A nonclassical light source is used to demonstrate experimentally the absolute efficiency calibration of a photon-number-resolving detector. The photon-pair detector calibration method developed by Klyshko for single-photon detectors is generalized to take advantage of the higher dynamic range and additional information provided by photon-number-resolving detectors. This enables the use of brighter twin-beam sources including amplified pulse pumped sources, which increases the relevant signal and provides measurement redundancy, making the calibration more robust.
A method for absolute calibration of a photon-number resolving detector producing analog signals as the output is developed using a twin beam. The method gives both analog-to-digital conversion parameters and quantum detection efficiency for the photon fields. Characteristics of the used twin beam are also obtained. A simplified variant of the method applicable to fields with high signal to noise ratios and suitable for more intense twin beams is suggested.
The scheme for building stronger multi-mode twin beams from a greater number of identical twin beams sufficiently weak so that single-photon sensitive on/off detectors suffice in their detection is studied. Statistical properties of these compound twin beams involving the non-classicality are analyzed for intensities up to hundreds of photon pairs. Their properties are compared with those of the genuine twin beams that require photon-number-resolving detectors in their experimental investigations. The use of such compound twin beams for the generation of sub-Poissonian light and measurement of…
We generate nonclassical conditional states by exploiting the quantum correlations of multi-mode twin-beam states endowed with a sizeable number of photons. A strong relation between the sub-shot-noise correlations exhibited by twin beams and the sub-Poissonian character of the conditional states is experimentally revealed. It determines optimal conditions for sub-Poissonian light generation.
A method for the determination of absolute quantum detection efficiency is suggested based on the measurement of photocount statistics of twin beams. The measured histograms of joint signal-idler photocount statistics allow to eliminate an additional noise superimposed on an ideal calibration field composed of only photon pairs. This makes the method superior above other approaches presently used. Twin beams are described using a paired variant of quantum superposition of signal and noise.
We report on the absolute calibration of a CCD camera by exploiting quantum correlation. This novel method exploits a certain number of spatial pairwise quantum correlated modes produced by spontaneous parametric-down-conversion. We develop a measurement model taking into account all the possible source of losses and noise that are not related to the quantum efficiency,accounting for all the uncertainty contributions, and we reach the relative uncertainty of 0.3% in low photon flux regime. This represents a significant step forward for the characterizaion of (scientific) CCDs used in mesoscopi…
The variance of difference of photocounts (VDPs) is an established measure of quantum correlations for quantum states of light. It enables us to discriminate between the classical correlation of a two-mode coherent state and the quantum correlation of a twin-beam state. We study the effect of loss and saturation of the photon-number-resolving detector on the measurement of the VDPs. An analytic function is derived for this variance, both for the coherent and the twin-beam states. It is found that the VDPs is no longer a reliable entanglement measure in the nonlinear regime of the detector resp…
We present improved method of sending-or-not-sending twin-field quantum key distribution (SNS TF-QKD) based on its structure and the application of error rejection. %And we present iteration formula for bit-flip error rate of the survived bits after error rejection. Taking the finite key effect into consideration with only $10^{11}$ total pulses, we show that the method here exceeds the absolute limit of repeater-less key rate with whatever detection efficiency. We also make comparative study of different protocols numerically. It shows that the method here presents advantageous results at lon…
Single-photon detectors are widely used in modern quantum optics experiments and applications. Like all detectors, it is important for these devices to be accurately calibrated. A single-photon detector is calibrated by determining its detection efficiency; the standard method to measure this quantity requires comparison to another detector. Here, we suggest a method to measure the detection efficiency of a single photon detector without requiring an external reference detector. Our method is valid for individual single-photon detectors as well as multiplexed detectors, which are known to be p…
The aim of this review paper is to enlighten some recent progresses in quantum optical metrology in the part of quantum efficiency measurements of photo-detectors performed with bi-photon states. The intrinsic correlated nature of entangled photons from Spontaneous Parametric Down Conversion phenomenon has opened wide horizons to a new approach for the absolute measurement of photo-detector quantum efficiency, outgoing the requirement for conventional standards of optical radiation; in particular the simultaneous feature of the creation of conjugated photons led to a well known technique of co…
Well characterized photon number resolving detectors are a requirement for many applications ranging from quantum information and quantum metrology to the foundations of quantum mechanics. This prompts the necessity for reliable calibration techniques at the single photon level. In this paper we propose an innovative absolute calibration technique for photon number resolving detectors, using a pulsed heralded photon source based on parametric down conversion. The technique, being absolute, does not require reference standards and is independent upon the performances of the heralding detector. …
Detector stochastic deviations from an ideal response can hamper the measurement of quantum properties of light especially in the mesoscopic regime where photon-number resolution is required. We demonstrate that, by a proper analysis of the output signal, nonclassicality of twin-beam states can be detected and exploited with commercial and cost effective silicon-based photon-number-resolving detectors.
