Five-Fold Reduction of Lasing Threshold near the First $ΓL$-Pseudogap of ZnO Inverse Opals

Ultrafast all-optical gated amplifier based on ZnO nanowire lasing

We present an ultrafast all-optical gated amplifier, or transistor, consisting of a forest of ZnO nanowire lasers. A gate light pulse creates a dense electron-hole plasma and excites laser action inside the nanowires. Source light traversing the nanolaser forest is amplified, partly as it is guided through the nanowires, and partly as it propagates diffusively through the forest. We have measured transmission increases at the drain up to a factor 34 for 385-nm light. Time-resolved amplification measurements show that the lasing is rapidly self-quenching, yielding pulse responses as short as 1.…

Waveguiding-assisted random lasing in epitaxial ZnO thin film

Zinc Oxide thin films were grown on c-sapphire substrates using pulsed laser deposition. Pump power dependence of surface emission spectra, acquired using a quadrupled 266 nm laser, revealed room temperature stimulated emission (threshold of 900 kW/cm2). Time dependent spectral analysis plus gain measurements of single-shot, side-emission, spectra pumped with a nitrogen laser revealed random lasing indicative of the presence of self-forming laser cavities. It is suggested that random lasing in an epitaxial system rather than a 3-dimensional configuration of disordered scattering elements, was …

Carrier density driven lasing dynamics in ZnO nanowires

We report on the temporal lasing dynamics of high quality ZnO nanowires using time-resolved micro-photoluminescence technique. The temperature dependence of the lasing characteristics and of the corresponding decay constants demonstrate the formation of an electron-hole plasma to be the underlying gain mechanism in the considered temperature range from 10 K to 300 K. We found that the temperature dependent emission onset-time ($t_{\text{on}}$) strongly depends on the excitation power and becomes smallest in the lasing regime, with values below 5 ps. Furthermore, the observed red shift of the d…

Bi-functional nonlinearities in monodisperse ZnO nano-grains - Self-consistent transport and random lasing

We report a quantum field theoretical description of light transport and random lasing. The Bethe-Salpeter equation is solved including maximally crossed diagrams and non-elastic scattering. This is the first theoretical framework that combines so called off-shell scattering and lasing in random media. We present results for the self-consistent scattering mean free path that varies over the width of the sample. Further we discuss the density dependent correlation length of self-consistent transport in disordered media composed of semi-conductor Mie scatterers.

非线性等离子体随机激光器中的反常激射行为

Anomalous Lasing Behavior in a Nonlinear Plasmonic Random Laser

本文报道了Au纳米岛修饰ZnO纳米棒的等离子体随机激光器中由模式强耦合吸收与Au非线性光学效应共同导致的双阈值激射现象，并用统计方法验证了该行为。

Tuning nanowire lasers via hybridization with two-dimensional materials

Mixed dimensional hybrid structures have recently gained increasing attention as promising building blocks for novel electronic and optoelectronic devices. In this context, hybridization of semiconductor nanowires with two-dimensional materials could offer new ways to control and modulate lasing at the nanoscale. In this work, we deterministically fabricate hybrid mixed-dimensional heterostructures composed of ZnO nanowires and MoS2 monolayers with micrometer control over their relative position. First, we show that our deterministic fabrication method does not degrade the optical properties o…

Laser emission with excitonic gain in a ZnO planar microcavity

The lasing operation of a ZnO planar microcavity under optical pumping is demonstrated from T=80 K to 300 K. At the laser threshold, the cavity switches from the strong coupling to the weak coupling regime. A gain-related transition, which appears while still observing polariton branches and, thus, with stable excitons, is observed below 240K. This shows that exciton scattering processes, typical of II-VI semiconductors, are involved in the gain process.

Fabrication and Optical Properties of a Fully Hybrid Epitaxial ZnO-Based Microcavity in the Strong Coupling Regime

In order to achieve polariton lasing at room temperature, a new fabrication methodology for planar microcavities is proposed: a ZnO-based microcavity in which the active region is epitaxially grown on an AlGaN/AlN/Si substrate and in which two dielectric mirrors are used. This approach allows as to simultaneously obtain a high-quality active layer together with a high photonic confinement as demonstrated through macro-, and micro-photoluminescence (μ-PL) and reflectivity experiments. A quality factor of 675 and a maximum PL emission at k=0 are evidenced thanks to μ-PL, revealing an efficient p…

紫外混合等离激元纳米线激光器的尺寸依赖与衬底依赖性能的光学表征

Optical characterization of size- and substrate-dependent performance of ultraviolet hybrid plasmonic nanowire lasers

本文通过单纳米线光学表征与高通量PL光谱，研究Ag、Al衬底上ZnO纳米线紫外混合等离激元激光器，揭示衬底色散与纳米线直径对激子-表面等离激元耦合及器件性能的调控作用。

ZnO-Based Polariton Laser Operating at Room Temperature: From Excitonic to Photonic Condensate

A laser threshold is determined by the gain condition, which has been progressively reduced by the use of heterostructures and of quantum confinement. The polariton laser is the ultimate step of this evolution: coherent emission is obtained from the spontaneous decay of an exciton-polariton condensate, without the achievement of any gain condition. ZnO, with its unique excitonic properties, is the best choice for a blue/UV-emitting polariton laser device. We report on the fabrication of a new family of fully hybrid microcavities that combine the best-quality ZnO material available (bulk substr…

Low-threshold, highly stable colloidal quantum dot short-wave infrared laser enabled by suppression of trap-assisted Auger recombination

Pb-chalcogenide colloidal quantum dots (CQDs) are attractive materials to be used as tuneable laser media across the infrared spectrum. However, excessive nonradiative Auger recombination due to the presence of trap states outcompetes light amplification by rapidly annihilating the exciton population, leading to high gain thresholds. Here, we employ a binary blend of CQDs and ZnO nanocrystals in order to passivate the in-gap trap states of PbS-CQD gain medium. Using transient absorption, we measure a five-fold increase in Auger lifetime demonstrating the suppression of trap-assisted Auger reco…