We consider electronic transport through a suspended voltage-biased nanowire. By coupling the tunneling current to a transverse magnetic field, vibrational modes of the wire are excited which influences the current-voltage characteristics of the system in novel ways through the induced electron-vibron interaction. From this analysis, we find that at high voltages the current through the suspended nanowire is offset from its non-vibrating ohmic value by an amount that is independent of both bias voltage and temperature. We also show that the corrections to the current from the back-action of the vibrating wire decay exponentially in the limit of high voltage, a result that holds even if the nanowire vibrational modes have been driven out of thermal equilibrium.
Nanowires are perfect transducers for ultra-sensitive detections of force and mass. For small mass sensing, recent advances in detecting more properties than their masses with high sensitivity for absorbed particles onto a nanowire rely on identifications of two orthogonal flexural vibration modes of the nanowire. The directions of these orthogonal flexural vibrations with respect to measurement direction are crucial parameters of vibration modes. However, previous method, which determines a nanowire's vibration direction using thermal vibrations, requires simultaneously detecting of two ortho…
The vibrations of gold nanowires and nanorods are investigated numerically in the framework of continuum elasticity using the Rayleigh-Ritz variational method. Special attention is paid to identify the vibrations relevant in Raman scattering experiments. A comprehensive description of the vibrations of nanorods is proposed by determining their symmetry, comparing with standing waves in the corresponding nanowires and estimating their Raman intensity. The role of experimentally relevant parameters such as the anisotropic cubic lattice structure, the presence of faceted lateral surfaces and the …
We review recent results on electronic and thermal transport in two different quasi one-dimensional systems: Silicon nanowires (SiNW) and atomic gold chains. For SiNW's we compute the ballistic electronic and thermal transport properties on equal footing, allowing us to make quantitative predictions for the thermoelectric properties, while for the atomic gold chains we evaluate microscopically the damping of the vibrations, due to the coupling of the chain atoms to the modes in the bulk contacts. Both approaches are based on a combination of density-functional theory, and nonequilibrium Green'…
We consider a new type of cooling mechanism for a suspended nanowire acting as a weak link between two superconductive electrodes. By applying a bias voltage over the system, we show that the system can be viewed as a refrigerator for the nanomechanical vibrations, where energy is continuously transferred from the vibrational degrees of freedom to the extended quasiparticle states in the leads through the periodic modulation of the inter-Andreev level separation. The necessary coupling between the electronic and mechanical degrees of freedom responsible for this energy-transfer can be achieved…
We obtain the the long-wavelength polar optical vibrational modes of semiconductor core-shell nanowires by means of a phenomenological continuum model. A basis for the space of solutions is derived, and by applying the appropriate boundary conditions, the transcendental equations for the coupled and uncoupled modes are attained. Our results are applied to the study of the GaAs-GaP core-shell nanowire, for which we calculate numerically the polar optical modes, analyzing the role of strain in the vibrational properties of this nanosystem.
Based on the molecular dynamics (MD) simulation and the classical Euler-Bernoulli beam theory, a fundamental study of the vibrational performance of the Ag nanowire (NW) is carried out. A comprehensive analysis of the quality (Q)-factor, natural frequency, beat vibration, as well as high vibration mode is presented. Two excitation approaches, i.e., velocity excitation and displacement excitation, have been successfully implemented to achieve the vibration of NWs. Upon these two kinds of excitations, consistent results are obtained, i.e., the increase of the initial excitation amplitude will le…
Vibrational optical spectroscopies can be enhanced by surface plasmons to reach molecular-sized limits of detection and characterization. The level of enhancement strongly depends on microscopic details of the sample that are generally missed by macroscopic techniques. Here we investigate phonons in h-BN by coupling them to silver-nanowire plasmons, whose energy is tuned by modifying the nanowire length. Specifically, we use electron beam milling to accurately and iteratively change the nanowire length, followed by electron energy-loss spectroscopy to reveal the plasmon-enhanced vibrational fe…
We present a first-principles study on lattice vibrational modes of Si/Ge core-shell nanowires (NWs). In addition to quantum confinement, the internal strain induced by the lattice mismatch between core and shell contributes to significant frequency shifts of characteristic optical modes. More importantly, our simulation shows that these frequency shifts can be detected by Raman scattering experiments, providing convenient and nondestructive ways to obtain structural information of core-shell materials. Meanwhile, another type of collective modes, radial breathing modes (RBMs), are identified …
We have performed first-principles calculations to study the lattice vibrational modes and their Raman activities in silicon nanowires (SiNWs). Two types of characteristic vibrational modes are examined: high-frequency optical modes and low-frequency confined modes. Their frequencies have opposite size dependence with a red shift for the optical modes and a blue shift for the confined modes as the diameter of SiNWs decreases. In addition, our calculations show that these vibrational modes can be detected by Raman scattering measurements, providing an efficient way to estimate the size of SiNWs…
