A spatial quantum model of spontaneous parametric down-conversion in nonlinear layered structures is developed expanding the interacting vectorial fields into monochromatic plane waves. A two-photon spectral amplitude depending on the signal- and idler-field frequencies and propagation directions is used to derive transverse profiles of the emitted fields as well as their spatial correlations. Intensity spatial profiles and their spatial correlations are mainly determined by the positions of transmission peaks formed in these structures with photonic bands. A method for geometry optimization of the structures with respect to efficiency of the nonlinear process is suggested. Several structures composed of GaN/AlN layers are analyzed as typical examples. They allow the generation of photon pairs correlated in several emission directions. Photon-pair generation rates increasing better than the second power of the number of layers can be reached. Also structures efficiently generated photon pairs showing anti-bunching and anti-coalescence can be obtained. Three reasons for splitting the correlated area in photonic-band-gap structures are revealed: zig-zag movement of photons inside the structure, spatial symmetry and polarization-dependent properties. Also spectral splitting can be observed in these structures.
Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that allows the spectral shaping of entangled photons with high resolution. We evaluate its performances by detecting sum frequency generation in a non-linear crystal. The efficiency of the process is compared when performed with classical or entangled light.
We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single…
Entangled photons are crucial for quantum technologies, but generating arbitrary entangled photon states deterministically, efficiently, and with high fidelity remains a challenge. Here, we demonstrate how hybridization and dipole-dipole interactions -- potentially simultaneously available in colloidal quantum dots and molecular aggregates -- leveraged in conjunction can couple simple, well understood emitters into composite emitters with flexible control over the level structure. We show that cascade decay through carefully designed level structures can result in emission of frequency-entangl…
In this paper, an experiment of quantum diffraction of position-momentum entangled photons from a straight sharp edge is presented. Path of a single photon of an entangled pair is partially blocked by a sharp edge whereas the other photon is detected at a stationary location without revealing the which-path information of the other photon. Quantum diffraction pattern of the sharp edge is revealed only in the correlated conditional detection of spatially separated photons and no diffraction pattern is formed in local detections of individual photons. Theoretical analysis of the quantum diffract…
We report measurements of time-frequency entangled photon pairs and heralded single photons at telecommunications wavelengths, generated using a periodically-poled, lithium niobate on insulator (LNOI) waveguide pumped optically by a diode laser. We achieve a high Coincidences-to-Accidentals Ratio (CAR) at high pair brightness, a low value of the conditional self-correlation function [$g^{(2)}$(0)], and high two-photon energy-time Franson interferometric visibility, which demonstrate the high quality of the entangled photon pairs and heralded single photons.
Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the excitonic fine-structure splitting. This work demonstrates that, even if this splitting is absent, the degree of entanglement cannot reach unity when the excitation pulse in a two-photon resonance scheme has a finite duration. The degradation of the entanglement has its origin in a dynamically induced splitting of the exciton states caused by the laser puls…
We consider six-photon entangled state emitted from a single third-order parametric down-conversion process. In the regime of weak nonlinearities, we present a symmetry detector which is capable of analyzing the twin-beam six-photon symmetric states. By cascading the symmetry detectors, as an application, it is shown that one can purify the desired six-photon entangled state from an arbitrary twin-beam six-photon symmetric state. With linear optics we propose a fruitful scheme for exploring a class of multimode-photon entangled states from third-order parametric down-conversion process. Furthe…
The mid-infrared (MIR) band entangled photon source is vital for the next generation of quantum communication, quantum imaging, and quantum sensing. However, the current entangled states are mainly prepared in visible or near-infrared bands. It is still lack of high-quality entangled photon sources in the MIR band. In this work, we optimize the poling sequence of lithium niobate to prepare two kinds of typical entangled states, the Hermit-Gaussian state and the comb-like entangled state at 3.2 $μ$m. We have also calculated the photon pair rates and estimated the effect of fabrication resolutio…
We present recent findings towards developing brighter entangled photon sources in critically phase matched (CPM) nonlinear crystals. Specifically, we use type-I collinear phase matching at non-degenerate wavelengths in parallel \b{eta}-Barium Borate (BBO) crystals to generate pairs of polarization entangled photons for free-space quantum key distribution (QKD). We first review the entangled source configuration and then discuss ways to further improve the source brightness by means of tailoring the pump and collection modes. We present preliminary results that may lead to brighter entangled p…
