By investigating the quantum properties of magnetically trapped nS Rydberg atoms, it is demonstrated that the composite nature of Rydberg atoms significantly alters their trapping properties opposed to point-like particles with the same magnetic moment. We show how the specific signatures of the Rydberg trapping potential can be probed by means of ground state atoms that are off-resonantly coupled to the Rydberg state via a two photon laser transition. In addition, it is demonstrated how this approach provides new possibilities for generating traps for ground state atoms. Simulated time-of-flight pictures mirroring the experimental situation are provided.
We explore the possibility to trap Rydberg atoms in tightly confining magnetic microtraps. The trapping frequencies for Rydberg atoms are expected to be influenced strongly by magnetic field gradients. We show that there are regimes where Rydberg atoms can be trapped. Moreover, we show that so-called magic trapping conditions can be found for certain states of rubidium, where both Rydberg atoms and ground state atoms have the same trapping frequencies. Magic trapping is highly beneficial for implementing quantum gate operations that require long operation times.
Intensity modulated optical lattice potentials can change sign for an alkali metal Rydberg atom, and the atoms are not always attracted to intensity minima in optical lattices with wavelengths near the CO$_2$ laser band. Here we demonstrate that such IR lattices can be tuned so that the trapping potential seen by the Rydberg atom can be made to vanish for atoms in \targeted" Rydberg states. Such state selective trapping of Rydberg atoms can be useful in controlled cold Rydberg collisions, cooling Rydberg states, and species-selective trapping and transport of Rydberg atoms in optical lattices.…
The Rydberg blockade mechanism has shown noteworthy promise for scalable quantum computation with neutral atoms. Both qubit states and gate-mediating Rydberg state belong to the same optically-trapped atom. The trapping fields, while being essential, induce detrimental decoherence. Here we theoretically demonstrate that this Stark-induced decoherence may be completely removed using powerful concepts of "magic" optical traps. We analyze "magic" trapping of a prototype three-level system: a Rydberg state along with two qubit states: hyperfine states attached to a J=1/2 ground state. Our numerica…
Cold atomic gases resonantly excited to Rydberg states can exhibit strong optical nonlinearity at the single photon level. We observe that in such samples radiation trapping leads to an additional mechanism for Rydberg excitation. Conversely we demonstrate that Rydberg excitation provides a novel in situ probe of the spectral, statistical, temporal and spatial properties of the trapped re-scattered light. We also show that absorption can lead to an excitation saturation that mimics the Rydberg blockade effect. Collective effects due to multiple scattering may co-exist with co-operative effects…
We theoretically investigate the quantum properties of nS, nP, and nD Rydberg atoms in a magnetic Ioffe-Pritchard trap. In particular, it is demonstrated that the two-body character of Rydberg atoms significantly alters the trapping properties opposed to point-like particles with identical magnetic moment. Approximate analytical expressions describing the resulting Rydberg trapping potentials are derived and their validity is confirmed for experimentally relevant field strengths by comparisons to numerical solutions of the underlying Schroedinger equation. In addition to the electronic propert…
We predict the possibility of "triply-magic" optical lattice trapping of neutral divalent atoms. In such a lattice, the ${^1}\!S_{0}$ and ${^3}\!P_{0}$ clock states and an additional Rydberg state experience identical optical potentials, fully mitigating detrimental effects of the motional decoherence. In particular, we show that this triply magic trapping condition can be satisfied for Yb atom at optical wavelengths and for various other divalent systems (Ca, Mg, Hg and Sr) in the UV region. We assess the quality of triple magic trapping conditions by estimating the probability of excitation …
Motivated by compelling advances in manipulating cold Rydberg (Ry) atoms in optical traps, we consider the effect of large extent of Ry electron wave function on trapping potentials. We find that when the Ry orbit lies outside inflection points in laser intensity landscape, the atom can stably reside in laser intensity maxima. Effectively, the free-electron AC polarizability of Ry electron is modulated by intensity landscape and can accept both positive and negative values. We apply these insights to determining magic wavelengths for Ry-ground-state transitions for alkali atoms trapped in infr…
We develop a theoretical understanding of trapping divalent Rydberg atoms in optical lattices. Because the size of the Rydberg electron cloud can be comparable to the scale of spatial variations of laser intensity, we pay special attention to averaging optical fields over the atomic wavefunctions. Optical potential is proportional to the ac Stark polarizability. We find that in the independent particle approximation for the valence electrons, this polarizability breaks into two contributions: the singly ionized core polarizability and the contribution from the Rydberg electron. Unlike the usua…
We demonstrate the coherent excitation of a mesoscopic ensemble of about 100 ultracold atoms to Rydberg states by driving Rabi oscillations from the atomic ground state. We employ a dedicated beam shaping and optical pumping scheme to compensate for the small transition matrix element. We study the excitation in a weakly interacting regime and in the regime of strong interactions. When increasing the interaction strength by pair state resonances we observe an increased excitation rate through coupling to high angular momentum states. This effect is in contrast to the proposed and previously ob…
Highly excited Rydberg states are usually extremely polarizable and exceedingly sensitive to electric fields. Because of this Rydberg ions confined in electric fields have state-dependent trapping potentials. We engineer a Rydberg state that is insensitive to electric fields by coupling two Rydberg states with static polarizabilities of opposite sign, in this way we achieve state-independent magic trapping. We show that the magically-trapped ion can be coherently excited to the Rydberg state without the need for control of the ion's motion.
