quartet spin-state combination, indicating strong suppression of Penning ionization loss by at least two orders of magnitude. For the other spin-mixtures we observe short lifetimes that depend linearly on the doublet character of the entrance channel. We compare the extracted loss rate coefficient with recent predi…
We have obtained accurate ab initio quartet potentials for the diatomic metastable triplet helium + alkali-metal (Li, Na, K, Rb) systems, using all-electron restricted open-shell coupled cluster singles and doubles with noniterative triples corrections [CCSD(T)] calculations and accurate calculations of the long-range $C_6$ coefficients. These potentials provide accurate ab initio quartet scattering lengths, which for these many-electron systems is possible, because of the small reduced masses and shallow potentials that results in a small amount of bound states. Our results are relevant for u…
Recently we have reported (Knoop et al. [arXiv:1404.4826]) on an experimental determination of metastable triplet $^4$He+$^{87}$Rb scattering length by performing thermalization measurements for an ultracold mixture in a quadrupole magnetic trap. Here we present our experimental apparatus and elaborate on these thermalization measurements. In particular we give a theoretical description of interspecies thermalization rate for a quadrupole magnetic trap, i. e. in the presence of Majorana heating, and a general procedure to extract the scattering length from the elastic cross section at finite t…
We report on the realization of Bose-Einstein condensation of metastable helium-4. After exciting helium to its metastable state in a novel pulse-tube cryostat source, the atomic beam is collimated and slowed. We then trap several 10^8 atoms in a magneto-optical trap. For subsequent evaporative cooling, the atoms are transferred into a magnetic trap. Degeneracy is achieved with typically a few 10^6 atoms. For detection of atomic correlations with high resolution, an ultrafast delay-line detector has been installed. Consisting of four quadrants with independent readout electronics that allow fo…
We report on the Bose-Einstein condensation of metastable Helium-4 atoms using a hybrid approach, consisting of a magnetic quadrupole and a crossed optical dipole trap. In our setup we cross the phase transition with 2x10^6 atoms, and we obtain pure condensates of 5x10^5 atoms in the optical trap. This novel approach to cooling Helium-4 provides enhanced cycle stability, large optical access to the atoms and results in production of a condensate every 6 seconds - a factor 3 faster than the state-of-the-art. This speed-up will dramatically reduce the data acquisition time needed for the measure…
We have measured the forbidden 2 3S1 - 2 1P1 transition at 887 nm in a quantum degenerate gas of metastable He-4 atoms confined in an optical dipole trap. The determined transition frequency is 338 133 594.4 (0.5) MHz, from which we obtain an ionization energy of the 2 1P1 state of 814 709 148.6 (0.5) MHz. This ionization energy is in disagreement by > 3 sigma with the most accurate quantum electrodynamics (QED) calculations available. Our measurements also provide a new determination of the lifetime of the 2 1P1 state of 0.551 (0.004)stat (+ 0.013,- 0.000)syst ns, which is the most accurate d…
Ultracold dilute gases provide ideal settings for measurements of atomic structure. Helium has an internal structure sufficiently simple to permit highly accurate predictions of its resonances and transition rates. Precise laser spectroscopy of helium thus yields empirical constraints on such calculations. These are desirable in the ongoing investigations seeking to reconcile the disagreement between independent determinations of nuclear charge radius data in both hydrogenic and helium atoms. Either the size of these particles are truly constant and quantum electrodynamics (QED) is flawed, or …
We demonstrate a simple scheme to reach Bose-Einstein condensation (BEC) of metastable triplet helium atoms using a single beam optical dipole trap with moderate power of less than 3 W. Our scheme is based on RF-induced evaporative cooling in a quadrupole magnetic trap and transfer to a single beam optical dipole trap that is located below the magnetic trap center. We transfer 1x10^6 atoms into the optical dipole trap, with an initial temperature of 14 μK, and observe efficient forced evaporative cooling both in a hybrid trap, in which the quadrupole magnetic trap operates just below the levit…
