We investigate the interaction of tightly focused light with the surface-plasmon-polariton resonances of metal nanospheres. In particular, we compute the scattering and absorption ratios as well as transmission and reflection coefficients. Inspired by our previous work in Ref. [1], we discuss how well a metal nanoparticle approximates a point-like dipolar radiator. We find that a 100 nm silver nanosphere is very close to such an ideal oscillator. Our results have immediate implications for single nanoparticle spectroscopy and microscopy as well as plasmonics.
All-dielectric nanostructures have recently emerged as a promising alternative to plasmonic devices, as they also possess pronounced electric and magnetic resonances and allow effective light manipulation. In this work, we study optical properties of a composite structure that consists of a silicon nanoparticle array (metasurface) and high-index substrate aiming at clarifying the role of substrate on reflective properties of the nanoparticles. We develop a simple semi-analytical model that describes interference of separate contributions from nanoparticle array and the bare substrate to the to…
The study of high-index dielectric nanoparticles currently attracts a lot of attention. They do not suffer from absorption but promise to provide control on the properties of light comparable to plasmonic nanoparticles. To further advance the field, it is important to identify versatile dielectric nanoparticles with unconventional properties. Here, we show that breaking the symmetry of an all-dielectric nanoparticle leads to a geometrically tunable magneto-electric coupling, i.e. an omega-type bianisotropy. The suggested nanoparticle exhibits different backscatterings and, as an interesting co…
The heat-shielding properties of random metasurface, composed of spherical or spheroidal nanoparticles with random displacements and/or random deformation, were theoretically investigated using the finite difference time domain method. The effective coverage was defined using the total area of nanoparticles in the metasurface, and the robustness of the near-infrared light reflection against randomness was investigated. When the effective coverage was high, the near-infrared light reflection was reduced by at least 20% in both nanoparticle arrangement and shape randomness compared to the hexago…
Single particle tracking has found broad applications in the life and physical sciences, enabling the observation and characterisation of nano- and microscopic motion. Fluorescence-based approaches are ideally suited for high-background environments, such as tracking lipids or proteins in or on cells, due to superior background rejection. Scattering-based detection is preferable when localisation precision and imaging speed are paramount due to the in principle infinite photon budget. Here, we show that micromirror-based total internal reflection dark field microscopy enables background suppre…
The study of metallic nanoparticles has a long tradition in linear and nonlinear optics [1], with current emphasis on the ultrafast dynamics, size, shape and collective effects in their optical response [2-6]. Nanoparticles also represent the ultimate confined geometry:high surface-to-volume ratios lead to local field enhancements and a range of dramatic modifications of the material's properties and phase diagram [7-9]. Confined gallium has become a subject of special interest as the light-induced structural phase transition recently observed in gallium films [10, 11] has allowed for the demo…
Reflection of near-infrared light is important for preventing heat transfer in energy saving applications. A large-area, mass-producible reflector that contains randomly distributed disk-shaped silver nanoparticles and that exhibits high reflection at near-infrared wavelengths was demonstrated. Although resonant coupling between incident light and the nanostructure of the reflector plays some role, what is more important is the geometrical randomness of the nanoparticles, which serves as the origin of a particle-dependent localization and hierarchical distribution of optical near-fields in the…
We study the optical responses of metal nanoparticle chains. Multiple scattering calculations are used to study the extinction cross sections of silver nanosphere chains of finite length embedded in a glass matrix. The transmission and reflection coefficients of periodic 2D arrays of silver nanospheres are also calculated to understand the interaction between nanoparticle chains. The results are in agreement with recent experiments. The splitting of plasmon-resonance modes for different polarizations of the incident light are explored. Results on the effect of disorder are also presented.
