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arXiv 1004.3759cond-mat.str-elcond-mat.mtrl-scicond-mat.supr-con
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金属Fe $_{1.087}$ Te的芯-孔介导非弹性X射线散射的证据

Evidence for core-hole-mediated inelastic x-ray scattering from metallic Fe$_{1.087}$Te

J. N. Hancock, R. Viennois, D. van der Marel, H. M. Rønnow, M. Guarise, P. -H. Lin, M. Grioni, M. Moretti Sala, G. Ghiringhelli, V. N. Strocov, J. Schlappa, T. Schmitt

摘要:

我们提出了一个详细的分析共振非弹性散射(RIXS)从Fe $_{1.087}$ Te前所未有的能量分辨率。与在过渡金属$L_3$边缘的绝缘系统中通常看到的尖峰相反,我们观察到显示不同特征的光谱。对于低能量转移,我们从实验上观察到理论预测的共振拉曼散射从非相互作用的费米子气体的多体效应。此外,我们发现,这种多体电子理论的局限性,实现在高拉曼位移,其中指数线形揭示了能量尺度不存在于这些考虑。这种制度,确定为发射,需要考虑晶格自由度,以了解线形。我们认为,这两个观察是内在的一般特征的多体物理的金属。

英文摘要:

We present a detailed analysis of resonant inelastic scattering (RIXS) from Fe$_{1.087}$Te with unprecedented energy resolution. In contrast to the sharp peaks typically seen in insulating systems at the transition metal $L_3$ edge, we observe spectra which show different characteristic features. For low energy transfer, we experimentally observe theoretically predicted many-body effects of resonant Raman scattering from a non-interacting gas of fermions. Furthermore, we find that limitations to this many-body electron-only theory are realized at high Raman shift, where an exponential lineshape reveals an energy scale not present in these considerations. This regime, identified as emission, requires considerations of lattice degrees of freedom to understand the lineshape. We argue that both observations are intrinsic general features of many-body physics of metals.

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