Temporal growth of an optical Kerr frequency comb generated in a microresonator is studied both experimentally and numerically. We find that the comb emerges from vacuum fluctuations of the electromagnetic field on timescales significantly exceeding the ringdown time of the resonator modes. The frequency harmonics of the comb spread starting from the optically pumped mode if the microresonator is characterized with anomalous group velocity dispersion. The harmonics have different growth rates resulting from sequential four-wave mixing process that explains intrinsic modelocking of the comb.
Dissipative structures are the result of spontaneous symmetry breaking in a dynamic open system, which is induced by either the nonlinear effect or loss fluctuations. While optical temporal dissipative solitons in nonlinear Kerr cavities has been widely studied, they are operated in a red-detuned regime that is non-trivial to access. Here, we demonstrate an emergent dissipative soliton state in optical cavities in the presence of loss fluctuations, which is accessible by self-evolution of the system and is operated in resonance. We numerically investigate both the effect of loss modulation and…
Soliton microcombs based on Kerr nonlinearity in microresonators have been a prominent miniaturized coherent light source. Here, for the first time, we demonstrate the existence of Kerr solitons in an optomechanical microresonator, for which a nonlinear model is built by incorporating a single mechanical mode and multiple optical modes. Interestingly, an exotic vibrational Kerr soliton state is found, which is modulated by a self-sustained mechanical oscillation. Besides, the soliton provides extra mechanical gain through the optical spring effect, and results in phonon lasing with a red-detun…
The deep ultraviolet, the bandgap region of dielectrics, is not readily accessible for established methods of ultrafast spectroscopy. Here, a miniature beamline, where a tailored deep ultraviolet field is used immediately after the noncollinear generation without subsequent optical elements, is introduced for transient absorption and dispersion spectroscopy. The near-bandgap region of diamond in the presence of a few-femtosecond pump pulse is explored where the delayed dynamical Franz-Keldysh effect and the almost instantaneous optical Kerr effect coexist.
Optical frequency combs are crucial for both fundamental science and applications demanding wide frequency spanning and ultra-precision resolutions. Recent advancements of nonlinear Kerr effect based optical frequency combs in microcavities open up new opportunities in a compact platform, however, internal cavity-enhanced nonlinearities are still unclear. Here we demonstrate transient nonlinear dynamics during optical frequency comb formation inside a Kerr microcavity. We show that gain spiking forms due to nonlinear phase modulation, causing comb lines' self-detuning nearby a cavity resonance…
We experimentally demonstrate phase retrieval of a single-soliton Kerr comb using electric field cross-correlation implemented via dual-comb interferometry. The phase profile of the Kerr comb is acquired through the heterodyne beat between the Kerr comb and a reference electro-optical comb with a pre-characterized phase profile. The soliton Kerr comb has a nearly flat phase profile, and the pump line is observed to show a phase offset which depends on the pumping parameters. The experimental results are in agreement with numerical simulations. Our all-linear approach enables rapid measurements…
Optical injection locking is implemented to faithfully transfer the phase noise of a dissipative Kerr microresonator soliton comb in addition to the amplification of the Kerr comb. Unlike Er-doped fiber and semiconductor optical amplifiers, the optical injection locking amplifies the comb mode without degrading the optical signal-to-noise ratio. In addition, we show that the residual phase noise of the optical injection locking is sufficiently small to transfer the relative phase noise of comb modes (equivalent to the repetition frequency) of low phase noise Kerr combs, concluding that the opt…
In a uniform microresonator, the generation of a broadband Kerr frequency comb is triggered by Turing patterns. Here, we study a distinctly different route to initiate the Kerr frequency comb by Faraday ripples. Momentum conservation is ensured by azimuthal modulation of the cavity dispersion. With a good agreement with the theoretical analysis, we demonstrate a multispectral Kerr frequency comb covering telecommunication O, C, L, and 2 μm bands. Comb coherence and absence of a subcomb offset are confirmed by cw heterodyne beat note and amplitude noise spectra measurements. The device can be u…
Kerr optical frequency combs generated in a coherently driven Kerr nonlinear resonator has the potential for a wide range of applications. However, in a single cavity which is a widely adopted configuration for Kerr optical frequency combs generation, modulation instability is suppressed in normal dispersion regime and the pump-to-comb conversion efficiency is extremely low for a single dissipative Kerr soliton in anomalous dispersion regime. Dual-coupled cavities have been proposed to generate Kerr optical frequency combs in normal dispersion regime, and have potential to remarkably increase …
We show via numerical simulation that Kerr frequency combs can be generated in a nonlinear resonator characterized with normal group velocity dispersion (GVD). We find the spectral shape of the comb and temporal envelope of the corresponding optical pulses formed in the resonator.
