We have studied the collective properties of two-dimensional (2D) excitons immersed within a quantum well which contains 2D excitons and a two-dimensional electron gas (2DEG). We have also analyzed the excitations for a system of 2D dipole excitons with spatially separated electrons and holes in a pair of quantum wells (CQWs) when one of the wells contains a 2DEG. Calculations of the superfluid density and the Kosterlitz-Thouless (K-T) phase transition temperature for the 2DEG-exciton system in a quantum well have shown that the K-T transition temperature increases with increasing exciton density and that it might be possible to have fast long range transport of excitons. The superfluid density and the K-T transition temperature for dipole excitons in CQWs in the presence of a 2DEG in one of the wells increases with increasing inter-well separation.
We predict the formation and superfluidity of polaritons in an optical microcavity formed by excitons in gapped graphene embedded there and microcavity photons. The Rabi splitting related to the creation of an exciton in a graphene layer in the presence of the band gap is obtained. The analysis of collective excitations as well as the sound velocity is presented. We show that the superfluid density and temperature of the Kosterlitz-Thouless phase transition are decreasing functions of the energy gap.
Double-layer electron systems in the quantum Hall regime have excitonic condensate ground states when the layers are close together and the total Landau level filling factor is close to an odd integer. In this paper we discuss the microscopic physics of these states and recent progress toward building a theory of the anomalous collective transport effects that occur in separately contacted bilayers when the condensate is present.
Fingerprints of Excitonic Collective Modes in the Two-Dimensional Electron Gas
Friedrich-Schiller-Universät Jena（耶拿弗里德里希·席勒大学）；Ruhr University Bochum（波鸿鲁尔大学）；École Polytechnique, Institut Polytechnique de Paris（巴黎综合理工学院，巴黎理工学院）；Synchrotron SOLEIL（SOLEIL同步辐射中心）
Excitonic insulators host a condensate of electron-hole pairs at equilibrium, giving rise to collective many-body effects. Although several materials have emerged as excitonic insulator candidates, evidence of long-range coherence is lacking and the origin of the ordered phase in these systems remains controversial. Here, using ultrafast pump-probe microscopy, we investigate the possible excitonic insulator Ta$_2$NiSe$_5$. Below 328 K, we observe the anomalous micrometer-scale propagation of coherent modes at velocities of the order of $\sim10^5$ m/s, which we attribute to the hybridization be…
The layered chalcogenide Ta$_{2}$NiSe$_{5}$ has been proposed to host an excitonic condensate in its ground state, a phase that could offer a unique platform to study and manipulate many-body states at room temperature. However, identifying the dominant microscopic contribution to the observed spontaneous symmetry breaking remains challenging, perpetuating the debate over the ground state properties. Here, using broadband ultrafast spectroscopy we investigate the out-of-equilibrium dynamics of Ta$_{2}$NiSe$_{5}$ and demonstrate that the transient reflectivity in the near-infrared range is conn…
The collective decay of excitons from initial Bose-Einstein condensate state is investigated theoretically. As practically more interesting case we consider excitons of the yellow series in the semiconductor cuprous oxide where we have collective photon and phonon assisted decay of excitons. It is shown that because of intrinsic instability of recoilless two-boson decay of Bose-Einstein condensate, the spontaneously emitted bosonic pairs are amplified leading to an exponential buildup of a macroscopic population into the certain modes. The collective decay rate has a nonlinear dependence on th…
The photoluminescence dynamics of a microscopic gas of indirect excitons trapped in coupled quantum wells is probed at very low bath temperature (approximately 350 mK). Our experiments reveal the non linear energy relaxation characteristics of indirect excitons. Particularly, we observe that the excitons dynamics is strongly correlated with the screening of structural disorder by repulsive exciton-exciton interactions. For our experiments where two-dimensional excitonic states are gradually defined, the distinctive enhancement of the exciton scattering rate towards lowest energy states with in…
Bose-Einstein condensation of the excitons in graphene is considered. We suggested the model spinor equation for neutral particles with short range interaction described the microscopic graphene excitons dynamic. Using this equation we derived quantum hydrodynamic equations for description of collective properties of excitons in graphene, particularly for the case when excitons being in the Bose-Einstein condensate (BEC) state. The dispersion of collective excitations in graphene excitons BEC is studied. We shown that frequency of collective excitations is proportional to the square root of th…
We consider a two-band spinless model describing an excitonic insulator (EI) on the two-dimensional square lattice with anisotropic hopping parameters and electron-phonon (el-ph) coupling, inspired by the EI candidate Ta$_2$NiSe$_5$. We systematically study the nature of the collective excitations in the ordered phase which originates from the interband Coulomb interaction and the el-ph coupling. When the ordered phase is stabilized only by the Coulomb interaction (pure EI phase), its collective response exhibits a massless phase mode in addition to the amplitude mode. We show that in the BEC …
We discuss light-heavy hole beats observed in transient optical experiments in GaAs quantum wells in terms of a free-boson coherent state model. This approach is compared with descriptions based on few-level representations. Results lead to an interpretation of the beats as due to classical electromagnetic interference. The boson picture correctly describes photon excitation of extended states and accounts for experiments involving coherent control of the exciton density and Rayleigh scattering beating.
