We generate a 200-nm optical frequency comb at 1.5 microns by injecting two single-frequency lasers into a highly nonlinear fiber, and explore its spectral phase properties and high power to demonstrate full nonlinear conversion into its second harmonic. Combs of optical frequencies with 100-nm (~ 48 THz) bandwidths, centered at 790-800 nm and spaced by 0.8-1 nm (380-470 GHz) were produced by second harmonic and multiple sum frequency generation simply by focusing into a 2-mm long nonlinear crystal. Conventional birefringence phase matching was used in normal incidence configuration without tilting the crystal.
We demonstrate, for the first time, a scheme that generates radially-polarized light using Goos-Hanchen shift of a cylindrically symmetric Total Internal Reflection. It allows ultra-broadband radial polarization conversion for wavelengths differing >1 micron.
Frequency conversion of light can be dramatically enhanced using high quality factor ($Q$-factor) cavities. Unfortunately, the achievable conversion efficiencies and conversion bandwidths are fundamentally limited by the time-bandwidth limit of the cavity, restricting their use in frequency conversion of ultrashort pulses. Here, we propose and numerically demonstrate sum-frequency generation based frequency conversion using a metasurface-based cavity configuration that could overcome this limitation. The proposed experimental configuration takes use of the spatially dispersive responses of per…
We propose a design for broadband waveguide mode conversion based on gradient index metamaterials (GIMs). Numerical simulations demonstrate that the zeroth order of transverse magnetic mode or the first order of transverse electric mode (TM0/TE1) can be converted into the first order of transverse magnetic mode or the second order of transverse electric mode (TM1/TE2) for a broadband of frequencies. As an application, an asymmetric propagation is achieved by integrating zero index metamaterials inside the GIM waveguide.
A comprehensive physical model of adiabatic three wave mixing is developed for the fully nonlinear regime, i.e. without making the undepleted pump approximation. The conditions for adiabatic evolution are rigorously derived, together with an estimate of the bandwidth of the process. Furthermore, these processes are shown to be robust and efficient. Finally, numerical simulations demonstrate adiabatic frequency conversion in a wide variety of physically attainable configurations.
We investigate the up-conversion process of broadband light from parametric down-conversion (PDC), focusing on the spatio-temporal spectral properties of the sum-frequency generated (SFG) radiation. We demonstrate that the incoherent component of the SFG spectrum is characterized by a skewed geometry in space-time, which originates from a compensation between the group-velocity mismatch and the spatial walk-off of the fundamental and the SFG fields. The results are illustrated both by a theoretical modeling of the optical system and by experimental measurements.
We investigate the up-conversion process of broadband light from parametric down-conversion (PDC), focusing on the spatio-temporal spectral properties of the sum-frequency generated (SFG) radiation. We demonstrate that the incoherent component of the SFG spectrum is characterized by a skewed cigar-shaped geometry in space-time due to the compensation of spatial walk-off and group-velocity mismatch between the fundamental and the generated SFG fields. The results are illustrated both by a theoretical modeling of the optical system and by experimental measurements.
Using a hydrodynamic approach we examine bulk- and surface-induced second and third harmonic generation from semiconductor nanowire gratings having a resonant nonlinearity in the absorption region. We demonstrate resonant, broadband and highly efficient optical frequency conversion: contrary to conventional wisdom, we show that harmonic generation can take full advantage of resonant nonlinearities in a spectral range where nonlinear optical coefficients are boosted well beyond what is achievable in the transparent, long-wavelength, non-resonant regime. Using femtosecond pulses with approximate…
An influence of multi-line CO laser focusing on spectral characteristics of broadband sum-frequency generation in ZnGeP2 nonlinear crystal was experimentally and numerically studied. Maximal frequency conversion was experimentally observed under tight focusing of the multi-line rather than single-line CO laser. The tight focusing resulted in broadening sum-frequency generation spectrum and increasing total, i.e. integrated over the spectrum, frequency conversion efficiency. These effects were due to increasing phase-matching bandwidth and angular dispersion. Maximal conversion efficiency of th…