Using numerical simulations of an extended Lugiato-Lefever equation, we analyze the stability and nonlinear dynamics of Kerr frequency combs generated in microresonators and fiber resonators taking into account third-order dispersion effects. We show that cavity solitons underlying Kerr frequency combs, normally sensitive to oscillatory and chaotic instabilities, are stabilized in a wide range of parameter space by third-order dispersion. Moreover, we demonstrate how the snaking structure organizing compound states of multiple cavity solitons is qualitatively changed by third-order dispersion,…
A generalized Lugiato-Lefever equation is numerically solved with a Newton-Raphson method to model Kerr frequency combs. We obtain excellent agreement with past experiments, even for an octave-spanning comb. Simulations are much faster than with any other technique despite including more modes than ever before. Our study reveals that Kerr combs are associated with temporal cavity solitons and dispersive waves, and opens up new avenues for the understanding of Kerr comb formation.
We investigate the effects of Raman and Kerr gain in crystalline microresonators and determine the conditions required to generate modelocked frequency combs. We show theoretically that strong, narrowband Raman gain determines a maximum microresonator size allowable to achieve comb formation. We verify this condition experimentally in diamond and silicon microresonators and show that there exists a competition between Raman and Kerr effects that leads to the existence of two different comb states.
It is demonstrated that Kerr frequency comb generation described by coupled mode equations can be numerically simulated using Fast Fourier Transform methods. This allows broadband frequency combs spanning a full octave to be efficiently simulated using standard algorithms, resulting in orders of magnitude improvements in the computation time.
Synchronization is a ubiquitous phenomenon in nature that manifests as the spectral or temporal locking of coupled nonlinear oscillators. In the field of photonics, synchronization has been implemented in various laser and oscillator systems, enabling applications including coherent beam combining and high precision pump-probe measurements. Recent experiments have also shown time-domain synchronization of Kerr frequency combs via coupling of two separate oscillators operating in the dissipative soliton [i.e., anomalous group-velocity dispersion (GVD)] regime. Here, we demonstrate all-optical s…
We use numerical simulations based on an extended Lugiato-Lefever equation (LLE) to investigate the stability properties of Kerr frequency combs generated in microresonators. In particular, we show that an ensemble average calculated over sequences of output fields separated by a fixed number of resonator roundtrips allows the coherence of Kerr combs to be quantified in terms of the complex-degree of first-order coherence. We identify different regimes of comb coherence, linked to the solutions of the LLE. Our approach provides a practical and unambiguous way of assessing the stability of Kerr…
A single closed-form analytical solution of the driven nonlinear Schrödinger equation is developed, reproducing a large class of the behaviors in Kerr-comb systems, including bright-solitons, dark-solitons, and a large class of periodic wavetrains. From this analytical framework, a Kerr-comb area theorem and a pump-detuning relation are developed, providing new insights into soliton- and wavetrain-based combs along with concrete design guidelines for both. This new area theorem reveals significant deviation from the conventional soliton area theorem, which is crucial to understanding cavity so…
We demonstrate an approach for automated Kerr comb generation in the normal group-velocity dispersion (GVD) regime. Using a coupled-ring geometry in silicon nitride, we precisely control the wavelength location and splitting strength of avoided mode crossings to generate low-noise frequency combs with pump-to-comb conversion efficiencies of up to 41%, which is the highest reported to date for normal-GVD Kerr combs. Our technique enables on-demand generation of a high-power comb source for applications such as wavelength-division multiplexing in optical communications.