We perform laser absorption spectroscopy with ultracold $^4$He atoms to measure the energy intervals between the $2^{3\!} P_2$ level and five levels in the n = 5 manifold. The laser light perturbs the cold atomic cloud during the production of Bose-Einstein condensates and decreases the phase space density, causing a measurable decrease in the number of atoms in the final condensate. We improve on the precision of previous measurements by at least an order of magnitude, and report the first observation of the spin-forbidden $2^{3\!}P_2 - 5^{1\!}D_2$ transition in helium. Theoretical transition…
The bound states of the fermionic ^3He(2 ^3S_1)+ ^3He(2 ^3P_j)system, where j=0,1,2, are investigated using the recently available ab initio short-range ${}^{1,3,5}Σ^{+}_{g,u}$ and ${}^{1,3,5}Π_{g,u}$ potentials computed by Deguilhem et al. (J. Phys. B: At. Mol. Opt. Phys., 2009, 42, 015102). Single-channel and multichannel calculations have been undertaken in order to investigate the effects of Coriolis and non-adiabatic couplings. The possible experimental observability of the theoretical levels is assessed using criteria based upon the short-range character of each level and their coupling …
We report the realization of a BEC of metastable helium-4 atoms (4He*) in an all optical potential. Up to 10^5 spin polarized 4He* atoms are condensed in an optical dipole trap formed from a single, focused, vertically propagating far off-resonance laser beam. The vertical trap geometry is chosen to best match the resolution characteristics of a delay-line anode micro-channel plate detector capable of registering single He* atoms. We also confirm the instability of certain spin state combinations of 4He* to two-body inelastic processes, which necessarily affects the scope of future experiments…
We report the realisation of Bose-Einstein condensation (BEC) of metastable helium atoms using an in-vacuum coil magnetic trap and a crossed beam optical dipole trap. A novel quadrupole-Ioffe configuration (QUIC) magnetic trap made from in-vacuum hollow copper tubes provides fast switching times while generating traps with a 10G bias, without compromising optical access. The bias enables in-trap 1D doppler cooling to be used, which is the only cooling stage between the magneto-optic trap (MOT) and the optical dipole trap. This allows direct transfer to the dipole trap without the need for any …
Quantum science with arrays of metastable helium-3 atoms
The University of Illinois at Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校）；HRL Laboratories（HRL实验室）；Rice University（莱斯大学）；Purdue University（普渡大学）；University of Chicago（芝加哥大学）
In several settings of physics and chemistry one has to deal with molecules interacting with some kind of an external environment, be it a gas, a solution, or a crystal surface. Understanding molecular processes in the presence of such a many-particle bath is inherently challenging, and usually requires large-scale numerical computations. Here, we present an alternative approach to the problem - that based on the notion of the angulon quasiparticle. We show that molecules rotating inside superfluid helium nanodroplets and Bose-Einstein Condensates form angulons, and therefore can be described …
We report on the measurement of the scattering properties of ultracold $^{174}$Yb bosons in a three-dimensional (3D) optical lattice. Site occupancy in an atomic Mott insulator is resolved with high-precision spectroscopy on an ultranarrow optical clock transition. Scattering lengths and loss rate coefficients for $^{174}$Yb atoms in different collisional channels involving the ground state $^1$S$_0$ and the metastable $^3$P$_0$ are derived. These studies set important constraints for future experimental studies of two-electron atoms for quantum-technological applications.
A paradigm model of modern atom optics is studied, strongly interacting ultracold bosons in an optical lattice. This many-body system can be artificially opened in a controlled manner by modern experimental techniques. We present results based on a non-hermitian effective Hamiltonian whose quantum spectrum is analyzed. The direct access to the spectrum of the metastable many-body system allows us to easily identify relatively stable quantum states, corresponding to previously predicted solitonic many-body structures.
