The formation of rf-dressed Rydberg dark states in thermal Rb vapour is demonstrated. It is shown that such states exhibit enhanced sensitivity to dc electric fields compared to their bare counterparts and enable precise measurement of the dc field independent of laser frequency fluctuations.
We propose and demonstrate the laser cooling and trapping of Rydberg-dressed Sr atoms. By off-resonantly coupling the excited state of a narrow (7 kHz) cooling transition to a high-lying Rydberg state, we transfer Rydberg properties such as enhanced electric polarizability to a stable magneto-optical trap operating at $< 1 μK$. By increasing the density to $1 \times 10^{12} \rm{cm^{-3}}$, we show that it is possible to reach a regime where the long-range interaction between Rydberg-dressed atoms becomes comparable to the kinetic energy, opening a route to combining laser cooling with tunable l…
Atom-atom interactions within a small volume were investigated through the excitation of ultracold Rb atoms. The application of microwaves enhances these interactions, causing the suppression of Rydberg state excitation. The suppression of Rydberg atom excitation was both qualitatively observed and quantitatively analyzed using a universal scaling law, giving a measure of the atom-atom interaction strength in agreement with theoretical prediction.
The giant electro-optical response of Rydberg atoms manifests itself in the emergence of sidebands in the Rydberg excitation spectrum if the atom is exposed to a radio-frequency (RF) electric field. Here we report on the study of RF-dressed Rydberg atoms inside hollow-core photonic crystal fibres (HC-PCF), a system that enables the use of low modulation voltages and offers the prospect of miniaturised vapour-based electro-optical devices. Narrow spectroscopic features caused by the RF field are observed for modulation frequencies up to 500 MHz.
We consider two clouds of ground state alkali atoms in two distinct hyperfine ground states. Each level is far off-resonantly coupled to a Rydberg state, which leads to dressed ground states with a weak admixture of the Rydberg state properties. Due to this admixture, for a proper choice of the Rydberg states, the atoms experience resonant dipole-dipole interactions that induce mechanical forces acting on all atoms within both clouds. This behavior is in contrast to the dynamics predicted for bare dipole-dipole interactions between Rydberg superatoms, where only a single atom per cloud is subj…
We present the experimental realization and characterization of a Ramsey interferometer based on optically trapped ultracold potassium atoms, where one state is continuously coupled by an off-resonant laser field to a highly-excited Rydberg state. We show that the observed interference signals can be used to precisely measure the Rydberg atom-light coupling strength as well as the population and coherence decay rates of the Rydberg-dressed states with sub-kilohertz accuracy and for Rydberg state fractions as small as one part in $10^{6}$. We also demonstrate an application for measuring small,…
We perform a comprehensive investigation of the coupling between a Rydberg-dressed atomic gas and an ultra-cold plasma. Using simultaneous time-resolved measurements of both neutral atoms and ions, we show that plasma formation occurs via a Coulomb anti-blockade mechanism, in which background ions DC Stark shift nearby atoms into resonance at specific distances. The result is a highly correlated growth of the Rydberg population that shares some similarities with that previously observed for van der Waals interactions. We show that a rate equation model that couples the laser-driven Rydberg gas…
The non-linear and non-local effects in atomic Rydberg media under electromagnetically induced transparency (EIT) make it a versatile platform for fundamental studies and applications in quantum information. In this paper, we study the dynamics of a Rydberg-EIT system in an ensemble that allows for more than one Rydberg excitation in the propagation direction. The density of two-level atoms is such that transient superradiant effects occur. We experimentally observe a cross-over between coherent collective emission (`flash') of two-level atoms to a Rydberg dressed regime ('dressed flash') unde…
We theoretically analyze the interactions and decay rates for atoms dressed by multiple laser fields to strongly interacting Rydberg states using a quantum master equation approach. In this framework a comparison of two-level and three-level Rydberg-dressing schemes is presented. We identify a resonant enhancement of the three-level dressed interaction strength which originates from cooperative multiphoton couplings as well as small distance dependent decay rates. In this regime the soft-core shape of the potential is independent of the sign of the bare Rydberg-Rydberg interaction, while its s…