We investigate the various routes to spatiotemporal chaos in Kerr optical frequency combs obtained through pumping an ultra-high quality whispering-gallery mode resonator with a continuous-wave laser. The Lugiato-Lefever model is used to build bifurcation diagrams with regards to the parameters that are externally controllable, namely, the frequency and the power of the pumping laser. We show that the spatiotemporal chaos emerging from Turing patterns and solitons display distinctive dynamical features. Experimental spectra of chaotic Kerr combs are also presented for both cases, in excellent …
We explore the dynamical response of dissipative Kerr solitons to changes in pump power and detuning and show how thermal and nonlinear processes couple these parameters to the frequency-comb degrees of freedom. Our experiments are enabled by a Pound-Drever-Hall (PDH) stabilization approach that provides on-demand, radiofrequency control of the frequency comb. PDH locking not only guides Kerr-soliton formation from a cold microresonator, but opens a path to decouple the repetition and carrier-envelope-offset frequencies. In particular, we demonstrate phase stabilization of both Kerr-comb degre…
Optical frequency combs enable coherent data transmission on hundreds of wavelength channels and have the potential to revolutionize terabit communications. Generation of Kerr combs in nonlinear integrated microcavities represents a particularly promising option enabling line spacings of tens of GHz, compliant with wavelength-division multiplexing (WDM) grids. However, Kerr combs may exhibit strong phase noise and multiplet spectral lines, and this has made high-speed data transmission impossible up to now. Recent work has shown that systematic adjustment of pump conditions enables low phase-n…
Anomalous group velocity dispersion is a key parameter for generating bright solitons, and thus wideband Kerr frequency combs. Extension of frequency combs to visible wavelength in conventional photonic materials and structures has been a major challenge due to strong normal material dispersion at the relevant frequencies. Extension of frequency combs toward the normal dispersion region is possible via dispersive waves through soliton-induced Cherenkov radiation. However, this potentially powerful technique has not been used for extending frequency combs to the visible spectrum. In this paper,…
We theoretically study the stability conditions and excitation regimes of hyper-parametric oscillation and Kerr frequency comb generation in continuously pumped nonlinear optical resonators possessing anomalous group velocity dispersion. We show that both hard and soft excitation regimes are possible in the resonators. Selection between the regimes is achieved via change in the parameters of the pumping light.
We demonstrate various regimes of synchronization in systems of two coupled cavity soliton-based Kerr frequency combs. We show sub-harmonic, harmonic and harmonic-ratio synchronization of coupled microresonators, and reveal their dynamics in the form of Arnold tongues, structures that are ubiquitous in nonlinear dynamical systems. Our experimental results are well corroborated by numerical simulations based on coupled Lugiato-Lefever equations. This study illustrates the newfound degree of flexibility in synchronizing Kerr combs across a wide range of comb spacings and could find applications …
Self-referencing turns pulsed laser systems into self-referenced frequency combs. Such frequency combs allow counting of optical frequencies and have a wide range of applications. The required optical bandwidth to implement self-referencing is typically obtained via nonlinear broadening in optical fibers. Recent advances in the field of Kerr frequency combs have provided a path towards the development of compact frequency comb sources that provide broadband frequency combs, exhibit microwave repetition rates and that are compatible with on-chip photonic integration. These devices have the pote…
Intraresonance frequency combs in Kerr microresonators
Faculty of Physics, Lomonosov Moscow State University（莫斯科国立大学物理系）；Russian Quantum Center（俄罗斯量子中心）；Moscow Institute of Physics and Technology（莫斯科物理技术学院）；International Quantum Academy（国际量子研究院）；Hefei National Laboratory, University of Science and Technology of China（中国科学技术大学合肥国家实验室）；Lebedev Physical Institute, Russian Academy of Sciences（俄罗斯科学院列别捷夫物理研究所）
Optical frequency combs allow for precise measurement of optical frequencies and are used in a growing number of applications beyond spectroscopy and optical frequency metrology. A class of compact microresonator based frequency comb generators has emerged recently based on (hyper)-parametric frequency conversion, mediated by the Kerr-non-linearity, of a continuous wave laser beam. Despite the rapid progress and the emergence of a wide variety of micro-resonator Kerr-comb platforms, an understanding of the dynamics of the Kerr comb formation is still lacking. In particular the question in whic…
Using the known solutions of the Lugiato-Lefever equation, we derive universal trends of Kerr frequency combs. In particular, normalized properties of temporal cavity soliton solutions lead us to a simple analytic estimate of the maximum attainable bandwidth for given pump-resonator parameters. The result is validated via comparison with past experiments encompassing a diverse range of resonator configurations and parameters.