We investigate Coherent Population Trapping in a strongly interacting ultracold Rydberg gas. Despite the strong van der Waals interactions and interparticle correlations, we observe the persistence of a resonance with subnatural linewidth at the single-particle resonance frequency as we tune the interaction strength. This narrow resonance cannot be understood within a meanfield description of the strong Rydberg--Rydberg interactions. Instead, a many-body density matrix approach, accounting for the dynamics of interparticle correlations, is shown to reproduce the observed spectral features.
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit the experimental time-scale to about 100$μ$s. Here, we demonstrate laser trapping of long-lived circular Rydberg states for up to 10ms. Our method is very general and opens many opportunities for quantum simulation. The 10ms trapping time corresponds to thousands of interaction cycles in a circular-state-based quantum simulator. It is also promising for quantu…
Metastable (1s)(2s) $^3{\rm S}_1$ helium atoms produced in a supersonic beam were excited to Rydberg-Stark states (with $n$ in the $27-30$ range) in a cryogenic environment and subsequently decelerated by, and trapped above, a surface-electrode decelerator. In the trapping experiments, the Rydberg atoms were brought to rest in 75~$μ$s and over a distance of 33~mm and kept stationary for times $t_{\mathrm{trap}}$ in the $0-525$~$μ$s range, before being re-accelerated for detection by pulsed field ionization. The use of a home-built valve producing short gas pulses with a duration of about 20~$μ…
Beams of helium atoms in Rydberg-Stark states with principal quantum number $n=48$ and electric dipole moments of 4600~D have been decelerated from a mean initial longitudinal speed of 2000~m/s to zero velocity in the laboratory-fixed frame-of-reference in the continuously moving electric traps of a transmission-line decelerator. In this process accelerations up to $-1.3\times10^{7}$~m/s$^2$ were applied, and changes in kinetic energy of $ΔE_{\mathrm{kin}}=1.3\times10^{-20}$~J ($ΔE_{\mathrm{kin}}/e = 83$~meV) per atom were achieved. Guided and decelerated atoms, and those confined in stationar…
We propose a scheme for the creation of stable three dimensional bright solitons in Bose-Einstein condensates, i.e., the matter-wave analog of so-called spatio-temporal "light bullets". Off-resonant dressing to Rydberg $nD$-states is shown to provide nonlocal attractive interactions, leading to self-trapping of mesoscopic atomic clouds by a collective excitation of a Rydberg atom pair. We present detailed potential calculations, and demonstrate the existence of stable solitons under realistic experimental conditions by means of numerical simulations.
