We performed scanning tunneling spectroscopy of c-axis oriented YBCO films on top of which ferromagnetic SRO islands were grown epitaxially in-situ. When measured on the ferromagnetic islands, the density of states exhibits small gap-like features consistent with the expected short range penetration of the order parameter into the ferromagnet. However, anomalous split-gap structures are measured on the superconductor in the vicinity of ferromagnetic islands. This observation may provide evidence for the recently predicted induced magnetization in the superconductor side of a superconductor/ ferromagnet junction. The length scale of the effect inside the superconductor was found to be an order of magnitude larger than the superconducting coherence length. This is inconsistent with the theoretical prediction of a penetration depth of only a few superconducting coherence lengths. We discuss a possible origin for this discrepancy.
In this work, we study the spin transport at the Ferromagnet$|$Noncentrosymmetric Superconductor (F$|$NCSC) junction of a Ferromagnet$|$Noncentrosymmetric Superconductor$|$Ferromagnet (F$|$NCSC$|$F) spin valve. We investigate the Tunnelling Spin-Conductance (TSC), spin current and Spin Tunnelling Magneto-Resistance (STMR), and their dependence on various important parameters like Rashba Spin-Orbit Coupling (RSOC), strength and orientation of magnetization, an external in-plane magnetic field, barrier strength and a significant Fermi Wavevector Mismatch (FWM) at the ferromagnetic and supercondu…
In this paper, we study the quantum transport at the Ferromagnet$|$Noncentrosymmetric Superconductor (F$|$NCSC) interface of an F$|$S$|$F spin valve. In this context, we investigate the tunneling conductance and its dependence on Rashba Spin-Orbit Coupling (RSOC) considering different barrier strength and a significant Fermi Wave-vector Mismatch (FWM) at the ferromagnetic and superconducting regions. The study is carried out for different magnetization orientations and its strength. We developed Bogoliubov de Gennes (BdG) Hamiltonian introducing RSOC and exchange interaction for such an hybrid…
We have measured the tunnelling current in Nb/Nb$_x$O$_y$/Ni planar tunnel junctions at different temperatures. The junctions are in the intermediate transparency regime. We have extracted the current polarization of the metal/ferromagnet junction without applying a magnetic field. We have used a simple theoretical model, that provides consistent fitting parameters for the whole range of temperatures analyzed. We have also been able to gain insight into the microscopic structure of the oxide barriers of our junctions.%
We propose a novel platform for the creation and manipulation of Majorana zero modes consisting of a ferromagnetic metallic wire placed between conventional superconductors which are in proximity to ferromagnetic insulators. Our device relies on the interplay of applied supercurrents and exchange fields emerging from the ferromagnetic insulators. We assert that the proposed superconductor/ferromagnet heterostructures exhibit enhanced controllability, since topological superconductivity can be tuned apart from gate voltages applied on the ferromagnetic wire, also by manipulating the applied sup…
A normal conductor placed in good contact with a superconductor can inherit its remarkable electronic properties. This proximity effect microscopically originates from the formation in the conductor of entangled electron-hole states, called Andreev states. Spectroscopic studies of Andreev states have been performed in just a handful of systems. The unique geometry, electronic structure and high mobility of graphene make it a novel platform for studying Andreev physics in two dimensions. Here we use a full van der Waals heterostructure to perform tunnelling spectroscopy measurements of the prox…
Heterostructures made of itinerant ferromagnets and superconductors are studied. In contrast to most previous models, ferromagnetism is not enforced as an external Zeeman field but induced in a correlated single-band model (CSBM) that displays itinerant ferromagnetism as a mean-field ground state. This allows us to investigate the influence of an adjacent superconducting layer on the properties of the ferromagnet in a self-consistent Bogoliubov-de Gennes approach. The CSBM displays a variety features not present in the Zeeman exchange model that influence the behavior of order parameters close…
We present a theoretical study of spin screening effects in a ferromagnet/superconductor (F/S) heterojunction. It is shown that the magnetic moment of the ferromagnet is screened or antiscreened, depending on the polarization of the electrons at the Fermi level. If the polarization is determined by the electrons of the majority (minority) spin band then the magnetic moment of the ferromagnet is screened (antiscreened) by the electrons in the superconductor. We propose experiments that may confirm our theory: for ferromagnetic alloys with certain concentration of Fe or Ni ions there will be scr…
We study the shift of the the superconducting transition temperature $T_c$ in ferromagnetic-superconducting bi-layers and in a superconducting film supplied a square array of ferromagnetic dots. We find that the transition temperature in these two cases change presumably in opposite direction and that its change is not too small. We extend these results to multilayer structures. We predict that rather small external magnetic field $\sim 10$ Oe can change the transition temperature of the bilayer by 10% .