Stabilizing important physical quantities to atom-based standards lies at the heart of modern atomic, molecular and optical physics, and is widely applied to the field of precision metrology. Of particular importance is the atom-based microwave field amplitude stabilizer, the so-called atomic candle. Previous atomic candles are realized with atoms in their ground state, and hence suffer from the lack of frequency band tunability and small stabilization bandwidth, severely limiting their development and potential applications. To tackle these limitations, we employ microwave-dressed Rydberg ato…
We investigate the impact of an electric field on the structure of ultralong-range polar diatomic Rydberg molecules. Both the s-wave and p-wave interactions of the Rydberg electron and the neutral ground state atom are taken into account. In the presence of the electric field the angular degree of freedom between the electric field and the internuclear axis acquires vibrational character and we encounter two-dimensional oscillatory adiabatic potential energy surfaces with an antiparallel equilibrium configuration. The electric field allows to shift the corresponding potential wells in such a m…
We predict the existence of a universal class of ultralong-range Rydberg molecular states whose vibrational spectra form trimmed Rydberg series. A dressed ion-pair model captures the physical origin of these exotic molecules, accurately predicts their properties, and reveals features of ultralong-range Rydberg molecules and heavy Rydberg states with a surprisingly small Rydberg constant. The latter is determined by the small effective charge of the dressed anion, which outweighs the contribution of the molecule's large reduced mass. This renders these molecules the only known few-body systems …
We develop the research achievement of recent work [M. Gärttner, et.al., Phys. Rev. Letts. 113, 233002 (2014)], in which an anomalous excitation enhancement is observed in a three-level Rydberg-atom ensemble with many-body coherence. In our novel theoretical analysis, this effect is ascribed to the existence of a quasi-dark state as well as its avoided crossings to nearby Rydberg-dressed states. Moreover, we show that with an appropriate control of the optical detuning to the intermediate state, the enhancement can evoke a direct facilitation to atom-light coupling that even breaks through the…
We demonstrate finite range binding potentials between pairs of Rydberg atoms interacting with each other via attractive and repulsive van der Waals potentials and driven by a microwave field. We show that, using destructive quantum interference to cancel single-atom Rydberg excitation, the Rydberg-dimer states can be selectively and coherently populated from the two-atom ground state. This can be used to realize a two-qubit interaction gate which is not susceptible to mechanical forces between the atoms and is therefore immune to motional decoherence.
In Rydberg dressed ultra-cold gases, ground state atoms inherit properties of a weakly admixed Rydberg state, such as sensitivity to long-range interactions. We show that through hyperfine-state dependent interactions, a pair of atom clouds can evolve into a spin and subsequently into a spatial Schrödinger's cat state: The pair, containing 20 atoms in total, is in a coherent superposition of two configurations, with cloud locations separated by micrometers. The mesoscopic nature of the superposition state can be proven with absorption imaging, while the coherence can be revealed though recombi…
We study rotating quasi-two-dimensional Bose-Einstein-condensates, in which atoms are dressed to a highly excited Rydberg state. This leads to weak effective interactions that induce a transition to a mesoscopic supersolid state. Considering slow rotation, we determine its superfluidity using Quantum Monte-Carlo simulations as well as mean field calculations. For rapid rotation, the latter reveal an interesting competition between the supersolid crystal structure and the rotation-induced vortex lattice that gives rise to new phases, including arrays of mesoscopic vortex crystals.
We propose a method to realize the Frenkel-Kontorova model using an array of Rydberg dressed atoms. Our platform can be used to study this model with a range of realistic interatomic potentials. In particular, we concentrate on two types of interaction potentials: a springlike potential and a repulsive long-range potential. We numerically calculate the phase diagram for such systems and characterize the Aubry-like and commensurate-incommensurate phase transitions. Experimental realizations of this system that are possible to achieve using current technology are discussed.