We report the first observation of stochastic resonance in confined exciton-polaritons. We evidence this phenomena by tracking the polaritons behavior through two stochastic resonance quantifiers namely the spectral magnification factor and the signal-to-noise ratio. The evolution of the stochastic resonance in function of the modulation amplitude of the periodic excitation signal is studied. Our experimental observations are well reproduced by numerical simulations performed in the framework of the Gross-Pitaevskii equation under stochastic perturbation.
Collective (elementary) excitations of quantum bosonic condensates, including condensates of exciton polaritons in semiconductor microcavities, are a sensitive probe of interparticle interactions. In anisotropic microcavities with momentum-dependent TE-TM splitting of the optical modes, the excitations dispersions are predicted to be strongly anisotropic, which is a consequence of the synthetic magnetic gauge field of the cavity, as well as the interplay between different interaction strengths for polaritons in the singlet and triplet spin configurations. Here, by directly measuring the disper…
Photogenerated excitonic ensembles confined in coupled GaAs quantum wells are probed by a complementary approach of emission spectroscopy and resonant inelastic light scattering. Lateral electrostatic trap geometries are used to create dense systems of spatially indirect excitons and excess holes with similar densities in the order of 10$^{11}$ cm$^{-2}$. Inelastic light scattering spectra reveal a very sharp low-lying collective mode that is identified at an energy of 0.44 meV and a FWHM of only ~50 $μ$eV. This mode is interpreted as a plasmon excitation of the excess hole system coupled to t…
The spin dynamics of an interwell excitons gas has been investigated in n-i-n GaAs/AlGaAs coupled quantum wells (CQWs). In these heterostructures the electron and the hole are spatially separated in neighboring quantum wells by a narrow AlAs barrier, when an electric field is applied. The time evolution kinetics of the interwell exciton photoluminescence has been measured under resonant excitation of the 1sHH intrawell exciton, using a pulsed tunable laser. The formation of a collective exciton phase in time and the temperature dependence of its spin relaxation rate have been studied. The spin…
The influence of a random field induced by impurities, boundary irregularities etc. on the superfluidity of a quasi-two-dimensional (2D) system of spatially indirect excitons in coupled quantum wells is studied. The interaction between excitons is taken into account in the ladder approximation. The random field is allowed to be large compared to the dipole-dipole repulsion between excitons. The coherent potential approximation (CPA) allows us to derive the exciton Green's function for a wide range of the random field, and the CPA results are used in the weak-scattering limit, which results in …
I develop a theory of combined exciton-cyclotron resonance (ExCR) in a low-density two-dimensional electron gas in high magnetic fields. In the presence of excess electrons an incident photon creates an exciton and simultaneously excites one electron to higher-lying Landau levels. I derive exact ExCR selection rules that follow from the existing dynamical symmetries, magnetic translations and rotations about the magnetic field axis. The nature of the final states in the ExCR is elucidated. The relation between ExCR and shake-up processes is discussed. The double-peak ExCR structure for transit…
An emergent quantized field enriches quantum many-body systems. We propose an antiparticle analog of the exciton in semimetals as an emergent collective mode in interacting electron systems. We show that inter-band excitations in semimetals are generally comprised of both excitons and antiparticles of excitons. These two stand for two distinct inter-band collective modes in semimetals, having different energies and opposite conserved charges. The conserved charge here is a quantity conjugate to a joint U(1) symmetry of two electron's bands associated with the inter-band excitations. The opposi…
A doped graphene layer in the integer quantum Hall regime reveals a highly unusual particle-hole excitation spectrum, which is calculated from the dynamical polarizability in the random phase approximation. We find that the elementary neutral excitations in graphene in a magnetic field are unlike those of a standard two-dimensional electron gas (2DEG): in addition to the upper-hybrid mode, the particle-hole spectrum is reorganized in linear magneto-plasmons that disperse roughly parallel to $ω=v_F q$, instead of the usual horizontal (almost dispersionless) magneto-excitons. These modes could b…