We stabilize a chip-scale Si3N4 phase-locked Kerr frequency comb via locking the pump laser to an independent stable high-Q reference microresonator and locking the comb spacing to an external microwave oscillator. In this comb, the pump laser shift induces negligible impact on the comb spacing change. This scheme is a step towards miniaturization of the stabilized Kerr comb system as the microresonator reference can potentially be integrated on-chip. Fractional instability of the optical harmonics of the stabilized comb is limited by the microwave oscillator used for comb spacing lock below 1…
Transfer of amplitude and phase noise from a continuous wave optical pump to the repetition rate of a Kerr frequency comb is studied theoretically, with focus on generation of spectrally pure radio frequency (RF) signals via demodulation of the frequency comb on a fast photodiode. It is shown that both the high order chromatic dispersion of the resonator spectrum and frequency-dependent quality factor of the resonator modes facilitate the optical-to-RF noise conversion that limits spectral purity of the RF signal.
We demonstrate experimentally, and explain theoretically, generation of a wide, fundamentally phase locked Kerr frequency comb in a nonlinear resonator with a normal group velocity dispersion. A magnesium fluoride whispering gallery resonator characterized with 10 GHz free spectral range and pumped either at 780 nm or 795 nm is used in the experiment. The envelope of the observed frequency comb differs significantly from the Kerr frequency comb spectra reported previously. We show via numerical simulation that, while the frequency comb does not correspond to generation of short optical pulses,…
Mode interaction in silicon nitride micro-resonators is investigated. We provide clear experimental evidence of mode interaction between two family modes and mode interaction is demonstrated to be the cause of the comb generation in resonators with normal dispersion.
Frequency modulated (FM) frequency combs constitute an exciting alternative to generate equidistant spectra. The full set of Maxwell-Bloch equations is reduced to a single master equation for FM combs with fast dynamics to provide insight into the governing mechanisms behind phase-locking. It reveals that the recently observed linear frequency chirp is caused by the combined effects of spatial hole burning, group velocity dispersion and Kerr due to asymmetric gain. The comparison to observation in various semiconductor lasers suggests that the linear chirp is general to self-starting FM combs.
We theoretically and experimentally investigated the transition between modulation instability and Raman gain in a small silica microcavity with a large free-spectral range (FSR), which reveals that we can selectively switch from a four-wave mixing dominant state to a stimulated Raman scattering dominant state. Both the theoretical analysis and the experiment show that a Raman-dominant region is present between transitions of Kerr combs with different free-spectral range spacings. We can obtain a stable Kerr comb and a stable Raman state selectively by changing the driving power, coupling betw…
We show that scattering-based interaction among nearly degenerate optical modes is the key factor in low threshold generation of Kerr frequency combs in nonlinear optical resonators possessing small group velocity dispersion (GVD). The mode interaction is capable of producing drastic change in the local GVD, resulting in either a significant reduction or increase of the oscillation threshold. It is also responsible for the majority of observed combs in resonators characterized with large normal GVD. We present results of our numerical simulations as well as supporting experimental data.
A method of retrieving the complex intracavity pump field from the through port is proposed, and verified through characterizing the time-domain waveform of a mode-locked comb related to dark soliton formation in a normal-dispersion microresonator.