We consider a nanoelectromechanical Josephson junction, where a suspended nanowire serves as a superconducting weak link, and show that an applied DC bias voltage an result in suppression of the flexural vibrations of the wire. This cooling effect is achieved through the transfer of vibronic energy quanta first to voltage driven Andreev states and then to extended quasiparticle electronic states. Our analysis, which is performed for a nanowire in the form of a metallic carbon nanotube and in the framework of the density matrix formalism, shows that such self-cooling is possible down to a level…
We consider dc-electronic transport through a nanowire suspended between normal- and spin-polarized metal leads in the presence of an external magnetic field. We show that magnetomotive coupling between the electrical current through the nanowire and vibrations of the wire may result in self excitation of mechanical vibrations. The self-excitation mechanism is based on correlations between the occupancy of the quantized electronic energy levels inside the nanowire and the velocity of the nanowire. We derive conditions for the occurrence of the instability and find stable regimes of mechanical …
Presented here is a nanowire model, consisting of coupled elastic membranes with the purpose of investigating thermal transport in quasi-one-dimensional quantum systems. The vibrations of each elastic membrane are quantized and the flow of the vibrational energy between adjacent membranes is allowed. The ends of the nanowire are attached to thermal baths held at different temperatures. We derived quantum master equation for energy flow across the nanowire and obtained thermal currents and other key observables. We study the effects of a disordered boundary on the thermal current by randomizing…
We study InAs nanowire resonators fabricated on sapphire substrate with a local gate configuration. The key advantage of using an insulating sapphire substrate is that it results in a reduced parasitic capacitance thus allowing both wide bandwidth actuation and detection using a network analyzer as well as signal detection at room temperature. Both in-plane and out-of-plane vibrational modes of the nanowire can be driven and the non-linear response of the resonators studied. In addition this technique enables the study of variation of thermal strains due to heating in nanostructures
We demonstrate that a suspended nanowire forming a weak link between two superconductors can be cooled to its motional ground state by a supercurrent flow. The predicted cooling mechanism has its origins in magnetic field induced inelastic tunneling of the macroscopic superconducting phase associated with the junction. Furthermore, we show the voltage-drop over the junction is proportional to the average population of the vibrational modes in the stationary regime, a phenomena which can be used to probe the level of cooling.
We investigate electron-phonon coupling in a narrow suspended metallic wire, in which the phonon modes are restricted to one dimension but the electrons behave three-dimensionally. Explicit theoretical results related to the known bulk properties are derived. We find out that longitudinal vibration modes can be cooled by electronic tunnel refrigeration far below the bath temperature provided the mechanical quality factors of the modes are sufficiently high. The obtained results apply to feasible experimental configurations.
Engineering of the cross-section shape and size of ultra-scaled Si nanowires (SiNWs) provides an attractive way for tuning their structural properties. The acoustic and optical phonon shifts of the free-standing circular, hexagonal, square and triangular SiNWs are calculated using a Modified Valence Force Field (MVFF) model. The acoustic phonon blue shift (acoustic hardening) and the optical phonon red shift (optical softening) show a strong dependence on the cross-section shape and size of the SiNWs. The triangular SiNWs have the least structural symmetry as revealed by the splitting of the d…
We study thermal transport through Pt nanowires that bridge planar contacts as a function of wire length and vibrational frequency of the contacts. When phonons in the contacts have lower average frequencies than those in the wires thermal transport occurs under conditions away from local equilibrium with low-frequency phonons experiencing a higher thermal gradient than high-frequency ones. This results in a size-dependent increase in the effective thermal conductivity of the wire with decreasing vibrational frequencies of the contacts. The interfacial resistivity when heat flows from the wire…
We study theoretically electron spins in nanowire quantum dots placed inside a transmission line resonator. Because of the spin-orbit interaction, the spins couple to the electric component of the resonator electromagnetic field and enable coherent manipulation, storage, and read-out of quantum information in an all-electrical fashion. Coupling between distant quantum-dot spins, in one and the same or different nanowires, can be efficiently performed via the resonator mode either in real time or through virtual processes. For the latter case we derive an effective spin-entangling interaction a…
Self-organized silicide nanowires are considered as main building blocks of future nanoelectronics and have been intensively investigated. In nanostructures, the lattice vibrational waves (phonons) deviate drastically from those in bulk crystals, which gives rise to anomalies in thermodynamic, elastic, electronic, and magnetic properties. Hence, a thorough understanding of the physical properties of these materials requires a comprehensive investigation of the lattice dynamics as a function of the nanowire size. We performed a systematic lattice dynamics study of endotaxial FeSi$_2$ nanowires,…
Suspended nanowires are shown to provide mechanically-controlled coherent mixing/splitting of the spin states of transmitted electrons, caused by the Rashba spin-orbit interaction. The sensitivity of the latter to mechanical bending makes the wire a tunable nano-electro-mechanical (NEM) weak link between reservoirs. When the reservoirs are populated with misbalanced "spin up/down" electrons, the wire becomes a source of split spin currents, which are not associated with electric charge transfer and which do not depend on temperature or driving voltages. The mechanical vibrations of the bended …
