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arXiv 0812.3732cond-mat.str-elcond-mat.supr-con
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Bandwidth tuning triggers interplay of charge order and superconductivity in two-dimensional organic materials

S. Kaiser, M. Dressel, Y. Sun, A. Greco, J. A. Schlueter, G. L. Gard, N. Drichko

英文摘要:

We observe charge-order fluctuations in the quasi-two-dimensional organic superconductor $β^{\prime\prime}$-(BEDT-TTF)2 SF5 CH2 CF2 SO3 both by means of vibrational spectroscopy, locally probing the fluctuating charge order, and investigating the in-plane dynamical response by infrared reflectance spectroscopy. The decrease of effective electronic interaction in an isostructural metal suppresses both charge-order fluctuations and superconductivity, pointing on their interplay. We compare the results of our experiments with calculations on the extended Hubbard model.

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