Reflection at relativistically moving plasma mirrors is a well-known approach for frequency conversion as an alternative to nonlinear techniques. A key issue with plasma mirrors is the need for a high carrier concentration, of order 10^21 cm^-3, to achieve an appreciable reflectivity. To generate such high carrier concentrations, short laser pulses with extreme power densities of the order >10^15 W/cm^2 are required. Here, we introduce a novel waveguide-based method for generating relativistically moving plasma mirrors that requires much lower pump powers and much less carrier concentration. S…
Hopping of nanoparticles in optical tweezers governed by Mie resonances
Nonlinear Physics Center, Research School of Physics, Australian National University（澳大利亚国立大学物理研究学院非线性物理中心）；School of Optoelectronic Engineering and Instrumentation Science, Dalian University of Technology（大连理工大学光电工程与仪器科学学部）；Department of Electrical and Electronic Engineering, The University of Melbourne（墨尔本大学电气与电子工程系）；Photonics Laboratory, Physics Unit, Tampere University（坦佩雷大学物理学单元光子学实验室）
The goal of nanophotonics is to control and manipulate light at length scales below the diffraction limit. Typically nanostructured metals are used for this purpose, light being confined by exploiting the surface plasmon-polaritons such structures support. Recently excitonic (molecular) materials have been identified as an alternative candidate material for nanophotonics. Here we use theoretical modelling to explore how hybridisation of surface exciton-polaritons can be achieved through appropriate nanostructuring. We focus on the extent to which the frequency of the hybridised modes can be sh…
To achieve efficient light control at subwavelength dimensions, plasmonic and all-dielectric nanoparticles have been utilized both as a single element as well as in the arrays. Here we study 2D periodic nanoparticle arrays (metasurfaces) that support lattice resonances near the Rayleigh anomaly due to the electric dipole (ED) and magnetic dipole (MD) resonant coupling between the nanoparticles. Silicon and core-shell particles are considered. We demonstrate for the first time that, choosing of lattice periods independently in each mutual-perpendicular direction, it is possible to achieve a ful…
A thorough theoretical study of the optical properties of periodic Si nanosphere arrays is undertaken, placing particular emphasis on the synergy between electric and magnetic Mie resonances, which occur in high-refractive-index nanoparticles and can lead to a rich variety of phenomena ranging from perfect reflection to controlled diffraction. By means of systematic calculations using the layer-multiple-scattering method that we properly extended so as to describe periodic arrays with many scatterers per unit cell, in conjunction with finite-element simulations, we optimized surfaces of Si nan…
The features of polarization control of multiple multiresonances for quasi-trapped modes excited by synchronization of bianisotropic dipole responses in MoS$_2$ disks with a hole are considered. Using the numerical calculations with analytical multipole analysis, we showed that the presence of a strong optical anisotropy of MoS$_2$ nanoparticles provides an additional degree of freedom and allows to observe several resonances of electric and magnetic dipoles at once in a narrow spectral range. Based on the simulation results, we obtained the frequency dependences for the dipole polarizabilitie…
Transport properties of a single plasmon interacting with a hybrid system composed of a semiconductor quantum dot (SQD) and a metal nanoparticle (MNP) coupled to one-dimensional surface plasmonic waveguide are investigated theoretically via the real-space approach. We considered that the MNP-SQD interaction leads to the formation of a hybrid exciton and the transmission and reflection of a single incident plasmon could be controlled by adjusting the frequency of the classical control field applied to the MNP-SQD hybrid nanosystem, the kinds of metallic nanoparticles and the background media, r…
Excitation of surface plasmons supported by doped graphene sheets at terahertz frequencies is investigated numerically. To alleviate the momentum mismatch between the highly-confined plasmon modes and the incident radiation, it is proposed to increase the surface conductivity of graphene through high doping levels or with few-layer graphene. For currently achievable doping levels, our analysis shows that surface plasmons on monolayer graphene may be excited at operating frequencies up to about 10 THz (~ 41.3 meV) with a high-index coupling prism, and higher frequencies/energies are possible fo…
Metal-insulator-metal (MIM) nanogaps in canonical nanoparticle-on-mirror geometry (NPoM) provide deep-subwavelength confinement of light with mode volumes smaller than $V/V_0$ $<$ $10^{-6}$. However, access to these hotspots is limited by the impendence mismatch between the high in-plane $k_{//}$ of trapped light and free-space plane-waves, making the in- and out-coupling of light difficult. Here, by constructing a nanoparticle-on-foil (NPoF) system with thin metal films, we show the mixing of insulator-metal-insulator (IMI) modes and MIM gap modes resulting in MIMI modes. This mixing provides…