An intriguing athermal uniform elongation and accelerated radial shrinkage in amorphous SiOx nanowire (a-SiOx NW) as purely induced by uniform electron beam (e-beam) irradiation were in-situ investigated in transmission electron microscope. It was observed that at room temperature the straight and uniform a-SiOx NW demonstrated a uniform plastic elongation (without any external tensile pulling) and a corresponding uniform radial shrinkage. According to a new model taking into account the NW nanocurvature over its surface as well as the beam-induced athermal activation, a kinetic relationship b…
We settle a general expression for the Hamiltonian of the electron-phonon deformation potential (DP) interaction in the case of non-polar core-shell cylindrical nanowires (NWs). On the basis of long range phenomenological continuum model for the optical modes and by taking into account the bulk phonon dispersions, we study the size dependence and strain-induced shift of the electron-phonon coupling strengths for Ge-Si and Si-Ge NWs. We derive analytically the DP electron-phonon Hamiltonian and report some numerical results for the frequency core modes and vibrational amplitudes. Our approach a…
Planar driven nanowire oscillators are susceptible to undergo whirling motion due to coupling between flexural planar and nonplanar modes of vibration. This investigation is concerned with planar to whirling motion transition in the oscillation of an electrostatically actuated nanowire, which is pre-deflected due to applied DC voltage. We have derived dynamical equations of motion using Euler-Bernoulli beam theory and Galerkin formulation as reduced order model of the governing coupled partial differential equations. The dynamical equations have been solved using second-order averaging method …
We consider a nanowire suspended on two spin-polarized leads and subject to a nonuniform magnetic field. We show that in such a system a temperature drop between leads can significantly affect the nanowire dynamics. In particular, it is demonstrated that under certain conditions the stationary distribution of the mechanical subsystem has Boltzmann form with effective temperature which is smaller than the temperature of the "cold" lead; this seems rather counterintuitive. We also find that the change of the direction of the temperature gradient results in generation of mechanical vibrations rat…
A III-V compound semiconductor nanowire is an attractive material for a novel hybrid quantum interface that interconnects photons, electrons, and phonons through a wavelength-tunable quantum structure embedded in its free-standing structure. In such a nanomechanical element, however, a challenge is how to detect and manipulate a small number of phonons via its tiny mechanical motion. A solution would be to couple an optical cavity to a nanowire by introducing the ``cavity optomechanics'' framework, but the typical size difference between them becomes a barrier to achieving this. Here, we demon…
We examine theoretically the effects of the bonding geometries at the gold-thiol interfaces on the inelastic tunneling spectra of propanedithiolate (PDT) molecules bridging gold electrodes and show that inelastic tunneling spectroscopy combined with theory can be used to determine these bonding geometries experimentally. With the help of density functional theory, we calculate the relaxed geometries and vibrational modes of extended molecules each consisting of one or two PDT molecules connecting two gold nanoclusters. We formulate a perturbative theory of inelastic tunneling through molecules…
Half a century ago Brian Josephson made a series of striking predictions related to a tunnelling barrier sandwiched between two superconductors. One particular prediction, later became known as the a.c.-Josephson effect, said that under a finite d.c. bias the tunnelling current contains an a.c. supercurrent component, oscillating at microwave frequency. This prediction was experimentally verified through observation of the junction current-voltage characteristics modified by the interaction with the electromagnetic radiation, and direct detection of the microwave radiation emitted from the jun…
Passivation effect of heterogeneous Au nanoparticles (AuNPs) on the nonuniform structure changes of amorphous SiOx nanowire (a-SiOx NW) as athermally induced by focused electron beam (e-beam) irradiation is investigated in an in-situ transmission electron microscope. It is found that at room temperature the straight and uniform a-SiOx NW demonstrates an accelerated necking at the nanoscale along with a fast, plastic elongation and a local S-type deformation in the axial direction. However, once being modified with uniform AuNPs, the nanocurved sidewall surface of a-SiOx NW becomes intriguingly…
Recent progress in nanotechnology has allowed to fabricate new hybrid systems where a single two-level system is coupled to a mechanical nanoresonator. In such systems the quantum nature of a macroscopic degree of freedom can be revealed and manipulated. This opens up appealing perspectives for quantum information technologies, and for the exploration of quantum-classical boundary. Here we present the experimental realization of a monolithic solid-state hybrid system governed by material strain: a quantum dot is embedded within a nanowire featuring discrete mechanical resonances corresponding …
We study theoretically the detection and possible utilization of electric current-induced mechanical torques in ferromagnetic-normal metal heterostructures that are generated by spin-flip scattering or the absorption of transverse spin currents by a ferromagnet. To this end, we analyze the DC voltage signals over a spin valve that is driven by an AC current. In agreement with recent studies, this "rectification", measured as a function of AC frequency and applied magnetic field, contains important information on the magnetostatics and --dynamics. Subsequently, we show that the vibrations excit…
Long metallic nanowires combine crucial factors for non-conservative current-driven atomic mo- tion. These systems have degenerate vibrational frequencies, clustered about a Kohn anomaly in the dispersion relation, that can couple under current to form non-equilibrium modes of motion growing exponentially in time. Such motion is made possible by non-conservative current-induced forces on atoms, and we refer to it generically as the waterwheel effect. Here the connection be- tween the waterwheel effect and the stimulated directional emission of phonons propagating along the electron flow is dis…