At the interface between a superconductor and a ferromagnetic metal spin-singlet Cooper pairs can penetrate into the ferromagnetic part of the heterostructure with an oscillating and decaying spin-singlet Cooper pair density. However, if the interface allows for a spin-mixing effect, equal-spin spin-triplet Cooper pairs can be generated that can penetrate much further into the ferromagnetic part of the heterostructure, known as the long-range proximity effect. Here, we present results of spin-mixing based on self-consistent solutions of the microscopic Bogoliubov-de Gennes equations incorporat…
Coexistence of ferromagnetic and superconducting orders and their interplay in ferromagnet-superconductor heterostructures is a topic of intense research. While it is well known that proximity of a ferromagnet suppresses superconducting order in the superconductor, there exist few studies indicating the proximity of a superconductor suppressing ferromagnetic order in a ferromagnet. Here we demonstrate a rare observation of the suppression of ferromagnetic order in a LaCaMnO3 layer separated from a YBa2Cu3O7-δ layer by a thin insulator (SrTiO3). Polarized neutron reflectivity measurements on La…
The theory of superconductivity developed by Bardeen, Cooper and Schrieffer (BCS) explains the stabilization of electron pairs into a spin-singlet, even frequency, state by the formation of an energy gap within which the density of states is zero. At a superconductor interface with an inhomogeneous ferromagnet, a gapless odd frequency superconducting state is predicted, in which the Cooper pairs are in a spin-triplet state. Although indirect evidence for such a state has been obtained, the gap structure and pairing symmetry have not so far been determined. Here we report scanning tunnelling sp…
Thin film heterostructures provide a powerful means to study the antagonism between superconductivity (SC) and ferromagnetism (FM). One interesting issue in FM-SC hybrids which defies the notion of antagonistic orders is the observation of magnetic field induced superconductivity (FIS). Here we show that in systems where the FM domains/islands produce spatial inhomogeneities of the SC order parameter, the FIS can derive significant contribution from different mobilities of the magnetic flux identified by two distinct critical states in the inhomogeneous superconductor. Our experiments on nanoe…
First experimental observations of the ferromagnetic shielding effect in high-Tc superconducting coated conductors were carried out. Experimental results were compared to simulations calling upon finite-element calculations based on the H-formulation of Maxwell equations to model superconducting strips with ferromagnetic shields. Samples of copper-stabilized coated conductors were electroplated with nickel shields and afterwards characterized. Both externally applied oscillating transverse magnetic fields as well as transport currents were studied. Having observed promising gains with respect …
Superconductor/ferromagnet/superconductor heterostructures exhibit a so-called long-range proximity effect provided some layers of conical magnet Holmium are included in the respective interface regions. The Ho layers lead to a spin-flip process at the interface generating equal-spin spin-triplet pairing correlations in the ferromagnet. These equal-spin spin-triplet pairing correlations penetrate much further into the heterostructure compared to the spin-singlet and unequal-spin spin-triplet correlations which occur in the absence of Ho. Here we present calculations of this effect based on the…
Superconductor/ferromagnet (S/F) proximity effect theory predicts that the superconducting critical temperature of the F1/F2/S or F1/S/F2 trilayers for the parallel orientation of the F1 and F2 magnetizations is smaller than for the antiparallel one. This suggests a possibility of a controlled switching between the superconducting and normal states in the S layer. Here, using the spin switch design F1/F2/S theoretically proposed by Oh et al. [Appl. Phys. Lett. 71, 2376 (1997)], that comprises a ferromagnetic bilayer separated by a non-magnetic metallic spacer layer as a ferromagnetic component…
Based on the technique of quasiclassical Green's functions, we construct a theoretical framework for describing heterostructures consisting of superconductors and/or spin-polarized materials. The necessary boundary conditions at the interfaces separating different metals are formulated in terms of hopping amplitudes in a t-matrix approximation. The theory is applicable for an interface with arbitrary transmission and exhibiting scattering with arbitrary spin dependence. Also, it can be used in describing both ballistic and diffusive systems. We establish the connection between the standard sca…
In a setup where two ferromagnetic electrodes are attached to a superconductor, Andreev bound states are induced at both ferromagnet/superconductor (FM/SC) interfaces. We study how these states propagate through the SC and interact with each other. As a result of this interaction, the energetic positions of the Andreev states are not anymore determined solely by the magnetic properties of a single interface, but also depend on the interface distance and the relative magnetization orientation of the FM contacts. We discuss how these bound states show up as distinct peaks in the nonlocal conduct…
Ferromagnetic half-metal Co$_2$CrAl films and tunnel contacts Co$_2$CrAl - insulator (I) - Pb are fabricated and investigated. It is found that the normalized differential conductivity $σ^{\rm FS} $ of such tunnel junctions with low resistance is larger than the normalized differential conductivity $σ^{\rm NS} $ of known normal metal - I - superconductor type tunnel junctions. It is shown that the observed increase in $σ^{\rm FS} $ is caused by the accumulation of spin polarized electrons in a superconductor and can be used for estimating the spin polarization degree $P$ in ferromagnets. This …
We study the Josephson effect in clean heterojunctions that consist of superconductors connected through two metallic ferromagnets with insulating interfaces. We solve the scattering problem based on the Bogoliubov--de Gennes equation for any relative orientation of in-plane magnetizations, arbitrary transparency of interfaces, and mismatch of Fermi wave vectors. Both spin singlet and triplet superconducting correlations are taken into account, and the Josephson current is calculated as a function of the ferromagnetic layers thicknesses and of the angle $α$ between their magnetizations. We fin…
We have studied the local critical current density, jc, in the superconductor thin film of bilayer structures consisting of YBa2Cu3O7 and the ferromagnets La2/3Ca1/3MnO3 and SrRuO3, respectively, by means of quantitative magneto-optics. A pronounced hysteresis of jc was observed which is ascribed to the magnetization state of the ferromagnetic layer. The results are discussed within the frame of magnetic vortex - wall interactions.