Time resolved photoluminescence is a powerful technique to study the collective dynamics of excitons and polaritons in semiconductor nanostructures. We present a two excitation pulses technique to induce the ultrafast and controlled quenching of the exciton emission in a quantum well. The depth of the dip is given by the magnitude of the warming of the carriers induced by the arrival of a laser pulse when an exciton population is already present in the sample. We use this technique to study the relaxation mechanisms of polaritons in semiconductor microcavities, which are of great importance to…
Achieving and controlling strong light-matter interactions in many-body systems is of paramount importance both for fundamental understanding and potential applications. In this paper we demonstrate both experimentally and theoretically how to manipulate strong coupling between the Bragg-plasmon mode supported by a organo-metallic array and molecular excitons in the form of J-aggregates dispersed on the hybrid structure. We observe experimentally the transition from a conventional strong coupling regime exhibiting the usual upper and lower polaritonic branches to a more complex regime, where a…
We study the metal-insulator transition in individual self-assembled quantum wires and report optical evidences of metallic liquid condensation at low temperatures. Firstly, we observe that the temperature and power dependence of the single nanowire photoluminescence follow the evolution expected for an electron-hole liquid in one dimension. Secondly, we find novel spectral features that suggest that in this situation the expanding liquid condensate compresses the exciton gas in real space. Finally, we estimate the critical density and critical temperature of the phase transition diagram at $n…
Higgs modes in condensed matter physics have drawn attention because of analogies to the Higgs bosons of particle physics. Here we use a microscopic time-dependent mean-field theory to study the collective mode spectra of two-dimensional spatially indirect exciton (electron-hole pair) condensates, focusing on the Higgs modes, i.e., those that have a large weight in electron-hole pair amplitude response functions. We find that in the low exciton density (BEC) limit, the dominant Higgs modes of spatially indirect exciton condensates correspond to adding electron-hole pairs that are orthogonal to…
Layered bosonic dipolar fluids have been suggested to host a condensate of interlayer molecular bound states. However, its experimental observation has remained elusive. Motivated by two recent experimental works [Hubert et al., Phys. Rev. X 9, 021026 (2019) and D. J. Choksy et al., Phys. Rev. B 103 045126 (2021)], we theoretically study, using numerically exact quantum Monte Carlo calculations, the experimental signatures of collective interlayer pairing in vertically stacked indirect exciton (IX) layers. We find that IX energy shifts associated with each layer evolve non trivially as a funct…
We demonstrate the strong coupling of direct transition excitons in tungsten disulfide (WS2) with collective plasmonic resonances at room temperature. We use open plasmonic cavities formed by periodic arrays of metallic nanoparticles. We show clear anti-crossings with monolayer, bilayer and thicker multilayer WS2 on top of the nanoparticle array. The Rabi energy of such hybrid system varies from 50 to 110 meV from monolayer to sixteen layers, while it does not scale with the square root of the number of layers as expected for collective strong coupling. We prove that out-of-plane coupling comp…
A theory of non-linear emission of quantum dot ensembles coupled to the optical mode of the microcavity is presented. Numerical results are compared with analytical approaches. The effects of exciton-exciton interaction within the quantum dots and with the reservoir formed by nonresonant pumping are considered. It is demonstrated, that the nonlinearity due to the interaction strongly affects the shape of the emission spectra. The collective superradiant mode of the excitons is shown to be stable against the non-linear effects.
A Mach-Zehnder interferometer with spatial and spectral resolution was used to probe spontaneous coherence in cold exciton gases, which are implemented experimentally in the ring of indirect excitons in coupled quantum wells. A strong enhancement of the exciton coherence length is observed at temperatures below a few Kelvin. The increase of the coherence length is correlated with the macroscopic spatial ordering of excitons.