Cold Rydberg atoms exposed to strong magnetic fields possess unique properties which open the pathway for an intriguing many-body dynamics taking place in Rydberg gases consisting of either matter or anti-matter systems. We review both the foundations and recent developments of the field in the cold and ultracold regime where trapping and cooling of Rydberg atoms have become possible. Exotic states of moving Rydberg atoms such as giant dipole states are discussed in detail, including their formation mechanisms in a strongly magnetized cold plasma. Inhomogeneous field configurations influence t…
We propose blue-detuned optical traps that are suitable for trapping of both ground state and Rydberg excited atoms. Addition of a background compensation field or suitable choice of the trap geometry provides a magic trapping condition for ground and Rydberg atoms at the trap center. Deviations from the magic condition at finite temperature are calculated. Designs that achieve less than 200 kHz differential trap shift between Cs ground and 125s Rydberg states for 10 μK Cs atoms are presented. Consideration of the trapping potential and photoionization rates
We demonstrate three-dimensional trapping of individual Rydberg atoms in holographic optical bottle beam traps. Starting with cold, ground-state $^{87}$Rb atoms held in standard optical tweezers, we excite them to $nS_{1/2}$, $nP_{1/2}$, or $nD_{3/2}$ Rydberg states and transfer them to a hollow trap at 850 nm. For principal quantum numbers $60 \leqslant n \leqslant 90$, the measured trapping time coincides with the Rydberg state lifetime in a 300~K environment. We show that these traps are compatible with quantum information and simulation tasks by performing single qubit microwave Rabi flopp…
We propose to apply atom-chip techniques to the trapping of a single atom in a circular Rydberg state. The small size of microfabricated structures will allow for trap geometries with microwave cut-off frequencies high enough to inhibit the spontaneous emission of the Rydberg atom, paving the way to complete control of both external and internal degrees of freedom over very long times. Trapping is achieved using carefully designed electric fields, created by a simple pattern of electrodes. We show that it is possible to excite, and then trap, one and only one Rydberg atom from a cloud of groun…
In this letter we investigate the possibility to attain strongly confined atomic localization using interacting Rydberg atoms in a Coherent Population Trapping (CPT) ladder configuration, where a standing-wave (SW) is used as a coupling field in the second leg of the ladder. Depending on the degree of compensation of the Rydberg level energy shift induced by the van der Waals (vdW) interaction, by the coupling field detuning, we distinguish between two antiblockade regimes, i.e. a partial antiblockade (PA) and a full antiblockade (FA). While a periodic pattern of tightly localized regions can …
We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which provides the gross energetic and spatial scales, and on the distribution of ground state atoms within the volume of the Rydberg wave function, which sculpt the electronic states. The latter range from the "trilobites", for small numbers of scatterers, to delocalized and chaotic eigenstates for disordered scatterer arrays, culminating in the dense scatterer …
Atoms excited into high-lying Rydberg states and under strong dipole-dipole interactions exhibit phenomena associated with highly correlated and complex systems. We perform first principles numerical simulations on the dynamics of such systems. The emergence of a roton minimum in the excitation spectrum, as expected in strongly correlated gases and accurately described by Feynman's theory of liquid helium, is shown to significantly inhibit particle transport, with a strong suppression of the diffusion coefficient, due to the emerging spatial order. We also demonstrate how the ability to tempor…
The properties and behaviour of a Ring Rydberg Composite are explicated. This system consists of a ring of ground state atoms centered on a Rydberg atom, whose electron elastically scatters off the ground state atoms. We transform the electronic Hamiltonian into a discrete tight-binding representation in which the on-site energies and long-range hopping between sites are controlled and mediated by the Rydberg electron. From this new representation, which to a large extent enables an analytic treatment, we derive scaling laws and analytic expressions for the wave functions and eigenspectrum. Th…
Single neutral atoms trapped in optical tweezers and laser-coupled to Rydberg states provide a fast and flexible platform to generate configurable atomic arrays for quantum simulation. The platform is especially suited to study quantum spin systems in various geometries. However, for experiments requiring continuous trapping, inhomogeneous light shifts induced by the trapping potential and temperature broadening impose severe limitations. Here we show how Raman sideband cooling allows one to overcome those limitations, thus, preparing the stage for Rydberg dressing in tweezer arrays.
We discuss a candidate solution for the controlled trapping and manipulation of two individual Rydberg atoms by means of a magnetic Ioffe-Pritchard trap that is superimposed by a constant electric field. In such a trap Rydberg atoms experience a permanent electric dipole moment that can be of the order of several hundred Debye. The interplay of electric dipolar repulsion and three dimensional magnetic confinement leads to a well controllable equilibrium configuration with tunable trap frequency and atomic distance. We thoroughly investigate the trapping potentials and analyze the interaction-i…
We explore how the extraordinary properties of Rydberg atoms can be employed to impact the motion of ultracold ground state atoms. Specifically, we use an off-resonant two-photon laser dressing to map features of the Rydberg states on ground state atoms. It is demonstrated that the interplay between the spatially varying quantization axis of the considered Ioffe-Pritchard field and the fixed polarizations of the laser transitions provides the possibility of substantially manipulating the ground state trapping potential.