We examine interactions between atoms continuously and coherently driven between the ground state and a Rydberg state, producing "Rydberg-dressed atoms." Because of the large dipolar coupling between two Rydberg atoms, a small admixture of Rydberg character into a ground state can produce an atom with a dipole moment of a few Debye, the appropriate size to observe interesting dipolar physics effects in cold atom systems. We have calculated the interaction energies for atoms that interact via the dipole-dipole interaction and find that due to blockade effects, the R-dependent two-atom interacti…
We show that ultracold chemical reactions can be manipulated and controlled by using Rydberg-dressed interactions. Scattering in the ultracold regime is sensitive to long-range interactions, especially when weakly bound (or quasi-bound) states exist near the collision threshold. We investigate how, by Rydberg-dressing a reactant, one enhances its polarizability and modifies the long-range van der Waals collision complex, which can alter chemical reaction rates by shifting the position of near threshold bound states. We carry out a full quantum mechanical scattering calculation for the benchmar…
We theoretically study trapped ions that are immersed in an ultracold gas of Rydberg-dressed atoms. By off-resonant coupling on a dipole-forbidden transition, the adiabatic atom-ion potential can be made repulsive. We study the energy exchange between the atoms and a single trapped ion and find that Langevin collisions are inhibited in the ultracold regime for these repulsive interactions. Therefore, the proposed system avoids recently observed ion heating in hybrid atom-ion systems caused by coupling to the ion's radio frequency trapping field and retains ultracold temperatures even in the pr…
We demonstrate that Ramsey spectroscopy can be used to observe Rydberg-dressed interactions. In contrast to many prior proposals, our scheme operates comfortably within experimentally measured lifetimes, and accesses a regime where quantum superpositions are crucial. The key idea is to build a spin-1/2 from one level that is Rydberg-dressed and another that is not. These levels may be hyperfine or long-lived electronic states. An Ising spin model governs the Ramsey dynamics, for which we derive an exact solution. Due to the structure of Rydberg interactions, the dynamics differs significantly …
We study the dynamics of an atomic Bose-Einstein condensate in an optical lattice in which the electronic groundstate of each atom is weakly coupled to a highly excited Rydberg state by a far off-resonant laser. This dressing induces a switchable effective soft-core interaction between groundstate atoms which, in the lattice, gives rise to on-site as well as long-range interaction terms. Upon switching on the dressing laser the Bose-Einstein condensate undergoes a nontrivial collapse and revival dynamics which can be observed in the interference pattern that is created after a release of the a…
Neutral atoms are building blocks of ground-up quantum many-body systems. Well-controlled and high-fidelity entangling gates are an essential component for realizing complex neutral atom architectures for quantum computing, quantum simulation, and measurement with precision better than the standard quantum limit. In this Letter we report the realization of a Mølmer-Sørensen unitary between two neutral atoms, based on adiabatic single-photon dressing to Rydberg levels. We show that this technique is highly robust to noise sources and experimental imperfections that have limited the fidelity of …
We study theoretically the deformation of the Fermi surface (FS) of a three-dimensional gas of Rydberg-dressed $^6$Li atoms. The laser dressing to high-lying Rydberg $D$ states results in angle-dependent soft-core-shaped interactions whose anisotropy is described by multiple spherical harmonics. We show that this can drastically modify the shape of the FS and that its deformation depends on the interplay between the Fermi momentum $k_F$ and the reciprocal momentum $\bar{k}$ corresponding to the characteristic soft-core radius of the dressing-induced potential. When $k_F< \bar{k}$, the dressed …
We study an architecture for implementing adiabatic quantum computation with trapped neutral atoms. Ground state atoms are dressed by laser fields in a manner conditional on the Rydberg blockade mechanism, thereby providing the requisite entangling interactions. As a benchmark we study the performance of a Quadratic Unconstrained Binary Optimization (QUBO) problem whose solution is found in the ground state spin configuration of an Ising-like model. We model a realistic architecture, including details of the atomic implementation, with qubits encoded into the clock states of 133Cs, effective B…
The effect of an ac modulation on a 2-level or 3-level system is studied theoretically. The absorption spectrum is calculated by solving the optical Bloch equations and is interpreted by reference to the Floquet quasienergy spectrum. The dependence of the absorption sidebands on the intensity of the coupling laser field in Rydberg systems submitted to a radio-frequency (rf) field is analysed in detail. It is shown that for sufficiently strong coupling fields additional sidebands appear in the probe absorption spectrum in ladder 3-level systems. These additional sidebands are induced by the cou…