We experimentally demonstrate an efficient broadband second harmonic generation process with tunable mode-locked Ti: sapphire oscillator. We have achieved a robust broadband and efficient flat conversion of more than 35nm wavelength, by designing an adiabatic aperiodically poled potassium titanyl phosphate (KTP) crystal. Moreover, we have shown that with such efficient flat conversion, we can shape and control broadband second harmonic pulses. More specifically, we assign spectral-phase of abs-value and π-step, which allows wavelength tunable intense pump-probe and amplitude modulation of the …
The modern information networks are built on hybrid systems working at disparate optical wavelengths. Coherent interconnects for converting photons between different wavelengths are highly desired. Although coherent interconnects have conventionally been realized with nonlinear optical effects, those systems require demanding experimental conditions such as phase matching and/or cavity enhancement, which not only bring difficulties in experimental implementation but also set a narrow operating bandwidth (typically in MHz to GHz range as determined by the cavity linewidth). Here, we propose and…
We investigate terahertz emission from two-color fs-laser-induced microplasmas. Under strongest focusing conditions, microplasmas are shown to act as point-sources for broadband terahertz-to-far-infrared radiation, where the emission bandwidth is determined by the plasma density. Semi-analytical modeling allows us to identify scaling laws with respect to important laser parameters. In particular, we find that the optical-to-THz conversion efficiency crucially depends on the focusing conditions. We use this insight to demonstrate by means of Maxwell-consistent 3D simulations, that for only 10-$…
We propose to use the integrated aluminum nitride waveguide with engineered width variation to achieve optical frequency conversion based on $χ^{(2)}$ nonlinear effect on a photonic chip. We show that in an adiabatically tapered waveguide, the frequency conversion has a much broader bandwidth and the efficiency within the bandwidth is almost constant, which is favorable for short pulses. We demonstrate both analytically and numerically an "area law" for the frequency conversion, i.e. the product of bandwidth and efficiency is conserved as long as peak conversion efficiency does not saturate. T…
Ultra-broadband imaging devices with high performance are in great demand for a variety of technological applications, including imaging, remote sensing, and communications. An ultra-broadband up-converter is realized based on a p-GaAs homojunction interfacial workfunction internal photoemission (HIWIP) detector-light emitting diode (LED) device. The device demonstrates an ultra-broad response ranging from visible to terahertz (THz) with good reproducibility. The peak responsivity in the mid-infrared (MIR) region is 140 mA/W at 10.5 microns. The HIWIP-LED shows enormous potential for ultra-bro…
The recent development of devices based on novel nonlinear materials like chalcogenides (ChGs), silicon (Si) and other semi-conductors has revolutionized the field of nonlinear photonics [1,2,3]. Among the nonlinear effects observed in these materials, four-wave mixing (FWM) is the process that finds the most applications including wavelength conversion [4], optical regeneration [5,6], optical delay [7], time-domain demultiplexing[8], temporal cloaking[9] and negative refraction[10]. Although FWM has been observed in several media including chalcogenides [11,12,13,14], silicon[15, 16], bismuth…
Cavity optomagnonics has emerged as a promising platform for studying coherent photon-spin interactions as well as tunable microwave-to-optical conversion. However, current implementation of cavity optomagnonics in ferrimagnetic crystals remains orders of magnitude larger in volume than state-of-the-art cavity optomechanical devices, resulting in very limited magneto-optical interaction strength. Here, we demonstrate a cavity optomagnonic device based on integrated waveguides and its application for microwave-to-optical conversion. By designing a ferrimagnetic rib waveguide to support multiple…
We report design of an efficient ~ 50 cm long all-fiber compact microstructured optical fiber-based 3-4.25 um mid-IR light source with power conversion efficiency > 28% by exploiting FWM with Er3+-doped ZBLAN fiber as the pump.
We propose an operating principle to achieve broadband and highly tunable mode conversion and amplification exploiting inter-modal four wave mixing in a multimode fiber. A bandwidth of 30 nanometers is demonstrated by properly designing a simple step-index silica fiber.