We employ metastable ultracold $^{173}$Yb atoms to study dynamics in the 1D dissipative Fermi-Hubbard model experimentally and theoretically, and observe a complete inhibition of two-body losses after initial fast transient dynamics. We attribute the suppression of particle loss to the dynamical generation of a highly entangled Dicke state. For several lattice depths and for two- and six-spin component mixtures we find very similar dynamics, showing that the creation of strongly correlated states is a robust and universal phenomenon. This offers interesting opportunities for precision measurem…
We have analyzed our recently-measured three-body loss rate coefficient for a Bose-Einstein condensate of spin-polarized metastable triplet 4He atoms in terms of Efimov physics. The large value of the scattering length for these atoms, which provides access to the Efimov regime, arises from a nearby potential resonance. We find the loss coefficient to be consistent with the three-body parameter (3BP) found in alkali-metal experiments, where Feshbach resonances are used to tune the interaction. This provides new evidence for a universal 3BP, the first outside the group of alkali-metal elements.…
Recently it has been shown that pairs of atoms can form metastable bonds due to non-conservative forces induced by dissipation [Lemeshko&Weimer, Nature Comm. 4, 2230 (2013)]. Here we study the dynamics of interaction-induced coherent population trapping - the process responsible for the formation of dissipatively bound molecules. We derive the effective dissipative potentials induced between ultracold atoms by laser light, and study the time evolution of the scattering states. We demonstrate that binding occurs on short timescales of ~10 microseconds, even if the initial kinetic energy of the …
Magnetic Feshbach resonances have allowed great success in the production of ultracold diatomic molecules from bi-alkali mixtures, but have so far eluded observation in mixtures of alkali and alkaline-earth-like atoms. Inelastic collisional properties of ultracold atomic systems exhibit resonant behavior in the vicinity of such resonances, providing a detection signature. We study magnetic field dependent inelastic effects via atom loss spectroscopy in an ultracold heteronuclear mixture of alkali $^6$Li in the ground state and alkaline-earth-like $^{174}$Yb in an excited electronic metastable …
Helium atoms in the metastable $2^3{S_{1}}$ state (He$^*$) have unique advantages for ultracold atomic experiments. However, there is no known accessible Feshbach resonance in He$^*$, which could be used to manipulate the scattering length and hence unlock several new experimental possiblities. Previous experimental and theoretical studies for He$^*$ have produced contradictory results. We aimed to resolve this discrepancy with a theoretical search for Feshbach resonances, using a new close-coupled model of He$^*$ collisions in the presence of an external magnetic field. Several resonances wer…
Liquid helium 4 had been the only bosonic superfluid available in experiments for a long time. This situation was changed in 1995, when a new superfluid was born with the realization of the Bose-Einstein condensation in ultracold atomic gases. The liquid helium 4 is strongly interacting and has no spin; there is almost no way to change its parameters, such as interaction strength and density. The new superfluid, Bose-Einstein condensate (BEC), offers various aspects of advantages over liquid helium. On the one hand, BEC is weakly interacting and has spin degrees of freedom. On the other hand, …
The phenomenon of metastability can shape dynamical processes on all temporal and spatial scales. Here, we induce metastable dynamics by pumping ultracold bosonic atoms from the lowest band of an optical lattice to an excitation band, via a sudden quench of the unit cell. The subsequent relaxation process to the lowest band displays a sequence of stages, which include a metastable stage, during which the atom loss from the excitation band is strongly suppressed. Using classical-field simulations and analytical arguments, we provide an explanation for this experimental observation, in which we …
We report on the experimental realization of a state-dependent lattice for a two-orbital fermionic quantum gas with strong interorbital spin exchange. In our state-dependent lattice, the ground and metastable excited electronic states of $^{173}$Yb take the roles of itinerant and localized magnetic moments, respectively. Repulsive on-site interactions in conjunction with the tunnel mobility lead to spin exchange between mobile and localized particles, modeling the coupling term in the well-known Kondo Hamiltonian. In addition, we find that this exchange process can be tuned resonantly by varyi…
