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arXiv 1010.1192quant-phcond-mat.other
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金刚石单氮空位中心光循环中的自旋动力学

Spin dynamics in the optical cycle of single nitrogen-vacancy centres in diamond

Lucio Robledo, Hannes Bernien, Toeno van der Sar, Ronald Hanson

摘要:

本文研究了金刚石中单个负电荷氮空位中心的自旋相关衰变和光循环中的系间交叉。我们使用自旋控制和脉冲光激发来提取自旋分辨的激发态寿命和光诱导自旋极化的程度。通过用一系列皮秒脉冲光激发中心,我们确定了每个光学周期的自旋翻转概率,以及系统间交叉的自旋相关概率。这些信息,连同独立测量的单重态布居的衰变率提供了一个完整的描述在NV中心的光学循环的自旋动力学。单重态布居衰减速率的温度依赖性提供了光循环中所涉及的单重态数量的信息。

英文摘要:

We investigate spin-dependent decay and intersystem crossing in the optical cycle of single negatively-charged nitrogen-vacancy (NV) centres in diamond. We use spin control and pulsed optical excitation to extract both the spin-resolved lifetimes of the excited states and the degree of optically-induced spin polarization. By optically exciting the centre with a series of picosecond pulses, we determine the spin-flip probabilities per optical cycle, as well as the spin-dependent probability for intersystem crossing. This information, together with the indepedently measured decay rate of singlet population provides a full description of spin dynamics in the optical cycle of NV centres. The temperature dependence of the singlet population decay rate provides information on the number of singlet states involved in the optical cycle.

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