We report a broadband microwave frequency converter based on a coherent Kerr optical micro-comb generated by an integrated micro-ring resonator. The coherent micro-comb displays features that are consistent with soliton crystal dynamics with an FSR of 48.9GHz. We use this to demonstrate a high-performance millimeter-wave local oscillator at 48.9GHz in the Q-band for microwave frequency conversion. We experimentally verify the microwave performance up to 40 GHz, achieving a ratio of 6.8 dB between output RF power and IF power and a spurious suppression ratio of > 43.5 dB. The experimental resul…
Phase-matched nonlinear processes exhibit a tradeoff between the conversion efficiency and the acceptance bandwidth. Adiabatic nonlinear processes, in which the phase mismatch varies slowly along the interaction length, enable us to overcome this tradeoff, allowing an efficient frequency conversion with broad spectral and thermal bandwidths. Until now, the variation in the phase mismatch condition was mainly based on quasi-phase matching in ferroelectric crystals. However, this solution is limited to low power sources. Here, instead, we study the adiabatic second harmonic in birefringently pha…
Future wireless communication networks have to handle data rates of tens or even hundreds of Gbit/s per link, requiring carrier frequencies in the unallocated terahertz (THz) spectrum. In this context, seamless integration of THz links into existing fiber-optic infrastructures is of great importance to complement the inherent portability and flexibility advantages of wireless networks by the reliable and virtually unlimited capacity of optical transmission systems. On the technological level, this requires novel device and signal processing concepts for direct conversion of data streams betwee…
We report on generation and control of tunable, broad orbital angular momentum (OAM) spectrum of a vortex beam. Using two spiral phase plates (SPPs), we have converted the Gaussian beam of Yb-fiber femtosecond laser at 1064 nm into optical vortices of orders, l=1-6, with conversion efficiency >95%. By adjusting the transverse shift of the SPPs with respect to the incident Gaussian beam axis, we have transformed the symmetric (intensity distribution) optical vortex of order, l, into an asymmetric vortex beam of broad OAM spectrum of orders, l, l-1, l-2,..,0. While the position of the SPPs deter…
Optical frequency conversion processes in nonlinear materials are limited in wavelength by the accessible phase matching and the required high pump powers. In this letter, we report a novel broadband phase matching (PM) technique in high quality factor (Q) whispering gallery mode (WGM) resonators made of birefringent crystalline materials. This technique relies on two interacting WGMs, one with constant and the other with spatially oscillating phase velocity. Thus, phase matching occurs cyclically. The technique can be implemented with a WGM resonator with its disk plane parallel to the optic …
Thin-film lithium niobate (TFLN) is an emerging platform for compact, low-power nonlinear-optical devices, and has been used extensively for near-infrared frequency conversion. Recent work has extended these devices to mid-infrared wavelengths, where broadly tunable sources may be used for chemical sensing. To this end, we demonstrate efficient and broadband difference frequency generation between a fixed 1-micron pump and a tunable telecom source in uniformly-poled TFLN-on-sapphire by harnessing the dispersion-engineering available in tightly-confining waveguides. We show a simultaneous 1-2 o…
We demonstrated broadband highly efficient optical nonlinear processes in on-chip integrated lithium niobate (LN) microdisk resonators. The Q factors of the micro-resonators fabricated by femtosecond laser writing and chemo-mechanical polishing are reliably above 10^8, approaching the intrinsic material absorption limit of LN. Broadband nonlinear processes, including optical parametric oscillation (OPO), second harmonic generation (SHG), third harmonic generation, and fourth harmonic generation, were observed with ultrahigh efficiencies in the same LN microdisk without introducing domain inver…
We theoretically investigate photothermal heating of ultra-flexible metamaterials, which are obtained by randomly mixing TiN nanoparticles in polydimethylsiloxane (PDMS). Due to the plasmonic properties of TiN nanoparticles, incident light is perfectly absorbed in a broadband range (300-3000 nm) to generate heat within these metamaterials. Under irradiation of an 808 nm near-infrared laser with different intensities, our predicted temperature rises as a function of time agree well with recent experimental data. For a given laser intensity, the temperature rise varies non-monotonically with con…
High-efficiency photon-pair production is a long-sought-after goal for many optical quantum technologies, and coherent photon conversion processes are promising candidates for achieving this. We show theoretically how to control coherent conversion between a narrow-band pump photon and broadband photon pairs in nonlinear optical waveguides by tailoring frequency dispersion for broadband quantum frequency mixing. We reveal that complete deterministic conversion as well as pump-photon revival can be achieved at a finite propagation distance. We also find that high conversion efficiencies can be …
Efficient, low noise conversion between different colors of light is a necessary tool for interfacing quantum optical technologies that have different operating wavelengths. Optomechanically mediated wavelength conversion and amplification is a potential method for realizing this technology, and is demonstrated here in microdisks fabricated from single crystal diamond--a material that can host a wide range of quantum emitters. Frequency up--conversion is demonstrated with internal conversion efficiency of $\sim$45% using both narrow and broadband probe fields, and optomechanical frequency conv…
