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arXiv 0910.5310cond-mat.str-elcond-mat.other
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RAu_{2} Ge_{2}(R = La,Ce,Pr)单晶的磁晶各向异性

Magnetocrystalline anisotropy in RAu_{2}Ge_{2} (R = La, Ce and Pr) single crystals

Devang A. Joshi, A. K. Nigam, S. K. Dhar, A. Thamizhavel

摘要:

报道了单晶RAu_{2} Ge_{2}(R = La,Ce,Pr)化合物的各向异性磁性。LaAu_{2} Ge_{2}表现出Pauli顺磁行为,而CeAu_{2} Ge_{2}和PrAu_{2} Ge_{2}表现出反铁磁有序,N \grave{e} el温度T_{N}分别为13.5和9 K。Ce和Pr化合物的各向异性磁响应确定[001]为易磁化轴,在磁性等温线中观察到尖锐的自旋翻转型变磁转变。这些化合物,特别是LaAu_{2} Ge_{2}的电阻和磁阻行为表明了各向异性费米表面。CeAu_{2} Ge_{2}的磁电阻率显然揭示了残余近藤相互作用的存在。晶体电场分析的各向异性的磁化率结合实验推断的肖特基热容量,使我们能够提出一个晶体电场水平计划的Ce和Pr化合物。对于CeAu_{2} Ge_{2},我们的值与以前关于中子衍射的报道非常一致。LaAu_{2} Ge_{2}的热容数据清楚地表明了爱因斯坦对热容的贡献。

英文摘要:

Anisotropic magnetic properties of single crystalline RAu_{2}Ge_{2} (R = La, Ce and Pr) compounds are reported. LaAu_{2}Ge_{2} exhibit a Pauli-paramagnetic behavior whereas CeAu_{2}Ge_{2} and PrAu_{2}Ge_{2} show an antiferromagnetic ordering with N\grave{e}el temperatures T_{N} = 13.5 and 9 K, respectively. The anisotropic magnetic response of Ce and Pr compounds establishes [001] as the easy axis of magnetization and a sharp spin-flip type metamagnetic transition is observed in the magnetic isotherms. The resistance and magnetoresistance behavior of these compounds, in particular LaAu_{2}Ge_{2}, indicate an anisotropic Fermi surface. The magnetoresistivity of CeAu_{2}Ge_{2} apparently reveals the presence of a residual Kondo interaction. A crystal electric field analysis of the anisotropic susceptibility in conjunction with the experimentally inferred Schottky heat capacity enables us to propose a crystal electric field level scheme for Ce and Pr compounds. For CeAu_{2}Ge_{2} our values are in excellent agreement with the previous reports on neutron diffraction. The heat capacity data in LaAu_{2}Ge_{2} show clearly the existence of Einstein contribution to the heat capacity.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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