Controlling quantum entanglement between parts of a many-body system is the key to unlocking the power of quantum information processing for applications such as quantum computation, high-precision sensing, and simulation of many-body physics. Spin degrees of freedom of ultracold neutral atoms in their ground electronic state provide a natural platform given their long coherence times and our ability to control them with magneto-optical fields, but creating strong coherent coupling between spins has been challenging. We demonstrate a Rydberg-dressed ground-state blockade that provides a strong…
Measurement-based quantum computing relies on the rapid creation of large-scale entanglement in a register of stable qubits. Atomic arrays are well suited to store quantum information, and entanglement can be created using highly-excited Rydberg states. Typically, isolating pairs during gate operation is difficult because Rydberg interactions feature long tails at large distances. Here, we engineer distance-selective interactions that are strongly peaked in distance through off-resonant laser coupling of molecular potentials between Rydberg atom pairs. Employing quantum gas microscopy, we veri…
Trapping potentials and quantum gates for microwave-dressed Rydberg atoms on an atom chip
Freie Universität Berlin(柏林自由大学);Center for Quantum Science and Technologies, FORTH(量子科学与技术中心,FORTH);University of Crete(克里特大学);German Research Center for Artificial Intelligence(德国人工智能研究中心);Eberhard Karls Universität Tübingen(蒂宾根大学)
Charge dynamics in an ultra-cold setup involving a laser dressed atom and an ion is studied here. This transfer of charge is enabled through molecular Rydberg states that are accessed via a laser. The character of the charge exchange crucially depends on the coupling between the electronic dynamics and the vibrational motion of the atoms and ion. The molecular Rydberg states are characterized and a criterion for distinguishing coherent and incoherent regimes is formulated. Furthermore the concept is generalized to the many-body setup as the ion effectively propagates through a chain of atoms. …
We investigate the transport of excitations through a chain of atoms with non-local dissipation introduced through coupling to additional short-lived states. The system is described by an effective spin-1/2 model where the ratio of the exchange interaction strength to the reservoir coupling strength determines the type of transport, including coherent exciton motion, incoherent hopping and a regime in which an emergent length scale leads to a preferred hopping distance far beyond nearest neighbors. For multiple impurities, the dissipation gives rise to strong nearest-neighbor correlations and …
Comment on "Determining angle of arrival of radio-frequency fields using subwavelength, amplitude-only measurements of standing waves in a Rydberg atom sensor"
We propose a technique for engineering momentum-dependent dissipation in Bose-Einstein condensates with non-local interactions. The scheme relies on the use of momentum-dependent dark-states in close analogy to velocity-selective coherent population trapping. During the short-time dissipative dynamics, the system is driven into a particular finite-momentum phonon mode, which in real space corresponds to an ordered structure with non-local density-density correlations. Dissipation-induced ordering can be observed and studied in present-day experiments using cold atoms with dipole-dipole or off-…
Dynamic control of atomic dressing to the highly-excited Rydberg state in multi-level systems has special appeals owing to the development of flexible and precise measurement. In this study we develop an experimentally-accessible proposal to robustly control the dressing probability via a three-step cascaded excitation with double electromagnetically induced transparency (EIT) technique. The system can function as an optical switch where the third addressing laser serving as the control knob can switchably engineer the dressing probability with time. Differing from a conventional two-photon EI…
Recent experiments have illustrated that long range two-body interactions can be induced by laser coupling atoms to highly excited Rydberg states. Stimulated by this achievement, we study supersolidity of lattice bosons in an experimentally relevant situation. In our setup, we consider two-component atoms on a square lattice, where one species is weakly dressed to an electronically high-lying (Rydberg) state, generating a tunable, soft-core shape long-range interaction. Interactions between atoms of the second species and between the two species are characterized by local inter- and intra-spec…
We study the dynamics of bosonic atoms on a two-dimensional square lattice, where atomic interactions are long-ranged with either a box or soft-core shape. The latter can be realized through laser dressing ground-state atoms to electronically excited Rydberg states. When the range of interactions is equal or larger than the lattice constant, the system is governed by an extended Bose-Hubbard model. We propose a quench process by varying the atomic hopping linearly across phase boundaries of the Mott insulator-supersolid and supersolid-superfluid phases. Starting from a Mott insulating state, t…
Extended Hubbard models have proven to bear novel quantum states, but their experimental realization remains challenging. In this work we propose to use bosonic quantum gases dressed with molecular bound states in Rydberg interaction potentials for the observation of these quantum states. We study the molecular Rabi coupling with respect to principal quantum number and trapping frequency of the ground state atoms for various molecular potentials of Rubidium and Potassium, and the hereby resulting dressed interaction strength. Additionally, we propose a two-color excitation scheme which signifi…