Nanostructured superconductor/ferromagnet heterocontacts are studied in the different transport regimes of point-contact spectroscopy. Direct measurements of the nanocontact size by scanning electron microscopy allow a comparison with theoretical models for contact-size estimates of heterocontacts. Our experimental data give evidence that size estimates yield reasonable values for the point-contact diameter $d$ as long as the samples are carefully characterized with respect to the local electronic parameters.
The interplay between superconductivity and ferromagnetism in the superconductor/ferromagnet (SC/FM) heterostructures generates many interesting physical phenomena, including spin-triplet superconductivity, superconducting order parameter oscillation, and topological superconductivity. The unique physical properties make the SC/FM heterostructures as promising platforms for future superconducting spintronics and quantum computation applications. In this article, we review important research progress of SC/FM heterostructures from superconducting spintronics to quantum computation, and it is or…
We study spectroscopic properties of ferromagnetic-superconductor heterostructures with strong spin-orbit coupling of the Rashba type and in the presence of exchange fields. The superconducting layer (film) experiences both an intrinsic spin-orbit field and an exchange field due to the proximity to ferromagnetic layers (films). We analyse the temperature dependence of the order parameter for superconductivity at various values of exchange field and spin-orbit coupling, and describe momentum-dependent properties that exhibit parity violation. Furthermore, we show that parity violation can be pr…
We provide a derivation of a spin Skyrmion number classification for two-dimensional topological superconductors constructed from ferromagnetic and Rashba spin-orbit coupled semiconductor-superconductor heterostructures. We show that in the non-trivial topological phase, characterized by a non-zero Chern number, there is always a topological spin texture in the occupied bands represented by a Skyrmion number. The Skyrmion number has the advantage of being both physically intuitive and directly measurable using spin-sensitive band structure imaging techniques. In addition, we show that the Skyr…
The very special characteristic of the proximity effect in superconductor-ferromagnet systems is the damped oscillatory behavior of the Cooper pair wave function in a ferromagnet. In some sense, this is analogous to the inhomogeneous superconductivity, predicted long time ago by Larkin and Ovchinnikov (1964), and Fulde and Ferrell (1964), and constantly searched since that. After the qualitative analysis of the peculiarities of the proximity effect in the presence of the exchange field, the author provides a unified description of the properties of the superconductor-ferromagnet heterostructur…
A novel state is predicted for a S/F heterostructure. It is shown that the equilibrium F/S bilayer can be in a bistable state: one state is ground and the other is metastable. One of these states is always normal and the other is superconducting. One can switch between these states by an external control parameter, for example, by an applied magnetic field. This phenomenon can manifest itself through the hysteresis behavior upon varying the applied magnetic field or, even, temperature. It can also lead to transition of the heterostructure into the superconducting state upon increase of the tem…
Employment of the non-trivial proximity effect in superconductor/ferromagnet (S/F) heterostructures for the creation of novel superconducting devices requires accurate control of magnetic states in complex thin-film multilayers. In this work, we study experimentally in-plane transport properties of microstructured Nb/Co multilayers. We apply various transport characterization techniques, including magnetoresistance, Hall effect, and the first-order-reversal-curves (FORC) analysis. We demonstrate how FORC can be used for detailed in situ characterization of magnetic states. It reveals that upon…
We review the present status of the experimental and theoretical research on the proximity effect in heterostructures composed of superconducting (S) and ferromagnetic (F) thin films. First, we discuss traditional effects originating from the oscillatory behavior of the superconducting pair wave function in the F-layer. Then, we concentrate on recent theoretical predictions for S/F layer systems. These are a) generation of odd triplet superconductivity in the F-layer and b) ferromagnetism induced in the S-layer below the superconducting transition temperature $T_{c}$ (inverse proximity effect)…
