局域场因子和微观级联：一种应用于分子受限体系的自洽方法
The Local Field Factor and Microscopic Cascading: A Self-Consistent Method Applied to Confined Systems of Molecules
摘要：
我们使用一个简化的自洽方法来解决非线性光学级联现象，这表明增加了微观级联的贡献，在高阶非线性介电常数通过五阶。这些级联项在微观范围内包括所有可能的标量级联配置。几何约束的施加进一步影响了预测的级联贡献，并为非线性光学材料开辟了额外的设计参数。这些结果被用于近似的有效五阶极化率在薄膜的C60单体的不同厚度和浓度。本文包含了对《物理学杂志B》上发表的原始论文的更正，这些更正反映在随后的勘误表中。
英文摘要：
We use a simplified self-consistent method to address nonlinear-optical cascading phenomena, which shows added microscopic cascading contributions in high-ordered nonlinear susceptibilities through fifth order. These cascading terms in the microscopic regime encompass all possible scalar cascading configurations. The imposition of geometric constraints further influences the predicted cascading contributions and opens up additional design parameters for nonlinear-optical materials. These results are used in approximating the effective fifth-order susceptibility in thin films of C60 monomers of varying thickness and concentration. This paper contains the corrections to the original paper that appeared in the Journal of Physics B as reflected in the content of the corrigendum that followed.
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