We propose and demonstrate the laser cooling and trapping of Rydberg-dressed Sr atoms. By off-resonantly coupling the excited state of a narrow (7 kHz) cooling transition to a high-lying Rydberg state, we transfer Rydberg properties such as enhanced electric polarizability to a stable magneto-optical trap operating at $< 1 μK$. By increasing the density to $1 \times 10^{12} \rm{cm^{-3}}$, we show that it is possible to reach a regime where the long-range interaction between Rydberg-dressed atoms becomes comparable to the kinetic energy, opening a route to combining laser cooling with tunable l…
Rydberg states of atomic helium with principal quantum numbers ranging from n=20 to n=100 have been prepared by non-resonance-enhanced single-color two-photon excitation from the metastable 2 {^3}S{_1} state. Photoexcitation was carried out using linearly and circularly polarized pulsed laser radiation. In the case of excitation with circularly polarized radiation, Rydberg states with azimuthal quantum number |m_{\ell}|=2 were prepared in zero electric field, and in homogeneous electric fields oriented parallel to the propagation axis of the laser radiation. In sufficiently strong electric fie…
Beams of helium atoms in Rydberg states with principal quantum number $n=52$, and traveling with an initial speed of 1950 m/s, have been accelerated, decelerated and guided while confined in moving electric traps generated above a curved, surface-based electrical transmission line with a segmented center conductor. Experiments have been performed with atoms guided at constant speed, and with accelerations exceeding $10^7$ m/s$^2$. In each case the manipulated atoms were detected by spatially resolved, pulsed electric field ionization. The effects of tangential and centripetal accelerations on …
Trapped Rydberg ions are a promising new system for quantum information processing. They have the potential to join the precise quantum operations of trapped ions and the strong, long-range interactions between Rydberg atoms. Technically, the ion trap will need to stay active while exciting the ions into the Rydberg state, else the strong Coulomb repulsion will quickly push the ions apart. Thus, a thorough understanding of the trap effects on Rydberg ions is essential for future applications. Here we report the observation of two fundamental trap effects. First, we investigate the interaction …
Long ground-Rydberg coherence lifetime is interesting for implementing high-fidelity quantum logic gates, many-body physics, and other quantum information protocols. However, the potential formed by a conventional far-off-resonance red-detuned optical-dipole trap (ODT) is usually repulsive for Rydberg atoms, which will result in fast atom loss and low repetition rate of the experimental sequence. These issues can be addressed by a magic ODT. We performed the calculation of ODT's magic detuning for confinement of cesium ground state and Rydberg state with the same potential well. We used a sum-…
Usually the influence of the quadratic Stark effect on an ion's trapping potential is minuscule and only needs to be considered in atomic clock experiments. In this work we excite a trapped ion to a Rydberg state with polarizability $\sim$~eight orders of magnitude higher than a low-lying electronic state; we find that the highly-polarizable ion experiences a vastly different trapping potential owing to the Stark effect. We observe changes in trap stiffness, equilibrium position and minimum potential, which can be tuned using the trapping electric fields. These effects lie at the heart of prop…
We demonstrate excitation of a single trapped cold $^{40}$Ca$^+$ ion to Rydberg levels by laser radiation in the vacuum-ultraviolet at 122 nm wavelength. Observed resonances are identified as 3d$^2$D$_{3/2}$ to 51 F, 52 F and 3d$^2$D$_{5/2}$ to 64F. We model the lineshape and our results imply a large state-dependent coupling to the trapping potential. Rydberg ions are of great interest for future applications in quantum computing and simulation, in which large dipolar interactions are combined with the superb experimental control offered by Paul traps.