Non-resonant dressing fields can make the transition frequency between two circular Rydberg states insensitive to second order variations in the dc electric field. Perturbation theory can be used to establish the required dressing field amplitude and frequency. The same perturbative approach may be used to understand removal of the first order dependence of the transition frequency on electric field about a bias dc electric field [Hyafil et al. Phys. Rev. Lett., v. 93, 103001 (2004)]. The directional alignment of the dressing and dc fields is critical in determining the electric field sensitiv…
We experimentally studied the Rydberg level shift caused by the electric field, which is generated by Rydberg atom collision induced ionization in a cesium atomic ensemble. The density of charged particles caused by collisions between Rydberg atoms is changed by controlling the ground-state atomic density and optical excitation process. We measured the Rydberg level shift using Rydberg electromagnetically-induced-transparency (EIT) spectroscopy, and interpreted the physical origin using a semi-classical model. The experimental results are in good agreement with the numerical simulation. These …
We explore the external electric field control of a species of ultralong-range molecules that emerge from the interaction of a ground state polar molecule with a Rydberg atom. The external field mixes the Rydberg electronic states and therefore strongly alters the electric field seen by the polar diatomic molecule due to the Rydberg electron. As a consequence, the adiabatic potential energy curves responsible for the molecular binding can be tuned in such a way that an intersection with neighboring curves occurs. The latter leads to admixture of s-wave character in the Rydberg wave function an…
Rydberg states of atomic helium with principal quantum numbers ranging from n=20 to n=100 have been prepared by non-resonance-enhanced single-color two-photon excitation from the metastable 2 {^3}S{_1} state. Photoexcitation was carried out using linearly and circularly polarized pulsed laser radiation. In the case of excitation with circularly polarized radiation, Rydberg states with azimuthal quantum number |m_{\ell}|=2 were prepared in zero electric field, and in homogeneous electric fields oriented parallel to the propagation axis of the laser radiation. In sufficiently strong electric fie…
Dipole-dipole interactions between helium atoms in Rydberg-Stark states with principal quantum number $n=53$ and approximately linear Stark energy shifts, resulting from induced electric dipole moments of approximately 7900 D, have been investigated experimentally. The experiments were performed in pulsed supersonic metastable helium beams, with particle number densities of up to $\sim10^9$ cm$^{-3}$. In the presence of amplitude-modulated, radio-frequency electric fields, changes in the spectral intensity distributions associated with the transitions to these states that are attributed to dip…
High resolution laser Stark excitation of np (60 < n < 85) Rydberg states of ultra-cold cesium atoms shows an efficient blockade of the excitation attributed to long-range dipole-dipole interaction. The dipole blockade effect is observed as a quenching of the Rydberg excitation depending on the value of the dipole moment induced by the external electric field. Effects of eventual ions which could match the dipole blockade effect are discussed in detail but are ruled out for our experimental conditions. Analytic and Monte-Carlo simulations of the excitation of an ensemble of interacting Rydberg…
Resonant electric dipole-dipole interactions between cold Rydberg atoms were observed using microwave spectroscopy. Laser-cooled Rb atoms in a magneto-optical trap were optically excited to 45d Rydberg states using a pulsed laser. A microwave pulse transferred a fraction of these Rydberg atoms to the 46p state. A second microwave pulse then drove atoms in the 45d state to the 46d state, and was used as a probe of interatomic interactions. The spectral width of this two-photon probe transition was found to depend on the presence of the 46p atoms, and is due to the resonant electric dipole-dipol…
We demonstrate a continuous frequency electric field measurement based on the far off-resonant AC stark effect in a Rydberg atomic vapor cell. In this configuration, a strong far off-resonant field, denoted as a local oscillator (LO) field, acts as a gain shifting the Rydberg level to a high sensitivity region. An incident weak signal field with a few hundreds of kHz difference from the LO field is mixed with the LO field in Rydberg system to generate an intermediate frequency (IF) signal, which is read out by the Rydberg electromagnetically induced transparency (Rydberg-EIT) spectroscopy. Not…
Resonant energy transfer between cold Rydberg atoms was used to determine Rydberg atom energy levels, at precisions approaching those obtainable in microwave spectroscopy. Laser cooled Rb atoms from a magneto-optical trap were optically excited to 32d Rydberg states. The two-atom process 32d(j=5/2) + 32d(j=5/2) -> 34p(j=3/2) + 30g is resonant at an electric field of approximately 0.3 V/cm. This process is driven by the electric dipole-dipole interaction, which is allowed due to the partial f character that the g state acquires in an electric field. The experimentally observed resonant field, t…