We study the loading of a nonequilibrium, dissipative system of composite bosons -- exciton polaritons -- into a one dimensional periodic lattice potential. Utilizing momentum resolved photoluminescence spectroscopy, we observe a transition between an incoherent Bose gas and a polariton condensate, which undergoes further transitions between different energy states in the band-gap spectrum of the periodic potential with increasing pumping power. We demonstrate controlled loading into distinct energy bands by modifying the size and shape of the excitation beam. The observed effects are comprehe…
A theory of the spin exciton capture by a magnetic impurity in a 2D electron gas is developed. We consider the resonance model for electron scattering by a transition metal impurity and calculate the binding potential for spin excitons. This potential is spin selective and is capable of binding a spin exciton with zero angular momentum. In order to trap an exciton with a nonzero angular momentum m, the potential must exceed a certain threshold value, depending on m.
We study the collective interaction of excitons in closely spaced artificial molecules and arrays of nearly identical quantum dots with the electromagnetic modes. We discuss how collective fluorescence builds up in the presence of a small mismatch of the transition energy. We show that a superradiant state of a single exciton in a molecule of two dots with realistic energy mismatch undergoes a two-rate decay. We analyze also the stability of subdecoherent states for non-identical systems.
Charge separated interlayer excitons in transition metal dichalcogenide (TMDC) heterobilayers are being explored for moiré exciton lattices and exciton condensates. The presence of permanent dipole moments and the poorly screened Coulomb interaction make many body interactions particularly strong for interlayer excitons. Here we reveal two distinct phase transitions for interlayer excitons in the MoSe2/WSe2 heterobilayer using time and spatially resolved photoluminescence imaging: from trapped excitons in the moiré-potential to the modestly mobile exciton gas as exciton density increases to ne…
We study the kinetics of 2D Bose gas cooling provided Bose particles interact with 3D phonons. At low temperatures phonon emission is prohibited by the energy and the momentum conservation. We show that both particle-particle scattering and impurity scattering assist the Bose gas cooling.
We study the spontaneous emission from a coherently delocalized exciton state in a double quantum dot as a function of the distance between the dots, focusing on the similarities and differences between the cases of radiative (long-range, dipole) and tunnel coupling between the excitons in the dots. We show that there may be no qualitative difference between the collective emission induced by these two coupling types in spite of their essentially different physical properties.
Excitons, bound pairs of electrons and holes, form a model system to explore the quantum physics of cold bosons in solids. Cold exciton gases can be realized in a system of indirect excitons, which can cool down below the temperature of quantum degeneracy due to their long lifetimes. Here, we report on the measurement of spontaneous coherence in a gas of indirect excitons. We found that extended spontaneous coherence of excitons emerges in the region of the macroscopically ordered exciton state and in the region of vortices of linear polarization. The coherence length in these regions is much …
We report on the observation of a spin texture in a cold exciton gas in a GaAs/AlGaAs coupled quantum well structure. The spin texture is observed around the exciton rings. The observed phenomena include: a ring of linear polarization, a vortex of linear polarization with polarization perpendicular to the radial direction, an anisotropy in the exciton flux, a skew of the exciton fluxes in orthogonal circular polarizations and a corresponding four-leaf pattern of circular polarization, a periodic spin texture, and extended exciton coherence in the region of the polarization vortex. The data ind…
Spin currents and spin textures are observed in a coherent gas of indirect excitons. Applied magnetic fields bend the spin current trajectories and transform patterns of linear polarization from helical to spiral and patterns of circular polarization from four-leaf to bell-like-with-inversion.