Octave-spanning, self-referenced frequency combs are applied in diverse fields ranging from precision metrology to astrophysical spectrometer calibration. In the past decade, Kerr frequency comb generators have emerged as alternative scheme offering chip-scale integration, high repetition rate and bandwidths that are only limited by group velocity dispersion. The recent observation of Kerr frequency combs operating in the dissipative Kerr soliton (DKS) regime, along with dispersive wave formation, has provided the means for fully coherent, broadband Kerr frequency comb generation with engineer…
We establish an exact partial differential equation to model Kerr comb generation in whispering-gallery mode resonators. This equation is a variant of the Lugiato-Lefever equation that includes higher-order dispersion and nonlinearity. This spatio-temporal model, whose main variable is the total intracavity field, is significantly more suitable than the modal expansion approach for the theoretical understanding and the numerical simulation of wide-span combs. It allows us to explore pulse formation in which a large number of modes interact cooperatively. This versatile approach can be straight…
Recent experiments have demonstrated the generation of widely-spaced parametric sidebands that can evolve into "clustered" optical frequency combs in Kerr microresonators. Here we describe the physics that underpins the formation of such clustered comb states. In particular, we show that the phase-matching required for the initial sideband generation is such that (at least) one of the sidebands experiences anomalous dispersion, enabling that sideband to drive frequency comb formation via degenerate and non-degenerate four-wave mixing. We validate our proposal through a combination of experimen…
Taking advantage of an extended Lugiato--Lefever equation with third-order dispersion, we numerically show that dark cavity solitons formed in normal dispersion of microresonators are capable of emitting dispersive waves in both normal and anomalous dispersion regions, resembling the behavior of the commonly encountered bright cavity solitons. The generated dispersive waves can be accurately predicted by the dissipative radiation theory. In addition, we demonstrate the stability enhancement of Kerr frequency combs in normal dispersion regime in case the dispersive wave is emitted by dark solit…
We present the experimental realization of transverse mode conversion in an optical fiber via an optically induced long-period grating. The transient gratings are generated by femtosecond laser pulses, exploiting the Kerr effect to translate intensity patterns emerging from multimode interference into a spatial refractive index modulation. Since these modulations exist only while the pump beam is present, they can be used for optical switching of transverse modes. As only a localized part of the grating was written at a time and the probe beam was co-propagating with the pump beam the required…
The model, that is usually called Lugiato-Lefever equation (LLE), was introduced in 1987 with the aim of providing a paradigm for dissipative structure and pattern formation in nonlinear optics. This model, describing a driven, detuned and damped nonlinear Schroedinger equation, gives rise to dissipative spatial and temporal solitons. Recently, the rather idealized conditions, assumed in the LLE, have materialized in the form of continuous wave driven optical microresonators, with the discovery of temporal dissipative Kerr solitons (DKS). These experiments have revealed that the LLE is a perfe…
By generating a Brillouin laser in an optical microresonator, we realize a soliton Kerr microcomb through exciting the Kerr frequency comb using the generated Brillouin laser in the same cavity. The intracavity Brillouin laser pumping scheme enables us to access the soliton states with a blue-detuned input pump. Due to the ultra-narrow linewidth and the low-noise properties of the generated Brillouin laser, the observed soliton microcomb exhibits narrow-linewidth comb lines and stable repetition rate even by using a diode laser with relatively broad linewidth. Also, we demonstrate a low-noise …
Dissipative Kerr solitons are localized structures that exist in optical microresonators. They lead to the formation of microcombs --- chip-scale frequency combs that could facilitate precision frequency synthesis and metrology by capitalizing on advances in silicon photonics. Previous demonstrations have mainly focused on anomalous dispersion microresonators. Notwithstanding, localized structures also exist in the normal dispersion regime in the form of circulating dark pulses, but their physical dynamics is far from being understood. Here, we report the discovery of reversible switching betw…
We study the impact of inherent mode coupling between clockwise (CW) and counter-clockwise (CCW) modes on Kerr comb generation in a small whispering-gallery mode microcavity. Our numerical analysis using a coupled Lugiato-Lefever equation reveals the range of the coupling strength in which a soliton pulse can be obtained in the CW direction. It also showed that CCW comb power depends on the coupling strength between the CW and CCW modes. In addition to the simulation, we conducted an experiment to confirm that the power ratio between the CW and CCW comb modes depends on the coupling strength, …
Optical frequency comb (OFC) technology has been the cornerstone for scientific breakthroughs such as precision frequency metrology, redefinition of time, extreme light-matter interaction, and attosecond sciences. While the current mode-locked laser-based OFC has had great success in extending the scientific frontier, its use in real-world applications beyond the laboratory setting remains an unsolved challenge. Microresonator-based OFCs, or Kerr frequency comb, have recently emerged as a candidate solution to the challenge because of their preferable size, weight, and power consumption (SWaP)…
Laser frequency combs are coherent light sources that simultaneously provide pristine frequency spacings for precision metrology and the fundamental basis for ultrafast and attosecond sciences. Recently, nonlinear parametric conversion in high-Q microresonators has been suggested as an alternative platform for optical frequency combs, though almost all in 100 GHz frequencies or more. Here we report a low-phase-noise on-chip Kerr frequency comb with mode spacing compatible with high-speed silicon optoelectronics. The waveguide cross-section of the silicon nitride spiral resonator is designed to…
Kerr microresonators generate interesting and useful fundamental states of electromagnetic radiation through nonlinear interactions of continuous-wave (CW) laser light. Using photonic-integration techniques, functional devices with low noise, small size, low-power consumption, scalable fabrication, and heterogeneous combinations of photonics and electronics can be realized. Kerr solitons, which stably circulate in a Kerr microresonator, have emerged as a source of coherent, ultrafast pulse trains and ultra-broadband optical-frequency combs. Using the f-2f technique, Kerr combs support carrier-…
We show that both the power and repetition rate of a frequency comb generated in a nonlinear ring resonator, pumped with continuous wave (cw) coherent light, are modulated. The modulation is brought about by the interaction of the cw background with optical pulses excited in the resonator, and occurs in resonators with nonzero high-order chromatic dispersion and wavelength-dependent quality factor. The modulation frequency corresponds to the detuning of the pump frequency from the eigenfrequency of the pumped mode in the resonator.
