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arXiv 0907.4572cond-mat.supr-concond-mat.mtrl-sci
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Holstein模型中的极化子质量和电子-声子关联

Polaron Mass and Electron-Phonon Correlations in the Holstein Model

Marco Zoli

摘要:

Holstein分子晶体模型研究了强耦合微扰方法,与标准的Lang-Firsov方法不同,该方法考虑了极化子尺寸扩展引起的延迟效应。计算的有效质量的第二微扰阶在任何晶格维数为广泛的(反)绝热制度和电子-声子耦合。从一个大的到一个小的极化子状态的交叉被发现在绝热和中间绝热制度的所有维度。声子色散在很大程度上平滑了这种交叉,这是由极化子质量增强和现场本地化的关联函数。自陷的概念与光极化子的存在条件,主要是在二维和三维,进行了讨论。通过虚时间路径积分形式主义,我展示了如何非本地的电子-声子的相关性,由于色散声子,向下重整化的{ \it e-ph}耦合证明光和基本上小的2D Holstein极化子的可能性。

英文摘要:

The Holstein Molecular Crystal Model is investigated by a strong coupling perturbative method which, unlike the standard Lang-Firsov approach, accounts for retardation effects due to the spreading of the polaron size. The effective mass is calculated to the second perturbative order in any lattice dimensionality for a broad range of (anti)adiabatic regimes and electron-phonon couplings. The crossover from a large to a small polaron state is found in all dimensionalities for adiabatic and intermediate adiabatic regimes. The phonon dispersion largely smooths such crossover which is signalled by polaron mass enhancement and on site localization of the correlation function. The notion of self-trapping together with the conditions for the existence of light polarons, mainly in two- and three-dimensions, are discussed. By the imaginary time path integral formalism I show how non local electron-phonon correlations, due to dispersive phonons, renormalize downwards the {\it e-ph} coupling justifying the possibility for light and essentially small 2D Holstein polarons.

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