Joint photocount distributions of a weak twin beam acquired by an iCCD camera are analyzed with respect to the beam spatial correlations. A method for extracting these correlations from the experimental joint photocount distributions is suggested using a suitable statistical model that quantifies the contribution of spatial correlations to the joint photocount distributions. In detail, the profile of twin-beam intensity spatial cross-correlation function is revealed from the curve that gives the genuine mean photon-pair number (both photons from a pair are detected) as a function of the extent…
Numerous inequalities involving moments of integrated intensities and revealing nonclassicality and entanglement in bipartite optical fields are derived using the majorization theory, non-negative polynomials, the matrix approach, as well as the Cauchy-Schwarz inequality. Different approaches for deriving these inequalities are compared. Using the experimental photocount histogram generated by a weak noisy twin beam monitored by a photon-number-resolving iCCD camera the performance of the derived inequalities is compared. A basic set of ten inequalities suitable for monitoring the entanglement…
We propose a new method to measure the absolute photon absorption cross section of neutral molecules in a molecular beam. It is independent of our knowledge of the particle beam density, nor does it rely on photo-induced fragmentation or ionization. The method is based on resolving the recoil resulting from photon absorption by means of near-field matter-wave interference, and it thus applies even to very dilute beams with low optical densities. Our discussion includes the possibility of internal state conversion as well as fluorescence. We assess the influence of various experimental uncertai…
The problem of on-demand generation of entanglement between single-atom qubits via a common photonic channel is examined within the framework of optical interferometry. As expected, for a Mach-Zehnder interferometer with coherent laser beam as input, a high-finesse optical cavity is required to overcome sensitivity to spontaneous emission. We show, however, that with a twin-Fock input, useful entanglement can in principle be created without cavity-enhancement. Both approaches require single-photon resolving detectors, and best results would be obtained by combining both cavity-feedback and twi…
A non-classical light source emitting pairs of identical photons represents a versatile resource of interdisciplinary importance with applications in quantum optics and quantum biology. Emerging research fields, which benefit from such type of quantum light source, include quantum-optical spectroscopy or experiments on photoreceptor cells sensitive to photon statistics. To date, photon twins have mostly been generated using parametric downconversion sources, relying on Poissonian number distributions, or atoms, exhibiting low emission rates. Here, we propose and experimentally demonstrate the …
Two twin beams with a shared signal beam and separated idler beams are used together with the photon-number-resolving postselection in the signal beam to arrive at two coupled beams with anticorrelations in photon-number fluctuations. Moreover, the beams exhibit the sub-Poissonian photon-number statistics in their marginal distributions under suitable conditions. The postselected fields with the increasing mean photon numbers are reconstructed from the experimental photocount histograms by the maximum likelihood approach. Also a suitable Gaussian fit of both original twin beams and simulation …
Due to their strict photon-number correlation, the twin beams produced in parametric down-conversion (PDC) work well for heralded state generation. Often, however, this state manipulation is distorted by the optical losses in the herald and by the higher photon-number contributions inevitable in the PDC process. In order to find feasible figures of merit for characterizing the heralded states, we investigate their normalized factorial moments of the photon number that can be accessed regardless of the optical losses in the detection. We then perform a measurement of the joint photon statistics…
We show that quantum mechanics predicts a contradiction with local hidden variable theories for photon number measurements which have limited resolving power, to the point of imposing an uncertainty in the photon number result which is macroscopic in absolute terms. We show how this can be interpreted as a failure of a new premise, macroscopic local realism.
We present a novel interferometric technique for performing ellipsometric measurements. This technique relies on the use of a non-classical optical source, namely, polarization-entangled twin photons generated by spontaneous parametric down-conversion from a nonlinear crystal, in conjunction with a coincidence-detection scheme. Ellipsometric measurements acquired with this scheme are absolute; i.e., they do not require source and detector calibration.
Loss measurements are at the base of spectroscopy and imaging, thus perme- ating all the branches of science, from chemistry and biology to physics and material science. However, quantum mechanics laws set the ultimate limit to the sensitivity, constrained by the probe mean energy. This can be the main source of uncertainty, for example when dealing with delicate system such as biological samples or photosensitive chemicals. It turns out that ordinary (clas- sical) probe beams, namely with Poissonian photon number distribution, are fundamentally inadequate to measure small losses with the high…
Performing reliable measurements in optical metrology, such as those needed in ellipsometry, requires a calibrated source and detector, or a well-characterized reference sample. We present a novel interferometric technique to perform reliable ellipsometric measurements. This technique relies on the use of a non-classical optical source, namely polarization-entangled twin photons generated by spontaneous parametric downconversion from a nonlinear crystal, in conjunction with a coincidence-detection scheme. Ellipsometric measurements acquired with this scheme are absolute, i.e., they require nei…
This paper's purpose is to review the results recently obtained in the Quantum Optics labs of the National Institute of Metrological Research (INRIM) in the field of single- and few-photon detectors calibration, from both the classical and quantum viewpoint. In the first part of the paper is presented the calibration of a single-photon detector with absolute methods, while in the second part we focus on photon-number-resolving detectors, discussing both the classical and quantum characterization of such devices.
The measurement of circular dichroism (CD) has widely been exploited to distinguish the different enantiomers of chiral structures. It has been applied to natural materials (e.g. molecules) as well as to artificial materials (e.g. nanophotonic structures). However, especially for chiral molecules the signal level is very low and increasing the signal-to-noise ratio is of paramount importance to either shorten the necessary measurement time or to lower the minimum detectable molecule concentration. As one solution to this problem, we propose here to use quantum states of light in CD sensing to …