An indirect exciton is a bound state of an electron and a hole in spatially separated layers. Two-dimensional indirect excitons can be created optically in heterostructures containing double quantum wells or atomically thin semiconductors. We study theoretically transmission of such bosonic quasiparticles through nano-constrictions. We show that quantum transport phenomena, e.g., conductance quantization, single-slit diffraction, two-slit interference, and the Talbot effect, are experimentally realizable in systems of indirect excitons. We discuss similarities and differences between these phe…
Topological Frenkel excitons in 2D molecular crystals
Université de Strasbourg（斯特拉斯堡大学）；CNRS（法国国家科学研究中心）；Institute of Physics, Czech Academy of Sciences（捷克科学院物理研究所）；Georg-August-Universität Göttingen（哥廷根大学）；Donostia International Physics Center（多诺斯蒂亚国际物理中心）；Ikerbasque, Basque Foundation for Science（伊克尔巴斯克科学基金会）
We report on the kinetics of a low-temperature gas of indirect excitons in the optically-induced exciton trap. The excitons in the region of laser excitation are found to rapidly -- within 4 ns -- cool to the lattice temperature T = 1.4 K, while the excitons at the trap center are found to be cold -- essentially at the lattice temperature -- even during the excitation pulse. The loading time of excitons to the trap center is found to be about 40 ns, longer than the cooling time yet shorter than the lifetime of the indirect excitons. The observed time hierarchy is favorable for creating a dense…
We discuss a theory of the ultrafast non-linear optical response of excitons in the Quantum Hall system. Our theory focusses on the role of the low energy collective electronic excitations of the cold, strongly correlated, two-dimensional electron gas (2DEG) present in the ground state. It takes into account ground state electron correlations and Pauli exchange and interaction effects between the photoexcited excitons and the collective excitations. Our formulation addresses both the initial coherent regime, where the dynamics is determined by exciton and 2DEG polarizations, and the subsequent…
We predict the existence of exchange broadening of optical lineshapes in disordered molecular aggregates and a nonuniversal disorder scaling of the localization characteristics of the collective electronic excitations (excitons). These phenomena occur for heavy-tailed Lévy disorder distributions with divergent second moments - distributions that play a role in many branches of physics. Our results sharply contrast with aggregate models commonly analyzed, where the second moment is finite. They bear a relevance for other types of collective excitations as well.
Systems of up to twelve electrons and six holes on the Haldane sphere are studied by exact numerical diagonalization. The low lying states of the system involve bound excitonic complexes such as (X^n)-. The angular momenta of these complexes and the pseudopotentials describing their interaction are determined. The similarity to the electron pseudopotential suggests the possibility of incompressible ground states of a gas of X- ions for nu<=1/3. The nu=1/3 state of three X-'s is found.
Flat-band systems are a promising platform for realizing exotic collective ground states with spontaneously broken symmetry because the electron-electron interactions dominate over the kinetic energy. A collective ground state of particular interest is the chased after exciton condensate (EC). However, in flat band systems other collective ground states can compete with an EC phase, and the conventional treatment of the effect of thermal and quantum fluctuations predicts the EC phase should be unstable. Here, using double twisted bilayer graphene (TBLG) heterostructures as an example, we show …
The high-temperature superfluidity of two-dimensional dipolar excitons in two parallel TMDC layers is predicted. We study Bose-Einstein condensation in the two-component system of dipolar A and B excitons. The effective mass, energy spectrum of the collective excitations, the sound velocity and critical temperature are obtained for different TMDC materials. It is shown that in the Bogolubov approximation the sound velocity in the two-component dilute exciton Bose gas is always larger than in any one-component. The difference between the sound velocities for two-component and one-component dilu…
Traditional spintronics relies on spin transport by charge carriers, such as electrons in semiconductor crystals. This brings several complications: the Pauli principle prevents the carriers from moving with the same speed; Coulomb repulsion leads to rapid dephasing of electron flows. Spin-optronics is a valuable alternative to traditional spintronics. In spin-optronic devices the spin currents are carried by electrically neutral bosonic quasi-particles: excitons or exciton-polaritons. They can form highly coherent quantum liquids and carry spins over macroscopic distances. The price to pay is…
We study collective electronic excitations in graphene in the integer quantum Hall regime, concentrating mainly on excitations with spin reversal such as spin-flip and spin-wave excitations. We show that these excitations are correctly accounted for in the time-dependent Hartree-Fock and strong magnetic field approximations, in contrast to spin-conserving (magneto-exciton) modes which involve a strong Landau-level mixing at non-zero wave vectors. The collective excitations are discussed in view of prominent theorems, such as Kohn's and Larmor's. Whereas the latter remains valid in graphene and…