The shaping of group velocity dispersion in microresonators is an important component in the generation of wideband optical frequency combs. Small resonators - with tight bending radii - offer the large free-spectral range desirable for wide comb formation. However, the tighter bending usually limit comb formation as it enhances normal group velocity dispersion. We experimentally demonstrate that engineering the sidewall angle of small-radius (100 $μ$m), 3 $μ$m-thick silica wedge microdisks enables dispersion tuning in both normal and anomalous regimes, without significantly affecting the free…
Nonlinear Kerr micro-resonators have enabled fundamental breakthroughs in the understanding of dissipative solitons, as well as in their application to optical frequency comb generation. However, the conversion efficiency of the pump power into a soliton frequency comb typically remains below a few percent. We introduce a hybrid Mach-Zehnder ring resonator geometry, consisting of a micro-ring resonator embedded in an additional cavity with twice the optical path length of the ring. The resulting interferometric back coupling enables to achieve an unprecedented control of the pump depletion: pu…
We theoretically investigate the phase-locking phenomena between the spectral components of Kerr optical frequency combs in the dynamical regime of Turing patterns. We show that these Turing patterns display a particularly strong and robust phase-locking, originating from a cascade of phase-locked triplets which asymptotically lead to a global phase-locking between the modes. The local and global phase-locking relationship defining the shape of the optical pulses are analytically determined. Our analysis also shows that solitons display a much weaker phase-locking which can be destroyed more e…
Kerr soliton frequency comb generation in monolithic microresonators recently attracted great interests as it enables chip-scale few-cycle pulse generation at microwave rates with smooth octave-spanning spectra for self-referencing. Such versatile platform finds significant applications in dual-comb spectroscopy, low-noise optical frequency synthesis, coherent communication systems, etc. However, it still remains challenging to straightforwardly and deterministically generate and sustain the single-soliton state in microresonators. In this paper, we propose and theoretically demonstrate the ex…
Optical frequency combs enable state-of-the-art applications including frequency metrology, optical clocks, astronomical measurements, and sensing. Recent demonstrations of microresonator-based Kerr frequency combs or microcombs pave the way to scalable and stable comb sources on a photonic chip. Generating microcombs in the visible wavelength range, however, has been limited by large material dispersion and optical loss. Here we demonstrate a scheme for efficiently generating visible microcomb in a high Q aluminum nitride microring resonator. Enhanced Pockels effect strongly couples infrared …
Microresonator-based Kerr frequency comb (microcomb) generation can potentially revolutionize a variety of applications ranging from telecommunications to optical frequency synthesis. However, phase-locked microcombs have generally had low conversion efficiency limited to a few percent. Here we report experimental results that achieve ~30% conversion efficiency (~200 mW on-chip comb power excluding the pump) in the fiber telecommunication band with broadband mode-locked dark-pulse combs. We present a general analysis on the efficiency which is applicable to any phase-locked microcomb state. Th…
The experimental realization of a Kerr frequency comb represented the convergence of research in materials, physics, and engineering, and this symbiotic relationship continues to underpin efforts in comb innovation today. While the initial focus developing cavity-based frequency combs relied on existing microresonator architectures and classic optical materials, in recent years, this trend has been disrupted. This paper reviews the latest achievements in frequency comb generation using resonant cavities, placing them within the broader historical context of the field. After presenting well-est…