We introduce a general technique to generate compressed broadband terahertz pulses based on difference frequency generation of optical pump radiation using aperiodically poled structures. The pump pulse format and poling of the crystals conceived are such that the emergent terahertz pulse is compressed. The approach circumvents pump pulse distortions that result from non-collinear approaches and the need for external compression. It is particularly efficient for the generation of pulses of intermediate durations of few to tens of cycles. For instance, conversion efficiencies in the few percent…
We observe at record-high speed the nonclassical nature of ultra-broadband bi-photons, reducing the measurement time by four orders of magnitude compared to standard techniques of Hong-Ou-Mandel interference or sum-frequency generation. We measure the quantum state of the broadband bi-photons, amplitude and phase, with a pairwise "Mach-Zehnder" quantum interferometer, where bi-photons that are generated in one nonlinear crystal are enhanced (constructive interference) or diminished (destructive interference) in another crystal, depending on the bi-photon phase. We verify the quantum nature of …
Broadband-tunable sources of circularly-polarized light are crucial in fields such as laser science, biomedicine and spectroscopy. Conventional sources rely on nonlinear wavelength conversion and polarization control using standard optical components, and are limited by the availability of suitably transparent crystals and glasses. Although gas-filled hollow-core photonic crystal fiber provides pressure-tunable dispersion, long well-controlled optical path-lengths, and high Raman conversion efficiency, it is unable to preserve circular polarization state, typically exhibiting weak linear biref…
Segment-chirped periodically poled lithium niobate waveguides for broadband supercontinuum generation
National University of Singapore（新加坡国立大学）；Sichuan University（四川大学）；A ∗ STAR Quantum Innovation Centre (Q.InC), Agency for Science, Technology and Research (A ∗ STAR)（A*STAR量子创新中心（Q.InC），科学技术研究局（A*STAR））；Nanyang Technological University（南洋理工大学）
The nonlinear metamaterials have been shown to provide nonlinear properties with high nonlinear conversion efficiency and in a myriad of light manipulation. Here we study terahertz generation from nonlinear metasurface consisting of single layer nanoscale split-ring resonator array. The terahertz generation due to optical rectification by the second-order nonlinearity of the split-ring resonator is investigated by a time-domain implementation of the hydrodynamic model for electron dynamics in metal. The results show that the nonlinear metasurface enables us to generate broadband terahertz radi…
High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped periodically poled lithium niobate waveguides driven by phase-stable $\leq$12-nJ, 100 fs pulses at 3 $μ$m with 100 MHz repetition rate. A mid-infrared to ultraviolet-visible conversion efficiency as high as 10% is observed, amongst an overall 23% conversion of the fundamental to all harmonics. We verify the coherence of the harmonic frequency combs despite the complex …
Metadevices based on dielectric nanostructured surfaces with both electric and magnetic Mie-type resonances have resulted in the best efficiency to date for functional flat optics with only one disadvantage: a narrow operational bandwidth. Here we experimentally demonstrate broadband transparent all-dielectric metasurfaces for highly efficient polarization manipulation. We utilize the generalized Huygens principle, with a superposition of the scattering contributions from several electric and magnetic multipolar modes of the constituent meta-atoms, to achieve destructive interference in reflec…
Non-linear optical characteristics of a new BaGa2GeSe6 crystal were numerically studied and compared with well-known mid-IR nonlinear crystals ZnGeP2, GaSe, and AgGaSe2.The calculations demonstrated for the new crystal to be probably the most efficient crystal for second harmonic generation of CO and CO2laser radiation. It was found that a broadband two-stage frequency conversion of multi-line CO-laser radiation in this crystal is possible within 2.5-9.0 μm wavelength range with higher efficiency than in ZnGeP2 and AgGaSe2 crystals.
Developments in integrated photonics have led to stable, compact, and broadband comb generators that support a wide range of applications. Current on-chip comb generators, however, are still limited by low optical pump-to-comb conversion efficiencies. Here, we demonstrate an integrated electro-optic frequency comb with a conversion efficiency of 30% and an optical bandwidth of 132 nm, featuring a 100-times higher conversion efficiency and 2.2-times broader optical bandwidth compared with previous state-of-the-art integrated electro-optic combs. We further show that, enabled by the high efficie…
The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses with center frequency tunable between 2-4 THz. The coherent THz light source with pulse energy of 1.2 microjoule can be generated from a low-cost crystalline quartz pumped by an ultrashort tilted wave-front pulse. Thanks to the wide transparent spectral window and high damage threshold, our theoretical analysis and experiment show that the optical rectification…
As shown in the early 1960s, the gain in stimulated Raman scattering (SRS) is drastically suppressed when the rate of creation of phonons (via pump-to-Stokes conversion) is exactly balanced by the rate of phonon annihilation (via pump-to-anti-Stokes conversion). This occurs when the phonon coherence waves synchronized vibrations of a large population of molecules have identical propagation constants for both processes, i.e., they are phase-velocity matched. As recently demonstrated, hydrogen-filled photonic crystal fiber pumped in the vicinity of its zero dispersion wavelength provides an idea…
We present a new approach to engineering broadband sources of entangled photon pairs for quantum interferometry. The source is based on quasi-phase-matched spontaneous parametric down conversion in a titanium diffused periodically poled lithium niobate waveguide with a strongly-chirped poling period. The proposed non-standard asymmetric poling mitigates phase distortions associated with the process of chirping. Asymmetric poling significantly broadens the entangled source bandwidth while preserving high visibility quantum interferometric sensing.