We study the exciton condensate (EC) in a bilayer two-dimension-electron-gas (2DEG) adjacent to a type-II superconductor thin film with an array of pinned vortex lattices. By applying continuum low energy theory and carrying numerical simulations of lattice model within mean-field approximation, we find that if the order parameter of EC has a vortex profile, there are exact zero modes and associated \emph{rational} fractional charge for zero pseudospin potential ($μ$) and average chemical potential ($h$): $μ$=0 and $h$=0; while for $μ\mathtt{\neq}0$ and $h$=0, intervalley mixing splits the zer…
We report a comprehensive experimental study and detailed model analysis of the terahertz dielectric response and density kinetics of excitons and unbound electron-hole pairs in GaAs quantum wells. A compact expression is given, in absolute units, for the complex-valued terahertz dielectric function of intra-excitonic transitions between the 1s and higher-energy exciton and continuum levels. It closely describes the terahertz spectra of resonantly generated excitons. Exciton ionization and formation are further explored, where the terahertz response exhibits both intra-excitonic and Drude feat…
Negative diffusivity of excitons in electron-hole plasmas
Instituto Superior de Engenharia de Lisboa, Instituto Politécnico de Lisboa（里斯本高等工程学院，里斯本理工学院）；GoLP/Instituto de Plasmas e Fusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa（等离子体与核聚变研究所，里斯本高等工学院，里斯本大学）；Physics Department, Lomonosov Moscow State University（莫斯科国立大学物理系）
Interlayer excitons are bound states of electrons and holes confined in separate two-dimensional layers. Due to their repulsive dipolar interaction, interlayer excitons can form a correlated liquid. If another electron-hole bilayer is present, excitons from different bilayers can exhibit mutual attraction. We study such a quadrilayer system by a hypernetted chain formalism. We compute ground state energies, pair correlation functions, and collective mode velocities as functions of the exciton densities. We estimate the critical density for the transition to a paired biexciton phase. For a stro…
The mechanisms for generation of long-lived spin coherence in a two-dimensional electron gas (2DEG) have been studied experimentally by means of a picosecond pump-probe Kerr rotation technique. CdTe/(Cd,Mg)Te quantum wells with a diluted 2DEG were investigated. The strong Coulomb interaction between electrons and holes, which results in large binding energies of neutral excitons and negatively charged excitons (trions), allows one to address selectively the exciton or trion states by resonant optical excitation. Different scenarios of spin coherence generation were analyzed theoretically, amon…
We study the exciton gas-liquid transition in GaAs/AlGaAs coupled quantum wells. Below a critical temperature, Tc=4.8K, and above a threshold laser power density the system undergoes a phase transition into a liquid state. We determine the density temperature phase diagram over the temperature range 0.1 to 4.8K. We find that the latent heat increases linearly with temperature at T<1.1K, similarly to a Bose Einstein condensate transition, and becomes constant at 1.1<T<4.8K. Resonant Rayleigh scattering measurements reveal that the disorder in the sample is strongly suppressed and the diffusion …
We report on the principle and realization of a new trap for excitons -- the diamond electrostatic trap -- which uses a single electrode to create a confining potential for excitons. We also create elevated diamond traps which permit evaporative cooling of the exciton gas. We observe collection of excitons towards the trap center with increasing exciton density. This effect is due to screening of disorder in the trap by the excitons. As a result, the diamond trap behaves as a smooth parabolic potential which realizes a cold and dense exciton gas at the trap center.
The Andreev-Bashkin effect, or superfluid drag, is predicted in a system of Bose-condensed excitonic polaritons in optical microcavity coupled by electron-exciton interaction with a superconducting layer. Two possible setups with spatially indirect dipole excitons or direct excitons are considered. The drag density characterizing a magnitude of this effect is found by many-body calculations with taking into account dynamical screening of electron-exciton interaction. For the superconducting electronic layer, we assume the recently proposed polaritonic mechanism of Cooper pairing, although the …
We study the phase diagram of the inverted InAs/GaSb bilayer quantum wells. For small tunneling amplitude between the layers, we find that the system is prone to formation of an s-wave exciton condensate phase, where the spin-structure of the order parameter is uniquely determined by the small spin-orbit coupling arising from the bulk inversion asymmetry. The phase is topologically trivial and does not support edge transport. On the contrary, for large tunneling amplitude, we obtain a topologically non-trivial quantum spin Hall insulator phase with a p-wave exciton order parameter, which enhan…