A theory of light reflection and transmission by an optically thin nanocomposite slab which contains randomly distributed metal nanoparticles (NPs) is developed. The underlying model takes into account the reflection of light scattered by NPs from the slab boundaries, enhanced decay of localized surface plasmons in dense NP arrays and light scattering at the slab surface -- the factors which are beyond the scope of the Maxwell Garnett approximation. It is demonstrated that the first two effects lead to broadband perfect absorption observed in such nanocomposites, whereas the last one is respon…
Absorption of electromagnetic energy by a dissipative material is one of the most fundamental electromagnetic processes that underlies a plethora of applied problems, including sensing and molecular detection, radar detection, wireless power transfer, and photovoltaics. Perfect absorption is a particular regime when all of the incoming electromagnetic energy is absorbed by the system without scattering. Commonly, the incident energy is delivered to the absorbing system by a plane wave, hence perfect absorption of this wave requires an infinitely extended planar structure. Here, we demonstrate …
A general metallic mirror (i.e., a flat metallic surface) has been a popular optical component that can contribute broadband light absorption to thin-film optoelectronic devices; nonetheless, such electric mirror with a reversal of reflection phase inevitably causes the problem of minimized electric field near at the mirror surface (maximized electric field at one quarter of wavelength from mirror). This problem becomes more elucidated, when the deep-subwavelength-scaled two-dimensional (2D) material (e.g., graphene and molybdenum disulfide) is implemented into optoelectronic device as an acti…
Realizing strong light-matter interactions between individual 2-level systems and resonating cavities in atomic and solid state systems opens up possibilities to study optical nonlinearities on a single photon level, which can be useful for future quantum information processing networks. However, these efforts have been hampered by the unfavorable experimental conditions, such as cryogenic temperatures and ultrahigh vacuum, required to study such systems and phenomena. Although several attempts to realize strong light-matter interactions at room-temperature using so-called plasmon resonances h…
We investigate the resonant optical response of single material-anisotropic nanoparticles (NPs) of molybdenum disulfide (MoS$_2$) and their two-dimensional arrays (metasurfaces) irradiated by plane waves of the telecomunication optical range. Nanoparticles in the form of a disk with centered and shifted hole are considered. Using the recently experimental measured the MoS$_2$ dielectric permittivity and numerical calculations with analytical multipole analysis, we show that the material-anisotropy of NPs can lead to specific nonlocal contributions in their magnetic and electric dipole response…
We propose and theoretically analyze a new vibrational spectroscopy, termed electron- and light-induced stimulated Raman (ELISR) scattering, that combines the high spatial resolution of electron microscopy with the molecular sensitivity of surface-enhanced Raman spectroscopy. With ELISR, electron-beam excitation of plasmonic nanoparticles is utilized as a spectrally-broadband but spatially-confined Stokes beam in the presence of a diffraction-limited pump laser. To characterize this technique, we develop a numerical model and conduct full-field electromagnetic simulations to investigate two di…
The interaction of swift, free-space electrons with confined optical near fields has recently sparked much interest. It enables a new type of photon-induced near-field electron microscopy, mapping local optical near fields around nanoparticles with exquisite spatial and spectral resolution and lies at the heart of quantum state manipulation and attosecond pulse shaping of free electrons. The corresponding interaction of optical near fields with slow electrons has achieved much less attention, even though the lower electron velocity may enhance electron-near-field coupling for small nanoparticl…
We present an analytical study for the scattering amplitudes (Reflection $|R|$ and Transmission $|T|$), of the periodic ${\cal{PT}}$ symmetric optical potential $ V(x) = \displaystyle W_0 \left( \cos ^2 x + i V_0 \sin 2x \right) $ confined within the region $0 \leq x \leq L$, embedded in a homogeneous medium having uniform potential $W_0$. The confining length $L$ is considered to be some integral multiple of the period $ π$. We give some new and interesting results. Scattering is observed to be normal ($|T| ^2 \leq 1, \ |R|^2 \leq 1$) for $V_0 \leq 0.5 $, when the above potential can be mappe…