We use the sensitive response to electric fields of Rydberg atoms to characterize all three vector components of the local electric field close to an atom-chip surface. We measured Stark-Zeeman maps of $S$ and $D$ Rydberg states using an elongated cloud of ultracold Rubidium atoms ($T\sim2.5$ $μ$K) trapped magnetically $100$ $μ$m from the chip surface. The spectroscopy of $S$ states yields a calibration for the generated local electric field at the position of the atoms. The values for different components of the field are extracted from the more complex response of $D$ states to the combined …
We characterize the two-photon excitation of an ultracold gas of Rubidium atoms to Rydberg states analysing the induced atomic losses from an optical dipole trap. Extending the duration of the Rydberg excitation to several ms, the ground state atoms are continuously coupled to the formed positively charged plasma. In this regime we measure the $n$-dependence of the blockade effect and we characterise the interaction of the excited states and the ground state with the plasma. We also investigate the influence of the quasi-electrostatic trapping potential on the system, confirming the validity o…
We theoretically study trapped ions that are immersed in an ultracold gas of Rydberg-dressed atoms. By off-resonant coupling on a dipole-forbidden transition, the adiabatic atom-ion potential can be made repulsive. We study the energy exchange between the atoms and a single trapped ion and find that Langevin collisions are inhibited in the ultracold regime for these repulsive interactions. Therefore, the proposed system avoids recently observed ion heating in hybrid atom-ion systems caused by coupling to the ion's radio frequency trapping field and retains ultracold temperatures even in the pr…
We present a theoretical quasiclassical study of the formation, during Coulomb explosion, of two highly excited neutral H atoms (double H$^{*}$) of strongly driven H$_2$. In this process, after the laser field is turned off each electron occupies a Rydberg state of an H atom. We show that two-electron effects are important in order to correctly account for double H$^{*}$ formation. We find that the route to forming two H$^{*}$ atoms is similar to pathway B that was identified in Phys. Rev. A {\bf 85} 011402 (R) as one of the two routes leading to single H$^{*}$ formation. However, instead of o…
We review Rydberg aggregates, assemblies of a few Rydberg atoms exhibiting energy transport through collective eigenstates, considering isolated atoms or assemblies embedded within clouds of cold ground-state atoms. We classify Rydberg aggregates, and provide an overview of their possible applications as quantum simulators for phenomena from chemical or biological physics. Our main focus is on flexible Rydberg aggregates, in which atomic motion is an essential feature. In these, simultaneous control over Rydberg-Rydberg interactions, external trapping and electronic energies, allows Born-Oppen…
We describe the fabrication and construction of a setup for creating lattices of magnetic microtraps for ultracold atoms on an atom chip. The lattice is defined by lithographic patterning of a permanent magnetic film. Patterned magnetic-film atom chips enable a large variety of trapping geometries over a wide range of length scales. We demonstrate an atom chip with a lattice constant of 10 $μ$m, suitable for experiments in quantum information science employing the interaction between atoms in highly-excited Rydberg energy levels. The active trapping region contains lattice regions with square …
Trapping a Rydberg atom close to a surface is an important step towards the realisation of many proposals of quantum information or hybrid quantum systems. One of the challenges in these experiments is to overcome the electric field emanating from contaminations on the surface. Here we report on measurements of an electric field created by $^{87}$Rb atoms absorbed on a 25$\,$nm thick layer of SiO$_2$, covering a 90$\,$nm layer of Au. The electric field is measured using a two-photon transition to the 23$D_{5/2}$ and 25$S_{1/2}$ state. The electric field value that we measure is higher than typ…
Atoms in highly excited (Rydberg) states have a number of unique properties which make them attractive for applications in quantum information. These are large dipole moments, lifetimes and polarizabilities, as well as strong long-range interactions between Rydberg atoms. Experimental methods of laser cooling and precision spectroscopy enable the trapping and manipulation of single Rydberg atoms and applying them for practical implementation of quantum gates over qubits of a quantum computer based on single neutral atoms in optical traps. In this paper, we give a review of the experimental and…
This article proposes quantum processing in an optical lattice, using Rydberg electron's Fermi scattering from ground-state atoms in spin-dependent lattices as a source of interaction. Instead of relying on Rydberg pair potentials, the interaction is controlled by engineering the electron cloud of a sole Rydberg atom. Here we specifically propose the implementation of two prominent multi-qubit gates i.e. the stabilizer-phase operator and the Toffoli gate. The new scheme addresses the main bottleneck in Rydberg quantum simulation by suppressing the population of short-lived Rydberg states over …
The binding and trapping of particles usually rely on conservative forces, described by unitary quantum dynamics. We show that both can also arise solely from spatially dependent dephasing, the simplest type of decoherence. This can be based on continuous weak position measurements in only selected regions of space, for which we propose a practical realisation. For a single particle, we demonstrate a quantum particle-in-the-box based on dephasing. For two particles, we demonstrate their binding despite repulsive interactions, if their molecular states are dephased at large separations only. Bo…
The large electric dipole moments associated with highly excited Rydberg states of atoms and molecules make gas-phase samples in these states very well suited to deceleration and trapping using inhomogeneous electric fields. The methods of Rydberg-Stark deceleration with which this can be achieved are reviewed here. Using these techniques, the longitudinal motion of beams of atoms and molecules moving at speeds as high as 2500~m/s have been manipulated, with changes in kinetic energy of up to $|ΔE_{\mathrm{kin}}|=1.3\times10^{-20}$~J ($|ΔE_{\mathrm{kin}}|/e=80$~meV or $|ΔE_{\mathrm{kin}}|/hc=6…
